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Exploring of quantum many-body effect in strongly frustrated spin systems

Research Project

Project/Area Number 23244072
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Condensed matter physics II
Research InstitutionTokyo Institute of Technology

Principal Investigator

HIDEKAZU Tanaka  東京工業大学, 理工学研究科, 教授 (80188325)

Co-Investigator(Kenkyū-buntansha) ONO Toshio  大阪府立大学, 理学系研究科, 准教授 (40332639)
KURITA Nobuyuki  東京工業大学, 大学院理工学研究科, 助教 (80566737)
Co-Investigator(Renkei-kenkyūsha) SATO Taku  東北大学, 多元物質科学研究所, 教授 (70354214)
Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥47,840,000 (Direct Cost: ¥36,800,000、Indirect Cost: ¥11,040,000)
Fiscal Year 2013: ¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2012: ¥30,940,000 (Direct Cost: ¥23,800,000、Indirect Cost: ¥7,140,000)
Fiscal Year 2011: ¥7,410,000 (Direct Cost: ¥5,700,000、Indirect Cost: ¥1,710,000)
Keywords磁性 / 量子スピン系 / フラストレーション / 強磁場 / 量子多体効果 / 三角格子反強磁性体 / 籠目格子反強磁性体 / スピンダイマー磁性体 / 物性実験 / 量子磁性 / 強相関電子系 / 強磁場物性 / スピンダイマー系 / 低温物性
Research Abstract

We investigated remarkable quantum effects in strongly frustrated spin systems. We performed magnetization measurement on Ba3CoSb2O9, and provide evidence that a spin-1/2 Heisenberg antiferromagnet on a regular triangular lattice is actually realized in Ba3CoSb2O9. We found that the entire magnetization curve is in excellent quantitative agreement with the theoretical calculations.
Magnetic excitations in the spin-1/2 kagome lattice antiferromagnet Cs2Cu3SnF12 with an ordered ground state were studied using inelastic neutron scattering. Although the spin-wave dispersion can be qualitatively understood in terms of linear spin-wave theory (LSWT), the excitation energies are renormalized by a factor of approximately 0.6 from those calculated by LSWT. This result provides the first evidence of negative quantum renormalization. We determined the crystal structure of the spin dimer magnet Ba2CoSi2O6Cl2, and observed quantization of magnetization at half of the saturation magnetization.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (40 results)

All 2014 2013 2012 2011 Other

All Journal Article (24 results) (of which Peer Reviewed: 24 results) Presentation (13 results) (of which Invited: 2 results) Remarks (3 results)

  • [Journal Article] Ghost modes and continuum scattering in the dimerized distorted kagome lattice antiferromagnet Rb_2Cu_3SnF_<12>2014

    • Author(s)
      K. Matan, Y. Nambu, T. J. Sato, Y. Fukumoto, T. Ono, H. Tanaka, Y. Zhao, C. Broholm, A. Podlesnyak, and G. Ehlers
    • Journal Title

      Phys. Rev. B

      Volume: 89 Issue: 2 Pages: 24414-24414

    • DOI

      10.1103/physrevb.89.024414

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] スピンが1/2の三角格子反強磁性体の磁化過程と量子多体効果2014

    • Author(s)
      田中秀数,栗田伸之,松尾晶,金道浩一
    • Journal Title

      日本物理学会誌

      Volume: 69 Pages: 24-28

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] スピン1/2の正規三角格子反強磁性体Ba_3CoSb_2O_9 の量子磁化過程とESR2013

    • Author(s)
      薄 拓哉,栗田伸之,田中秀数,野尻浩之
    • Journal Title

      電子スピンサイエンス

      Volume: 11 Pages: 86-91

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Magnetization Process and Collective Excitations in the S=1/2 Triangular-Lattice Heisenberg Antiferromagnet Ba_3CoSb_2O_92013

    • Author(s)
      T. Susuki, N. Kurita, T. Tanaka, H. Nojiri, A. Matsuo, K. Kindo and H. Tanaka
    • Journal Title

      Phys. Rev. Lett

      Volume: 110

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Microscopic Properties of the "Pinwheel" Kagome Compound Rb_2Cu_3SnF_<12>2013

    • Author(s)
      M. S. Grbić, S. Krämer, C. Berthier, F. Trousselet, O. Cépas, H. Tanaka, and M. Horvatić
    • Journal Title

      Phys. Rev. Lett

      Volume: 110 Issue: 24

    • DOI

      10.1103/physrevlett.110.247203

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] The magnetization process of the spin-one triangular-lattice Heisenberg antiferromagnet2013

    • Author(s)
      J. Richter, O. Götze, R. Zinke, D. J. J. Farnell and H. Tanaka
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 82 Issue: 1 Pages: 015002-015002

    • DOI

      10.7566/jpsj.82.015002

    • NAID

      210000132369

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Magnetization Process and Collective Excitations in the S=1/2 Triangular-Lattice Heisenberg Antiferromagnet Ba3CoSb2O92013

    • Author(s)
      T. Susuki, N. Kurita, T. Tanaka, H. Nojiri, A. Matsuo, K. Kindo and H. Tanaka
    • Journal Title

      Phys. Rev. Lett.

      Volume: 110 Issue: 26

    • DOI

      10.1103/physrevlett.110.267201

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] スピン1/2の正規三角格子反強磁性体Ba3CoSb2O9の量子磁化過程とESR2013

    • Author(s)
      薄 拓哉,栗田伸之,田中秀数,野尻浩之
    • Journal Title

      電子スピンサイエンス

      Volume: 11 Pages: 86-91

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantum renormalization effects in one-dimensional Heisenberg antiferromagnets Rb2Mn0.6Mg0.4F42012

    • Author(s)
      S. Itoh, T. Yokoo, S. Yano, D. Kawana, H. Tanaka and Y. Endoh
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 81 Issue: 8 Pages: 084706-084706

    • DOI

      10.1143/jpsj.81.084706

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ferromagnetism induced in the anisotropic stacked kagome lattice antiferromagnet Cs_2Cu_3CeF_<12>2012

    • Author(s)
      T. Amemiya, I. Umegaki, H. Tanaka, T. Ono, A. Matsuo and K. Kindo
    • Journal Title

      Phys. Rev. B

      Volume: 85

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Thermodynamic properties of quantum sine-Gordon spin chain system KCuGaF_62012

    • Author(s)
      I. Umegaki, H. Tanaka, T. Ono, M. Oshikawa and K Sakai
    • Journal Title

      Phys. Rev. B

      Volume: 85

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Experimental Realization of Spin-1/2 Triangular-Lattice Heisenberg Antiferromagnet2012

    • Author(s)
      Y. Shirata, H. Tanaka, A. Matsuo and K. Kindo
    • Journal Title

      Phys. Rev. Lett

      Volume: 108 Issue: 5

    • DOI

      10.1103/physrevlett.108.057205

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Longitudinal magnetic excitation in KCuCl_3 studied by Raman scattering under hydrostatic pressures2012

    • Author(s)
      H. Kuroe, N. Takami, N. Niwa, T. Sekine, M. Matsumoto, F. Yamada, H. Tanaka and K. Takemura
    • Journal Title

      J. Phys : Conf. Ser

      Volume: 400 Issue: 3 Pages: 032042-4

    • DOI

      10.1088/1742-6596/400/3/032042

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Thermodynamic properties of quantum sine-Grordon spin chain system KCuGaF62012

    • Author(s)
      I.Umegaki, H.Tanaka, T.Ono, M.Oshikawa, K.Sakai
    • Journal Title

      Physical Review B

      Volume: 85 Issue: 14 Pages: 144423-19

    • DOI

      10.1103/physrevb.85.144423

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ferromagnetism induced in the anisotropic stacked kagome lattice antiferromagnet Cs2Cu3CeF122012

    • Author(s)
      T. Amemiya
    • Journal Title

      Phys. Rev. B

      Volume: 85 Issue: 14 Pages: 144409-19

    • DOI

      10.1103/physrevb.85.144409

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantum Magnetization Plateau in Spin-1 Triangular-Lattice Antiferromagnet Ba3NiSb2O92011

    • Author(s)
      Y.Shirata
    • Journal Title

      Journal of Physical Society of Japan

      Volume: 80 Issue: 9 Pages: 093702-093702

    • DOI

      10.1143/jpsj.80.093702

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Change in magnetic ground states in nonmagnetic-impurity-doped spin-gap systems TlCu_<1-x>Mg_xCl_3 using muon spin relaxation2011

    • Author(s)
      T. Suzuki, M. Yamada, Y. Ishii, I. Watanabe, T. Goto, H. Tanaka and K. Kubo
    • Journal Title

      Phys. Rev. B

      Volume: 83 Issue: 17

    • DOI

      10.1103/physrevb.83.174436

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Reply to Comment on 'Transition from Bose glass to a condensate of triplons in Tl_<1-x>K_xCuCl_3'2011

    • Author(s)
      F.Yamada, H.Tanaka, et al.
    • Journal Title

      Phys.Rev.B

      Volume: 83 Issue: 21

    • DOI

      10.1103/physrevb.83.216402

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Elementary excitations and specific heat in quantum sine-Gordon spin chain KCuGaF_62011

    • Author(s)
      I.Umegaki, H.Tanaka, et al.
    • Journal Title

      Physica E

      Volume: 43 Pages: 741-747

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic-Field Induced Quantum Phase Transitions in Triangular-Lattice Antiferromagnets2011

    • Author(s)
      T.Ono
    • Journal Title

      Journal of Physics : Conference Series

      Volume: 302 Pages: 012003-012003

    • DOI

      10.1088/1742-6596/302/1/012003

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ^<63, 65> Cu-NMR study on Mg-doped quantum spin system TlCu_<1-x> Mg_xCl_32011

    • Author(s)
      S Atarashi, T. Goto, M Yamada, F Yamada, A Oosawa, H Tanaka and T Suzuki
    • Journal Title

      J. Phys.: Conf. Ser

      Volume: 302 Pages: 12009-12009

    • DOI

      10.1088/1742-6596/302/1/012009

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Antiferromagnetic resonance modes for the S=1/2 kagome antiferromagnet Cs_2Cu_3SnF_<12>2011

    • Author(s)
      S.Sharmin, H.Tanaka, et al.
    • Journal Title

      J.Phys : Conf.Ser.

      Volume: 302 Pages: 012011-012011

    • DOI

      10.1088/1742-6596/302/1/012011

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ^<19>F-NMR Study on Antiferromagnetic Heisenberg Chain KCuGaF_62011

    • Author(s)
      Y.Mori, H.Tanaka, et al.
    • Journal Title

      J.Phys : Conf.Ser.

      Volume: 302 Pages: 012012-012012

    • DOI

      10.1088/1742-6596/302/1/012012

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effect of DM interaction in a quantum antiferromagnet on a deformed Kagome lattice R_2Cu_3SnF_<12>2011

    • Author(s)
      H. Tashiro, M. Nishiyama, A. Oyamada, T. Itou, S. Maegawa, M. Yano, T. Ono and H. Tanaka
    • Journal Title

      J.of Phys. : Conf. Ser.

      Volume: Vol.320 Pages: 12052-12052

    • DOI

      10.1088/1742-6596/320/1/012052

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] スピン1/2擬2次元正方格子反強磁性体Sr_2CuTeO_6におけるスピンフラストレーション効果2014

    • Author(s)
      古賀智之,栗田伸之,田中秀数
    • Organizer
      日本物理学会2014年年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Final Research Report
  • [Presentation] S=1/2 スピンダイマー系Ba_2CoSi_2O_6Cl_2の強磁場磁化過程と量子多体効果2013

    • Author(s)
      田 中秀数
    • Organizer
      東京大学物性研究所短期研究会「極限強磁場科学-場,物質,プローブのリンクから融合へ」
    • Place of Presentation
      東京大学物性研究所
    • Related Report
      2013 Final Research Report
  • [Presentation] S=1 三角格子反強磁性体 Ba_3NiSb_2O_9 の強磁場磁化過程2013

    • Author(s)
      田中秀数,松尾晶,金道浩一
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2013 Final Research Report
  • [Presentation] S=1/2 三角格子反強磁性体 Ba_3CoSb_2O_9 の磁場中量子相転移と磁気励起2013

    • Author(s)
      薄拓哉,栗田伸之,田中秀数,野尻浩之,田中卓也,松尾晶,金道浩一
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2013 Final Research Report
  • [Presentation] S=1/2 XY スピンダイマー系 Ba2CoSi2O6Cl2 の強磁場磁化過程2013

    • Author(s)
      田中秀数,松尾晶,金道浩一
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Related Report
      2013 Final Research Report
  • [Presentation] Experimental Realization of Spin-1/2 Triangular-Lattice Heisenberg Antiferromagnets2013

    • Author(s)
      H. Tanaka
    • Organizer
      Collaborative Conference on Material Research
    • Place of Presentation
      Jeju Island South Korea
    • Related Report
      2013 Annual Research Report 2013 Final Research Report
  • [Presentation] Ground States and Magnetic Excitations in S=1/2 Kagome-Lattice Antiferromagnets Rb_2Cu_3SnF_<12> and Cs_2Cu_3SnF_<12>2013

    • Author(s)
      H. Tanaka
    • Organizer
      JAEA Synchrotron Radiation Research Symposium "Magnetism in Quantum Beam Science"
    • Place of Presentation
      Harima Science Garden City, Hyogo, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] S=1/2スピンダイマー系Ba2CoSi2O6Cl2の強磁場磁化過程と量子多体効果2013

    • Author(s)
      田中秀数
    • Organizer
      東京大学物性研究所短期研究会「極限強磁場科学-場,物質,プローブのリンクから融合へ」
    • Place of Presentation
      東京大学物性研究所
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Ground States and Magnetic Excitations in S=1/2 Kagome-Lattice Antiferromagnets Rb2Cu3SnF12 and Cs2Cu3SnF122013

    • Author(s)
      H. Tanaka
    • Organizer
      JAEA Synchrotron Radiation Research Symposium&#8232;"Magnetism in Quantum Beam Science"
    • Place of Presentation
      Harima Science Garden City, Hyogo, Japan
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Ground states and magnetic excitations in a fluoride family of S=1/2 kagome-lattice antiferromagnet2012

    • Author(s)
      H. Tanaka
    • Organizer
      International Conference on Highly Frustrated Magnetism
    • Place of Presentation
      Hamilton, Canada
    • Related Report
      2013 Final Research Report 2012 Annual Research Report
  • [Presentation] Ordered Perovskite 型三角格子反強磁性体の量子磁性2012

    • Author(s)
      田中秀数
    • Organizer
      京都大学基礎物理学研究所研究会「量子スピン系の物理」
    • Place of Presentation
      京都大学基礎物理学研究所
    • Related Report
      2013 Final Research Report
  • [Presentation] フラストレーションの強いスピン系における量子多体効果の新展開2011

    • Author(s)
      田中秀数
    • Organizer
      日本物理学会
    • Place of Presentation
      富山大学(招待講演)
    • Year and Date
      2011-09-21
    • Related Report
      2011 Annual Research Report
  • [Presentation] フラストレーションの強いスピン系における量子多体効果の新展開2011

    • Author(s)
      田中秀数
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学五福キャンパス
    • Related Report
      2013 Final Research Report
  • [Remarks]

    • URL

      http://www.lee.phys.titech.ac.jp/index.html

    • Related Report
      2013 Final Research Report
  • [Remarks] 東京工業大学大学院理工学研究科物性物理学専攻 田中研究室

    • URL

      http://www.lee.phys.titech.ac.jp/index.html

    • Related Report
      2013 Annual Research Report
  • [Remarks]

    • URL

      http://www.lee.phys.titech.ac.jp/~tanakalb/tanakalb.html

    • Related Report
      2011 Annual Research Report

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Published: 2011-04-06   Modified: 2020-05-15  

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