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Theoretical Study of Neuromorphic Devices Based on Two-dimensional-based Magnetic Tunnel Junctions

Research Project

Project/Area Number 22KJ2092
Project/Area Number (Other) 21J22520 (2021-2022)
Research Category

Grant-in-Aid for JSPS Fellows

Allocation TypeMulti-year Fund (2023)
Single-year Grants (2021-2022)
Section国内
Review Section Basic Section 29020:Thin film/surface and interfacial physical properties-related
Research InstitutionOsaka University

Principal Investigator

Harfah Halimah  大阪大学, 基礎工学研究科, 特別研究員(DC1)

Project Period (FY) 2023-03-08 – 2024-03-31
Project Status Completed (Fiscal Year 2023)
Budget Amount *help
¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 2023: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 2022: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 2021: ¥800,000 (Direct Cost: ¥800,000)
Keywordsmagnetic tunnel junction / 2D materials / monoatomic vacancy / spintronics / hexagonal boron nitride / graphene (Gr) / localized state / spin coupling / vacancy / magnetic proximity / neuromorphic device / magnetoresistance (MR) / proximity effect / optical-based MTJ / new MTJ mechanism
Outline of Research at the Start

Research on exploring and designing a neuromorphic device based on 2D materials magnetic tunnel junction is proposed. The 2D materials such as graphene and hBN have unique physical and chemical properties when doping or a vacancy occur. One of the example is the appearance of localized state. A neuromorphic device by utilizing and controlling the localized state of the doped or defected 2D materials to create a multi-level memory state are expected to be the the outcome. This result will be an insight to create in-materio synapses weight based on 2D materials based MTJ.

Outline of Annual Research Achievements

The study on vacancies in 2D materials impacting magnetic tunnel junction (MTJ) device performance has progressed significantly. Utilizing density functional theory (DFT), monoatomic vacancies in hexagonal boron nitride (hBN) and graphene layers were investigated. Vacancies were found to create distinct transmission channels for spin-majority and spin-minority channels, influenced by the proximity effect and vacancy layer's localized state.

A novel van der Waals-based MTJ design was proposed, comprising hBN(VB)/Graphene(Gr)/hBN(VB) with strategically positioned monoatomic vacancies. Non-equilibrium Green's function (NEGF) simulations, coupled with DFT data, showed a TMR ratio of approximately 400%, marking a significant advancement in thin structure MTJs. This design underscores the potential of defective 2D materials in enhancing magnetic random-access memory (MRAM) devices and optimizing neuromorphic devices.

The research reveals the intricate relationship between vacancies in 2D materials and MTJ device performance, offering new avenues for device optimization. The proposed MTJ design with monoatomic vacancies demonstrates remarkable potential for improving TMR ratios and advancing MRAM devices, highlighting the importance of defective 2D materials in next-generation electronic and magnetic devices. Furthermore, the engineering of the vacancy opens up the possible application of 2D materials MTJ as a potential neuromorphic device.

Report

(3 results)
  • 2023 Annual Research Report
  • 2022 Annual Research Report
  • 2021 Annual Research Report
  • Research Products

    (10 results)

All 2024 2023 2022 2021

All Journal Article (4 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 4 results,  Open Access: 4 results) Presentation (6 results) (of which Int'l Joint Research: 2 results)

  • [Journal Article] Ultra-thin van der Waals magnetic tunnel junction based on monoatomic boron vacancy of hexagonal boron nitride2024

    • Author(s)
      Harfah Halimah、Wicaksono Yusuf、Sunnardianto Gagus Ketut、Majidi Muhammad Aziz、Kusakabe Koichi
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 26 Issue: 12 Pages: 9733-9740

    • DOI

      10.1039/d4cp00218k

    • Related Report
      2023 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Spin-Topological Electronic Valve in Ni/hBN-Graphene-hBN/Ni Magnetic Junction2023

    • Author(s)
      Wicaksono Yusuf、Harfah Halimah、Sunnardianto Gagus Ketut、Majidi Muhammad Aziz、Kusakabe Koichi
    • Journal Title

      Magnetochemistry

      Volume: 9 Issue: 5 Pages: 113-113

    • DOI

      10.3390/magnetochemistry9050113

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Colossal in-plane magnetoresistance ratio of graphene sandwiched with Ni nanostructures2022

    • Author(s)
      Wicaksono Yusuf、Harfah Halimah、Sunnardianto Gagus Ketut、Majidi Muhammad Aziz、Kusakabe Koichi
    • Journal Title

      RSC Advances

      Volume: 12 Issue: 22 Pages: 13985-13991

    • DOI

      10.1039/d2ra00957a

    • Related Report
      2022 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] High magnetoresistance of a hexagonal boron nitride?graphene heterostructure-based MTJ through excited-electron transmission2022

    • Author(s)
      Harfah Halimah、Wicaksono Yusuf、Sunnardianto Gagus Ketut、Majidi Muhammad Aziz、Kusakabe Koichi
    • Journal Title

      Nanoscale Advances

      Volume: 4 Issue: 1 Pages: 117-124

    • DOI

      10.1039/d1na00272d

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Application of Monoatomic Boron Vacancy of Hexagonal Boron Nitride as Ultra-thin Van der Waals Magnetic Tunnel Junction2023

    • Author(s)
      Halimah Harfah, Yusuf Wicaksono, Gagus Ketut Sunnardianto, Muhammad Aziz Majidi, and Koichi Kusakabe
    • Organizer
      the 71st JSAP Spring Meeting
    • Related Report
      2023 Annual Research Report
  • [Presentation] Spin-mechatronics device based on controllable mass gapped Dirac cone of graphene in aNi/hBN-graphene-hBN/Ni magnetic junction2022

    • Author(s)
      Yusuf Wicaksono, Halimah Harfah, Gagus Ketut Sunnardianto, Muhammad Aziz Majidi, and Koichi Kusakabe
    • Organizer
      the 70th JSAP Spring Meeting
    • Related Report
      2022 Annual Research Report
  • [Presentation] Realizing a Novel Functionality on 2D Materials Based Magnetic Tunnel Junction2021

    • Author(s)
      Halimah Harfah, Yusuf Wicaksono, Gagus Ketut Sunnardianto, Muhammad Aziz Majidi, and Koichi Kusakabe
    • Organizer
      Materials Info 2022
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High magnetoresistance of hexagonal boron nitride-graphene heterostructure-based MTJ through excited-electron transmission2021

    • Author(s)
      Halimah Harfah, Yusuf Wicaksono, Gagus Ketut Sunnardianto, Muhammad Aziz Majidi, and Koichi Kusakabe
    • Organizer
      the 69th JSAP Spring Meeting
    • Related Report
      2021 Annual Research Report
  • [Presentation] Controlling the Gapped Dirac Cone of Graphene through Pseudospin to Achieve Colossal in-Plane Magnetoresistance2021

    • Author(s)
      Yusuf Wicaksono, Halimah Harfah, Gagus Ketut Sunnardianto, Muhammad Aziz Majidi, and Koichi Kusakabe
    • Organizer
      Materials Info 2022
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] The Importance of Interface in Controlling Mass Gapped Dirac Cone of Graphene through Pseudospin via Magnetic Proximity Effect2021

    • Author(s)
      Yusuf Wicaksono, Halimah Harfah, Gagus Ketut Sunnardianto, Muhammad Aziz Majidi, and Koichi Kusakabe
    • Organizer
      the 69th JSAP Spring Meeting
    • Related Report
      2021 Annual Research Report

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Published: 2021-05-27   Modified: 2024-12-25  

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