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Clarification and exploration of novel transport phenomena caused by electron-electron interactions and spin degrees of freedom in molecular crystals

Research Project

Project/Area Number 22740237
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Condensed matter physics II
Research InstitutionNational Institute for Materials Science

Principal Investigator

YAMAGUCHI Takahide  独立行政法人物質・材料研究機構, 超伝導線材ユニット, 主任研究員 (70399385)

Project Period (FY) 2010 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2011: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2010: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywords分子性結晶 / モット絶縁体 / 電荷秩序 / 非線形伝導 / 巨大磁気抵抗 / スピン依存伝導 / 誘電率 / 電子間クーロン相互作用 / 量子トンネル効果
Research Abstract

We have measured the low-temperature nonlinear current-voltage characteristics, dielectric properties, and magnetoconductance of organic crystalline insulators caused by electron-electron Coulomb interaction and clarified their transport mechanism. The Mott and charge-order insulators exhibit the same transport properties at zero magnetic field, but their magnetoconductances differ due to different spin states of the carriers that contribute to the conductivity. We have also performed measurements using micro-fabricated electrodes and under microwave irradiation.

Report

(3 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • Research Products

    (34 results)

All 2012 2011 2010 Other

All Journal Article (15 results) (of which Peer Reviewed: 15 results) Presentation (14 results) Remarks (5 results)

  • [Journal Article] Charge Transport in Charge-Ordered States of Two-Dimensional Organic Conductors,α-(BEDT-TTF)_2I_3 andα'-(BEDT-TTF)_2IBr_22012

    • Author(s)
      Kota Kodama, Motoi Kimata, Yamaguchi Takahide, Nobuyuki Kurita, Atsushi Harada, Hidetaka Satsukawa, Taichi Terashima, Shinya Uji, Kaoru Yamamoto, and Kyuya Yakushi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 81

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Two-dimensional superconductivity in the layered organic superconductorK_H-(DMEDO-TSeF)_2[Au(CN)_4](THF) with thick dielectric insulating layers2012

    • Author(s)
      Tadashi Kawamoto, Takehiko Mori, Yamaguchi Takahide, Taichi Terashima, Shinya Uji, Takashi Shirahata, Tatsuro Imakubo
    • Journal Title

      Physical Review B

      Volume: 85

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Charge Transport in Charge-Ordered States of Two-Dimensional Organic Conductors, alpha-(BEDT-TTF)_2I_3 and alpha2012

    • Author(s)
      K.Kodama
    • Journal Title

      JPSJ

      Volume: 81 Issue: 4 Pages: 44703-44703

    • DOI

      10.1143/jpsj.81.044703

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Two-dimensional superconductivity in the layered organic superconductor κ_H-(DMEDO-TSeF)_2[Au(CN)_4](THF) with thick dielectric insulating layers2012

    • Author(s)
      T.Kawamoto, T.Mori, Y.Takahide, T.Terashima, S.Uji, T.Shirahata, T.Imakubo
    • Journal Title

      Phys.Rev.B

      Volume: 85(17) Issue: 1

    • DOI

      10.1103/physrevb.85.014504

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Highly nonlinear current-voltage characteristics of the organic Mott insulator_K-(BEDT-TTF)_2Cu[N(CN)_2] Cl2011

    • Author(s)
      Yamaguchi Takahide, Motoi Kimata, Kouta Kodama, Taichi Terashima, Shinya Uji, Megumi Kobayashi, and Hiroshi M. Yamamoto
    • Journal Title

      Physical Review B

      Volume: 84

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fermi surface and interlayer transport in the two-dimensional magnetic organic conductor(Me-3, 5-DIP)[Ni(dmit)_2]_22011

    • Author(s)
      K. Hazama, S. Uji, Yamaguchi Takahide, M. Kimata, H. Satsukawa, A. Harada, T. Terashima, Y. Kosaka, H. M. Yamamoto and R Kato
    • Journal Title

      Physical Review B

      Volume: 83

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fermi surface and in-plane anisotropy of the layered organic superconductorK_L-(DMEDO-TSeF)_2[Au(CN)_4](THF) with domain structures2011

    • Author(s)
      Tadashi Kawamoto, Takehiko Mori, Yamaguchi Takahide, Shinya Uji, David Graf, James S. Brooks, Takashi Shirahata, Megumi Kibune, Hiroko Yoshino, and Tatsuro Imakubo
    • Journal Title

      Physical Review B

      Volume: 83

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Highly nonlinear current-voltage characteristics of the organic Mott insulator kappa-(BEDT-TTF)2Cu[N(CN)2]C]2011

    • Author(s)
      Yamaguchi Takahide, Motoi Kimata, Kouta Kodama, Taichi Terashima, Shinya Uji, Megumi Kobayashi, Hiroshi M.Yamamoto
    • Journal Title

      Physical Review B

      Volume: 84 Issue: 3

    • DOI

      10.1103/physrevb.84.035129

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fermi Surface and Interlayer Transport in the Two-Dimensional Magnetic Organic Conductor (Me-3,5-DIP)[Ni(dmit)_2]_22011

    • Author(s)
      K.Hazama, S.Uji, Y.Takahide, M.Kimata, H.Satsukawa, A.Harada, T.Terashima, Y.Kosaka, H.M.Yamamoto, R.Kato
    • Journal Title

      Physical Review B

      Volume: 83 Issue: 16

    • DOI

      10.1103/physrevb.83.165129

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fermi surface and in-plane anisotropy of the layered organic superconductor kappa_L-(DMEDO-TSeF)_2[Au(CN)_4](THF) with domain structures2011

    • Author(s)
      川本正、森健彦、山口尚秀, 他
    • Journal Title

      Physical Review B

      Volume: 83

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 層状分子性結晶の非線形伝導と巨大磁気抵抗2011

    • Author(s)
      山口尚秀
    • Journal Title

      固体物理

      Volume: 46 Pages: 29-39

    • NAID

      40018712905

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Charge Transport in Charge-Ordered Layered Crystalsθ-(BEDT-TTF)_2MZn(SCN)_4(M=Cs, Rb): Effects of Long-Range Coulomb Interaction and Pauli Exclusion Principle2010

    • Author(s)
      Yamaguchi Takahide, Motoi Kimata, Kaori Hazama, Taichi Terashima, Shinya Uji, Takako Konoike, and Hiroshi M. Yamamoto
    • Journal Title

      Physical Review B

      Volume: 81

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Non-linear current-voltage characteristics inα-(BEDT-TTF)_2I_32010

    • Author(s)
      K. Kodama, M. Kimata, Yamaguchi Takahide, T. Terashima, H. Satsukawa, A. Harada, K. Hazama, S. Uji, K. Yamamoto, K. Yakushi
    • Journal Title

      Physica B

      Volume: 405

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Charge Transport in Charge-Ordered Layered Crystals theta-(BEDT-TTF)_2MZn(SCN)_4 (M=Cs, Rb) : Effects of Long-Range Coulomb Interaction and Pauli Exclusion Principle2010

    • Author(s)
      山口尚秀, 他
    • Journal Title

      Physical Review B

      Volume: 81

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Non-linear current-voltage characteristics in alpha-(BEDT-TTF)_2I_32010

    • Author(s)
      小玉恒太、木俣基、山口尚秀, 他
    • Journal Title

      Physica B

      Volume: 405

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] Charge dynamics in Mott-insulating and charge-ordered organic crystals : a possibility of Kosterlitz-Thouless metal-insulator transition2012

    • Author(s)
      Yamaguchi Takahide, Tohru Watanabe, Yoshihiko Takano, Kouta Kodama, Shinya Uji, Hiroshi M.Yamamoto
    • Organizer
      American Physical Society March meeting 2012
    • Place of Presentation
      Boston Convention Center, Boston, USA
    • Year and Date
      2012-02-27
    • Related Report
      2011 Annual Research Report
  • [Presentation] Charge dynamics in Mott-insulating and charge-ordered organic crystals : a possibility of Kosterlitz-Thouless metal-insulator transition2012

    • Author(s)
      Yamaguchi Takahide, Tohru Watanabe, Yoshihiko Takano, Kouta Kodama Shinya Uji, Hiroshi M. Yamamoto
    • Organizer
      American Physical Society March meeting
    • Place of Presentation
      Boston Convention Center(Boston, USA)
    • Related Report
      2011 Final Research Report
  • [Presentation] BEDT-TTF系分子性結晶の微小領域伝導2011

    • Author(s)
      山口尚秀、渡邊徹、高野義彦、小玉恒太、宇治進也、山本浩史
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学、富山
    • Year and Date
      2011-09-21
    • Related Report
      2011 Annual Research Report
  • [Presentation] 微小電極を用いて測定した分子性結晶の伝導特性2011

    • Author(s)
      山口尚秀
    • Organizer
      特定領域研究「配列ナノ空間を利用した新物質科学 ユビキタス元素戦略」第7回領域会議
    • Place of Presentation
      大阪大学
    • Year and Date
      2011-01-07
    • Related Report
      2010 Annual Research Report
  • [Presentation] K-(BEDT-TTF)_2Cu[N(CN)_2] Clのモット絶縁相における電荷輸送2011

    • Author(s)
      山口尚秀
    • Organizer
      有機固体若手の会冬の学校
    • Place of Presentation
      定山渓
    • Related Report
      2011 Final Research Report
  • [Presentation] Charge transport of insulating organic crystals measured with sub-micron electrodes2011

    • Author(s)
      Yamaguchi Takahide, Tohru Watanabe, Yoshihiko Takano, Kouta Kodama, Shinya Uji, and Hiroshi M. Yamamoto
    • Organizer
      International Conferentce of New Science Created by Materials with Nano Spaces
    • Place of Presentation
      Tohoku University, Sendai
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] BEDT-TTF系分子性結晶の微小領域伝導2011

    • Author(s)
      山口尚秀、渡邊徹、高野義彦、小玉恒太、宇治進也、山本浩史
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学(富山)
    • Related Report
      2011 Final Research Report
  • [Presentation] 微小電極による分子性結晶の伝導測定2010

    • Author(s)
      山口尚秀
    • Organizer
      有機固体若手の学校冬の学校
    • Place of Presentation
      上諏訪
    • Year and Date
      2010-12-10
    • Related Report
      2010 Annual Research Report
  • [Presentation] メタルマスクによる分子性結晶上へのサブミクロン電極の作製2010

    • Author(s)
      山口尚秀
    • Organizer
      日本物理学会 2010年秋季大会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2010-09-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] 層状分子性結晶theta-(BEDT-TTF)_2CsZn(SCN)_4の低周波誘電特性2010

    • Author(s)
      山口尚秀
    • Organizer
      特定領域研究「配列ナノ空間を利用した新物質科学 ユビキタス元素戦略」第6回領域会議
    • Place of Presentation
      名古屋大学
    • Year and Date
      2010-05-29
    • Related Report
      2010 Annual Research Report
  • [Presentation] 微小電極による分子性結晶の伝導測定2010

    • Author(s)
      山口尚秀
    • Organizer
      有機固体若手の会冬の学校
    • Place of Presentation
      上諏訪
    • Related Report
      2011 Final Research Report
  • [Presentation] メタルマスクによる分子性結晶上へのサブミクロン電極の作製2010

    • Author(s)
      山口尚秀、渡邊徹、高野義彦、小玉恒太、宇治進也、山本浩史
    • Organizer
      日本物理学会2010年秋季大会
    • Place of Presentation
      大阪府立大学(大阪)
    • Related Report
      2011 Final Research Report
  • [Presentation] Dielectric anisotropy of the organic crystalsθ-(BEDT-TTF)_2CsZn(SCN)_4 and K-(BEDT-TTF)_2Cu[N(CN)_2] Cl2010

    • Author(s)
      Yamaguchi Takahide, K. Kodama, M. Kimata, T. Terashima, S. Uji, Y. Takano, M. Kobayashi and H. M. Yamamoto
    • Organizer
      ICSM2010(International Conference on Science and Technology of Synthetic Metals)
    • Place of Presentation
      Kyoto
    • Related Report
      2011 Final Research Report
  • [Presentation] Spin Related Magnetotransport in Insulating BEDT-TTF Crystals2010

    • Author(s)
      Yamaguchi Takahide, Kouta Kodama, Motoi Kimata, Taichi Terashima, Shinya Uji, Tohru Watanabe, Yoshihiko Takano, Megumi Kobayashi, Hiroshi M. Yamamoto
    • Organizer
      ISSP-MDF Joint International Workshop Spin-related Phenomena in Organic Materials
    • Place of Presentation
      ISSP, Kashiwa
    • Related Report
      2011 Final Research Report
  • [Remarks]

    • URL

      http://samurai.nims.go.jp/YAMAGUCHI_Takahide-j.html

    • Related Report
      2011 Final Research Report
  • [Remarks]

    • URL

      http://www.nims.go.jp/NFM/member/yamaguchi/index_j.html

    • Related Report
      2011 Final Research Report
  • [Remarks]

    • URL

      http://samurai.nims.go.jp/YAMAGUCHI_Takahide-j.html

    • Related Report
      2011 Annual Research Report
  • [Remarks]

    • URL

      http://www.nims.go.jp/NFM/member/yamaguchi/index_j.html

    • Related Report
      2011 Annual Research Report
  • [Remarks]

    • URL

      http://www.nims.go.jp/NFM/member/yamaguchi/index.html

    • Related Report
      2010 Annual Research Report

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Published: 2010-08-23   Modified: 2020-05-15  

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