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Stress-responsive underwater adhesion using particle-stabilized bubble

Research Project

Project/Area Number 22K18891
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 26:Materials engineering and related fields
Research InstitutionOsaka Institute of Technology

Principal Investigator

Fujii Syuji  大阪工業大学, 工学部, 教授 (70434785)

Co-Investigator(Kenkyū-buntansha) 石田 尚之  岡山大学, 自然科学学域, 准教授 (80344133)
Project Period (FY) 2022-06-30 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥6,500,000 (Direct Cost: ¥5,000,000、Indirect Cost: ¥1,500,000)
Fiscal Year 2023: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2022: ¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Keywords泡 / 接着 / 高分子粒子 / 界面 / 刺激応答
Outline of Research at the Start

粒子が表面を覆うことで安定化した泡(内部に空気を含有するカプセル)を刺激応答性接着剤として捉え、応力印加によるカプセル崩壊・空気漏出が誘起する空気による基材の架橋に基づく水中接着技術を実現する。具体的には、まず「ぬれの化学」に基づき、基材の表面化学(親水性・疎水性バランス)と泡の基材への吸着性・ぬれ性の相関関係を解明する。さらに、接着部位の構造評価、および接着力の実測値とラプラス圧から算出される理論値の比較を行い、接着性発現メカニズムの解明に取り組む。無尽蔵の材料である空気を「水中接着剤」として捉え、新たな接着科学の開拓に挑戦する点で大きな意義がある。

Outline of Final Research Achievements

Based on the "wetting chemistry" the research was conducted to elucidate the correlation between the surface chemistry of the substrate (hydrophilic/hydrophobic balance) and the adsorption of the air bubble to the substrate. We also utilized particle-stabilized bubble as a stress-responsive adhesive and tried to realize a stimulus-responsive underwater adhesion technology. As a result, the following points were clarified. (1) The adsorption of the bubble improved as the hydrophobicity of the adherend increased. (2) The adherends were successfully bonded by the collapse of the particle-stabilized bubble and leakage of air. (3) The mechanism for adhesion phenomena using particle-stabilized aqueous bubble was clarified.

Academic Significance and Societal Importance of the Research Achievements

本研究では、基板の表面化学と泡の吸着性・形状の相関関係を解明し、目的箇所における任意タイミングでの接着を可能にする新規水中接着技術の開拓を目的とした。空気を「水中接着剤」として捉え、新たな接着科学を開拓した点で大きな意義がある。本研究課題で研究した接着技術は、空気を接着剤として使用するため環境適応型・簡便であり、表面に凹凸がある基材に対しても、空気がぬれ広がることで接着が可能になると期待でき、接着可能な基材の対象が広い。空気泡を用いた接着現象の理解が進むことは、様々な科学技術・日常生活の問題への解決に貢献し、各学術分野に変革をもたらす可能性を含んでいる。

Report

(3 results)
  • 2023 Annual Research Report   Final Research Report ( PDF )
  • 2022 Research-status Report
  • Research Products

    (37 results)

All 2024 2023 2022 Other

All Int'l Joint Research (9 results) Journal Article (11 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 11 results,  Open Access: 2 results) Presentation (12 results) (of which Int'l Joint Research: 8 results,  Invited: 10 results) Book (2 results) Remarks (3 results)

  • [Int'l Joint Research] Friedrich-Alexander-Universitat/Max Planck Institute(ドイツ)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Ariel University(イスラエル)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] University of Newcastle(オーストラリア)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Chulalongkorn University/Rajamangala Univ. Tech. Thanyaburi(タイ)

    • Related Report
      2023 Annual Research Report
  • [Int'l Joint Research] Friedrich-Alexander-Universitat/Max Planck Institute(ドイツ)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] Ariel University(イスラエル)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] University of Hull/University of Sheffield(英国)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] University of Newcastle(オーストラリア)

    • Related Report
      2022 Research-status Report
  • [Int'l Joint Research] Chulalongkorn University/Rajamangala University of Technology(タイ)

    • Related Report
      2022 Research-status Report
  • [Journal Article] Shape design of aqueous bubbles stabilized with millimeter-sized polymer plates2024

    • Author(s)
      Sakurai Yuri、Kakiuchi Rina、Hayashi Masaki、Hirai Tomoyasu、Nakamura Yoshinobu、Fujii Syuji
    • Journal Title

      New Journal of Chemistry

      Volume: 48 Issue: 1 Pages: 31-35

    • DOI

      10.1039/d3nj04411d

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Aqueous Bubbles Stabilized with Millimeter-Sized Polymer Plates2023

    • Author(s)
      Sakurai Yuri、Kakiuchi Rina、Hirai Tomoyasu、Nakamura Yoshinobu、Fujii Syuji
    • Journal Title

      Langmuir

      Volume: 39 Issue: 10 Pages: 3800-3809

    • DOI

      10.1021/acs.langmuir.3c00149

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electroless nickel plating on a biomineral-based sponge structure2022

    • Author(s)
      Takeoka Hiroaki、Seike Musashi、Nakamura Yoshinobu、Imai Hiroaki、Oaki Yuya、Fujii Syuji
    • Journal Title

      Materials Advances

      Volume: 3 Issue: 2 Pages: 931-936

    • DOI

      10.1039/d1ma00909e

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Driving Droplets on Liquid Repellent Surfaces via Light‐Driven Marangoni Propulsion2022

    • Author(s)
      Hwang Hyesun、Papadopoulos Periklis、Fujii Syuji、Wooh Sanghyuk
    • Journal Title

      Advanced Functional Materials

      Volume: 32 Issue: 15 Pages: 2111311-2111311

    • DOI

      10.1002/adfm.202111311

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Synthesis of Polypyrrole and Its Derivatives as a Liquid Marble Stabilizer via a Solvent-Free Chemical Oxidative Polymerization Protocol2022

    • Author(s)
      Seike Musashi、Uda Makoto、Suzuki Toyoko、Minami Hideto、Higashimoto Shinya、Hirai Tomoyasu、Nakamura Yoshinobu、Fujii Syuji
    • Journal Title

      ACS Omega

      Volume: 7 Issue: 15 Pages: 13010-13021

    • DOI

      10.1021/acsomega.2c00327

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Alcohol as Hydrophobizer for Polypyrrole2022

    • Author(s)
      Seike Musashi、Hirai Tomoyasu、Nakamura Yoshinobu、Fujii Syuji
    • Journal Title

      Chemistry Letters

      Volume: 51 Issue: 6 Pages: 598-600

    • DOI

      10.1246/cl.220109

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] “Foam Marble” Stabilized with One Type of Polymer Particle2022

    • Author(s)
      Aono Kodai、Ueno Kazuyuki、Hamasaki Sho、Sakurai Yuri、Yusa Shin-ichi、Nakamura Yoshinobu、Fujii Syuji
    • Journal Title

      Langmuir

      Volume: 38 Issue: 24 Pages: 7603-7610

    • DOI

      10.1021/acs.langmuir.2c00869

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] Photo/Thermo Dual Stimulus-Responsive Liquid Marbles Stabilized with Polypyrrole-Coated Stearic Acid Particles2022

    • Author(s)
      Tsumura Yusuke、Oyama Keigo、Fameau Anne-Laure、Seike Musashi、Ohtaka Atsushi、Hirai Tomoyasu、Nakamura Yoshinobu、Fujii Syuji
    • Journal Title

      ACS Applied Materials & Interfaces

      Volume: 14 Issue: 36 Pages: 41618-41628

    • DOI

      10.1021/acsami.2c12681

    • Related Report
      2022 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Liquid Marble as an Amphibious Carrier for the Controlled Delivery and Release of Substances2022

    • Author(s)
      Fujii Syuji
    • Journal Title

      Langmuir

      Volume: 38 Issue: 42 Pages: 12757-12763

    • DOI

      10.1021/acs.langmuir.2c02305

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] 界面吸着粒子による液液・気液分散体の安定化2022

    • Author(s)
      藤井秀司
    • Journal Title

      化学と工業

      Volume: 75-2 Pages: 102-102

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Journal Article] シランカップリング剤の反応性に関する研究動向2022

    • Author(s)
      中村吉伸,上辻靖智,平井智康,藤井秀司
    • Journal Title

      日本接着学会誌

      Volume: 58 Pages: 313-321

    • Related Report
      2022 Research-status Report
    • Peer Reviewed
  • [Presentation] 界面吸着粒子が拓く材料化学2024

    • Author(s)
      藤井秀司
    • Organizer
      応用化学セミナー2024~ 複合・融合が生み出す新技術~
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Liquid marbles and dry liquids2024

    • Author(s)
      Syuji FUJII
    • Organizer
      Research seminar at Fraunhofer-Institute Keramische Technologien und Systeme IKTS
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Biomimetic materials based on particles adsorbed at air-water interface2023

    • Author(s)
      Syuji FUJII
    • Organizer
      10th Nagoya Biomimetics International Symposium
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Polyhedral liquid marbles2023

    • Author(s)
      Syuji FUJII
    • Organizer
      Armesfest700
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Liquid marble engineering: From nature to materials2023

    • Author(s)
      Syuji FUJII
    • Organizer
      19th Asian Chemical Congress
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Fabrication of liquid marbles using biodegradable chitosan-stearic acid conjugated particles2023

    • Author(s)
      Apirak Kunanopparatn, Masaki Hayashi, Yamato Iwata, Kenshin-Yamamoto, Tomoyasu Hirai, Yoshinobu Nakamura, Apichat Imyim, Fuangfa Unob, Syuji Fujii
    • Organizer
      PCC & PETROMAT Symposium 2023
    • Related Report
      2023 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Liquid marble engineering: From nature to materials2023

    • Author(s)
      Syuji FUJII
    • Organizer
      Research seminar at Department of Chemistry, The Chinese University of Hong Kong
    • Related Report
      2023 Annual Research Report
    • Invited
  • [Presentation] Liquid marbles stabilized with polymer particles2023

    • Author(s)
      Syuji FUJII
    • Organizer
      Research seminar at Chung-Ang University
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Liquid marbles stabilized with polymer particles2023

    • Author(s)
      Syuji FUJII
    • Organizer
      Research seminar at Friedrich-Alexander-Universitat Erlangen-Nurnberg
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] 高分子微粒子安定化泡を利用した水中接着技術の開拓2022

    • Author(s)
      足羽奏来・平井智康・中村吉伸・藤井秀司
    • Organizer
      第73回コロイドおよび界面化学討論会
    • Related Report
      2022 Research-status Report
  • [Presentation] Liquid marble engineering: From nature to materials2022

    • Author(s)
      Syuji FUJII
    • Organizer
      GDR ISM Focus : Active Interfaces
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Liquid marble: Droplet covered by particulate membrane2022

    • Author(s)
      Syuji FUJII
    • Organizer
      The 60th Annual Meeting of the Biophysical Society of Japan
    • Related Report
      2022 Research-status Report
    • Int'l Joint Research / Invited
  • [Book] 高分子微粒子の最新技術動向 第27章 高分子粒子安定化ソフト分散体を基盤技術とする物質運搬・放出システムの構築2022

    • Author(s)
      藤井秀司
    • Total Pages
      289
    • Publisher
      シーエムシー出版
    • ISBN
      9784781316710
    • Related Report
      2022 Research-status Report
  • [Book] エポキシ樹脂の設計技術と市場 2022 第4章 エポキシ樹脂のフィラーと界面の設計2022

    • Author(s)
      中村吉伸,平井智康,藤井秀司
    • Total Pages
      231
    • Publisher
      シーエムシー出版
    • ISBN
      9784781316697
    • Related Report
      2022 Research-status Report
  • [Remarks] 大阪工業大学工学部応用化学科高分子材料化学領域webページ

    • URL

      https://www.chem.oit.ac.jp/cherry/4_lab/research2.html

    • Related Report
      2023 Annual Research Report 2022 Research-status Report
  • [Remarks] 藤井秀司 研究紹介webページ

    • URL

      https://www.youtube.com/watch?v=u2TArGB-79Y&list=UUxBwz6-418ToeacGKIBtVmw&index=5

    • Related Report
      2023 Annual Research Report 2022 Research-status Report
  • [Remarks] 日本化学会新領域研究グループ(分散凝集の学理構築への科学と技術戦略)

    • URL

      http://dispersion.chemistry.or.jp/

    • Related Report
      2023 Annual Research Report 2022 Research-status Report

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Published: 2022-07-05   Modified: 2025-01-30  

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