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Nonequilibrium Quantum Electron Transport Properties of Functional Interfaces

Research Project

Project/Area Number 22760500
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Physical properties of metals
Research InstitutionTohoku University

Principal Investigator

WANG Zhongchang  東北大学, 原子分子材料科学高等研究機構, 助教 (20510548)

Project Period (FY) 2010 – 2011
Project Status Completed (Fiscal Year 2011)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2011: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2010: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywords界面 / 電子顕微鏡 / 第一原理計算 / 粒界 / 二次元電子系 / 電子状態 / 電子材料 / 原子構造
Research Abstract

The origin of the long-standing contact issue in silicon carbide devices can be understood and technologically manipulated at atomic level. Using advanced transmission electron microscopy, we attributed qualitatively the formation of ohmic contacts to silicon carbide to an epitaxial, coherent, and atomically ordered interface. First principles calculations predict that this interface can trap an atomic layer of carbon and hence enable lowered Schottky barrier and enhanced quantum electron transport.
An unprecedented insulator-to-metal transition has been discovered in A-site excess, nonstoichiometric oxides, La_<0. 5> Sr_<n+ 1-0. 5> TinO_<3n+ 1>, which is found to be driven by an insulating SrTiO_3 unit cell. The transition is accompanied by electron localization due to a complex interplay of electrons and phonons, and is unusual as the majority of electrons in the conducting phase are confined to within an atomic layer forming a two-dimensional electron gas.

Report

(3 results)
  • 2011 Annual Research Report   Final Research Report ( PDF )
  • 2010 Annual Research Report
  • Research Products

    (50 results)

All 2012 2011 2010

All Journal Article (30 results) (of which Peer Reviewed: 30 results) Presentation (19 results) Book (1 results)

  • [Journal Article] Enhanced Gas-sensing Properties by SnO_2 Nanosphere Functionalized TiO_2 Nanobelts2012

    • Author(s)
      Wen Zeng, Tianmo Liu, Zhongchang Wang
    • Journal Title

      Journal of Materials Chemistry

      Volume: 22 Pages: 3544-3544

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Double Change Channel Angular Pressing of Magnesium Alloys AZ312012

    • Author(s)
      Liwei Lu, Tianmo Liu, Yong Chen, Liguang Wang, Zhongchang Wang
    • Journal Title

      Materials and Design

      Volume: 35 Pages: 138-138

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Microstructure and Corrosion Behavior of AZ31 Alloys Prepared by Dual Directional Extrusion2012

    • Author(s)
      Liwei Lu, Tianmo Liu, Jian Chen, Zhongchang Wang
    • Journal Title

      Materials and Design

      Volume: 36 Pages: 687-687

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Electrical Conductivity Optimization in Electrolyte-free Fuel Cells by Single-component Ce_<0. 8> Sm_<0. 2> O_<2-δ>-Li_<0. 15> Ni_<0. 45> Zn_<0. 4> Layer2012

    • Author(s)
      Yanjie Xia, Xiaojuan Liu, Yijia Bai, Hongping Li, Xiaolong Deng, Xiaodong Niu, Xiaojie Wu, Defeng Zhou, Minfeng Lv, Zhongchang Wang, Jian Meng
    • Journal Title

      RSC Advances

      Volume: 2 Pages: 3828-3828

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effect of Annealing on Microstructure Evolution and Mechanical Property of Cold Forged Magnesium Pipes2012

    • Author(s)
      Liwei Lu, Tianmo Liu, Ming-jen Tan, Jian Chen, Zhongchang Wang
    • Journal Title

      Materials and Design

      Volume: 39 Pages: 131-131

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Deformation and Fracture Behavior of Hot Extruded Mg Alloys AZ312012

    • Author(s)
      Liwei Lu, Tianmo Liu, Yong Chen, Zhongchang Wang
    • Journal Title

      Materials Characterization

      Volume: 67 Pages: 93-93

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Gas-sensing Property Performance Enhancement in ZnO Nanostructures by Hierarchical Morphology2012

    • Author(s)
      Weiwei Guo, Tianmo Liu, Hejing Zhang, Rong Sun, Yong Chen, Wen Zeng, Zhongchang Wang
    • Journal Title

      Sensors and Actuators B

      Volume: 492 Pages: 166-167

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Structural and Electronic Impact of SrTiO_3 Substrate on TiO_2 Thin Films2012

    • Author(s)
      Zhongchang Wang, Rong Sun, Chunlin Chen, Mitsuhiro Saito, Susumu Tsukimoto, Yuichi Ikuhara
    • Journal Title

      Journal of Materials Science

      Volume: 47 Pages: 5148-5148

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Insulator-Metal Transition Driven by Pressure and B-Site Disorder in Double Perovskite La_2CoMnO_62012

    • Author(s)
      Shuhui Lv, Xiaojuan Liu, Hongping Li, Lin Han, Zhongchang Wang, Jian Meng
    • Journal Title

      Journal of Computational Chemistry

      Volume: 33 Pages: 1433-1433

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Adhesion, Atomic Structure and Bonding Variation at TiN/VN Interface by Chemical Segregation2012

    • Author(s)
      Deqiang Yin, Xianghe Peng, Yi Qin, Zhongchang Wang
    • Journal Title

      Surface and Interface Analysis

      Volume: (In press)

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Microstructural Study of Forged Magnesium Pipes at Room Temperature2012

    • Author(s)
      Liwei Lu, Tianmo Liu, Ming-Jen Tan, Yong Chen, Zhongchang Wang
    • Journal Title

      Materials Science and Technology

      Volume: (In Press)

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Electrical Properties Optimization of Calcium Co-doping System : CeO_2-Sm_2O_32012

    • Author(s)
      Yanjie Xia, Xiaojuan Liu, Yijia Bai, Hongping Li, Xiaolong Deng, Xiaodong Niu, Xiaojie Wu, Defeng Zhou, Minfeng Lv, Zhongchang Wang, Jian Meng
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: (In Press)

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Structural and electronic impact of SrTiO3 substrate on T1O2 thin films2012

    • Author(s)
      ZC. Wang, R. Sun, CL Chen, M. Saito, S. Tsukimoto, Y. Ikuhara
    • Journal Title

      Journal of Materials Science

      Volume: 47(13) Issue: 13 Pages: 5148-5157

    • DOI

      10.1007/s10853-012-6392-4

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-Scale Ti_3SiC_2 Bilayers Embedded in SiC : Formation of Point Fermi Surface2011

    • Author(s)
      Zhongchang Wang, Susumu Tsukimoto, Rong Sun, Mitsuhiro Saito, Yuichi Ikuhara
    • Journal Title

      Applied Physics Letters

      Volume: 98 Pages: 104101-104101

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Gas-sensing Property Improvement of ZnO by Hierarchical Flower-like Architectures2011

    • Author(s)
      Weiwei Guo, Tianmo Liu, Wen Zeng, Dejun Liu, Yong Chen, Zhongchang Wang
    • Journal Title

      Materials Letters

      Volume: 65 Pages: 3384-3384

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Heterointerfaces : Atomic Structures, Electronic States, and Related Properties2011

    • Author(s)
      Zhongchang Wang, Mitsuhiro Saito, Susumu Tsukimoto, Yuichi Ikuhara
    • Journal Title

      Journal of the Ceramics Society of Japan

      Volume: 119 Pages: 783-783

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Quantifying Adhesion Energy of Mechanical Coatings at Atomistic Scale2011

    • Author(s)
      Deqiang Yin, Xianghe Peng, Yi Qin, Jiling Feng, Zhongchang Wang
    • Journal Title

      Applied Surface Science

      Volume: 258 Pages: 1451-1451

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atom-Resolved Imaging of Ordered Defect Superstructures at Individual Grain Boundaries2011

    • Author(s)
      Zhongchang Wang, Mitsuhiro Saito, Keith P. McKenna, Lin Gu, Susumu Tsukimoto, Alexander L. Shluger, Yuichi Ikuhara
    • Journal Title

      Nature

      Volume: 479 Pages: 380-380

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Strain Control of Orbital Polarization and Corrected Metal-Insulator Transition in La_2CoMnO_6 from First Principles2011

    • Author(s)
      Shuhui Lv, Hongping Li, Zhongchang Wang, Lin Han, Yao Liu, Xiaojuan Liu, Jian Meng
    • Journal Title

      Applied Physics Letters

      Volume: 99 Pages: 202110-202110

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atom-resolved imaging of ordered defect superstructures at individual grain boundaries2011

    • Author(s)
      Z.C.Wang, M.Saito, K.P.McKenna, L.Gu, S.Tsukimoto, A.L.Shluger, Y.Ikuhara
    • Journal Title

      NATURE

      Volume: 479 Issue: 7373 Pages: 380-383

    • DOI

      10.1038/nature10593

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Heterointerfaces: atomic structures, electronic states, and related properties2011

    • Author(s)
      Z.C.Wang, M.Saito, S.Tsukimoto, Y.Ikuhara
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 119 Issue: 1395 Pages: 783-793

    • DOI

      10.2109/jcersj2.119.783

    • NAID

      130001310502

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-scale Ti_3SiC_2 bilayers embedded in SiC : Formation of point Fermi surface2011

    • Author(s)
      Z.C.Wang, S.Tsukimoto, R.Sun, M.Saito, Y.Ikuhara
    • Journal Title

      Applied Physics Letters

      Volume: 98

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Microstructure and Gas-Sensing Property of Titania-Added ZnSnO_32010

    • Author(s)
      Wen Zeng, Tianmo Liu, Zhongchang Wang
    • Journal Title

      Materials Transactions

      Volume: 51 Pages: 1326-1326

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Electronic Property and Bonding Configuration at the TiN(111)/VN(111)Interface2010

    • Author(s)
      Deqiang Yin, Xianghe Peng, Yi Qin, Zhongchang Wang
    • Journal Title

      Journal of Applied Physics

      Volume: 108 Pages: 33714-33714

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Microstructure Evolution of Dual-Directional-Extruded Mg Alloy AZ31 : An Experimental and Simulation Study2010

    • Author(s)
      Liwei Lu, Tianmo Liu, Yong Chen, Liguang Wang, Zhongchang Wang
    • Journal Title

      Materials Transactions

      Volume: 51 Pages: 2088-2088

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dimensionality-Driven Insulator-Metal Transition in A-Site Excess Nonstoichiometric Perovskites2010

    • Author(s)
      Zhongchang Wang, Masaki Okude, Mitsuhiro Saito, Susumu Tsukimoto, Akira Ohtomo, Masaru Tsukada, Masashi Kawasaki, Yuichi Ikuhara
    • Journal Title

      Nature Communications

      Volume: 1 Pages: 106-106

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Sensitivity Improvement of TiO_2-doped SnO_2 to Volatile Organic Compounds2010

    • Author(s)
      Wen Zeng, Tianmo Liu, Zhongchang Wang
    • Journal Title

      Physica E

      Volume: 43 Pages: 633-633

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-Scale Structure and Electronic Property of the LaAlO_3/TiO_2 Interface2010

    • Author(s)
      Zhongchang Wang, Wen Zeng, Lin Gu, Mitsuhiro Saito, Susumu Tsukimoto, Yuichi Ikuhara
    • Journal Title

      Journal of Applied Physics

      Volume: 108 Pages: 113701-113701

    • Related Report
      2011 Final Research Report
    • Peer Reviewed
  • [Journal Article] Atomic-scale structure and electronic property of the LaAlO_3/TiO_2 interface2010

    • Author(s)
      Z.C.Wang, W.Zeng, L.Gu, M.Saito, S.Tsukimoto, Y.Ikuhara
    • Journal Title

      Journal of Applied Physics

      Volume: 108

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dimensionality-driven insulator-metal transition in A-site excess non-stoichiometric perovskites2010

    • Author(s)
      Z.C.Wang, M.Okude, M.Saito, S.Tsukimoto, A.Ohtomo, (他3名)
    • Journal Title

      Nature Communications

      Volume: 1

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Presentation] Atom-by-Atom Analysis of Functional Ceramics Interfaces and Grain Boundaries2012

    • Author(s)
      Z. C. Wang, M. Saito, S. Tsukimoto, Y. Ikuhara
    • Organizer
      The 3^<rd> International Symposium on Advanced Microscopy and Theoretical Calculations (AMTC3)
    • Place of Presentation
      Nagaragawa Convention Center, Gifu City, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Atomic-Scale Structure and Electronic Property of the SrTiO_3/TiO_2 Interface2012

    • Author(s)
      Z. C. Wang, M. Saito, R. Sun, C. L. Chen, S. Tsukimoto, Y. Ikuhara
    • Organizer
      International Symposium on Role of Electron Microscopy in Industry
    • Place of Presentation
      Nagoya University, Nagoya, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Atom-by-atom Analysis of Functional Ceramics Interfaces2011

    • Author(s)
      Z.C.Wang, M.Saito, S.Tsukimoto, Y.Ikuhara
    • Organizer
      The 21st Academic Symposium of Materials Research Society-Japan (MRS-J)
    • Place of Presentation
      Yokohama, Japan(招待講演)
    • Year and Date
      2011-12-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] Insulator-to-Metal Transition Induced by Insulating Layers in A-site Excess Nonstoichiometric Oxides2011

    • Author(s)
      Z.C.Wang, M.Okude, M.Saito, S.Tsukimoto, A.Ohtomo, M.Tsukada, M.Kawasaki, Y.Ikuhara
    • Organizer
      Materials Science and Technology (MS&T2011)
    • Place of Presentation
      Columbus, Ohio, USA
    • Year and Date
      2011-10-19
    • Related Report
      2011 Annual Research Report
  • [Presentation] Direct Imaging of Ordered Defect Superstructures at Grain Boundaries2011

    • Author(s)
      Z.C.Wang, M.Saito, K.McKenna, L.Gu, S.Tsukimoto, A.Shluger, Y.Ikuhara
    • Organizer
      Materials Science and Technology (MS&T2011)
    • Place of Presentation
      Columbus, Ohio, USA
    • Year and Date
      2011-10-17
    • Related Report
      2011 Annual Research Report
  • [Presentation] Atom-by-atom Analysis of of Functional Ceramics Interfaces2011

    • Author(s)
      Z.C.Wang, M.Saito, S.Tsukimoto, Y.Ikuhara
    • Organizer
      The 3rd International Conference on Heterogeneous Materials Mechanics (ICHMM 2011)
    • Place of Presentation
      Shanghai, China(招待講演)
    • Year and Date
      2011-05-24
    • Related Report
      2011 Annual Research Report
  • [Presentation] Atom-by-Atom Analysis of Functional Ceramics Interfaces2011

    • Author(s)
      Z. C. Wang, M. Saito, S. Tsukimoto, Y. Ikuhara
    • Organizer
      The 21^<st> Academic Symposium of MRS-J
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Insulating-Layer-Induced Insulator-to-Metal Transition in A-site Excess Nonstoichiometric Perovskites2011

    • Author(s)
      Z. C. Wang, M. Okude, M. Saito, S. Tsukimoto, A. Ohtomo, M. Tsukada, M. Kawasaki, Y. Ikuhara
    • Organizer
      15^<th> International Conference on Thin Films
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Insulator-to-Metal Transition Induced by Insulating Layers in A-site Excess Nonstoichiometric Oxides2011

    • Author(s)
      Z. C. Wang, M. Okude, M. Saito, S. Tsukimoto, A. Ohtomo, M. Tsukada, M. Kawasaki, Y. Ikuhara
    • Organizer
      Materials Science and Technology
    • Place of Presentation
      Columbus, Ohio, US
    • Related Report
      2011 Final Research Report
  • [Presentation] Direct Imaging of Ordered Defect Superstructures at Grain Boundaries2011

    • Author(s)
      Z. C. Wang, M. Saito, K. McKenna, L. Gu, S. Tsukimoto, A. Shluger, Y. Ikuhara
    • Organizer
      Materials Science and Technology
    • Place of Presentation
      Columbus, Ohio, US
    • Related Report
      2011 Final Research Report
  • [Presentation] Insulating-Layer-Induced Insulator-to-Metal Transition in Ruddlesden-Popper Series2011

    • Author(s)
      Z. C. Wang, M. Saito, S. Tsukimoto, T. Mizoguchi, M. Okude, A. Ohtomo, T. Kita, M. Tsukada, M. Kawasaki, Y. Ikuhara
    • Organizer
      International Workshop on Advanced Electron Microscopy and Applications in Materials Science
    • Place of Presentation
      Shenyang, China
    • Related Report
      2011 Final Research Report
  • [Presentation] Atom-by-atom Analysis of Functional Ceramics Interfaces2011

    • Author(s)
      Z. C. Wang, M. Saito, S. Tsukimoto, Y. Ikuhara
    • Organizer
      The 3^<rd> International Conference on Heterogeneous Materials Mechanics (ICHMM 2011)
    • Place of Presentation
      Chongming island, Shanghai, China
    • Related Report
      2011 Final Research Report
  • [Presentation] Insulator-to-metal transition driven by an insulating layer in Ruddlesden-Popper series2010

    • Author(s)
      Z.C.Wang, M.Okude, M.Saito, S.Tsukimoto, A.Ohtomo, (他3名)
    • Organizer
      The 20th Academic Symposium of MRS-J
    • Place of Presentation
      Yokohama, Japan
    • Year and Date
      2010-12-21
    • Related Report
      2010 Annual Research Report
  • [Presentation] Quantum electron transport through function interfaces2010

    • Author(s)
      Z.C.Wang, S.Tsukimoto, M.Saito, Y.Ikuhara
    • Organizer
      The 2nd International Symposium on Advanced Microscopy and Theoretical Calculations (AMTC2)
    • Place of Presentation
      Nagoya Congress Center, Nagoya
    • Year and Date
      2010-06-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] Insulator-to-Metal Transition Driven by an Insulating Layer in Ruddlesden-Popper Series2010

    • Author(s)
      Z. C. Wang, M. Okude, M. Saito, S. Tsukimoto, A. Ohtomo, M. Tsukada, M. Kawasaki, Y. Ikuhara
    • Organizer
      The 20^<th> Academic Symposium of MRS-J
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Introducing Ohmic Contacts into SiC Technology2010

    • Author(s)
      Z. C. Wang, S. Tsukimoto, M. Saito, Y. Ikuhara
    • Organizer
      The 6^<th> International Conference on Physical and Numerical Simulation of Materials Processing (ICPNS 2010)
    • Place of Presentation
      Cuilin, Guxi Province, China
    • Related Report
      2011 Final Research Report
  • [Presentation] Atomic-Scale Structure and Electron Transport of SiC/Ti_3SiC_2 Interface2010

    • Author(s)
      Z. C. Wang, S. Tsukimoto, M. Saito, Y. Ikuhara
    • Organizer
      The 13^<th> International Conference on Intergranular and Interphase Boundaries in Materials (iib2010)
    • Place of Presentation
      Shima, Mie, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Quantum Electron Transport through Functional Interfaces2010

    • Author(s)
      Z. C. Wang, S. Tsukimoto, M. Saito, Y. Ikuhara
    • Organizer
      The 2^<nd> International Symposium on Advanced Microscopy and Theoretical Calculations (AMTC2)
    • Place of Presentation
      Nagoya, Japan
    • Related Report
      2011 Final Research Report
  • [Presentation] Interface Atomic-Scale Structure and its Impact on Quantum Electron Transport2010

    • Author(s)
      Z. C. Wang
    • Organizer
      The Third International Conference on Modeling and Simulation (ICMS2010)
    • Place of Presentation
      WuXi, JiangSu, China
    • Related Report
      2011 Final Research Report
  • [Book] Silicon Carbide. Materials, Processing and Applications in Electronic Device2011

    • Author(s)
      Z. C. Wang
    • Publisher
      INTECH open
    • Related Report
      2011 Final Research Report

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Published: 2010-08-23   Modified: 2016-04-21  

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