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Emergent nonlinear optical effects in two-dimensional materials using ultrahigh-Q optical microcavities

Research Project

Project/Area Number 22K14625
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 30020:Optical engineering and photon science-related
Research InstitutionKeio University

Principal Investigator

Fujii Shun  慶應義塾大学, 理工学部(矢上), 助教 (80897950)

Project Period (FY) 2022-04-01 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2023: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2022: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywords微小光共振器 / 二次元材料 / 非線形光学効果 / 第二高調波発生 / 非線形波長変換 / 非線形光学変換 / 高Q値微小光共振器
Outline of Research at the Start

超高Q値微小光共振器と二次元材料の融合によるナノスケール非線形フォトニクスの開拓を目指す.高い光の閉じ込め性能(高Q値)を有するマイクロ共振器とよばれる微小デバイスを用いることで,非常に弱い光励起でも様々なの非線形光学効果を発現できることが知られている.この素子を原子数層程度の厚みしか持たない二次元材料と組み合わせることで,従来観測されてこなかった非線形光学物性を発現させることを狙う.超高Q値微小光共振器の非線形フォトニクスを,ナノ材料の光学特性評価,顕微分光技術と組み合わせることで,二次元材料の新たなナノフォトニクスの開拓への足がかりとする.

Outline of Final Research Achievements

High-efficiency second-order nonlinear optical processes have been demonstrated by using a hybrid device, where an atomically-thin two-dimensional material is integrated into a high-Q silica optical microcavity. By performing the layer-dependence and excitation power dependence measurements, it is confirmed that the strong nonlinearity was enhanced by a microcavity via strong light-matter interaction at the surface. Although silica does not inherently show second-order nonlinearities, this approach provides a method to drastically alter the nonlinear properties of high-Q optical microcavities by functionalizing with semiconductor two-dimensional materials without significant losses.

Academic Significance and Societal Importance of the Research Achievements

高Q値微小光共振器の非線形光学特性を,原子層二次元材料の転写というプロセスで自由に制御できる可能性を示した.特に,連続光レーザー励起で高効率な非線形光学効果の観測に成功したことは,微小光共振器と二次元材料の親和性の高さを証明する重要な結果である.また,本手法を適用することで将来的なナノフォトニクスデバイスの設計の自由度を飛躍的に高めることが期待される.

Report

(3 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • Research Products

    (16 results)

All 2024 2023 2022

All Journal Article (8 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 8 results,  Open Access: 7 results) Presentation (8 results) (of which Int'l Joint Research: 5 results,  Invited: 1 results)

  • [Journal Article] Synchronization of two chaotic microresonator frequency combs2024

    • Author(s)
      Moreno David、Fujii Shun、Nakashima Ayata、Lemcke Deniz、Uchida Atsushi、Sanchis Pablo、Tanabe Takasumi
    • Journal Title

      Optics Express

      Volume: 32 Issue: 2 Pages: 2460-2460

    • DOI

      10.1364/oe.511097

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] van der Waals Decoration of Ultra-High-Q Silica Microcavities for χ(2)–χ(3) Hybrid Nonlinear Photonics2024

    • Author(s)
      Fujii Shun、Fang Nan、Yamashita Daiki、Kozawa Daichi、Fong Chee Fai、Kato Yuichiro K.
    • Journal Title

      Nano Letters

      Volume: 24 Issue: 14 Pages: 4209-4216

    • DOI

      10.1021/acs.nanolett.4c00273

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Room-temperature quantum emission from interface excitons in mixed-dimensional heterostructures2024

    • Author(s)
      Fang N.、Chang Y. R.、Fujii S.、Yamashita D.、Maruyama M.、Gao Y.、Fong C. F.、Kozawa D.、Otsuka K.、Nagashio K.、Okada S.、Kato Y. K.
    • Journal Title

      Nature Communications

      Volume: 15 Issue: 1 Pages: 2871-2871

    • DOI

      10.1038/s41467-024-47099-6

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Mechanically Actuated Kerr Soliton Microcombs2024

    • Author(s)
      Fujii Shun、Wada Koshiro、Kogure Soma、Kumazaki Hajime、Tanabe Takasumi
    • Journal Title

      Laser & Photonics Reviews

      Volume: - Issue: 9 Pages: 2301329-2301329

    • DOI

      10.1002/lpor.202301329

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Stability and mutual coherence of Raman combs in high-Q silica microresonators2023

    • Author(s)
      Sugawara Shuto、Fujii Shun、Kawanishi Satoki、Tanabe Takasumi
    • Journal Title

      Optics Continuum

      Volume: 2 Issue: 7 Pages: 1588-1588

    • DOI

      10.1364/optcon.493749

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Resonant exciton transfer in mixed-dimensional heterostructures for overcoming dimensional restrictions in optical processes2023

    • Author(s)
      Fang N.、Chang Y. R.、Yamashita D.、Fujii S.、Maruyama M.、Gao Y.、Fong C. F.、Otsuka K.、Nagashio K.、Okada S.、Kato Y. K.
    • Journal Title

      Nature Communications

      Volume: 14 Issue: 1 Pages: 8152-8159

    • DOI

      10.1038/s41467-023-43928-2

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Versatile tuning of Kerr soliton microcombs in crystalline microresonators2023

    • Author(s)
      Fujii Shun、Wada Koshiro、Sugano Ryo、Kumazaki Hajime、Kogure Soma、Kato Yuichiro K.、Tanabe Takasumi
    • Journal Title

      Communications Physics

      Volume: 6 Issue: 1 Pages: 1-1

    • DOI

      10.1038/s42005-022-01118-4

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] <i>ortho</i>-Substituted Aryldiazonium Design for the Defect Configuration-Controlled Photoluminescent Functionalization of Chiral Single-Walled Carbon Nanotubes2022

    • Author(s)
      Yu Boda、Naka Sadahito、Aoki Haruka、Kato Koichiro、Yamashita Daiki、Fujii Shun、Kato Yuichiro K.、Fujigaya Tsuyohiko、Shiraki Tomohiro
    • Journal Title

      ACS Nano

      Volume: 16 Issue: 12 Pages: 21452-21461

    • DOI

      10.1021/acsnano.2c09897

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Presentation] Emerging second-order nonlinearity in two-dimensional material functionalized silica microcavities2024

    • Author(s)
      Shun Fujii, Nan Fang, Daiki Yamashita, Daichi Kozawa, Chee Fai Fong, and Yuichiro K. Kato
    • Organizer
      APS March Meeting
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nonlinear optics and soliton frequency combs in ultrahigh-Q microresonators2024

    • Author(s)
      Shun Fujii
    • Organizer
      The International Conference on Nano-photonics and Nano-optoelectronics 2024
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Second-order Nonlinear Optics in Ultrahigh-Q Silica Microcavities Decorated by Two-Dimensional Materials2024

    • Author(s)
      Shun Fujii, Nan Fang, Daiki Yamashita, Daichi Kozawa, Chee Fai Fong, and Yuichiro K. Kato
    • Organizer
      CLEO Pacific Rim 2024
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Mechanical Actuation of Kerr Soliton Microcombs in Ultrahigh-Q Crystalline Microresonators2024

    • Author(s)
      S. Fujii, K. Wada, S. Kogure, H. Kumazaki, and T. Tanabe
    • Organizer
      CLEO Pacific Rim 2024
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 超高Q値微小光共振器を用いた機械駆動型ソリトンマイクロコム2023

    • Author(s)
      藤井 瞬、和田幸四郎、木暮蒼真、田邉 孝純
    • Organizer
      第84回秋季応用物理学会学術講演会
    • Related Report
      2023 Annual Research Report
  • [Presentation] Extending Spectral Tunability of Soliton Microcombs in Ultrahigh-Q Microresonators2023

    • Author(s)
      S. Fujii, K. Wada, H. Kumazaki, S. Kogure, and T. Tanabe
    • Organizer
      PhotonIcs and Electromagnetics Research Symposium
    • Related Report
      2023 Annual Research Report
  • [Presentation] ソリトンマイクロコムの広範囲精密チューニング2023

    • Author(s)
      藤井瞬,和田幸四郎,菅野凌,熊崎基,木暮蒼真,加藤雄一郎,田邉孝純
    • Organizer
      第70回応用物理学春季学術講演会
    • Related Report
      2022 Research-status Report
  • [Presentation] Nonlinear frequency conversion in two-dimensional material integrated high-Q silica optical microresonators2022

    • Author(s)
      S. Fujii, N. Fang, D. Yamashita, and Y. K. Kato
    • Organizer
      The 10th RAP Symposium - The New Optical Science in Post-Corona Era
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research

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Published: 2022-04-19   Modified: 2025-01-30  

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