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Oxygen storage materials among transition-metal oxides : development of new materials and their applications

Research Project

Project/Area Number 22750181
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Inorganic industrial materials
Research InstitutionHokkaido University

Principal Investigator

MOTOHASHI Teruki  北海道大学, 大学院・工学研究院, 准教授 (00323840)

Co-Investigator(Renkei-kenkyūsha) KIKKAWA Shinichi  北海道大学, 大学院・工学研究院, 教授 (10127219)
MASUBUCHI Yuji  北海道大学, 大学院・工学研究院, 助教 (80466440)
Research Collaborator SETOYAMA Tohru  三菱化学科学技術研究センター, 無機系機能材料研究所, 所長
OSHIMA Kazunori  三菱化学科学技術研究センター, 無機系機能材料研究所, 主席研究員
Project Period (FY) 2010 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2011: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2010: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywords酸素貯蔵材料 / 遷移金属酸化物 / マンガン酸化物 / ペロブスカイト / 酸素貯蔵能 / 酸化還元触媒 / 酸素濃縮 / 燃料電池
Research Abstract

Oxides with remarkable oxygen intake/release capability are called "oxygen storage materials(OSMs)" which have attracted increased attention as potential candidates for energy production/environmental applications. The present work was aimed to search for new OSMs among transition-metal oxides. In this project, two manganese-based OSMs, BaYMn_2O_<5+δ> and Ca_2(AlxMn_<1-x>)_2O_<5+δ>, were developed and their oxygen intake/release mechanism was studied.

Report

(3 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • Research Products

    (24 results)

All 2012 2011 2010 Other

All Journal Article (5 results) (of which Peer Reviewed: 3 results) Presentation (14 results) Remarks (5 results)

  • [Journal Article] The oxygen-storage materials BaYMn_2O_<5+δ> from the quantum-chemical point of view2012

    • Author(s)
      M. Gillesen, M. Lumeij, J. George, R. Stoffel, T. Motohashi, S. Kikkawa, and R. Dronskowski
    • Journal Title

      Chemistry of Materials

      Volume: (in press)

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Enhanced oxygen intake/release kinetics of BaYMn_2O_<5+δ> fine powders prepared by a wet-chemical route2011

    • Author(s)
      T. Motohashi, T. Ueda, Y. Masubuchi, and S. Kikkawa
    • Journal Title

      Journal of the Ceramics Society of Japan

      Volume: 119 Pages: 894-897

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Enhanced oxygen intake/release kinetics of BaYMn2O5+.DELTA. fine powders prepared by a wet-chemical route2011

    • Author(s)
      T.Motohashi, T.Ueda, Y.Masubuchi, S.Kikkawa
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 119 Issue: 1395 Pages: 894-897

    • DOI

      10.2109/jcersj2.119.894

    • NAID

      130001310521

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ダブルペロブスカイト型マンガン酸化物BaYMn_2O_<5+δ>の酸素貯蔵能2010

    • Author(s)
      本橋輝樹, 上田拓, 鱒渕友治, 吉川信一, 滝口真, 瀬戸山亨, 大島一典
    • Journal Title

      燃料電池

      Volume: 10(No.1) Pages: 145-148

    • Related Report
      2011 Final Research Report
  • [Journal Article] ダブルペロブスカイド型マンガン酸化物BaYMn_2O_<5+δ>の酸素貯蔵能2010

    • Author(s)
      本橋輝樹, 上田拓, 鱒渕友治, 吉川信一, 滝口真, 瀬戸山亨, 大島一典
    • Journal Title

      燃料電池

      Volume: 10 Pages: 145-148

    • Related Report
      2010 Annual Research Report
  • [Presentation] ブラウンミラーライト型Ca_2(Al_xMn_<1-x>)_2O<5+δ>(x=0. 50~0. 67)の酸素貯蔵能2012

    • Author(s)
      平野佑佳,本橋輝樹,鱒渕友治,吉川信一,大島一典,瀬戸山亨
    • Organizer
      日本セラミックス協会2012年年会
    • Place of Presentation
      京都大学吉田キャンパス(京都)
    • Year and Date
      2012-03-20
    • Related Report
      2011 Final Research Report
  • [Presentation] ブラウンミラーライト型Ca_2(Al_xMn_<1-x>)_2O_<5+δ> (x=0.50~0.67)の酸素貯蔵能2012

    • Author(s)
      平野佑佳、本橋輝樹、鱒渕友治、吉川信一、大島一典、瀬戸山亨
    • Organizer
      日本セラミックス協会2012年年会
    • Place of Presentation
      京都大学吉田キャンパス(京都)
    • Year and Date
      2012-03-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] マンガンをベースにした酸素貯蔵材料の創製とその応用展開2012

    • Author(s)
      本橋輝樹
    • Organizer
      平成23年度日本化学会北海道支部奨励賞受賞講演
    • Place of Presentation
      北海道大学札幌キャンパス(札幌)
    • Year and Date
      2012-02-01
    • Related Report
      2011 Final Research Report
  • [Presentation] マンガンをベースにした酸素貯蔵材料の創製とその応用展開2012

    • Author(s)
      本橋輝樹
    • Organizer
      平成23年度日本化学会北海道支部奨励賞受賞講演
    • Place of Presentation
      北海道大学札幌キャンパス(札幌)(招待講演)
    • Year and Date
      2012-02-01
    • Related Report
      2011 Annual Research Report
  • [Presentation] 酸素貯蔵材料BaYMn_2O_<5+δ>(δ=0~1)の酸素吸収放出挙動2012

    • Author(s)
      上田拓,本橋輝樹,鱒渕友治,吉川信一
    • Organizer
      セラミックス基礎科学討論会第50回記念大会
    • Place of Presentation
      国際ファッションセンター(東京)
    • Year and Date
      2012-01-12
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] Oxygen intake/release kinetics of double-perovskite type BaYMn_2O_<5+δ>(δ=0~1)2011

    • Author(s)
      Taku Ueda, Teruki Motohashi, Yuji Masubuchi, and Shinichi Kikkawa
    • Organizer
      The third Symposium on Academic Exchange and Collaborative Research between the Faculty of Engineering, Hokkaido University & the Materials Research Center
    • Place of Presentation
      ETH Zurich(Zurich, Switzerland)
    • Year and Date
      2011-10-12
    • Related Report
      2011 Final Research Report
  • [Presentation] Oxygen intake/release kinetics of double-perovskite type BaYMn_2O_<5+δ>(δ=0~1)2011

    • Author(s)
      Taku Ueda, Teruki Motohashi, Yuji Masubuchi, Shinichi Kikkawa
    • Organizer
      The third Symposium on Academic Exchange and Collaborative Research between the Faculty of Engineering, Hokkaido University & the Materials Research Center, ETH Zurich
    • Place of Presentation
      ETH Zurich (Zurich, Switzerland)
    • Year and Date
      2011-10-12
    • Related Report
      2011 Annual Research Report
  • [Presentation] 酸素欠損ペロブスカイト型マンガン酸化物の顕著な酸素貯蔵能2011

    • Author(s)
      本橋輝樹,上田拓,平野佑佳,鱒渕友治,吉川信一,大島一典,瀬戸山享
    • Organizer
      日本セラミックス協会第24回秋季シンポジウム
    • Place of Presentation
      北海道大学札幌キャンパス(札幌)
    • Year and Date
      2011-09-07
    • Related Report
      2011 Annual Research Report 2011 Final Research Report
  • [Presentation] ブラウンミラーライト型Ca_2(Al_xMn_<1-x>)_2O_<5+δ>(x=0. 5~0. 67,δ=0~0.5)の合成と酸素吸収放出特性2011

    • Author(s)
      平野佑佳,本橋輝樹,鱒渕友治,大島一典,瀬戸山亨,吉川信一
    • Organizer
      日本化学会北海道支部2011年夏季研究発表会
    • Place of Presentation
      室蘭工業大学(室蘭市)
    • Year and Date
      2011-07-23
    • Related Report
      2011 Final Research Report
  • [Presentation] ブラウンミラーライト型Ca_2(Al_xMn_<1-x>)_2O_<5+δ> (x=0.5~0.67, δ=0~0.5)の合成と酸素吸収放出特性2011

    • Author(s)
      平野佑佳、本橋輝樹、鱒渕友治、大島一典、瀬戸山亨、吉川信一
    • Organizer
      日本化学会北海道支部2011年夏季研究発表会
    • Place of Presentation
      室蘭工業大学(室蘭市)
    • Year and Date
      2011-07-23
    • Related Report
      2011 Annual Research Report
  • [Presentation] ダブルペロブスカイト型BaYMn_2O_<5+δ>における酸素吸収放出の速度論研究2011

    • Author(s)
      上田拓,本橋輝樹,鱒渕友治,吉川信一
    • Organizer
      日本セラミックス協会2011年年会
    • Place of Presentation
      静岡大学(浜松)
    • Year and Date
      2011-03-18
    • Related Report
      2011 Final Research Report
  • [Presentation] ダブルペロブスカイト型BaYMn_2O_<5+δ>における酸素吸収放出の速度論研究2011

    • Author(s)
      上田拓, 本橋輝樹, 鱒渕友治, 吉川信一
    • Organizer
      日本セラミックス協会2011年年会
    • Place of Presentation
      静岡大学,浜松
    • Year and Date
      2011-03-18
    • Related Report
      2010 Annual Research Report
  • [Presentation] BaYMn_2O_<5+δ>: A Potential Material for Oxygen-Storage Applications2010

    • Author(s)
      T. Motohashi, T. Ueda, Y. Masubuchi, S. Kikkawa, M. Takiguchi, T. Setoyama, and K. Oshima
    • Organizer
      12th International Ceramics Congress(CIMTEC 2010)
    • Place of Presentation
      Plazzo dei Congressi, Montecatini Terme, Italy
    • Year and Date
      2010-06-10
    • Related Report
      2011 Final Research Report
  • [Presentation] BaYMn_2O_<5+δ> : A Potential Material for Oxygen-Storage Applications2010

    • Author(s)
      T.Motohashi, T.Ueda, Y.Masubuchi, S.Kikkawa, M.Takiguchi, T.Setoyama, K.Oshima
    • Organizer
      12th International Ceramics Congress (CIMTEC 2010)
    • Place of Presentation
      Plazzo dei Congressi, Montecatini Terme, Italy
    • Year and Date
      2010-06-10
    • Related Report
      2010 Annual Research Report
  • [Remarks] 「北大高性能な酸素貯蔵材料を汎用元素のみで製造」,化学工業日報, 2011年8月31日.新聞報道

    • Related Report
      2011 Final Research Report
  • [Remarks] 高性能な酸素貯蔵材料汎用元素のみで製造,「トピックス」,セラミックス47(No.1), 51(2012).学会誌の紹介記事

    • Related Report
      2011 Final Research Report
  • [Remarks] 本研究の成果により、日本化学会北海道支部奨励賞を受賞研究成果に関するWebページ

    • URL

      http://homepagel.nifty.com/csjh/23records/23syoureisyou/motohasi.pdf

    • Related Report
      2011 Annual Research Report
  • [Remarks] 研究成果の新聞記事掲載化学工業日報平成23年8月31日(3面)掲載「高性能な酸素貯蔵材料汎用元素のみで製造」

    • URL

      http://www.kagakukogyonippo.com/headline/2011/08/31-3379.html

    • Related Report
      2011 Annual Research Report
  • [Remarks] 研究成果の学術雑誌紹介記事セラミックス誌2012年1月号「高性能な酸素貯蔵材料汎用元素のみで製造」

    • URL

      http://www.ceramic.or.jp/ihensyub/topics/topics2012.1.pdf

    • Related Report
      2011 Annual Research Report

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Published: 2010-08-23   Modified: 2016-04-21  

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