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Highly-efficient two-photon reaction processes using entanglement of localized plasmons

Research Project

Project/Area Number 23246016
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied optics/Quantum optical engineering
Research InstitutionHokkaido University

Principal Investigator

SASAKI Keiji  北海道大学, 電子科学研究所, 教授 (00183822)

Co-Investigator(Renkei-kenkyūsha) FUJIWARA Hideki  北海道大学, 電子科学研究所, 准教授 (10374670)
TANAKA Yoshito  北海道大学, 電子科学研究所, 博士研究員 (50533733)
Project Period (FY) 2011-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥48,880,000 (Direct Cost: ¥37,600,000、Indirect Cost: ¥11,280,000)
Fiscal Year 2013: ¥11,050,000 (Direct Cost: ¥8,500,000、Indirect Cost: ¥2,550,000)
Fiscal Year 2012: ¥18,980,000 (Direct Cost: ¥14,600,000、Indirect Cost: ¥4,380,000)
Fiscal Year 2011: ¥18,850,000 (Direct Cost: ¥14,500,000、Indirect Cost: ¥4,350,000)
Keywords光プロセシング / 微小球共振器 / 顕微分光イメージング / 金属ナノ構造体 / 光局在 / 光反応増強 / 顕微分光イメージング / 金属ナノ構造体
Outline of Final Research Achievements

Utilizing the synergistic effect of the plasmonic enhancement and temporal entangled photons in plasmonic metal nanostructures, we have developed elemental technologies for the realization of highly-efficient two-photon reaction process. We performed theoretical evaluations of enhanced electric fields and found that further electric field enhancement could be expected by the periodic array of gold nano-gap structures. Then, we experimentally examined that two-photon excited fluorescence was enhanced by at least 5 order of magnitude in the periodic gold nanostructure. Furthermore, using a tapered-fiber coupled microsphere, we also developed a plasmonic-photonic hybrid system for highly-efficient plasmon excitation, which can focus an incident light to a small gold nanostructure with 100% efficiency. To experimentally verify the efficient plasmon excitation, we succeeded in the observation of SHG and two-photon excited fluorescence under a weak CW excitation (a few kW/cm2).

Report

(4 results)
  • 2014 Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (36 results)

All 2014 2013 2012 2011 Other

All Journal Article (16 results) (of which Peer Reviewed: 15 results,  Acknowledgement Compliant: 3 results) Presentation (18 results) (of which Invited: 5 results) Remarks (2 results)

  • [Journal Article] Efficient optical coupling into a single plasmonic nanostructure using a fiber-coupled microspherical cavity2014

    • Author(s)
      H. Takashima, K. Kitajima, Y. Tanaka, H. Fujiwara and K. Sasaki
    • Journal Title

      Phys. Rev. A

      Volume: 89(2) Issue: 2 Pages: 21801-21801

    • DOI

      10.1103/physreva.89.021801

    • NAID

      120005853093

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 酸化亜鉛サブマイクロメートル球状粒子を用いた新規ランダムレーザーの開発2014

    • Author(s)
      藤原英樹、煮雪亮、笹木敬司、辻剛志、石川善恵、越崎直人
    • Journal Title

      レーザー加工学会誌

      Volume: 21(1) Pages: 42-45

    • Related Report
      2013 Annual Research Report
  • [Journal Article] Two-photon excited fluorescence from a pseudoisocyanine-attached gold-coated tip via a thin tapered fiber under a weak continuous excitation2013

    • Author(s)
      Fang Ren, Hideaki Takashima, Yoshito Tanaka, Hideki Fujiwara, Keiji Sasaki
    • Journal Title

      Optics Express

      Volume: 21 Issue: 23 Pages: 27759-27769

    • DOI

      10.1364/oe.21.027759

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Near-field optical response of periodically arrayed plasmonic nanogap antennas2013

    • Author(s)
      Kyosuke Sakai, Kensuke Nomura, Yoshito Tanaka, and Keiji Sasaki
    • Journal Title

      Journal of Applied Physics

      Volume: 114 Issue: 2 Pages: 24-306

    • DOI

      10.1063/1.4813129

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nanostructured potential of optical trapping using a plasmonic potential of optical trapping using a plasmonic nanoblock pair2013

    • Author(s)
      Y. Tanaka, S. Kaneda and K. Sasaki
    • Journal Title

      Nano Lett.

      Volume: 13(5) Issue: 5 Pages: 2146-2150

    • DOI

      10.1021/nl4005892

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Nonlinear phenomena from a PIC attached gold tip using a plasmonic-whispering gallery mode hybrid system2013

    • Author(s)
      R. Fang, H. Takashima, Y. Tanaka, H. Fujiwara and K. Sasaki
    • Journal Title

      Proc. SPIE-Int.

      Volume: 8816 Pages: 881612-881612

    • DOI

      10.1117/12.2022626

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Low-threshold and quasi-single-mode random laser within a submicrometer-sized ZnO spherical particle film2013

    • Author(s)
      Hideki Fujiwara, Ryo Niyuki, Yoshie Ishikawa, Naoto Koshizaki, Takeshi Tsuji, Keiji Sasaki
    • Journal Title

      Appl. Phys. Lett

      Volume: 102 Issue: 6 Pages: 61110-61110

    • DOI

      10.1063/1.4792349

    • NAID

      120005228342

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Analysis of Trap State Dynamics of Single CdSe/ZnS Quantum Dots on an Indium Tin Oxide Thin Film with Applying External Electric Field2013

    • Author(s)
      Takashi Chiba, Jun Qi, Hideki Fujiwara, Keiji Sasaki
    • Journal Title

      J. Phys. Chem. C

      Volume: 117 Issue: 6 Pages: 2507-2510

    • DOI

      10.1021/jp306408s

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Second harmonic generation from the top of an Au-coated tip via a tapered fiber coupled microsphere resonator2012

    • Author(s)
      F. Ren, K. Kitajima, H. Takashima, H. Fujiwara and K. Sasaki
    • Journal Title

      Proc. SPIE

      Volume: 8463

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nanoscale interference patterns of gap-mode multipolar plasmonic fields2012

    • Author(s)
      Yoshito Tanaka, Akio Sanada and Keiji Sasaki
    • Journal Title

      Scientific Reports

      Volume: 2 Issue: 1 Pages: 764-764

    • DOI

      10.1038/srep00764

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental evaluation of diffusion constant in a thin polymer film by triplet lifetime analysis of single molecules2012

    • Author(s)
      Takashi Chiba, Hideki Fujiwara, Jun-ichi Hotta, Shigeki Takeuchi, Keiji Sasaki
    • Journal Title

      Journal of Photochemistry and Photobiology A: Chemistry

      Volume: 238 Pages: 24-28

    • DOI

      10.1016/j.jphotochem.2012.04.013

    • NAID

      120005946705

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Efficient optical trapping using small arrays of plasmonic nanoblock pairs2012

    • Author(s)
      Yoshito Tanaka, Keiji Sasaki
    • Journal Title

      Applied Physics Letters

      Volume: 100 Issue: 2 Pages: 21102-21102

    • DOI

      10.1063/1.3675550

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Optical trapping through the localized surfaceplasmon resonance of engineered gold nanoblock pairs2011

    • Author(s)
      Y. Tanaka
    • Journal Title

      Opt. Exp.

      Volume: 19(18) Pages: 17462-17468

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temporal response analysis of trap states of single CdSe/ZnS quantum dots on a thin metal substrate2011

    • Author(s)
      H. Fujiwara
    • Journal Title

      J. Photochem. Photobiol., A

      Volume: 221(2-3) Pages: 160-163

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Detection of superposition in the orbital angular momentum of photons without excess components and its application in the verification of non-classical correlation2011

    • Author(s)
      Y.Miyamoto, D.Kawase, M.Takeda, K.Sasaki S.Takeuchi
    • Journal Title

      Journal of Optics

      Volume: Vol.13 Issue: 6 Pages: 064027-064027

    • DOI

      10.1088/2040-8978/13/6/064027

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct imaging of nanogap-mode plasmon-resonant fields2011

    • Author(s)
      Y. Tanaka
    • Journal Title

      Opt. Exp.

      Volume: 19(8) Pages: 7726-7733

    • NAID

      120003025355

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] Two-photon excited fluorescence from a PIC-attached Au-coated tip via a thin tapered fiber under a weak CW excitation2013

    • Author(s)
      R. Fang, H. Takashima, Y. Tanaka, H. Fujiwara and K. Sasaki
    • Organizer
      THE 14th RIES-Hokudai International Symposium 網 [mou]
    • Place of Presentation
      Chateraise Gateaux Kingdom Sapporo(Sapporo,Hokkaido)
    • Year and Date
      2013-12-11
    • Related Report
      2013 Annual Research Report
  • [Presentation] Multipole Plasmons Excited by Optical Vortex Beams2013

    • Author(s)
      K. Sakai, K. Nomura, T. Yamamoto, Y. Tanaka and K. Sasaki
    • Organizer
      THE 14th RIES-Hokudai International Symposium 網 [mou]
    • Place of Presentation
      Chateraise Gateaux Kingdom Sapporo(Sapporo,Hokkaido)
    • Year and Date
      2013-12-11
    • Related Report
      2013 Annual Research Report
  • [Presentation] Nonlinear phenomena from a PIC-attached gold tip using a plasmonic-whispering gallery mode hybrid system2013

    • Author(s)
      R. Fang, H. Takashima, Y. Tanaka, H. Fujiwara and K. Sasaki
    • Organizer
      SPIE Optics & Photonics 2013
    • Place of Presentation
      San Diego(USA)
    • Year and Date
      2013-08-29
    • Related Report
      2013 Annual Research Report
  • [Presentation] Interference of Whispering Gallery Modes in Photonic and Plasmonic Microcavities2013

    • Author(s)
      K. Sasaki
    • Organizer
      PIERS2013 ( Progress in Electromagnetics Research Symposium) Stockholm
    • Place of Presentation
      Stockholm( Sweden)
    • Year and Date
      2013-08-15
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Multipole Nanodisk Plasmons Excited by Cylindrical Vector Beams2013

    • Author(s)
      K. Sakai, T. Yamamoto, K. Nomura, Y. Tanaka and K. Sasaki
    • Organizer
      PIERS2013 ( Progress in Electromagnetics Research Symposium) Stockholm
    • Place of Presentation
      Stockholm(Sweden)
    • Year and Date
      2013-08-15
    • Related Report
      2013 Annual Research Report
  • [Presentation] Multipolar Dark-Mode Plasmon Excitation with Laguerre-Gaussian Beams2013

    • Author(s)
      K. Sasaki
    • Organizer
      ICP 2013( The 26th International Conference on Photochemistry)
    • Place of Presentation
      Leuven( Belgium)
    • Year and Date
      2013-07-23
    • Related Report
      2013 Annual Research Report
  • [Presentation] Photon Manipulation with Plasmonic Nanostructures2013

    • Author(s)
      K. Sasaki
    • Organizer
      ICP 2013 (Pre-conference: Conference on Plasmonics )
    • Place of Presentation
      Leuven(Belgium)
    • Year and Date
      2013-07-20
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Direct imaging of localized fields in a gold nanostructure using a scattering-type near-field microscope2013

    • Author(s)
      H. Fujiwara, Y. Tanaka and K. Sasaki
    • Organizer
      CLEO-PR & OECC/PS 2013
    • Place of Presentation
      Kyoto International Conference Center(Sakyo-ku, Kyoto)
    • Year and Date
      2013-07-04
    • Related Report
      2013 Annual Research Report
  • [Presentation] Realization of Single-Mode Random Lasing Within a Zinc Oxide Nanoparticle Film2013

    • Author(s)
      K. Sasaki
    • Organizer
      CLEO-PR & OECC/PS 2013
    • Place of Presentation
      Kyoto International Conference Center(Sakyo-ku, Kyoto)
    • Year and Date
      2013-07-03
    • Related Report
      2013 Annual Research Report
  • [Presentation] Quasi-single mode random laser2013

    • Author(s)
      H. Fujiwara, R. Niyuki, T. Tsuji, Y. Ishikawa, N. Koshizaki and K. Sasaki
    • Organizer
      Collaborative Conference on Materials Research (CCMR) 2013
    • Place of Presentation
      Jeju(Korea)
    • Year and Date
      2013-06-27
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Nanoscale Photon Shaping with Engineered Plasmonic Materials2013

    • Author(s)
      K. Sasaki and Y. Tanaka
    • Organizer
      Collaborative Conference on Materials Research (CCMR) 2013
    • Place of Presentation
      Jeju(Korea)
    • Year and Date
      2013-06-26
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Random Lasing at a Defect Particle Intentionally Embedded in a ZnO Nanoparticle Film2013

    • Author(s)
      K. Sasaki, H. Fujiwara, R. Niyuki and T. Tsuji
    • Organizer
      The Third International Workshop on Microcavities and Their Applications
    • Place of Presentation
      Beijing(China)
    • Year and Date
      2013-05-29
    • Related Report
      2013 Annual Research Report
  • [Presentation] Photpn Localization with Plasmonic WGM Cavities2013

    • Author(s)
      K. Sasaki
    • Organizer
      The Third International Workshop on Microcavities and Their Applications
    • Place of Presentation
      Beijing(China)
    • Year and Date
      2013-05-28
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Highly efficient photon coupling into a plasmonic nanostructure using a fiber-coupled microspherical cavity2012

    • Author(s)
      K. Sasaki
    • Organizer
      2012 SPIE Photonics West
    • Place of Presentation
      The Moscone Center, San Francisco, USA
    • Related Report
      2011 Annual Research Report
  • [Presentation] Trap state lifetime analysis of single CdSe/ZnS quantum dots on a thin conductive film2012

    • Author(s)
      H. Fujiwara
    • Organizer
      2012 SPIE Photonics West
    • Place of Presentation
      The Moscone Center, San Francisco, USA
    • Related Report
      2011 Annual Research Report
  • [Presentation] Nano-optical trapping of small particles with plasmonic nanostructures2011

    • Author(s)
      A. Sanada
    • Organizer
      12th RIES-Hokudai International Symposium "KAN "
    • Place of Presentation
      Chateraise Gateaux Kingdom Sapporo, Japan
    • Related Report
      2011 Annual Research Report
  • [Presentation] Efficient excitation of localized plasmons via a tapered fiber coupled microresonator2011

    • Author(s)
      K. Kitajima
    • Organizer
      12th RIES-Hokudai International Symposium "KAN "
    • Place of Presentation
      Chateraise Gateaux Kingdom Sapporo, Japan
    • Related Report
      2011 Annual Research Report
  • [Presentation] Direct Observation of Nanogap-Mode Plasmon-Resonant Fields2011

    • Author(s)
      Y.Tanaka
    • Organizer
      Nanoplasmonic Sensors and Spectroscopy 2011
    • Place of Presentation
      Chalmers Johanneberg Campus, Sweden
    • Related Report
      2011 Annual Research Report
  • [Remarks] 光システム物理研究分野 笹木研究室ホームページ

    • URL

      http://optsys.es.hokudai.ac.jp/~optsys/

    • Related Report
      2013 Annual Research Report
  • [Remarks] 北海道大学電子科学研究所笹木研究室

    • URL

      http://optsys.es.hokudai.ac.jp/~optsys/index.html

    • Related Report
      2012 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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