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Study on high temperature radiolysis of water relevant to water chemistry

Research Project

Project/Area Number 23246168
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionThe University of Tokyo

Principal Investigator

KATSUMURA Yosuke  東京大学, 工学(系)研究科(研究院), 教授 (70111466)

Co-Investigator(Kenkyū-buntansha) KUDO Hisaaki  東京大学, 大学院工学系研究科, 教授 (00334318)
MUROYA Yusa  大阪大学, 産業科学研究所, 准教授 (40334320)
LIN Mingzhang  日本原子力研究開発機構, 原子力科学研究所, 任期付研究員 (50465994)
YAMASHITA Shinichi  東京大学, 大学院工学系研究科, 助教 (20511489)
Project Period (FY) 2011-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥28,860,000 (Direct Cost: ¥22,200,000、Indirect Cost: ¥6,660,000)
Fiscal Year 2014: ¥5,980,000 (Direct Cost: ¥4,600,000、Indirect Cost: ¥1,380,000)
Fiscal Year 2013: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2012: ¥5,850,000 (Direct Cost: ¥4,500,000、Indirect Cost: ¥1,350,000)
Fiscal Year 2011: ¥11,440,000 (Direct Cost: ¥8,800,000、Indirect Cost: ¥2,640,000)
Keywords高温水化学 / パルスラジオリシス / 超臨界水 / 10B(n,α)7Li反応 / モンテカルロシミュレーション / 水分解生成物 / G値 / 水化学 / 水の放射線分解 / モンテカルロ計算 / 水和電子 / OHラジカル / スパー反応 / 高温水・超臨界水
Outline of Final Research Achievements

The coolant water in nuclear reactor is exposed to intense radiations such as fast neutrons and gamma-rays at high temperatures and decomposed, which is one of the important factors to control the chemical conditions of the coolant water. Therefore, understanding of water radiolysis at elevated temperatures is inevitably important not only technologically but also scientifically. In the present research project, we have picked up three subjects: (1) ultrafast pulse radiolysis, (2) Inhibition of H2 evolution via H2 addition in high LET radiolysis of water, and (3) Monte Carlo simulation of water radiolysis by 10B(n,α)7Li reaction.

Report

(5 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (32 results)

All 2015 2014 2013 2012 2011

All Journal Article (9 results) (of which Peer Reviewed: 9 results) Presentation (23 results) (of which Invited: 1 results)

  • [Journal Article] Sequential radiation chemical reactions in aqueous bromide soluteons: pulse radiolysis experiment and spur model simulation2015

    • Author(s)
      S. Yamashita, K. Iwamatsu, Y. Maehashi, M. Taguchi, K. Hata, Y. Muroya and Y. Katsumura
    • Journal Title

      RSC Adv.

      Volume: 5 Pages: 25877-25886

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Simulation of the inhibition of water α-radiolysis via H2 addition2014

    • Author(s)
      P. Lertnaisat, Y. Katsumura, S. Mukai, R. Umehara, Y. Shimizu and M. Suzuki
    • Journal Title

      J. Nucl. Sci. and Technol.

      Volume: 51 Issue: 9 Pages: 1087-1095

    • DOI

      10.1080/00223131.2014.907548

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Time-dependent yield of the hydrated electron in subcritical and supercritical water studied by ultrafast pulse radiolysis and Monte-Carlo simulation.2012

    • Author(s)
      Y. Muroya, S. Sanguanmith, J. Meesungnoen, M.Z. Lin, Y. Yan, Y. Katsumura, J.-P. Jay-Gerin
    • Journal Title

      Phys. Chem. Chem. Phys.

      Volume: 14 Issue: 41 Pages: 14325-14333

    • DOI

      10.1039/c2cp42260c

    • Related Report
      2012 Annual Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] On the spur lifetime and its temperature dependence in the low linear energy transfer radiolysis of water.2012

    • Author(s)
      S. Sanguanmith, J. Meesungnoen, Y. Muroya, M. Lin, Y. Katsumura, J.-P. Jay-Gerin
    • Journal Title

      Phys. Chem. Chem. Phys.

      Volume: 14 Issue: 48 Pages: 16731-16736

    • DOI

      10.1039/c2cp42826a

    • Related Report
      2012 Annual Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mechanism of radiation-induced reactions in aqueous solution of coumarin-3-carboxylic acid: Effects of concentration, gas and additive on fluorescent product yield2012

    • Author(s)
      Yamashita, S., Baldacchino, G., Maeyama, T., Taguchi, M., Muroya, Y., Lin, M. Z., Kimura, A., Murakami, T., Katsumura, Y.
    • Journal Title

      Free Radical Research

      Volume: 46 Pages: 861-871

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temperature Dependent of Br-, Br2-. and Br3- Absorption Spectra in Aqueous Solutions2011

    • Author(s)
      M. Lin, P. Archirel, N. Thi Van-Oanh, Y. Muroya, H. Fu, Y. Yan, R. Nagaishi, Y. Kumagai, Y. Katsumura, M. Mostafavi
    • Journal Title

      J. Phys. Chem. A

      Volume: 115 Issue: 17 Pages: 4241-4247

    • DOI

      10.1021/jp1123103

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temperature dependence of the Fricke dosimeter and spur expansion time in the low-LET high-temperature radiolysis of water up to 350°C: A Monte-Carlo simulation study2011

    • Author(s)
      S. Sanguanmith, Y. Muroya, T. Tippayamontri, J. Meesungnoen, M. Lin, Y. Katsumura and J-P. Jay-Gerin
    • Journal Title

      Phys. Chem. Chem. Phys.

      Volume: 13 Issue: 22 Pages: 10690-10698

    • DOI

      10.1039/c1cp20293f

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Low-liner energy transfer radiolysis of liquid water at elevated temperatures up to 350°C: Monte-Carlo simulations2011

    • Author(s)
      S. Sanguanmith, Y. Muroya, J. Meesungnoen, M. Lin, Y. Katsumura, L. M. Kohan, D. A. Guzonus, C. R. Stuart, J.-P. Jay-Gerin
    • Journal Title

      Chem. Phys. Lett.

      Volume: 508 Issue: 4-6 Pages: 224-230

    • DOI

      10.1016/j.cplett.2011.04.059

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Time-Dependent Radiolytic Yield of OH Radical Studied by Picosecond Pulse Radiolysis2011

    • Author(s)
      A. K. El Omar, U. Schmidhammer, P. Jeunesse, J-P. Larbre, M. Lin, Y. Muroya, Y. Katsumura, P. Pernot and M. Mostafavi
    • Journal Title

      J. Phys. Chem. A

      Volume: 115 Issue: 44 Pages: 12212-12216

    • DOI

      10.1021/jp208075v

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] Effects of Dissolved Species on Radiolysis of Diluted Seawater2014

    • Author(s)
      Kuniki Hata, Satoshi Hanawa, Shigeki Kasahara, Takafumi Motooka, Takashi Tsukada,Yusa Muroya, Shinichi Yamashita, Yosuke Katsumura
    • Organizer
      NPC2014
    • Place of Presentation
      ロイヤル札幌ホテル、北海道
    • Year and Date
      2014-10-26 – 2014-10-31
    • Related Report
      2014 Annual Research Report
  • [Presentation] Sequential Radiation Chemical Reactions in Aqueous2014

    • Author(s)
      Kazuhiro IWAMATSU, Shinichi YAMASHITA, Yuki MAEHASHI, Mitsumasa TAGUCHI, Yusa MUROYA, Kuniki HATA, and Yosuke KATSUMURA
    • Organizer
      5th Asia Pacific Symposium on Radiation Chemistry
    • Place of Presentation
      東京大学、東京
    • Year and Date
      2014-09-08 – 2014-09-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] The Important Role of H + H2O → OH + H2 Reaction in2014

    • Author(s)
      Phantira Lertnaisat,Yosuke Katsumura,Satoru Mukai,Ryuji Umehara,Yuichi Shimizu,Masaru Suzuki
    • Organizer
      5th Asia Pacific Symposium on Radiation Chemistry
    • Place of Presentation
      東京大学、東京
    • Year and Date
      2014-09-08 – 2014-09-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] 高温高圧水中における水和電子の時間挙動と反応性2014

    • Author(s)
      鳩本大祐、室屋 裕佐、勝村庸介、山下真一、古澤孝弘
    • Organizer
      第51回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学、東京
    • Year and Date
      2014-07-07 – 2014-07-09
    • Related Report
      2014 Annual Research Report
  • [Presentation] 沸騰水の放射線分解2014

    • Author(s)
      勝村庸介、楊爽、山下真一、松浦千尋、田口光正
    • Organizer
      第51回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学、東京
    • Year and Date
      2014-07-07 – 2014-07-09
    • Related Report
      2014 Annual Research Report
  • [Presentation] 超臨界水の放射線分解反応機構2014

    • Author(s)
      室屋裕佐、鳩本大祐、勝村庸介、林 銘章、山下真一、Jintana Meesungnoen、Jean-Paul Jay-Gerin、古澤孝弘
    • Organizer
      第51回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学、東京
    • Year and Date
      2014-07-07 – 2014-07-09
    • Related Report
      2014 Annual Research Report
  • [Presentation] モンテカルロ計算による10B(n,α)7Li反応による水分解初期収量評価II2014

    • Author(s)
      ラートナイサット パンティラー、勝村庸介、メースングノエンジンタナ、ジェイジェラン ジャンポール、向井 悟、梅原隆二、志水雄一、鈴木 将
    • Organizer
      第51回アイソトープ・放射線研究発表会
    • Place of Presentation
      東京大学、東京
    • Year and Date
      2014-07-07 – 2014-07-09
    • Related Report
      2014 Annual Research Report
  • [Presentation] Current Understanding of Water Radiolysis at Elevated Temperatures2013

    • Author(s)
      Yosuke Katsumura, Phantira Lertnaisat
    • Organizer
      Symposium on Water Chemistry and Corrosion of NuclearPower Plants in Asia,2013
    • Place of Presentation
      Hotel Windsor,Taiching,Taiwan
    • Year and Date
      2013-10-14 – 2013-10-17
    • Related Report
      2013 Annual Research Report
  • [Presentation] Radiolysis of Water at High Temperature and Pressure Conditions2013

    • Author(s)
      Yusa Muroya, Yosuke Katsumura, Mingzhang Kin, Jean-Paul Jay-Gerin, Takahiro Kozawa
    • Organizer
      Symposium on Water Chemistry and Corrosion of NuclearPower Plants in Asia,2013
    • Place of Presentation
      Hotel Windsor,Taiching,Taiwan
    • Year and Date
      2013-10-14 – 2013-10-17
    • Related Report
      2013 Annual Research Report
  • [Presentation] Pulse Radiolysis Studies on High Temperature Water:the Behavious of Hydroxyl Radical2013

    • Author(s)
      Mingzhang Lin, Yosuke Katsumura, Yusa Muroya, Mehran Mostafavi, Jean-Paul Jay-Gerin
    • Organizer
      Symposium on Water Chemistry and Corrosion of NuclearPower Plants in Asia,2013
    • Place of Presentation
      Hotel Windsor,Taiching,Taiwan
    • Year and Date
      2013-10-14 – 2013-10-17
    • Related Report
      2013 Annual Research Report
  • [Presentation] Inter-comparison of Primary G-values, and reaction sets and rates constant of water radiolysis for computer simulation2013

    • Author(s)
      Phantira Lertnaisat,Yosuke Katsumura,Satoru Mukai,Ryuji Umehara,Yuichi Shimizu,Masaru Suzuki
    • Organizer
      第56回放射線化学討論会
    • Place of Presentation
      広島大学、広島
    • Year and Date
      2013-09-08 – 2013-09-11
    • Related Report
      2013 Annual Research Report
  • [Presentation] これからの水化学に期待する2012

    • Author(s)
      勝村庸介
    • Organizer
      第2回軽水炉燃料・材料・水化学3部会合同夏期セミナー
    • Place of Presentation
      島根・しんじ湖温泉
    • Related Report
      2012 Annual Research Report
  • [Presentation] Computer Modeling of Inhibition of α-radiolysis of water by H2 addition2012

    • Author(s)
      Phantira Lertnasiat、
    • Organizer
      Nuclear Plant Chemistry Conference 2012
    • Place of Presentation
      France・Paris
    • Related Report
      2012 Annual Research Report
  • [Presentation] 高温水の放射線化学反応初期過程:水素の発生機構2012

    • Author(s)
      室屋裕佐、勝村庸介、林銘章、Sunuchakan Sanguanmith、Jintana Meesungnoen、Jean-Paul Jay-Gerin、古澤孝弘
    • Organizer
      第55回放射線化学討論会
    • Place of Presentation
      宮城・モンタナリゾート岩沼
    • Related Report
      2012 Annual Research Report
  • [Presentation] 超臨界ピコ秒パルスラジオリシスの改良2012

    • Author(s)
      室屋裕佐、勝村庸介、林銘章、Jean-Paul Jay-Gerin、古澤孝弘
    • Organizer
      第55回放射線化学討論会
    • Place of Presentation
      宮城・モンタナリゾート岩沼
    • Related Report
      2012 Annual Research Report
  • [Presentation] Radiation Chemistry of Water – Past, Present and Future2012

    • Author(s)
      Y. Katsumura
    • Organizer
      The 4th Asia Pacific Symposium on Radiation Chemistry
    • Place of Presentation
      Huangshan, China
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Radiolysis of water at high temperature and high pressure- electron thermalization distance and spur diffusion reaction2012

    • Author(s)
      Yusa MUROYA, Mingzhang LIN, Sunuchakan SANGUANMITH,Jintana MEESUNGNOEN, Jean-Paul JAY-GERIN, Yosuke KATSUMURA
    • Organizer
      ワークショップ「原子力における放射線効果」
    • Place of Presentation
      東京大学、東京都
    • Related Report
      2011 Annual Research Report
  • [Presentation] Recent Progresses in the Studies on Water Radiolysis2012

    • Author(s)
      Mingzhang LIN, Yosuke KATSUMURA, Yusa MUROYA, Jintana MEESUNGNOEN, Mehran MOSTAFAVI, Jean-Paul JAY-GERIN
    • Organizer
      ワークショップ「原子力における放射線効果」
    • Place of Presentation
      東京大学、東京都
    • Related Report
      2011 Annual Research Report
  • [Presentation] Inhibition of radiolysis of water by H2 addition-II2012

    • Author(s)
      Phantira Lertnaisat, Yosuke Katsumura, Satoru Mukai, Ryuji Umehara, Yuichi Shimizu, Masaru Suzuki
    • Organizer
      ワークショップ「原子力における放射線効果」
    • Place of Presentation
      東京大学、東京都
    • Related Report
      2011 Annual Research Report
  • [Presentation] Direct measurement of hydroxyl radical by picosecond pulse radiolysis2011

    • Author(s)
      M. Lin, Y. Muroya, Y. Katsumura, A. K. El Omar, M. Mostafavi, J. Meesungneon,J.-P. jay-Gerin
    • Organizer
      第54回放射線化学討論会
    • Place of Presentation
      大阪大学、大阪市
    • Related Report
      2011 Annual Research Report
  • [Presentation] 高温水中における水和電子の拘束時間挙動:熱化距離およびスパー反応2011

    • Author(s)
      室屋裕佐、林銘章、Sunnuchakan Sanguanmith、Jintana Meesungnoen、Jean-Paul Jay-Gerin、勝村庸介
    • Organizer
      第54回放射線化学討論会
    • Place of Presentation
      大阪大学、大阪市
    • Related Report
      2011 Annual Research Report
  • [Presentation] Computer modeling of inhibition of α-radiolysis of water by H2 addition2011

    • Author(s)
      P. Lertnaisat, Y. Tamoto, Y. Katsumura, S. Mukai, R. Umehara,Y. Shimizu, M. Suzuki
    • Organizer
      第54回放射線化学討論会
    • Place of Presentation
      大阪大学、大阪市
    • Related Report
      2011 Annual Research Report
  • [Presentation] モンテカルロ法による高温高圧水の放射線分解反応シミュレーション2011

    • Author(s)
      室屋裕佐、林銘章、Sunnuchakan Sanguanmith、Jintana Meesungnoen、Jean-Paul Jay-Gerin、勝村庸介
    • Organizer
      第54回放射線化学討論会
    • Place of Presentation
      大阪大学、大阪市
    • Related Report
      2011 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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