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メソポーラスプラズモニック薄膜の合成と応用

Research Project

Project/Area Number 22KF0380
Project/Area Number (Other) 22F20370 (2022)
Research Category

Grant-in-Aid for JSPS Fellows

Allocation TypeMulti-year Fund (2023)
Single-year Grants (2022)
Section外国
Review Section Basic Section 26020:Inorganic materials and properties-related
Research InstitutionNational Institute for Materials Science

Principal Investigator

山内 悠輔  国立研究開発法人物質・材料研究機構, ナノアーキテクトニクス材料研究センター, NIMS招聘研究員 (10455272)

Co-Investigator(Kenkyū-buntansha) GUSELNIKOVA OLGA  国立研究開発法人物質・材料研究機構, ナノアーキテクトニクス材料研究センター, 外国人特別研究員
Project Period (FY) 2023-03-08 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥3,000,000 (Direct Cost: ¥3,000,000)
Fiscal Year 2023: ¥1,500,000 (Direct Cost: ¥1,500,000)
Fiscal Year 2022: ¥1,500,000 (Direct Cost: ¥1,500,000)
Keywordsメソ多孔体 / Porous materials
Outline of Research at the Start

The developed plasmon-active porous materials will be tested for SERS detection of environmental pollutants in the complex matrix containing different molecules and interfering matter. The mesoporous plasmon-active substrates will be tested in the light-driven reactions of environmental pollutants degradations. The experimental conditions for plasmon catalysis will be optimized to get the highest reaction rate, conversion and selectivity of reactions.

Outline of Annual Research Achievements

The objective of this project is to design novel functional porous materials by integrating mesoporous plasmonic films with chemically grafted organic layers to enhance selectivity. These materials will be applied to (i) monitoring food and water safety through optical sensing and (ii) utilizing greenhouse and related gases for organic synthesis.

New plasmon-active nanoporous materials were successfully prepared and their performance was investigated in terms of Surface-Enhanced Raman Scattering (SERS) detection of environmental pollutants in complex matrices containing various molecules and interfering substances. Particularly, hierarchical macro- and mesoporous Ag materials with organic layer coating achieved practical detections of microplastics, and the results were accepted for publication in Nature Communications (still not published). Additionally, the mesoporous plasmon-active substrates were evaluated in light-driven reactions for the degradation of environmental pollutants.

Report

(2 results)
  • 2023 Annual Research Report
  • 2022 Annual Research Report
  • Research Products

    (12 results)

All 2024 2023 2022

All Journal Article (12 results) (of which Int'l Joint Research: 12 results,  Peer Reviewed: 12 results)

  • [Journal Article] Amphipathic emulsion binder for enhanced performance of lithium-sulfur batteries2024

    • Author(s)
      He Yuan、Jing Xulong、Lai Tianxing、Jiang Dong、Wan Chao、Postnikov Pavel S.、Guselnikova Olga、Xu Lixin、He Xiaojun、Yamauchi Yusuke、Jin Biyu
    • Journal Title

      Journal of Materials Chemistry A

      Volume: -- Issue: 21 Pages: 12681-12690

    • DOI

      10.1039/d4ta01037j

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Uncovering the Role of Chemical and Electronic Structures in Plasmonic Catalysis: The Case of Homolysis of Alkoxyamines2023

    • Author(s)
      Votkina Darya、Petunin Pavel、Miliutina Elena、Trelin Andrii、Lyutakov Oleksiy、Svorcik Vaclav、Audran G?rard、Havot Jeffrey、Valiev Rashid、Valiulina Lenara I.、Joly Jean-Patrick、Yamauchi Yusuke、Mokkath Junais Habeeb、Henzie Joel、Guselnikova Olga、Marque Sylvain R. A.、Postnikov Pavel
    • Journal Title

      ACS Catalysis

      Volume: 13 Issue: 5 Pages: 2822-2833

    • DOI

      10.1021/acscatal.2c04685

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Waste PET upcycling to conductive carbon-based composite through laser-assisted carbonization of UiO-662023

    • Author(s)
      Kogolev Dmitry、Semyonov Oleg、Metalnikova Nadezhda、Fatkullin Maxim、Rodriguez Raul D.、Slepicka Petr、Yamauchi Yusuke、Guselnikova Olga、Boukherroub Rabah、Postnikov Pavel S.
    • Journal Title

      Journal of Materials Chemistry A

      Volume: 11 Issue: 3 Pages: 1108-1115

    • DOI

      10.1039/d2ta08127j

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Weak Bonds, Strong Effects: Enhancing the Separation Performance of UiO-66 toward Chlorobenzenes via Halogen Bonding2023

    • Author(s)
      Gulyaev Roman、Semyonov Oleg、Mamontov Georgy V.、Ivanov Alexey A.、Ivanov Daniil M.、Kim Minjun、Vaclav Svorcik、Resnati Giuseppe、Liao Ting、Sun Ziqi、Yamauchi Yusuke、Postnikov Pavel S.、Guselnikova Olga
    • Journal Title

      ACS Materials Letters

      Volume: 5 Issue: 5 Pages: 1340-1349

    • DOI

      10.1021/acsmaterialslett.2c01169

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Covalent functionalization of Ti3C2T MXene flakes with Gd-DTPA complex for stable and biocompatible MRI contrast agent2022

    • Author(s)
      Neubertova Viktoria、Guselnikova Olga、Yamauchi Yusuke、Olshtrem Anastasia、Rimpelova Silvie、Duchon Jan、Volfova Lenka、Lancok Jan、Herynek Vit、Fitl Premysl、Ulbrich Pavel、Jelinek Ludek、Schneider Patrik、Kosek Juraj、Postnikov Pavel、Kolska Zdenka、Svorcik Vaclav、Chertopalov Sergii、Lyutakov Oleksiy
    • Journal Title

      Chemical Engineering Journal

      Volume: 446 Pages: 136939-136939

    • DOI

      10.1016/j.cej.2022.136939

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Zwitterionic iodonium species afford halogen bond-based porous organic frameworks2022

    • Author(s)
      Soldatova Natalia S.、Postnikov Pavel S.、Ivanov Daniil M.、Semyonov Oleg V.、Kukurina Olga S.、Guselnikova Olga、Yamauchi Yusuke、Wirth Thomas、Zhdankin Viktor V.、Yusubov Mekhman S.、Gomila Rosa M.、Frontera Antonio、Resnati Giuseppe、Kukushkin Vadim Yu.
    • Journal Title

      Chemical Science

      Volume: 13 Issue: 19 Pages: 5650-5658

    • DOI

      10.1039/d2sc00892k

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] New Trends in Nanoarchitectured SERS Substrates: Nanospaces, 2D Materials, and Organic Heterostructures2022

    • Author(s)
      Guselnikova Olga、Lim Hyunsoo、Kim Hyun‐Jong、Kim Sung Hyun、Gorbunova Alina、Eguchi Miharu、Postnikov Pavel、Nakanishi Takuya、Asahi Toru、Na Jongbeom、Yamauchi Yusuke
    • Journal Title

      Small

      Volume: 18 Issue: 25 Pages: 2107182-2107182

    • DOI

      10.1002/smll.202107182

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Noble‐Metal‐Based Hollow Mesoporous Nanoparticles: Synthesis Strategies and Applications2022

    • Author(s)
      Sun Lizhi、Lv Hao、Feng Ji、Guselnikova Olga、Wang Yanzhi、Yamauchi Yusuke、Liu Ben
    • Journal Title

      Advanced Materials

      Volume: 34 Issue: 31 Pages: 2201954-2201954

    • DOI

      10.1002/adma.202201954

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Porous Nanoarchitectures of Nonprecious Metal Borides: From Controlled Synthesis to Heterogeneous Catalyst Applications2022

    • Author(s)
      Kang Yunqing、Tang Yi、Zhu Liyang、Jiang Bo、Xu Xingtao、Guselnikova Olga、Li Hexing、Asahi Toru、Yamauchi Yusuke
    • Journal Title

      ACS Catalysis

      Volume: 12 Issue: 23 Pages: 14773-14793

    • DOI

      10.1021/acscatal.2c03480

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Symmetry-Breaking Plasmonic Mesoporous Gold Nanoparticles with Large Pores2022

    • Author(s)
      Nugraha Asep Sugih、Guselnikova Olga、Henzie Joel、Na Jongbeom、Hossain Md Shahriar A.、Dag ?mer、Rowan Alan E.、Yamauchi Yusuke
    • Journal Title

      Chemistry of Materials

      Volume: 34 Issue: 16 Pages: 7256-7270

    • DOI

      10.1021/acs.chemmater.2c01125

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Phase engineering of dual active 2D Bi2O3-based nanocatalysts for alkaline hydrogen evolution reaction electrocatalysis2022

    • Author(s)
      Wu Ziyang、Mei Jun、Liu Qiong、Wang Sen、Li Wei、Xing Shihui、Bai Juan、Yang Jianping、Luo Wei、Guselnikova Olga、O'Mullane Anthony P.、Gu Yuantong、Yamauchi Yusuke、Liao Ting、Sun Ziqi
    • Journal Title

      Journal of Materials Chemistry A

      Volume: 10 Issue: 2 Pages: 808-817

    • DOI

      10.1039/d1ta09019d

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Surface Filtration in Mesoporous Au Films Decorated by Ag Nanoparticles for Solving SERS Sensing Small Molecules in Living Cells2022

    • Author(s)
      Guselnikova Olga、Nugraha Asep Sugih、Na Jongbeom、Postnikov Pavel、Kim Hyun-Jong、Plotnikov Evgenii、Yamauchi Yusuke
    • Journal Title

      ACS Applied Materials Interfaces

      Volume: 14 Issue: 36 Pages: 41629-41639

    • DOI

      10.1021/acsami.2c12804

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Int'l Joint Research

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Published: 2022-04-28   Modified: 2024-12-25  

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