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Simultaneous investigation of superconducting order parameter and charge excitations in cuprate superconductors via resonant inelastic x-ray scattering

Research Project

Project/Area Number 22K13994
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionTohoku University

Principal Investigator

Suzuki Hakuto  東北大学, 学際科学フロンティア研究所, 助教 (80922947)

Project Period (FY) 2022-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2023: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2022: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Keywords高温超伝導 / プラズモン / 長距離クーロン相互作用 / 共鳴非弾性X線散乱 / 銅酸化物 / 電荷励起 / 音響プラズモン / 電荷秩序 / 銅酸化物高温超伝導 / 超伝導秩序パラメータ
Outline of Research at the Start

銅酸化物における高温超伝導の発見以降、その超伝導発現機構解明のため膨大な研究がなされてきた。超伝導相は反強磁性モット絶縁体相に近接することから、磁気揺らぎ媒介の超伝導機構が最有力候補の一つである。一方近年の共鳴X線散乱の実験から、CuO2面内における電荷密度に周期性が現れること、また3次元的な分散関係を持つ電荷の集団励起モードが存在することが明らかとなった。本研究では高分解能共鳴非弾性X線散乱により超伝導秩序と電荷秩序・集団励起を統一的に観測し、電荷揺らぎの高温超伝導への役割を解明する。

Outline of Final Research Achievements

Superconductivity is a phenomenon where the electrical resistance of a metal becomes zero at low temperatures. Since the discovery of high-temperature superconductivity in cuprates, superconductivity has been found in various transition metal compounds. Superconductivity in cuprates cannot be explained by the conventional mechanism that involve lattice vibrations as a pairing glue but is considered to involve unconventional mechanisms mediated by the oscillations of electronic charge density or magnetic moments. This study aims to elucidate the behavior of charge oscillation modes using resonant inelastic x-ray scattering. It was found that the charge oscillation modes in the group of cuprates exhibiting the highest transition temperatures can only be explained by considering long-range Coulomb interactions between electrons in different CuO2 sheets.

Academic Significance and Societal Importance of the Research Achievements

本研究の結果、銅酸化物において電荷密度の集団的な振動が普遍的に存在し、かつその振る舞いが超伝導の発現するCuO2層の数に強く依存することが明らかとなった。この結果は3枚のCuO2層を含む銅酸化物において超伝導転移温度が最高になる理由を解明する可能性がある。また、鉄系やニッケル酸化物における非従来型超伝導一般においても同様の電荷の振動モードの存在が期待され、広く非従来型超伝導機構における電荷自由度の重要性を示唆するものである。
本研究で確立した散乱角度を連続的に変化させる共鳴非弾性X線散乱手法は、NanoTerasuにおける超高分解能RIXS測定において幅広い量子物質に対して適用可能である。

Report

(3 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • Research Products

    (33 results)

All 2024 2023 2022 Other

All Int'l Joint Research (12 results) Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (18 results) (of which Int'l Joint Research: 6 results,  Invited: 9 results) Funded Workshop (1 results)

  • [Int'l Joint Research] Max Planck Institute/DESY/Friedrich-Alexander-University(ドイツ)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] NSRRC(その他の国・地域)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Universite Paris-Saclay/College de France(フランス)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Flatiron Institute(米国)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Orebro University(スウェーデン)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research]

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Max Planck Institute/DESY/University of Nurnberg-Erlangen(ドイツ)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] Flatiron Insitutute/Columbia University(米国)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] Orebro University(スウェーデン)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] Ecole polytechnique/College de France(フランス)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] University of Geneva(スイス)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research]

    • Related Report
      2022 Research-status Report
  • [Journal Article] Distinct spin and orbital dynamics in Sr2RuO42023

    • Author(s)
      H. Suzuki, L. Wang, J. Bertinshaw, H. U. R. Strand, S. Kaser, M. Krautloher, Z. Yang, N. Wentzell, O. Parcollet, F. Jerzembeck, N. Kikugawa, A. P. Mackenzie, A. Georges, P. Hansmann, H. Gretarsson, B. Keimer
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 563-567

    • DOI

      10.1038/s41467-023-42804-3

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Magnetic Properties and Electronic Configurations of Mn Ions in the Diluted Magnetic Semiconductor Ba<sub>1-</sub><i><sub>x</sub></i>K<i><sub>x</sub></i>(Zn<sub>1-</sub><i><sub>y</sub></i>Mn<i><sub>y</sub></i>)<sub>2</sub>As<sub>2</sub> Studied by X-ray Magnetic Circular Dichroism and Resonant Inelastic X-ray Scattering2022

    • Author(s)
      Suzuki Hakuto、Zhao Guoqiang、Okamoto Jun、Sakamoto Shoya、Chen Zhi-Yin、Nonaka Yosuke、Shibata Goro、Zhao Kan、Chen Bijuan、Wu Wen-Bin、Chang Fan-Hsiu、Lin Hong-Ji、Chen Chien-Te、Tanaka Arata、Kobayashi Masaki、Gu Bo、Maekawa Sadamichi、Uemura Yasutomo J.、Jin Changqing、Huang Di-Jing、Fujimori Atsushi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 91 Issue: 6 Pages: 1-5

    • DOI

      10.7566/jpsj.91.064710

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Sr2RuO4におけるエネルギー的に分離したスピン・軌道励起の共鳴非弾性X線散乱による観測2024

    • Author(s)
      鈴木博人,L. Wang,J. Bertinshaw,H. U. R. Strand,S. Kaeser,M. Krautloher,Z. Yang,N. Wentzell,O. Parcolle,F. Jerzembeck,菊川直樹,A. P. Mackenzie,A. Georges,P. Hansmann,H. Gretarsson,B. Keimer
    • Organizer
      日本物理学会 2024年春季大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 酸素K端共鳴非弾性X線散乱による銅酸化物高温超伝導体Bi2223の電荷秩序・電荷励起の観測2024

    • Author(s)
      中田勝,岡本淳,志賀大亮,高橋龍之介,H. Y. Huang,A. Singh,組頭広志,和達大樹,石田茂之,永崎洋,藤森淳,D. J. Huang,鈴木博人
    • Organizer
      第37回日本放射光学会年会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 酸素K端共鳴非弾性X線散乱による銅酸化物高温超伝導体Bi2223の電荷秩序の観測2023

    • Author(s)
      中田勝,岡本淳,志賀大亮,高橋龍之介,H. Y. Huang,A. Singh,組頭広志,和達大樹,石田茂之,永崎洋,藤森淳,D. J. Huang,鈴木博人
    • Organizer
      日本物理学会第78回年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 酸素K吸収端共鳴非弾性 X 線散乱による三層系銅酸化物Bi2223のプラズモン分散の観測2023

    • Author(s)
      中田勝,岡本淳,志賀大亮,高橋龍之介,H. Y. Huang,A. Singh,組頭広志,和達大樹,石田茂之,永崎洋,藤森淳,D. J. Huang,鈴木博人
    • Organizer
      日本物理学会第78回年次大会
    • Related Report
      2023 Annual Research Report
  • [Presentation] 共鳴非弾性X線散乱によるBi系銅酸化物の電荷励起2023

    • Author(s)
      鈴木博人
    • Organizer
      高温超伝導フォーラム
    • Related Report
      2023 Annual Research Report
  • [Presentation] Distinct spin and orbital dynamics in Sr2RuO42023

    • Author(s)
      Hakuto Suzuki
    • Organizer
      RIXS/REXS workshop 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Exotic magnetism in honeycomb ruthenium compounds: Insights from IRIXS2023

    • Author(s)
      Hakuto Suzuki
    • Organizer
      International Conference on Strongly Correlated Electron Systems 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Exotic magnetism in honeycomb ruthenium compounds: Insights from IRIXS2023

    • Author(s)
      Hakuto Suzuki
    • Organizer
      NSRRC seminar
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 共鳴非弾性 X 線散乱による強相関物質の素励起の研究2023

    • Author(s)
      鈴木博人
    • Organizer
      日本物理学会 2023年春季大会
    • Related Report
      2022 Research-status Report
    • Invited
  • [Presentation] Distinct spin and orbital dynamics in Sr2RuO42023

    • Author(s)
      鈴木博人
    • Organizer
      令和4年度 TI-FRIS/FRIS シンポジウム
    • Related Report
      2022 Research-status Report
  • [Presentation] 共鳴非弾性X線散乱で見る量子物質の素励起2023

    • Author(s)
      鈴木博人
    • Organizer
      令和4年度 後期第5回 全領域合同研究交流会
    • Related Report
      2022 Research-status Report
  • [Presentation] Spin and orbital fluctuations in Sr2RuO4 revealed by resonant inelastic x-ray scattering2022

    • Author(s)
      Hakuto Suzuki
    • Organizer
      Integrated Spectroscopy for Strong Electron Correlation -Theory, Computation and Experiment
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research
  • [Presentation] Collective excitations from exotic quantum states in correlated materials2022

    • Author(s)
      Hakuto Suzuki
    • Organizer
      The 6th QST International Symposium: Innovation in Science and Technology from “NanoTerasu”
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 外場下・空間分解 RIXS による量子物質の相競合の解明2022

    • Author(s)
      鈴木博人, 宮脇淳
    • Organizer
      量研-東北大マッチング研究支援事業 2022年度キックオフ・ワークショップ
    • Related Report
      2022 Research-status Report
    • Invited
  • [Presentation] 共鳴非弾性X線散乱による酸化物研究の新展開2022

    • Author(s)
      鈴木博人
    • Organizer
      第83回 応用物理学会秋季学術講演会 先端計測と機能性酸化物研究の共進化
    • Related Report
      2022 Research-status Report
    • Invited
  • [Presentation] Ru L3端共鳴非弾性X線散乱によるRuX3 (X = Br, I)の多重項の観測2022

    • Author(s)
      藤原秀行, 佐藤楓貴, H.Gretarsson, B. Keimer, 今井良宗, 大串研也, 鈴木博人
    • Organizer
      日本物理学会 2022年秋季大会
    • Related Report
      2022 Research-status Report
  • [Presentation] 共鳴非弾性X線散乱で見る量子物質の素励起2022

    • Author(s)
      鈴木博人
    • Organizer
      令和4年度前期第2回 全領域合同研究交流会
    • Related Report
      2022 Research-status Report
    • Invited
  • [Presentation] Exotic magnetism in honeycomb ruthenium compounds: Insights from IRIXS2022

    • Author(s)
      Hakuto Suzuki
    • Organizer
      DESY Photon Science Seminar
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Funded Workshop] RIXS/REXS workshop 20232023

    • Related Report
      2023 Annual Research Report

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Published: 2022-04-19   Modified: 2025-01-30  

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