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Near-infrared nano-spectroscopy and emission energy control of semiconductor quantum dots using a phase-change mask method

Research Project

Project/Area Number 23360141
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionKeio University

Principal Investigator

SAIKI Toshiharu  慶應義塾大学, 理工学部, 教授 (70261196)

Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥19,110,000 (Direct Cost: ¥14,700,000、Indirect Cost: ¥4,410,000)
Fiscal Year 2013: ¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2012: ¥6,630,000 (Direct Cost: ¥5,100,000、Indirect Cost: ¥1,530,000)
Fiscal Year 2011: ¥7,280,000 (Direct Cost: ¥5,600,000、Indirect Cost: ¥1,680,000)
Keywords量子ドット / 相変化材料 / 近接場光学 / 応力光学 / 近赤外分光 / ナノ分光
Research Abstract

We have proposed a method to achieve near-field imaging spectroscopy of single semiconductor quantum dots with high sensitivity by using an optical mask layer of a phase-change material. An amorphous aperture allows imaging spectroscopy with high spatial resolution and high collection efficiency. We present numerical simulation and experimental result that show the effectiveness of this technique.
Inspired by this optical mask effect, a new approach which can precisely control the emission energy of semiconductor quantum dots has been proposed. This method uses the volume expansion of a phase-change material upon amorphization, which allows reversible emission energy tuning of quantum dots. We calculated the stress and energy shift distribution using finite element method. Simulation result is accompanied by two experimental studies; two-dimensional PL intensity mapping and an analysis on the relationship between PL intensity ratio and energy shift were performed.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (44 results)

All 2014 2013 2012 2011 Other

All Journal Article (8 results) (of which Peer Reviewed: 8 results,  Open Access: 1 results) Presentation (34 results) (of which Invited: 7 results) Remarks (2 results)

  • [Journal Article] Redshifted and blueshifted photoluminescence emission of InAs/InP quantum dots upon amorphization of phase change material2014

    • Author(s)
      Nurrul Syafawati Binti Humam, Y. Sato, M. Takahashi, S. Kanazawa, N. Tsumori, P. Regreny, M. Gendry, and T. Saiki
    • Journal Title

      Opt. Expr

      Volume: 22 Issue: 12 Pages: 14830-14839

    • DOI

      10.1364/oe.22.014830

    • Related Report
      2013 Final Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Near-infrared nano-spectroscopy and emission energy control of semiconductor quantum dots using a phase-change material2013

    • Author(s)
      N. Tsumori, M. Takahashi, Nurrul Syafawati Humam, P. Regreny, M. Gendry, and T. Saiki
    • Journal Title

      J. Phys. : Conf. Series

      Volume: 471 Pages: 012007-012007

    • DOI

      10.1088/1742-6596/471/1/012007

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Local control of emission energy of semiconductor quantum dots using volume expansion of a phase-change material2013

    • Author(s)
      M. Takahashi, Nurrul Syafawati Humam, N. Tsumori, T. Saiki, P. Regreny, and M. Gendry
    • Journal Title

      Appl. Phys. Lett

      Volume: 102 Issue: 9

    • DOI

      10.1063/1.4795291

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dependence of Switching Characteristics of GeTe/Sb2Te3 Superlattice Phase Change Materials on Electric Pulse Width and Optical Polarization Direction2013

    • Author(s)
      T. Shintani and T. Saiki
    • Journal Title

      Applied Physics Express

      Volume: 6 Issue: 11 Pages: 111401-111401

    • DOI

      10.7567/apex.6.111401

    • NAID

      210000136850

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Switching of localized surface plasmon resonance of gold nanoparticles on a GeSbTe film mediated by nanoscale phase change and modification of surface morphology2013

    • Author(s)
      T. Hira, T. Homma, T. Uchiyama, K. Kuwamura, and T. Saiki
    • Journal Title

      Applied Physics Letters

      Volume: 103 Issue: 24

    • DOI

      10.1063/1.4841975

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Near-Infrared Nano-Imaging Spectroscopy of Semiconductor Quantum Dots Using a Phase Change Mask Layer2012

    • Author(s)
      N.Tsumori
    • Journal Title

      Applied Physics Letters

      Volume: 100 Issue: 6

    • DOI

      10.1063/1.3683537

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Lateral Variation of Interface Disorder in the Wetting Layer on the Formation of InAs/InP Quantum Dots Visualized by Near-Field Imaging Spectroscopy2012

    • Author(s)
      H. Tojinbara et al.
    • Journal Title

      JOURNAL OF NANOPHOTONICS

      Volume: 6 Issue: 1 Pages: 063521-063521

    • DOI

      10.1117/1.jnp.6.063521

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental study of near-field light collection efficiency of aperture fiber probe at near-infrared wavelengths2011

    • Author(s)
      N.Tsumori, M.Takahashi, T.Saiki, Y.Sakuma
    • Journal Title

      Applied Optics

      Volume: 50 Issue: 29 Pages: 5710-5713

    • DOI

      10.1364/ao.50.005710

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] ドーナツ状結晶化を併用したサブ回折限界アモルファス領域の形成2014

    • Author(s)
      金澤翔平, 津守伸宏, ヌルーシャファワティビンティフマム, 佐藤悠, 斎木敏治
    • Organizer
      第14回 レーザー学会東京支部研究会
    • Place of Presentation
      東海大学高輪キャンパス(東京)
    • Related Report
      2013 Annual Research Report
  • [Presentation] アモルファス/結晶周期構造形成の解明に向けたGeTeにおける結晶化過程の観察2014

    • Author(s)
      森本悠介, 勝又洋介, 森田貴紀, 新谷俊通, 斎木敏治
    • Organizer
      第14回 レーザー学会東京支部研究会
    • Place of Presentation
      東海大学高輪キャンパス(東京)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 相変化材料による金ナノロッドプラズモン共鳴スイッチングの近赤外分光計測2014

    • Author(s)
      木原雄也, 平敬, 内山貴之, 鍬村健太, 矢渡将, 新谷俊通, 斎木敏治
    • Organizer
      第14回 レーザー学会東京支部研究会
    • Place of Presentation
      東海大学高輪キャンパス(東京)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 相変化材料と相互作用するプラズモン粒子系へのセルオートマトン機能の実装2014

    • Author(s)
      矢渡将, 内山貴之, 鍬村健太, 木原雄也, 平敬, 斎木敏治
    • Organizer
      第14回 レーザー学会東京支部研究会
    • Place of Presentation
      東海大学高輪キャンパス(東京)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Active nanophotonics using phase change materials and its possible applications to brain-inspired optical memory2014

    • Author(s)
      T. Saiki
    • Organizer
      UK-Japan Workshop on Photonics and Metamaterials Research
    • Place of Presentation
      英国大使館(東京)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Improvement of Spatial Resolution of Nano Spectroscopy Imaging using Phase-Change Mask2013

    • Author(s)
      Y. Sato and T. Saiki
    • Organizer
      25th Symposium on Phase Change Oriented Science (PCOS 2013)
    • Place of Presentation
      Sendai, Japan
    • Year and Date
      2013-11-28
    • Related Report
      2013 Final Research Report
  • [Presentation] Redshifted and Blueshifted Photoluminescence Spectra of InAs/InP Quantum Dots upon Amorphization of Phase Change Material2013

    • Author(s)
      Nurrul Syafawati Binti Humam and T. Saiki
    • Organizer
      25th Symposium on Phase Change Oriented Science (PCOS 2013)
    • Place of Presentation
      Sendai, Japan
    • Year and Date
      2013-11-28
    • Related Report
      2013 Final Research Report
  • [Presentation] Spectroscopy and Emission Energy Control of Individual InAs Quantum Dots Using a Phase Change Optical Mask2013

    • Author(s)
      N. Tsumori and T. Saiki
    • Organizer
      Collaborative Conference on 3D & Materials Research (CC3DMR 2013)
    • Place of Presentation
      Jeju, Korea
    • Year and Date
      2013-06-25
    • Related Report
      2013 Final Research Report
  • [Presentation] Visualization of local perturbation in GaAs quantum dot systems by near-field optical wavefunction mapping2013

    • Author(s)
      T. Saiki
    • Organizer
      18th Microscopy of Semiconducting Materials Meeting (MSMXVIII)
    • Place of Presentation
      Oxford, England
    • Year and Date
      2013-04-10
    • Related Report
      2013 Final Research Report
  • [Presentation] Visualization of local perturbation in GaAs quantum dot systems by near‐field optical wavefunction mapping2013

    • Author(s)
      T. Saiki
    • Organizer
      18th Microscopy of Semiconducting Materials Meeting (MSMXVIII)
    • Place of Presentation
      オックスフォード(イギリス)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Ultrafast nanoscale optical processes in chalcogenide phase change materials and their application to brain-inspired memory devices2013

    • Author(s)
      T. Saiki
    • Organizer
      Fundamentals of Laser Assisted Micro– and Nanotechnologies (FLAMN-13)
    • Place of Presentation
      サンクトペテルブルク(ロシア)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Spectroscopy and Emission Energy Control of Individual InAs Quantum Dots Using a Phase Change Optical Mask2013

    • Author(s)
      N. Tsumori, M. Takahashi, Nurrul Syafawati Humam, Y. Satoh, and T. Saiki
    • Organizer
      Collaborative Conference on 3D & Materials Research (CC3DMR 2013)
    • Place of Presentation
      チェジュ(韓国)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Active nanophotonics using phase change materials and its possible applications to neuron-inspired devices2013

    • Author(s)
      T. Saiki
    • Organizer
      The 9th Asia-Pacific Conference on Near-field Optics (APNFO2013)
    • Place of Presentation
      シンガポール(シンガポール)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] フェムト秒・ナノスケール相変化がもたらす時空間相関と記憶機能2013

    • Author(s)
      斎木敏治
    • Organizer
      ナノフォトニクスシンポジウム・ナノフォトニクスにおける複雑性・多様性と機能
    • Place of Presentation
      慶應義塾大学(横浜)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Nanophotonic Switching with Chalcogenide Phase Change Materials and its Application to Brain-Inspired Optical Memory2013

    • Author(s)
      T. Saiki
    • Organizer
      International Symposium on Optical Memory (ISOM2013)
    • Place of Presentation
      インチョン(韓国)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Electric and Optical Studies on Non-thermal Recording Mechanism of GeTe/Sb2Te3 Superlattice Phase Change Material2013

    • Author(s)
      T. Shintani and T. Saiki
    • Organizer
      12th European/Phase Change and Ovonics Symposium (E/PCOS2013)
    • Place of Presentation
      ベルリン(ドイツ)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Self-organization of a fringe pattern between amorphous and crystalline phases in GeTe induced by femtosecond laser pulse amorphization2013

    • Author(s)
      Y. Katsumata, T. Morita, and T. Saiki
    • Organizer
      12th European/Phase Change and Ovonics Symposium (E/PCOS2013)
    • Place of Presentation
      ベルリン(ドイツ)
    • Related Report
      2013 Annual Research Report
  • [Presentation] GeTeにおけるフェムト秒パルス照射による結晶相/アモルファス相周期構造の形成2013

    • Author(s)
      森田貴紀, 勝又洋介, 北村成章, 森本悠介, 斎木敏治
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] ナノフォトニクスの複雑性に潜む機能2013

    • Author(s)
      斎木敏治
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 相変化マスク顕微分光の高空間分解能化2013

    • Author(s)
      佐藤悠, 津守伸宏,ヌルーシャファワティビンティフマム, 金澤翔平, 斎木敏治
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 金ナノロッドを用いたナノ領域相変化および検出2013

    • Author(s)
      平敬, 本間貴士, 内山貴之, 斎木敏治
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Two-Dimensional Finite Element Modeling for Stress Analysis of Emission Energy Control of Quantum Dots using Phase Change Material2013

    • Author(s)
      ヌルーシャファワティビンティフマム, 佐藤悠, 津守伸宏, 斎木敏治
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 相変化光学マスクを用いたInAs量子ドットの局所的な発光エネルギー制御および発光分光2013

    • Author(s)
      津守伸宏, 高橋 基紀, ヌルーシャファワティビンティフマム, 佐藤悠, 斎木敏治
    • Organizer
      日本光学会年次学術講演会(OPJ2013)
    • Place of Presentation
      奈良県新公会堂(奈良)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Improvement of Spatial Resolution of Nano Spectroscopy Imaging using Phase-Change Mask2013

    • Author(s)
      Y. Sato, N. Tsumori, Nurrul Syafawari Binti Humam, S. Kanazawa, and T. Saiki
    • Organizer
      25th Symposium on Phase Change Oriented Science (PCOS 2013)
    • Place of Presentation
      ホテル瑞鳳(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Redshifted and Blueshifted Photoluminescence Spectra of InAs/InP Quantum Dots upon Amorphization of Phase Change Material2013

    • Author(s)
      Nurrul Syafawati Binti Humam, Y. Sato, N. Tsumori, T. Saiki
    • Organizer
      25th Symposium on Phase Change Oriented Science (PCOS 2013)
    • Place of Presentation
      ホテル瑞鳳(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Formation of a crystalline and amorphous periodic structure by femtosecond pulse excitation of GeTe2013

    • Author(s)
      T. Morita, Y. Katsumata, Y. Morimoto, and T. Saiki
    • Organizer
      25th Symposium on Phase Change Oriented Science (PCOS 2013)
    • Place of Presentation
      ホテル瑞鳳(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] High contrast optical switching of localized surface plasmon resonance in a single gold nanosandwich using a GeSbTe film2013

    • Author(s)
      K. Kuwamura, T. Hira, T. Uchiyama, Y. Kihara, and T. Saiki
    • Organizer
      25th Symposium on Phase Change Oriented Science (PCOS 2013)
    • Place of Presentation
      ホテル瑞鳳(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 相変化材料を用いたアクティブ・ナノフォトニクス2013

    • Author(s)
      斎木敏治
    • Organizer
      日本学術振興会アモルファス・ナノ材料第147委員会第119回研究会
    • Place of Presentation
      東京
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 近接場ファイバプローブを用いた相変化マスク顕微分光の高分解能化2013

    • Author(s)
      佐藤悠
    • Organizer
      第13回レーザー学会東京支部研究会
    • Place of Presentation
      東京
    • Related Report
      2012 Annual Research Report
  • [Presentation] Spatially inhomogeneous stress impression on semiconductor quantum dots using volume expansion of phase change material2012

    • Author(s)
      M. Takahashi and T. Saiki
    • Organizer
      The 22th Symposium on Phase Change Optical Information Storage
    • Place of Presentation
      Atami, Japan
    • Year and Date
      2012-11-29
    • Related Report
      2013 Final Research Report
  • [Presentation] Active nanophotonics with chalcogenide phase-change materials2012

    • Author(s)
      T. Saiki
    • Organizer
      The 2nd Sweden-Japan Workshop on Nanophotonics and Related Technologies
    • Place of Presentation
      Kista, Sweden
    • Year and Date
      2012-06-18
    • Related Report
      2013 Final Research Report 2012 Annual Research Report
  • [Presentation] Possibility of Emission Energy Control of Individual Quantum Dots using Volume Expansion of Phase Change Material2012

    • Author(s)
      Nurrul Syafawati Binti Humam
    • Organizer
      第73回応用物理学会学術講演会
    • Place of Presentation
      松山
    • Related Report
      2012 Annual Research Report
  • [Presentation] Spatially inhomogeneous stress impression on semiconductor quantum dots using volume expansion of phase change material2012

    • Author(s)
      M. Takahashi
    • Organizer
      The 22th Symposium on Phase Change Optical Information Storage
    • Place of Presentation
      Atami
    • Related Report
      2012 Annual Research Report
  • [Presentation] Near-Infrared Nano-Imaging Spectroscopy of Semiconductor Quantum Dots using a Phase Change Mask Layer2011

    • Author(s)
      N. Tsumori and T. Saiki
    • Organizer
      Conference on Lasers and Electro-Optics 2011
    • Place of Presentation
      Baltimore, USA
    • Year and Date
      2011-05-03
    • Related Report
      2013 Final Research Report 2011 Annual Research Report
  • [Remarks]

    • URL

      http://www.saiki.elec.keio.ac.jp/

    • Related Report
      2013 Final Research Report
  • [Remarks]

    • URL

      http://www.saiki.elec.keio.ac.jp/

    • Related Report
      2011 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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