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Demonstration of valley spin devices by coupling 2D semiconductors to chiral photonic crystal nanocavities

Research Project

Project/Area Number 22K14623
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 30020:Optical engineering and photon science-related
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

Fong CheeFai  国立研究開発法人理化学研究所, 開拓研究本部, 基礎科学特別研究員 (30881544)

Project Period (FY) 2022-04-01 – 2025-03-31
Project Status Granted (Fiscal Year 2023)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2023: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2022: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywords2D materials device / Photonic crystal / Optics and photonics / photonic crystal / optics and photonics / Valley spin devices / semiconductor / layered material
Outline of Research at the Start

In 2D semiconductors, the electron and holes possess coupled valley and spin properties which are referred to as valley spin. We propose the demonstration of valley spin devices by coupling 2D semiconductors to novel circularly polarized chiral photonic crystal nanocavities.

Outline of Annual Research Achievements

Using the photonic crystal (PhC) and 2D materials transfer technologies that we have developed previously, in this fiscal year, we have been focused on studying the self-aligned hybrid nanocavities. These hybrid nanocavities are formed by partially covering a photonic crystal waveguide post-fabrication with a suitably-sized 2D material flake. The presence of the flake increases the local refractive index causing a frequency mismatch of the optical fields in the regions with and without the flake results in the formation of a nanocavity. We successfully fabricated such hybrid nanocavity devices with hBN, WSe2 and MoTe2 flakes on silicon PhC waveguides.

Current Status of Research Progress
Current Status of Research Progress

1: Research has progressed more than it was originally planned.

Reason

In our hybrid nanocavity devices, we have obtained Q factors as high as 4.0×10^5. Remarkably, even monolayer flakes can provide sufficient local refractive index modulation to induce high Q nanocavity formation. We have also managed to observe cavity PL enhancement in a self-aligned MoTe2 cavity device, with a cavity Purcell enhancement factor of about 15. Our results highlight the potential of our devices to enhance light-matter coupling and to create functional optical devices.

Strategy for Future Research Activity

So far, we have fabricated hybrid nanocavities using a single flake per device. One of the key features of 2D materials is their amenability to heterogenous stacking i.e. stacking of 2D materials with different compositions and atomic lattices without having to worry about lattice matching. Such heterogeneous stacking has been used as encapsulation or passivation layer to sandwich and protect the 2D materials. Following from our results, our next step will be focused on coupling heterogenous stack of materials to the self-aligned hybrid nanocavities.

Report

(2 results)
  • 2023 Research-status Report
  • 2022 Research-status Report
  • Research Products

    (5 results)

All 2024 2023 2022

All Journal Article (1 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 1 results,  Open Access: 1 results) Presentation (4 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] Resonant exciton transfer in mixed-dimensional heterostructures for overcoming dimensional restrictions in optical processes2023

    • Author(s)
      Fang N.、Chang Y. R.、Yamashita D.、Fujii S.、Maruyama M.、Gao Y.、Fong C. F.、Otsuka K.、Nagashio K.、Okada S.、Kato Y. K.
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 8152-8159

    • DOI

      10.1038/s41467-023-43928-2

    • Related Report
      2023 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Emerging second-order nonlinearity in two-dimensional material functionalized silica microcavities2024

    • Author(s)
      Shun Fujii
    • Organizer
      March Meeting of the American Physical Society
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research
  • [Presentation] Intrinsically Circularly Polarized Modes Near Exceptional Points due to Symmetry Breaking in a H1 Photonic Crystal Cavity2023

    • Author(s)
      Chee Fai Fong
    • Organizer
      International Conference on Nano-photonics and Nano-electronics (ICNN2023)
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research
  • [Presentation] Nanocavity induced by atomically thin transition metal dichalcogenide in photonic crystal waveguide2023

    • Author(s)
      Chee Fai Fong
    • Organizer
      JSAP-Optica Joint Symposia, the 84th JSAP Autumn Meeting 2023
    • Related Report
      2023 Research-status Report
    • Int'l Joint Research
  • [Presentation] Formation of heterocavity by deposition of hexagonal boron nitride flake on photonic crystal waveguide2022

    • Author(s)
      C.F. Fong, D. Yamashita, N. Fang, T. Taniguchi, K. Watanabe and Y. K. Kato
    • Organizer
      JSAP-Optica Joint Symposia 2022
    • Related Report
      2022 Research-status Report

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Published: 2022-04-19   Modified: 2024-12-25  

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