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Determination on the photochemical reaction path from NO to nitrate in eastern Asian troposphere by using the triple oxygen isotopes as tracers

Research Project

Project/Area Number 23241001
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionNagoya University (2012-2013)
Hokkaido University (2011)

Principal Investigator

TSUNOGAI Urumu  名古屋大学, 環境学研究科, 教授 (50313367)

Co-Investigator(Kenkyū-buntansha) TANIMOTO Hiroshi  国立環境研究所, 地球環境研究センター, 室長 (30342736)
NOGUCHI Izumi  北海道立総合研究機構環境, 環境科学研究センター, 研究主幹 (10442617)
YAMAGUCHI Takashi  北海道立総合研究機構環境, 地質研究本部環境科学研究センター, 研究主任 (90462316)
SATO Keiichi  一般財団法人日本環境衛生センターアジァ大気汚染研究センター, 情報管理部, 上席研究員 (00391110)
TSUBOI Kazuhiro  気象庁気象研究所, 地球化学研究部, 主任研究官 (10553167)
MATSUEDA Hidekazu  気象庁気象研究所, 地球化学研究部, 室長 (60354552)
Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥32,760,000 (Direct Cost: ¥25,200,000、Indirect Cost: ¥7,560,000)
Fiscal Year 2013: ¥8,970,000 (Direct Cost: ¥6,900,000、Indirect Cost: ¥2,070,000)
Fiscal Year 2012: ¥9,230,000 (Direct Cost: ¥7,100,000、Indirect Cost: ¥2,130,000)
Fiscal Year 2011: ¥14,560,000 (Direct Cost: ¥11,200,000、Indirect Cost: ¥3,360,000)
Keywords東アジア / 大気 / 光化学反応 / 窒素酸化物 / 硝酸 / 三酸素同位体 / モニタリング / 大気光化学反応 / 大気沈着 / 汚染気塊 / オゾン / 連続観測 / 三酸素同位体組成 / 不均一反応
Research Abstract

Temporal variation in the triple oxygen isotopic compositions of atmospheric nitrate in precipitation (wet deposition) was monitored continuously in four observatories in Japan (Rishiri, Sado-seki, Kosugi, and Minami-torishima). We concluded the triple oxygen isotopic compositions of atmospheric nitrate were the useful tracer to estimate the major photochemical reaction path from NO to nitrate in eastern Asian troposphere. Besides, we found that the annual average values in the triple oxygen isotopic compositions of atmospheric nitrate was almost stable in mid-latitudes.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (49 results)

All 2014 2013 2012 2011

All Journal Article (23 results) (of which Peer Reviewed: 11 results) Presentation (24 results) (of which Invited: 5 results) Book (2 results)

  • [Journal Article] Quantifying the effects of clear-cutting and strip-cutting on nitrate dynamics in a forested watershed using triple oxygen isotopes as tracers2014

    • Author(s)
      Tsunogai, U., Komatsu, D. D., Ohyama, T., Suzuki, A., Nakagawa, F., Noguchi, I., Takagi, K., Nomura, M., Fukuzawa, K., and Shibata, H
    • Journal Title

      Biogeosciences Discuss

      Volume: 11 Pages: 7413-7450

    • Related Report
      2013 Final Research Report
  • [Journal Article] Tracing atmospheric nitrate in groundwater using triple oxygen isotopes : Evaluation based on bottled drinking water2013

    • Author(s)
      Nakagawa, F., A. Suzuki, S. Daita, T. Ohyama, D.D. Komatsu and U. Tsunogai
    • Journal Title

      Biogeosciences

      Volume: 10 Pages: 3547-3558

    • Related Report
      2013 Final Research Report
  • [Journal Article] Nitrogen isotopes in intra-crystal coralline aragonites2013

    • Author(s)
      Yamazaki, A., T. Watanabe, N. Takahata, Y. Sano, and U. Tsunogai
    • Journal Title

      Chemical Geology

      Volume: 351 Pages: 276-280

    • NAID

      120005446641

    • Related Report
      2013 Final Research Report
  • [Journal Article] Novel microbial populations colonized in deep granitic groundwater from Grimsel Test Site2013

    • Author(s)
      Konno, U., M. Kouduka, D.D. Komatsu, K. Ishii, A. Fukuda, U. Tsunogai, K. Ito, and Y. Suzuki
    • Journal Title

      Switzerland. Microbial Ecology

      Volume: 65 Pages: 626-637

    • Related Report
      2013 Final Research Report
  • [Journal Article] Strong relationship between dimethyl sulfide and net community production in the western subarctic Pacific2013

    • Author(s)
      Kameyama, S., H. Tanimoto, S. Inomata, H. Y. Inoue, U. Tsunogai, A. Tsuda, M. Uematsu, M. Ishii, and D. Sasano
    • Journal Title

      Geophys. Res. Lett

      Volume: 40 Pages: 3986-3990

    • Related Report
      2013 Final Research Report
  • [Journal Article] Validity of otolith δ18O of Pacific bluefin tuna (Thunnus orientalis) as an indicator of ambient water temperature2013

    • Author(s)
      Kitagawa, T., T. Ishimura, R. Uozato, K. Shirai, Y. Amano, A. Shinoda, T. Otake, U. Tsunogai, and S. Kimura
    • Journal Title

      Mar. Ecol. Prog. Ser

      Volume: 481 Pages: 199-209

    • Related Report
      2013 Final Research Report
  • [Journal Article] Megacities and large urban agglomerations in the Coastal Zone: Interactions between atmosphere, land and marine ecosystems.2013

    • Author(s)
      von Glasow, R., T. Jickells, A. Baklanov, G.R. Carmichael, T. Church, L. Gallardo, C. Hughes, M. Kanakidou, P. Liss, L. Mee, R. Raine, P. Ramachandran, R. Ramesh, K. Sundseth, U. Tsunogai, M. Uematsu, and T. Zhu
    • Journal Title

      AMBIO

      Volume: 42 Issue: 1 Pages: 13-28

    • DOI

      10.1007/s13280-012-0343-9

    • Related Report
      2013 Annual Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Otolith δ18O of Pacific bluefin tuna Thunnus orientalis as an indicator of ambient water temperature.2013

    • Author(s)
      Kitagawa, T., T. Ishimura, R. Uozato, K. Shirai, Y. Amano, A. Shinoda, T. Otake, U. Tsunogai, and S. Kimura
    • Journal Title

      Marine Ecology Progress Series

      Volume: 481 Pages: 199-209

    • DOI

      10.3354/meps10202

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Novel microbial populations colonized in deep granitic groundwater from Grimsel Test Site, Switzerland.2013

    • Author(s)
      Konno, U., M. Kouduka, D.D. Komatsu, K. Ishii, A. Fukuda, U. Tsunogai, K. Ito, and Y. Suzuki
    • Journal Title

      Microbial Ecology

      Volume: 65 Issue: 3 Pages: 626-637

    • DOI

      10.1007/s00248-013-0184-5

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tracing atmospheric nitrate in groundwater using triple oxygen isotopes: Evaluation based on bottled drinking water.2013

    • Author(s)
      Nakagawa, F., A. Suzuki, S. Daita, T. Ohyama, D.D. Komatsu and U. Tsunogai
    • Journal Title

      Biogeosciences

      Volume: 10 Issue: 6 Pages: 3547-3558

    • DOI

      10.5194/bg-10-3547-2013

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nitrogen isotopes in intra-crystal coralline aragonites2013

    • Author(s)
      Atsuko Yamazaki, Tsuyoshi Watanabe, Naoto Takahata, Yuji Sane, Urumu Tsunogai
    • Journal Title

      Chemical Geology

      Volume: 351 Pages: 276-280

    • DOI

      10.1016/j.chemgeo.2013.05.024

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Strong relationship between dimethyl sulfide and net community production in the western subarctic Pacific2013

    • Author(s)
      Kameyama, S., H. Tanimoto, S. Inomata, H. Yoshikawa-Inoue, U.Tsunogai, A. Tsuda, M. Uematsu, M. Ishii, D. Sasano, K. Suzuki, and Y. Nosaka
    • Journal Title

      Geophysical Research Letters

      Volume: 40 Issue: 15 Pages: 3986-3990

    • DOI

      10.1002/grl.50654

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Occurrence and potential activity of denitrifiers and methanogens in groundwater at 140 m depth in Pliocene diatomaceous mudstone of northern Japan.2013

    • Author(s)
      Katsuyama, C., Nashimoto, H., Nagaosa, K., Ishibashi, T., Kinoshita, T., Yoshikawa, H., Aoki, K., Asano, T., Sasaki, Y., Sohrin, R., Komatsu, D., Tsunogai, U., Kimura, H., Suwa, Y., Kato, K.
    • Journal Title

      FEMS Microbiology Ecology

      Volume: 86 Issue: 3 Pages: 532-543

    • DOI

      10.1111/1574-6941.12179

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tracing atmospheric nitrate in groundwater using triple oxygen isotopes: Evaluation based on bottled drinking water.2013

    • Author(s)
      Tsunogai, U.
    • Journal Title

      Biogeosciences Discuss

      Volume: 9 Pages: 16493-16519

    • DOI

      10.5194/bgd-9-16493-2012

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Coseimic massive methane release from a submarine mud volcano. Earth Planet2012

    • Author(s)
      Tsunogai, U., K. Maegawa, S. Sato, D.D. Komatsu, F. Nakagawa, T. Toki, and J. Ashi
    • Journal Title

      Sci. Lett

    • Related Report
      2013 Final Research Report
  • [Journal Article] Variation in stable carbon and oxygen isotopes of individual benthic foraminifera : Tracers for quantifying the magnitude of isotopic disequilibrium2012

    • Author(s)
      Ishimura, T., U. Tsunogai, S. Hasegawa, F. Nakagawa, T. Oi, H. Kitazato, H. Suga, and T. Toyofuku
    • Journal Title

      Biogeosciences

      Volume: 9 Pages: 4353-4367

    • Related Report
      2013 Final Research Report
  • [Journal Article] Biogeochemical processes involving acetate in sub-seafloor sediments from the Bering Sea shelf break2012

    • Author(s)
      Ijiri, A., N. Harada, A. Hirota, U. Tsunogai, (他4名)
    • Journal Title

      Organic Geochemistry

      Volume: 48 Pages: 47-55

    • Related Report
      2013 Final Research Report
  • [Journal Article] Stable hydrogen isotopic analysis of nanomolar molecular hydrogen by automatic multi-step gas chromatographic separation2011

    • Author(s)
      Komatsu, D.D., U. Tsunogai, K. Kamimura, U. Konno, T. Ishimura, and F. Nakagawa
    • Journal Title

      Rapid Commun. Mass Spec

      Volume: 25 Pages: 3351-3359

    • Related Report
      2013 Final Research Report
  • [Journal Article] δ15N in reef coral skeletons as a proxy of tropical nutrient dynamics2011

    • Author(s)
      Yamazaki, A., T.Watanabe, U.Isunogai
    • Journal Title

      Geophysical Research Letter

      Volume: 38 Issue: 19 Pages: 19605-19605

    • DOI

      10.1029/2011gl049053

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantifying nitrate dynamics in an oligotrophic lake using Δ^<17>O2011

    • Author(s)
      Tsunogai, U., S. Daita, D.D. Komatsu, F. Nakagawa, and A. Tanaka
    • Journal Title

      Biogeosciences

      Volume: 8 Pages: 687-702

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
  • [Journal Article] Application of PTR-MS to incubation experiments of the marine diatom Thalassiosira pseudonana2011

    • Author(s)
      Kameyama, S., H. Tanimoto, S. Inomata, K. Suzuki, D.D. Komatsu, A. Hirota, U. Konno, and U. Tsunogai
    • Journal Title

      Geochem. J

      Volume: 45 Pages: 355-363

    • NAID

      10030362941

    • Related Report
      2013 Final Research Report
  • [Journal Article] Stable carbon isotope ratios of ethane over the North Pacific : atmospheric measurements and global chemical transport modeling2011

    • Author(s)
      Saito, T., O. Stein, U. Tsunogai,(他4名)
    • Journal Title

      J. Geophys. Res

      Volume: 116 Issue: D2

    • DOI

      10.1029/2010jd014602

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen isotopes in volcanic plumes : Tracers for remote temperature sensing of fumaroles2011

    • Author(s)
      Tsunogai, U., K.Kamimura, S.Anzai, F.Nakagawa, D.D.Komatsu
    • Journal Title

      Geochimica et Cosmochimica Acta

      Volume: 75 Issue: 16 Pages: 4531-4546

    • DOI

      10.1016/j.gca.2011.05.023

    • NAID

      130005054211

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] 貧栄養・中栄養湖沼における大気沈着由来の硝酸の混合比 (A-2-1)2013

    • Author(s)
      角皆潤,宮内貴規,大山拓也,小松大祐,蓼沼雪衣,中川書子,梅田信,田中敦
    • Organizer
      第19回大気化学討論会
    • Place of Presentation
      石川県七尾市和倉温泉のと楽
    • Year and Date
      2013-11-17
    • Related Report
      2013 Final Research Report
  • [Presentation] 都市域における乾性沈着HNO3の起源について (ICO8)2013

    • Author(s)
      大山拓也,角皆潤,小松大祐,中川書子,野口泉
    • Organizer
      2013年度日本地球化学会第60回年会
    • Place of Presentation
      筑波大学第一エリア
    • Year and Date
      2013-09-11
    • Related Report
      2013 Final Research Report
  • [Presentation] 湧水系の溶存酸素の三酸素同位体組成 : なぜ富士山湧水系は酸素に富んでいるのか?2013

    • Author(s)
      角皆潤,南翔,佐久間博基,大山拓也,小松大祐,中川書子,加藤憲二
    • Organizer
      日本地球惑星科学連合2013年大会
    • Place of Presentation
      幕張メッセ国際会議場203
    • Year and Date
      2013-05-23
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 貧栄養・中栄養湖沼における大気沈着由来の硝酸の混合比2013

    • Author(s)
      角皆 潤
    • Organizer
      第19回大気化学討論会
    • Place of Presentation
      石川県七尾市和倉温泉のと楽
    • Related Report
      2013 Annual Research Report
  • [Presentation] 大胆予測:10年後の質量分析計はこうなる2013

    • Author(s)
      角皆 潤
    • Organizer
      2013年質量分析学会同位体比部会プレゼミ「10年後のIRMS」
    • Place of Presentation
      広島湯坂温泉郷賀茂川荘
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 都市域における乾性沈着 HNO3 の起源について2013

    • Author(s)
      大山 拓也, 角皆 潤, 小松 大祐, 中川 書子, 野口 泉
    • Organizer
      日本地球化学会第60回年会
    • Place of Presentation
      筑波大学第一エリア
    • Related Report
      2013 Annual Research Report
  • [Presentation] 硝酸の三酸素同位体組成を指標に用いたNOxの光化学反応過程解析2012

    • Author(s)
      大山拓也,角皆潤,小松大祐,中川書子,野口泉,山口高志,佐藤啓市,大泉毅,坪井一寛,木戸瑞佳
    • Organizer
      日本地球惑星科学連合2012年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Year and Date
      2012-05-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Quantifying nitrate dynamics in hydrosphere using the triple oxygen isotopes as tracers2012

    • Author(s)
      Tsunogai, U., Komatsu, D. D., and Nakagawa, F
    • Organizer
      Utilizing Rare isotopE for biogeochemistrY (UREY) Workshop
    • Place of Presentation
      Academia Sinica, Taipei, Taiwan
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 大気から沈着する窒素と衰退した森林生態系の相互作用定量化2012

    • Author(s)
      角皆潤,小松大祐,鈴木敦之,中川書子, 福澤加里部,柴田英昭,高木健太郎,野村睦
    • Organizer
      2012年度日本地球化学会第59回年会
    • Place of Presentation
      九州大学箱崎キャンパス
    • Related Report
      2013 Final Research Report 2012 Annual Research Report
  • [Presentation] Quantifying nitrate dynamics in hydrosphere using the triple oxygen isotopes as tracers2012

    • Author(s)
      Tsunogai, U., Tadenuma, Y., Ohyama, T., Komatsu, D. D., Nakagawa, F., Umeda, M, and Tanaka, A
    • Organizer
      2012 ASLO Aquatic Sciences Meeting
    • Place of Presentation
      Lake Biwa, Otsu, Shiga, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] 森林伐採に伴う窒素循環変化:流出する硝酸の三酸素同位体組成を指標に用いた評価2012

    • Author(s)
      角皆 潤
    • Organizer
      日本地球惑星科学連合2012年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Related Report
      2012 Annual Research Report
  • [Presentation] 硝酸の自然同位体組成を指標に用いた窒素循環速度定量化手法の開発:人工トレーサー添加法との比較検証2012

    • Author(s)
      角皆 潤
    • Organizer
      日本地球惑星科学連合2012年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Related Report
      2012 Annual Research Report
  • [Presentation] Quantifying nitrate dynamics in hydrosphere using the triple oxygen isotopes as tracers.2012

    • Author(s)
      角皆 潤
    • Organizer
      2012 ASLO Aquatic Sciences Meeting
    • Place of Presentation
      コラボしが21
    • Related Report
      2012 Annual Research Report
  • [Presentation] Quantifying nitrate dynamics in hydrosphere using the triple oxygen isotopes as tracers.2012

    • Author(s)
      角皆 潤
    • Organizer
      Utilizing Rare isotopE for biogeochemistrY (UREY) Workshop
    • Place of Presentation
      Academia Sinica, Taipei, Taiwan
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 試料前処理2012

    • Author(s)
      角皆 潤
    • Organizer
      2012年質量分析学会同位体比部会
    • Place of Presentation
      佐勘(宮城県仙台市)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Breakthrough in Isotope-Ratio Mass Spectrometry. Pre-seminar 2011 in Busan, Meeting on Isotope-ratio mass spectrometry2011

    • Author(s)
      Tsunogai. U., D.D. Komatsu, and F. Nakagawa
    • Organizer
      The Mass Spectrometry Society of Japan
    • Place of Presentation
      Haeundae Grand Hotel in Busan, Korea
    • Year and Date
      2011-11-23
    • Related Report
      2013 Final Research Report
  • [Presentation] Regional differences in the photochemical reaction paths of NOx estimated from the ^<17>0 tracer of nitrate. Meeting on Isotope-ratio mass spectrometry2011

    • Author(s)
      Ohayama, T., D.D. Komatsu, S. Daita, F. Nakagawa, U. Tsunogai, I. Noguchi, T. Yamaguchi, K. Sato, T. Ohizumi, K. Tsuboi
    • Organizer
      The Mass Spectrometry Society of Japan
    • Place of Presentation
      Haeundae Grand Hotel in Busan, Korea
    • Year and Date
      2011-11-23
    • Related Report
      2013 Final Research Report
  • [Presentation] 硝酸の三酸素同位体を指標に用いた貧栄養湖沼の窒素循環定量とその検証2011

    • Author(s)
      蓼沼雪衣,角皆潤,大山拓也,鈴木敦之,小松大祐,中川書子,田中敦
    • Organizer
      生物地球化学研究会10周年記念セッション
    • Place of Presentation
      北海道大学地球環境科学研究院
    • Year and Date
      2011-10-22
    • Related Report
      2013 Final Research Report
  • [Presentation] 硝酸の同位体組成を指標に用いた東京湾における窒素循環解析2011

    • Author(s)
      中川書子, 角皆潤, 小松大祐, 久保篤史, 神田穣太
    • Organizer
      2011年度日本地球化学会年会
    • Place of Presentation
      北海道大学学術交流会館(札幌)
    • Year and Date
      2011-09-16
    • Related Report
      2011 Annual Research Report
  • [Presentation] 170,180,15Nをトレーサーに用いた陸水環境における溶存硝酸の起源および窒素循環の解析法2011

    • Author(s)
      中川書子, 鈴木敦之, 大山拓也, 小松大祐, 角皆潤, 梅田信, 柴田英昭, 小畑元, 田副博文
    • Organizer
      2011年度日本地球化学会年会
    • Place of Presentation
      北海道大学学術交流会館(札幌)
    • Year and Date
      2011-09-16
    • Related Report
      2011 Annual Research Report
  • [Presentation] 硝酸の三酸素同位体組成を指標に用いたNOxの光化学反応過程の解析2011

    • Author(s)
      大山拓也, 角皆潤, 小松大祐, 代田里子, 中川書子, 野口泉, 山口高志, 佐藤啓市, 大泉毅, 坪井一寛, 木戸瑞佳
    • Organizer
      2011年度日本地球化学会年会
    • Place of Presentation
      北海道大学学術交流会館(札幌)
    • Year and Date
      2011-09-14
    • Related Report
      2011 Annual Research Report
  • [Presentation] 硝酸の三酸素同位体組成を指標に用いた水環境中の窒素循環の定量化 : 非培養・現場型の窒素同化速度定量法開発 (MISO23-042011

    • Author(s)
      角皆潤,小松大祐,中川書子
    • Organizer
      日本地球惑星科学連合2011年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Year and Date
      2011-05-22
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 硝酸の三酸素同位体組成を指標に用いた水環境中の窒素循環の定量化:非培養・現場型の窒素同化速度定量法開発2011

    • Author(s)
      角皆潤・小松大祐・中川書子
    • Organizer
      日本地球惑星科学連合2011年大会
    • Place of Presentation
      幕張メッセ国際会議場(千葉県)(招待講演)
    • Year and Date
      2011-05-22
    • Related Report
      2011 Annual Research Report
  • [Presentation] 硝酸の三酸素同位体組成を指標に用いたNOxの光化学反応過程の解析2011

    • Author(s)
      大山拓也,角皆潤,小松大祐,代田里子,中川書子,野口泉,山口高志,佐藤啓血,大泉毅,墨二寛,木戸瑞佳
    • Organizer
      2011年度日本地球化学会第58回年会
    • Place of Presentation
      北海道大学学術交流会館
    • Related Report
      2013 Final Research Report
  • [Book] 地球と宇宙の化学事典 (日本地球化学会編), (気体質量分析計(第一章) 温室効果気体(第五章) ガスハイドレート(第八章) 執筆)2012

    • Total Pages
      479
    • Publisher
      朝倉書店
    • Related Report
      2013 Final Research Report
  • [Book] 地球と宇宙の化学事典2012

    • Author(s)
      日本地球化学会
    • Total Pages
      472
    • Publisher
      朝倉書店
    • Related Report
      2012 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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