Development of high performance thermoelectric materials using information about fine electronic structure and phonon dispersions

• Project/Area Number: 23360278
• Research Category: Grant-in-Aid for Scientific Research (B)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Physical properties of metals
• Research Institution: Nagoya University
• Principal Investigator: TAKEUCHI Tsunehiro 名古屋大学, エコトピア科学研究所, その他 (00293655)
• Project Period (FY): 2011-04-01 – 2014-03-31
• Project Status: Completed (Fiscal Year 2013)
• Budget Amount: ¥19,630,000 (Direct Cost: ¥15,100,000、Indirect Cost: ¥4,530,000); Fiscal Year 2013: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000); Fiscal Year 2012: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000); Fiscal Year 2011: ¥14,170,000 (Direct Cost: ¥10,900,000、Indirect Cost: ¥3,270,000)
• Keywords: ゼーベック係数 / フォノン散乱 / 格子熱伝導度 / 熱電材料 / 熱電物性 / 第一原理計算 / 電子構造 / 電気伝導度 / 電子熱伝導度 / フォノン分散 / 電子物性 / 材料設計指針

Research Abstract

In this study, we constructed a guiding principle for the high-performance thermoelectric materials using detailed information about electronic structure and phonon dispersions, and developed new thermoelectric materials.
As a result of first principles calculations, we found that some of the selected alloys possess a electronic structure suitable for practical thermoelectric materials. Their possession of large of Seebeck coefficient and metallic electrical conduction was confirmed experimentally.
We also found, by using cluster calculation, that some of the heavy elements do not cause any variation in electrical properties but supposed to cause significant reduction in lattice thermal conductivity when they are partially substituted for the constituent elements. This tendency was confirmed experimentally, and the cheap, environmentally friendly thermoelectric materials usable at around 500 K were consequently developed.

Research Products

• [Journal Article] (2014)
  • Author(s): Y. Furuta, K. Kato, T. Miyawaki, H. Asano, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: (Accepted and now in press)
  • Peer Reviewed
• [Journal Article] (2014)
  • Author(s): R. Nakayama, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: (Accepted and now in press)
  • Peer Reviewed
• [Journal Article] Thermoelectric properties of Al-(Mn,X)-Si C54-phase (X = Ru and Re) (2014)
  • Author(s): A. Yamamoto, H. Miyazaki, T. Takeuchi
  • Journal Title: Journal of Applied Physics Volume: 115 Pages: 23708-23708
  • Peer Reviewed
• [Journal Article] (2014)
  • Author(s): 竹内恒博
  • Journal Title: 工業材料 Volume: 62巻 第4号 Pages: 22-25
• [Journal Article] 熱電材料の設計指針 (2014)
  • Author(s): 竹内恒博
  • Journal Title: 工業材料 Volume: 62 Pages: 22-25
• [Journal Article] Thermoelectric properties of Al-(Mn, X)-Si C54-phase (X=Ru, Re) (2014)
  • Author(s): 山本晃生, 宮崎秀俊, 竹内恒博
  • Journal Title: Joumal of Applied Physics Volume: 115 Issue: 2 Pages: 0237081-10
  • DOI: 10.1063/1.4861643
  • Peer Reviewed
• [Journal Article] Thermal rectification in bulk material through unusually increased electron thermal conductivity of Al-Cu-Fe icosahedral quasicrystal (2014)
  • Author(s): Ryu-suke Nakayama, Tsunehiro Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 43 Issue: 1 Pages: 356-361
  • DOI: 10.1007/s11664-014-3204-4
  • Peer Reviewed
• [Journal Article] Fe2VAl-Based Thermoelectric Thin Films Prepared by a Sputtering Technique (2014)
  • Author(s): Yukihiro Furuta, Keisuke Kato, Tetsuya Miyawaki, Hidefumi Asano, Tsunehiro Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 43 Issue: 6 Pages: 2157-2164
  • DOI: 10.1007/s11664-014-2994-8
• [Journal Article] (2013)
  • Author(s): T. Takeuchi, Y. Terazawa, Y. Furuta, A. Yamamoto, M. Mikami
  • Journal Title: Journal of Electronic Materials Volume: 42 Pages: 2084-2090
  • Peer Reviewed
• [Journal Article] (2013)
  • Author(s): M. Mikami, K. Ozaki, H. Takazawa, A. Yamamoto, Y. Terazawa, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 42 Pages: 1801-1806
  • Peer Reviewed
• [Journal Article] (2013)
  • Author(s): T. Kondo, Y. Nakashima, W. Malaeb, Y. Ishida, Y. Hamaya, T. Takeuchi, S. Shin
  • Journal Title: Physical Review Letters Volume: 110
  • Peer Reviewed
• [Journal Article] (2013)
  • Author(s): T. Kondo, A.D. Palczewski, Y. Hamaya, T. Takeuchi, J. S. Wen, Z. J. Xu, G. Gu, A. Kaminski
  • Journal Title: Physical Review Letters Volume: 111
  • Peer Reviewed
• [Journal Article] (2013)
  • Author(s): Y. He, Y. Yin, M. Zech, A. Soumyanarayanan, I. Zeljkovic, M. M. Yee, M. C. Boyer, K. Chatterjee, W. D. Wise, T. Kondo, T. Takeuchi, H. Ikuta, P. Mistark, R. S. Markiewicz, A. Bansil, S. Sachdev, E. W. Hudson, J. E. Hoffman
  • Journal Title: Science Volume: (Accepted and now in press)
  • Peer Reviewed
• [Journal Article] Effect of heavy element substitution and off-stoichiometric composition on thermoelectric properties of Fe2VAl thermoelectric material (2013)
  • Author(s): T. Takeuchi, Y. Terazawa, Y. Furuta, A. Yamamoto, M. Mikami.
  • Journal Title: Journal of Electronic Materials Volume: 42 Issue: 7 Pages: 2084-209
  • DOI: 10.1007/s11664-013-2532-0
  • Peer Reviewed
• [Journal Article] Effect of Ti Substitution on Thermoelectric Properties of W-Doped Heusler Fe2VAl Alloy (2013)
  • Author(s): M. Mikami, K. Ozaki, H. Takazawa, A. Yamamoto, Y. Terazawa, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 42 Pages: 1801-180
  • Peer Reviewed
• [Journal Article] Anomalous doping variation of the nodal low-energy feature of superconducting (Bi,Pb)2(Sr,La)2CuO6+d crystals revealed by laser-based angle-resolved photoemission spectroscopy (2013)
  • Author(s): T. Kondo, Y. Nakashima, W. Malaeb, Y. Ishida, Y. Hamaya, T. Takeuchi, S. Shin
  • Journal Title: Physical Review Letters Volume: 110 Issue: 21 Pages: 217006-217006
  • DOI: 10.1103/physrevlett.110.217006
  • Peer Reviewed
• [Journal Article] (2012)
  • Author(s): Y. Terazawa1, M. Mikami, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 41 Pages: 1348-1353
  • Peer Reviewed
• [Journal Article] (2012)
  • Author(s): A. Yamamoto, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 41 Pages: 1743-1748
  • Peer Reviewed
• [Journal Article] (2012)
  • Author(s): T. Takeuchi, H. Goto, R. Nakayama, Y. Terazawa, K. Ogawa, A. Yamamoto, T. Itoh, M. Mikami
  • Journal Title: Journal of Applied Physics Volume: 111
  • Peer Reviewed
• [Journal Article] (2012)
  • Author(s): M. Mikami, Y. Kinemuchi, K. Ozaki, Y. Terazawa, T. Takeuchi
  • Journal Title: Journal of Applied Physics Volume: 111
• [Journal Article] (2012)
  • Author(s): I. Zeljkovic, E. J. Main, T. L. Williams, M. C. Boyer, K. Chatterjee, W. D. Wise, Yi Yin, Martin Zech, A. Pivonka, T. Kondo, T. Takeuchi, H. Ikuta, J. Wen, Z. Xu, G. D. Gu, E. W. Hudson, J. E. Hoffman
  • Journal Title: Nature Materials Volume: 11 Pages: 585-589
  • Peer Reviewed
• [Journal Article] (2012)
  • Author(s): 寺澤佑一, 三上祐史, 伊藤孝至, 竹内恒博
  • Journal Title: 日本金属学会誌 Volume: 第76巻 第3号 Pages: 216-221
  • Peer Reviewed
• [Journal Article] (2012)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 第9巻 第1号 Pages: 27-31
• [Journal Article] (2012)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 第9巻 第2号 Pages: 21-26
• [Journal Article] Effect of Ru substitution for Mn in the Si2Ti-type Al-Mn-Si alloy. Journal of Electronic Materials (2012)
  • Author(s): A. Yamamoto
  • Journal Title: Journal of Electronic Materials Volume: 46 Issue: 6 Pages: 1743-1748
  • DOI: 10.1007/s11664-012-2101-y
  • Peer Reviewed
• [Journal Article] Improvement in rectification ratio of an Al-based bulk thermal rectifier working at high temperatures (2012)
  • Author(s): T. Takeuchi
  • Journal Title: Journal of Applied Physics Volume: 111 Issue: 9 Pages: 93517-93517
  • DOI: 10.1063/1.4712420
  • Peer Reviewed
• [Journal Article] Thermoelectric properties of tungsten-substituted Heusler Fe2VAl alloy (2012)
  • Author(s): M. Mikami
  • Journal Title: Journal of Applied Physics Volume: 111 Issue: 9 Pages: 93710-93710
  • DOI: 10.1063/1.4710990
  • Peer Reviewed
• [Journal Article] Scanning tunnelling microscopy imaging of symmetry-breaking structural distortion in the bismuth-based cuprate superconductors (2012)
  • Author(s): I. Zeljkovic
  • Journal Title: Nature Materials Volume: 11 Issue: 7 Pages: 585-589
  • DOI: 10.1038/nmat3315
  • Peer Reviewed
• [Journal Article] 金属と半導体の熱物性の基礎理論 第四回：熱電材料に求められる電子構造とフォノン分散の条件 (2012)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 9 (1) Pages: 21-36
• [Journal Article] 金属と半導体の熱物性の基礎理論 第五回：熱電材料開発におけるトレンドとZT > 1を示す材料の特徴 (2012)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 9 (2) Pages: 21-36
• [Journal Article] 金属と半導体の熱物性の基礎理論第三回:格子熱伝導度とフォノン分散 (2012)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 8(3) Pages: 27-31
  • Peer Reviewed
• [Journal Article] Fe_2VA1の電子構造と熱電物性における重元素部分置換効果 (2012)
  • Author(s): 寺澤佑一, 三上祐史, 伊藤孝至, 竹内恒博
  • Journal Title: 日本金属学会誌 Volume: 76(3) Pages: 216-221
  • Peer Reviewed
• [Journal Article] The Effects of Heavy Element Substitution on Electric Structure and Lattice Thermal Conductivity of Fe_2VA1 Thermoelectric Material (2012)
  • Author(s): Yu-ichi Terazawa, Masashi Mikami, Tsunehiro Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: (印刷中) Issue: 6 Pages: 1348-1353
  • DOI: 10.1007/s11664-011-1862-z
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): T. Kondo, Y. Hamaya, A. D. Palczewski, T. Takeuchi, J. S. Wen, Z. J. Xu, Genda Gu, Jorg Schmalian, A. Kaminski
  • Journal Title: Nature Physics Volume: 7 Pages: 21-25
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): Y. Okada, T. Kawaguchi, M. Ohkawa, K. Ishizaka, T. Takeuchi, S. Shin, H. Ikuta
  • Journal Title: Physical Review B Volume: 83
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): T. Takeuchi, H. Goto, Y. Toyama, T. Itoh, M. Mikami
  • Journal Title: Journal of Electronic Materials Volume: 40 Pages: 1129-1135
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): Y. Toyama, H. Hazama, R. Asahi, T. Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 40 Pages: 1052-1056
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): A. Yamamoto, K. Ogawa, T. Takeuchi
  • Journal Title: Materials Transactions Volume: 52 Pages: 1539-1545
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): H. Hazama, M. Matsubara, R. Asahi, T. Takeuchi
  • Journal Title: Journal of Applied Physics Volume: 110
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): T. Takeuchi, A. Yamamoto, K. Ogawa
  • Journal Title: Materials Research Society Proceedings Volume: Vol.1314
  • DOI: 10.1557/opl.2011.513
  • Peer Reviewed
• [Journal Article] (2011)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 第8巻 第2号 Pages: 18-23
• [Journal Article] (2011)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 第8巻 第3号 Pages: 27-31
• [Journal Article] 金属と半導体の熱物性の基礎理論第一回:熟電物性基礎理論と金属・半導体電子論の利用に関する問題点 (2011)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 8(1) Pages: 17-23
  • Peer Reviewed
• [Journal Article] 金属と半導体の熱物性の基礎理論第二回:線形応答理論を用いた電子物性の定量解析 (2011)
  • Author(s): 竹内恒博
  • Journal Title: 日本熱電学会誌 Volume: 8(2) Pages: 18-23
  • Peer Reviewed
• [Journal Article] Development of thermal rectifier usable at high temperature (2011)
  • Author(s): Tsunehiro Takeuchi, Hiroki Goto, Yasuhiro Toyama, Takashi Itoh, Masashi Mikami
  • Journal Title: Journal of Electronic Materials Volume: 40(5) Issue: 5 Pages: 1129-1135
  • DOI: 10.1007/s11664-011-1556-6
  • Peer Reviewed
• [Journal Article] Thermoelectric properties of Si_2Ti-type Al-(Mn, Cr, Fe)-Si alloys (2011)
  • Author(s): Yasuhiro Toyama, Hirofumi Hazama, Ryoji Asahi, Tsunehiro Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: 40(5) Issue: 5 Pages: 1052-1056
  • DOI: 10.1007/s11664-011-1531-2
  • Peer Reviewed
• [Journal Article] Effect of Chemical potential on thermoelectric power of Bi_2Te_3 and Bi_2Se_3 (2011)
  • Author(s): Yasuhiro Toyama, Hirofumi Hazama, Ryoji Asahi, Tsunehiro Takeuchi
  • Journal Title: Materials Transactions Volume: 52(8) Pages: 1539-1545
  • NAID: 10029297407
  • Peer Reviewed
• [Journal Article] Improvement of thermoelectric properties for half-Heusler TiNiSn by interstitial Ni defects (2011)
  • Author(s): Hirofumi Hazama, Masato Matsubara, Ryoji Asahi, Tsunehiro Takeuchi
  • Journal Title: Journal of Applied Physics Volume: 110
  • Peer Reviewed
• [Journal Article] Effect of Ru substitution for Mn in the Si_2Ti-type Al-Mn-Si alloy
  • Author(s): Akio Yamamoto, Tsunehiro Takeuchi
  • Journal Title: Journal of Electronic Materials Volume: (印刷中)
  • Peer Reviewed
• [Presentation] 狭い擬ギャップと準周期性を利用した熱整流材料の開発 (2014)
  • Author(s): 竹内恒博
  • Organizer: 日本物理学会第69回年次大会
  • Year and Date: 2014-03-29
  • Invited
• [Presentation] 高性能熱電材料における界面の役割 (2014)
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会2014年春期(第154回)講演大会
  • Year and Date: 2014-03-23
• [Presentation] Preparation of Thermal diode using plasma jet splaying technique (2014)
  • Author(s): Tsunehiro Takeuchi, Wataru Takahara, Akira Kobayashi
  • Organizer: The 7th International Workshop on Plasma Application and Hybrid Functionally Materials
  • Year and Date: 2014-03-08
• [Presentation] Thermal rectification in icosahedral quasicrystals (2013)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: The 12th International Conference on Quasicrystals
  • Year and Date: 2013-09-03
  • Invited
• [Presentation] Precise determination of superconducting gap of Bi_2(Sr,R)_2CuO_<6+d>(R = La and Sm) (2013)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: SRC Quantum Lunch Seminar
  • Year and Date: 2013-04-25
  • Invited
• [Presentation] Al-Mn-Si 系環境調和型熱電材料の創成 (2013)
  • Author(s): 竹内恒博, 山本晃生
  • Organizer: 平成25年電気学会全国大会
  • Year and Date: 2013-03-20
  • Invited
• [Presentation] 環境調和型高性能熱電材料の開発 (2013)
  • Author(s): 竹内恒博
  • Organizer: ６大学６研究所連携プロジェクト公開討論会
  • Place of Presentation: 名古屋大学，名古屋
  • Invited
• [Presentation] Al-Mn-Si系環境調和型熱電材料の創成 (2013)
  • Author(s): 竹内恒博
  • Organizer: 平成２５年電気学会全国大会
  • Place of Presentation: 名古屋大学，名古屋
  • Invited
• [Presentation] FeSb2の高分解能角度分解光電子分光 (2013)
  • Author(s): 島田崇史
  • Organizer: 第26回日本放射光学会年会・放射光科学合同シンポジウム
  • Place of Presentation: 名古屋大学，名古屋
• [Presentation] Al-Mn-Si系環境調和型熱電材料の創成 (2013)
  • Author(s): 竹内恒博
  • Organizer: 2013年応用物理学会春季学術講演大会
  • Place of Presentation: 神奈川工科大学，厚木
• [Presentation] FeSb2の電子構造と巨大ゼーベック係数 (2013)
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会2013年春季講演大会
  • Place of Presentation: 東京理科大学，東京
• [Presentation] Al-Cu-Fe準結晶の異常電子熱伝導度を利用した熱整流効果 (2013)
  • Author(s): 中山隆介
  • Organizer: 日本金属学会2013年春季講演大会
  • Place of Presentation: 東京理科大学，東京
• [Presentation] 重元素を部分置換したAl-(Mn,X)-Si系C５４相(X =Ru, Re)の熱電物性 (2013)
  • Author(s): 山本晃生
  • Organizer: 日本金属学会2013年春季講演大会
  • Place of Presentation: 東京理科大学，東京
• [Presentation] 熱電物性の支配因子とマイクロ・ナノ構造の影響 (2012)
  • Author(s): 竹内恒博
  • Organizer: 第4回日本機械学会マイクロナノ工学シンポジウム
  • Year and Date: 2012-10-23
  • Invited
• [Presentation] Improvement in thermoelectric performance of Fe_2VAl-based Heusler alloys by using electronic structure analysis (2012)
  • Author(s): Tsunehiro Takeuchi, Yuichi Terazawa, Yukihiro Furuta, Akio Yamamoto, Masashi Mikami
  • Organizer: International Union of Materials Research Societies-International Conference on Eelectronic Materials 2012
  • Year and Date: 2012-09-25
• [Presentation] Development of Thermal-Rectifier Using Al-Based Quasicrystals (2012)
  • Author(s): Tsunehiro Takeuchi, Ryu-suke Nakayamac, Masashi Mikamid, Hidetoshi Miyazakie
  • Organizer: APERIODIC 2012
  • Year and Date: 2012-09-06
• [Presentation] 「最先端スペクトロスコピーを用いた熱電変換材料の研究最前線」高性能熱電材料開発における高分解能光電子分光法の利用 (2012)
  • Author(s): 竹内恒博
  • Organizer: 日本熱電学会第15回研究会
  • Year and Date: 2012-08-02
  • Invited
• [Presentation] Improvement in thermoelectric performance of Fe_2VAl-based materials by means of heavy element partial substitutions (2012)
  • Author(s): Tsunehiro Takeuchi, Yuichi Terazawa, Yukihiro Furuta, Akio Yamamoto, Masashi Mikami
  • Organizer: The 31st International & 10th European Conference on Thermoelectrics
  • Year and Date: 2012-07-10
• [Presentation] 熱電材料開発研究における高分解能光電子分光の利用 (2012)
  • Author(s): 竹内恒博
  • Organizer: UVSOR 研究会熱電材料開発研
  • Year and Date: 2012-06-21
  • Invited
• [Presentation] 構成元素の部分置換によるAl-Mn-Si C54相熱電材料の物性改質 (2012)
  • Author(s): 山本晃生, 竹内恒博
  • Organizer: 日本金属学会2012年春期大会
  • Place of Presentation: 横浜国立大学
  • Year and Date: 2012-03-30
• [Presentation] 電子構造解析に基づくFe_2VAl系熱電材料の高性能化 (2012)
  • Author(s): 寺澤佑一, 三上祐史, 竹内恒博
  • Organizer: 日本金属学会2012年春期大会
  • Place of Presentation: 横浜国立大学
  • Year and Date: 2012-03-30
• [Presentation] フェルミ準位近傍の微細電子構造に起因する異常電子熱伝導度を利用した新規熱整流材料の開発 (2012)
  • Author(s): 中山隆介, 竹内恒博
  • Organizer: 日本金属学会2012年春期大会
  • Place of Presentation: 横浜国立大学
  • Year and Date: 2012-03-30
• [Presentation] 熱電物性における散乱因子の役割 (2012)
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会第3回熱電変換材料研究会
  • Year and Date: 2012-03-29
• [Presentation] 熱電物性における散乱因子の役割 (2012)
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会研究分科会第3回熱電変換材料研究会「熱電変換材料の性能向上にむけて」
  • Place of Presentation: 横浜国立大学(招待講演)
  • Year and Date: 2012-03-29
• [Presentation] 巨大ゼーベック係数を示すFeSb_2の高分解能角度分解光電子分光 (2012)
  • Author(s): 島田崇史, 竹内恒博
  • Organizer: 日本物理学会第67回年次大会
  • Place of Presentation: 関西学院大学
  • Year and Date: 2012-03-27
• [Presentation] 電子構造とフォノン分散を考慮した熱電材料設計指針の構築 (2012)
  • Organizer: 応用物理学会2012春季講演会
  • Year and Date: 2012-03-15
  • Invited
• [Presentation] 電子構造とフォノン分散を考慮した熱電材料設計指針の構築 (2012)
  • Author(s): 竹内恒博
  • Organizer: 日本応用物理学会2012春季講演会
  • Place of Presentation: 早稲田大学早稲田キャンパス(招待講演)
  • Year and Date: 2012-03-15
• [Presentation] ウエアラブルデバイスの電源となる無害で高性能な熱電発電材料の開発 (2012)
  • Author(s): 竹内恒博, 一野祐介, 伊藤孝至
  • Organizer: 第2回6大学連携プロジェクト公開討論会
  • Place of Presentation: 大阪府豊中市千里ライフサイエンスセンター
  • Year and Date: 2012-03-01
• [Presentation] 熱電材料の現状・課題と最近の研究 (2012)
  • Author(s): 竹内恒博
  • Organizer: 金属学会鉄鋼協会東海支部学術講演会
  • Year and Date: 2012-02-23
  • Invited
• [Presentation] FeSb_2の高分解能角度分解光電子分光 (2012)
  • Author(s): 島田崇史、小川古都、山本晃生、竹内恒博
  • Organizer: 第25回日本放射光学会・放射光科学合同シンポジウム
  • Place of Presentation: 佐賀県鳥栖市鳥栖市民文化会館・中央公民館
  • Year and Date: 2012-01-07
• [Presentation] Improvement in thermoelectric performance of Fe2VAl-based materials by means of heavy element partial substitutions (2012)
  • Author(s): T. Takeuchi
  • Organizer: The 31st International & 10th European Conference on Thermoelectrics
  • Place of Presentation: Aalborg, Denmark
• [Presentation] Development of Thermal-Rectifier Using Al-Based Quasicrystals (2012)
  • Author(s): T. Takeuchi
  • Organizer: APERIODIC 2012
  • Place of Presentation: Cairns Australia
• [Presentation] Improvement in thermoelectric performance of Fe2VAl-based materials by means of heavy element partial substitutions (2012)
  • Author(s): T. Takeuchi
  • Organizer: International Union of Materials Research Societies-International Conference on Eelectronic Materials 2012
  • Place of Presentation: Yokohama, Japan
• [Presentation] Improvement of the thermoelectric properties of Al-Mn-Si C54-phase by means of partial element substitution (2012)
  • Author(s): A. Yamamoto
  • Organizer: International Union of Materials Research Societies-International Conference on Eelectronic Materials 2012
  • Place of Presentation: Yokohama, Japan
• [Presentation] Relation between electronic structure and huge Seebeck coefficient of FeSb2 (2012)
  • Author(s): T. Shimada
  • Organizer: International Union of Materials Research Societies-International Conference on Eelectronic Materials 2012
  • Place of Presentation: Yokohama, Japan
• [Presentation] Development of bulk thermal rectifier using unusual increase of electron thermal conductivity of Al-Cu-Fe icosahedral quasicrystal (2012)
  • Author(s): R. Nakayama
  • Organizer: International Union of Materials Research Societies-International Conference on Eelectronic Materials 2012
  • Place of Presentation: Yokohama, Japan
• [Presentation] High Functional Coatings for Practical Thermoelectric Materials Using Gas Tunnel Type Plasma Spraying (2012)
  • Author(s): A. Kobayashi
  • Organizer: ISAEM-2012 & AMDI-3
  • Place of Presentation: Toyohashi, Japan
• [Presentation] Development of Environmentally-Friendly Al-Mn-Si Thermoelectric Materials (2012)
  • Author(s): T. Takeuchi
  • Organizer: ISAEM-2012 & AMDI-3
  • Place of Presentation: Toyohashi, Japan
• [Presentation] 熱電材料開発研究における高分解能光電子分光の利用 (2012)
  • Author(s): 竹内恒博
  • Organizer: UVSOR研究会
  • Place of Presentation: 分子科学研究所，岡崎
  • Invited
• [Presentation] 高性能熱電材料開発における高分解能光電子分光法の利用 (2012)
  • Author(s): 竹内恒博
  • Organizer: 日本熱電学会第15回研究会
  • Place of Presentation: 名古屋工業大学．名古屋
  • Invited
• [Presentation] Al-Cu-Fe準結晶を用いた熱整流材料の創成 (2012)
  • Author(s): 竹内恒博
  • Organizer: 第９回日本熱電学会学術講演会
  • Place of Presentation: 東京工業大学，東京
• [Presentation] 重元素部分置換によるAl-Mn-SiC54相熱電材料の物性改質 (2012)
  • Author(s): 山本晃生
  • Organizer: 第９回日本熱電学会学術講演会
  • Place of Presentation: 東京工業大学，東京
• [Presentation] Al-Cu-Fe準結晶とSiから構成される熱整流材料の熱整流効果の評価 (2012)
  • Author(s): 中山隆介
  • Organizer: 日本金属学会2012年秋季大会
  • Place of Presentation: 愛媛大学，松山
• [Presentation] Al-Mn-Si C54相熱電材料の構成元素部分置換効果 (2012)
  • Author(s): 山本晃生
  • Organizer: 日本金属学会2012年秋季大会
  • Place of Presentation: 愛媛大学，松山
• [Presentation] ZT>2を実現するための電子構造の条件 (2012)
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会2012年秋季大会
  • Place of Presentation: 愛媛大学，松山
• [Presentation] FeSb2の高分解能角度分解光電子分光 (2012)
  • Author(s): 島田崇史
  • Organizer: 日本物理学会 2012年秋季大会
  • Place of Presentation: 横浜国立大学．横浜
• [Presentation] 準結晶熱整流材料の開発 (2011)
  • Author(s): 竹内恒博
  • Organizer: 第16回準結晶研究会
  • Place of Presentation: 北海道大学
  • Year and Date: 2011-12-14
• [Presentation] Development of thermal rectifier using unusual electron thermal conductivity (2011)
  • Author(s): Ryu-suke Nakayama, Takashi Itoh, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2011
  • Place of Presentation: Nagoya University
  • Year and Date: 2011-12-10
• [Presentation] Thermoelectric properties of Si Ti-type Al-Mn-Ru-Si C54-phase (2011)
  • Author(s): Akio Yamamoto, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2011
  • Place of Presentation: Nagoya University
  • Year and Date: 2011-12-10
• [Presentation] High-resolution angle resolved photoemission spectroscopy of FeSb_2 (2011)
  • Author(s): Takafumi Shimada, Koto Ogawa, Akio Yamamoto, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2011
  • Place of Presentation: Nagoya University
  • Year and Date: 2011-12-10
• [Presentation] Effects of heavy element substitution on electric structure and lattice thermal conductivity of Fe thermoelectric materials (2011)
  • Author(s): Yu-ichi Terazawa, Masashi Mikami, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2011
  • Place of Presentation: Nagoya University
  • Year and Date: 2011-12-10
• [Presentation] FeSb_2の高分解能角度光電子分光 (2011)
  • Author(s): 島田崇史, 竹内恒博
  • Organizer: UVSORユーザーズミーティング
  • Place of Presentation: 自然科学研究機構岡崎コンファレンスセンター
  • Year and Date: 2011-11-18
• [Presentation] Effects of Ru substitution for Mn in the Si_2Ti-type Al-Mn-Si alloy (2011)
  • Author(s): Akio Yamamoto, Tsunehiro Takeuchi
  • Organizer: JSPS-CNRS Japan France Joint Seminar
  • Place of Presentation: 愛知県名古屋市Wincあいち
  • Year and Date: 2011-11-10
• [Presentation] Heavy Element Substitution on Electronic Structure and Lattice Thermal Conductivity of Fe2VAl-based Alloys (2011)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: JSPS Japan France Joint Seminar Effects
  • Year and Date: 2011-11-09
• [Presentation] Fe_2VAlの電子構造と熱電物性における重元素部分置換効果 (2011)
  • Author(s): 寺澤佑一, 三上祐史, 伊藤孝至, 竹内恒博
  • Organizer: 日本金属学会2011年秋期(第149回)大会
  • Place of Presentation: 沖縄県宜野湾市カルチャーリゾートフェストーネ
  • Year and Date: 2011-11-09
• [Presentation] Al-Mn-Ru-Si系C54相の熱電物性 (2011)
  • Author(s): 山本晃生, 竹内恒博
  • Organizer: 日本金属学会2011年秋期(第149回)大会
  • Place of Presentation: 沖縄県宜野湾市カルチャーリゾートフェストーネ
  • Year and Date: 2011-11-09
• [Presentation] Effects of Heavy Element Substitution on Electronic Structure and Lattice Therm al Conductivity of Fe_2VAl-based Alloys (2011)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: JSPS-CNRS Japan France Joint Seminar
  • Place of Presentation: 愛知県名古屋市Wincあいち(招待講演)
  • Year and Date: 2011-11-09
• [Presentation] 擬ギャップにより特徴づけられる準結晶と近似結晶の異常電子物性 (2011)
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会2011年秋期(第149回)大会
  • Place of Presentation: 沖縄県宜野湾市カルチャーリゾートフェストーネ(招待講演)
  • Year and Date: 2011-11-07
• [Presentation] フェルミ準位近傍の微細電子構造に起因する異常電子熱伝導度を利用した熱流制御材料の開発 (2011)
  • Author(s): 中山隆介, 竹内恒博
  • Organizer: 日本金属学会2011年秋期(第149回)大会
  • Place of Presentation: 沖縄県宜野湾市カルチャーリゾートフェストーネ
  • Year and Date: 2011-11-07
• [Presentation] FeSb_2の高分解能角度分解光電子分光-巨大熱電能発現における電子構造の役割- (2011)
  • Author(s): 島田崇史, 小川古都, 山本晃生, 竹内恒博
  • Organizer: 日本物理学会2011年秋季大会
  • Place of Presentation: 富山大学五福キャンパス
  • Year and Date: 2011-09-22
• [Presentation] 室温以上で動作する熱整流材料の創製 (2011)
  • Author(s): 竹内恒博, 中山隆介
  • Organizer: 第八回日本熱電学会学術講演会(TSJ2011)
  • Place of Presentation: 北海道大学
  • Year and Date: 2011-08-09
• [Presentation] Al-Mn-Ru-Si系C54相の熱電物性 (2011)
  • Author(s): 山本晃生、竹内恒博
  • Organizer: 第八回日本熱電学会学術講演会(TSJ2011)
  • Place of Presentation: 北海道大学
  • Year and Date: 2011-08-08
• [Presentation] Fe_2VAlの電子構造と熱電物性における重元素部分置換効果 (2011)
  • Author(s): 寺澤佑一、三上祐史、竹内恒博
  • Organizer: 第八回日本熱電学会学術講演会(TSJ2011)
  • Place of Presentation: 北海道大学
  • Year and Date: 2011-08-08
• [Presentation] Condition of electronic structure for practical thermoelectric materials (2011)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: The 30th International Conference on Thermoelectrics
  • Place of Presentation: Grand Traverse Resort and Spa, Traverse City, Michigan, USA(招待講演)
  • Year and Date: 2011-07-21
• [Presentation] The effects of heavy element substitution on electric structure and lattice thermal conductivity of Fe_2VAl thermoelectric material (2011)
  • Author(s): Yuichi Terazawa, Masashi Mikami, Tsunehiro Takeuchi
  • Organizer: The 30th International Conference on Thermoelectrics
  • Place of Presentation: Grand Traverse Resort and Spa, Traverse City, Michigan, USA
  • Year and Date: 2011-07-18
• [Presentation] Effects of Ru substitution for Mn in the Si_2Ti-type Al-Mn-Si alloy (2011)
  • Author(s): Akio Yamamoto, Tsunehiro Takeuchi
  • Organizer: The 30th International Conference on Thermoelectrics
  • Place of Presentation: Grand Traverse Resort and Spa, Traverse City, Michigan, USA
  • Year and Date: 2011-07-18
• [Presentation] Development of Thermal Rectifier Utilizing the Narrow Pseudogap at the Fermi Level (2011)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: The 6th Asian International Workshop on Quasicrystals
  • Place of Presentation: Seoul National University, Seoul, Korea(招待講演)
  • Year and Date: 2011-06-02
• [Presentation] 高性能熱電材料における界面の役割
  • Author(s): 竹内恒博
  • Organizer: 日本金属学会
  • Place of Presentation: 東京工業大学大岡山キャンパス
  • Invited
• [Presentation] Effect of heavy element substitution and off-stoichiometric composition on thermoelectric properties of Fe2VAl thermoelectric material
  • Author(s): T. Takeuchi, Y. Terazawa, Y. Furuta, A. Yamamoto, M. Mikami.
  • Organizer: The 32nd International Conference on Thermoelectrics (ICT2013)
  • Place of Presentation: 神戸コンペンションセンター
• [Presentation] RFスパッタ法を用いたFe2VAl系熱電材料の薄膜化
  • Author(s): 竹内恒博,古田幸大
  • Organizer: 日本応用物理学会2013年第74回応用物理学会秋季学術講演会
  • Place of Presentation: 同志社大学京田辺キャンパス
• [Presentation] Thermal rectification in icosahedral quasicrystals
  • Author(s): Tsunehiro Takeuchi
  • Organizer: The 12th International Conference on Quasicrystals
  • Place of Presentation: Krakow, Poland
  • Invited
• [Presentation] Fe2VAl based thermoelectric thin-films prepared by RF sputtering technique
  • Author(s): Yukihiro Furuta, Keisuke Kato, Tetsuya Miyawaki, Hidefumi Asano, ○Tsunehiro Takeuchi
  • Organizer: The 32nd International Conference on Thermoelectrics (ICT2013)
  • Place of Presentation: 神戸コンペンションセンター
• [Presentation] Thermal rectification using unusual increase of electron thermal conductivity of Al-Cu-Fe icosahedral quasicrystal
  • Author(s): Ryusuke Nakayama, Tsunehiro Takeuchi
  • Organizer: The 32nd International Conference on Thermoelectrics (ICT2013)
  • Place of Presentation: 神戸コンペンションセンター
• [Presentation] Effects of Chromium-doping on Thermoelectric Properties of (BiS)1.2(TiS2)2 Misfit Layer Sulfide
  • Author(s): Yulia Eka Putri, Chunlei Wan, Wataru Norimatsu, Michiko Kusunoki, Tsunehiro Takeuchi, Ruizhi Zhang, Takao Mori, Kunihito Koumoto
  • Organizer: The 32nd International Conference on Thermoelectrics (ICT2013)
  • Place of Presentation: 神戸コンペンションセンター
• [Presentation] 非化学量論組成Fe2VAlの熱電特性に及 ぼすTa及びSi同時置換の効果
  • Author(s): 加賀翔大、宮崎秀俊、井手直樹、竹内恒博、西野洋一
  • Organizer: 第10回日本熱電学会学術講演会
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] Thermoelectric properties of Al-(Mn,X)-Si C54-phase ( X = Ru, and Re )
  • Author(s): Akio Yamamoto, Tsunehiro Takeuchi
  • Organizer: The 32nd International Conference on Thermoelectrics (ICT2013)
  • Place of Presentation: 神戸コンペンションセンター
• [Presentation] Precise determination of superconducting gap of Bi2(Sr,R)2CuO6+d (R = La and Sm)
  • Author(s): Tsunehiro Takeuchi
  • Organizer: Synchrotron Radiation Center, Quantum Lunch Seminar
  • Place of Presentation: 米国ウイスコンシン州ストウトンSynchrotron Radiation Center
  • Invited
• [Presentation] 重元素を部分置換したAl-(Mn,X )-Si C54 相 (X = Ru, Ta, W, Re)の熱電物性
  • Author(s): 山本晃生、竹内恒博
  • Organizer: 第10回日本熱電学会学術講演会
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] MnをWで部分置換したMnSiγ (γ =1.75)の 熱電物性
  • Author(s): 広石尚也、山本晃生、竹内恒博
  • Organizer: 第10回日本熱電学会学術講演会
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] イオンビームスパッタリング法を用いた Fe2VAlエピタキシャル薄膜の作製
  • Author(s): 加藤恵介、岩崎航太、古田幸大、 宮脇哲也、浅野秀文、竹内恒博
  • Organizer: 第10回日本熱電学会学術講演会
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] Fe2VAl系薄膜熱電材料の作製
  • Author(s): 古田幸大，竹内恒博
  • Organizer: 日本金属学会2013年秋期講演大会
  • Place of Presentation: 金沢大学角間キャンパス
• [Presentation] Al基準結晶で観測される異常電子熱伝導度を利用した熱整流材料の開発
  • Author(s): 中山隆介，竹内恒博
  • Organizer: 日本金属学会2013年秋期講演大会
  • Place of Presentation: 金沢大学角間キャンパス
• [Presentation] Al-(Mn,X)-Si系C54相(X=Ta, W)の熱電物性
  • Author(s): 山本晃生，竹内恒博
  • Organizer: 日本金属学会2013年秋期講演大会
  • Place of Presentation: 金沢大学角間キャンパス
• [Presentation] MnをWで部分置換したMnSiγ (γ =1.75)の 熱電物性
  • Author(s): 広石尚也、山本晃生、竹内恒博
  • Organizer: 日本金属学会2013年秋期講演大会
  • Place of Presentation: 金沢大学角間キャンパス
• [Presentation] 中性子準弾性散乱によるNaxCoO2のNa拡散解析
  • Author(s): 野崎洋，梅垣いづみ，野村越子，竹内恒博，蒲沢和也，山田武，柴田薫，杉山純
  • Organizer: 日本物理学会2013年秋期大会
  • Place of Presentation: 高知大学朝倉キャンパス
• [Presentation] Al-Cu-Fe準結晶熱整流材料の高性能化
  • Author(s): 竹内恒博，中山隆介
  • Organizer: 日本物理学会2013年秋期大会
  • Place of Presentation: 高知大学朝倉キャンパス
• [Presentation] レーザーARPESによるBi2(Sr,R)2CuO6+dにおける超伝導ギャップの系統的評価
  • Author(s): 坂本英城，竹内恒博，近藤猛，辛埴
  • Organizer: 日本物理学会2013年秋期大会
  • Place of Presentation: 高知大学朝倉キャンパス
• [Presentation] Thermoelectric properties of Al―(Mn‚X)―Si C54-phase ( X = Ru‚ Ta‚ W‚ and Re )
  • Author(s): AkioYamamoto, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2013
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] Implovement of the thermoelectric properties of a Chimney-Ladder Mn(1-x)WxSiγ (γ=1.75) by means of partial element substitution
  • Author(s): Naoya Hiroishi, AkioYamamoto, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2013
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] The thermal rectifier using unusual increase of electron thermal conductivity of Al-Cu-Fe icosahedral quasicrystal
  • Author(s): Ryusuke Nakayama, Tsunehiro Takeuchi
  • Organizer: International Symposium on EcoTopia Science 2013
  • Place of Presentation: 名古屋大学東山キャンパス
• [Presentation] Preparation of Thermal diode using plasma jet splaying technique
  • Author(s): Tsunehiro Takeuchi, Wataru Takahara, Akira Kobayashi
  • Organizer: The 7th International Workshop on Plasma Application and Hybrid Functionally Materials
  • Place of Presentation: 香港理工大学
• [Presentation] Al-Mn-Si系C40相の熱電物性と 熱電材料としての可能性
  • Author(s): Tsunehiro Takekuchi
  • Organizer: 2014年 第61回応用物理学会春季学術講演会
  • Place of Presentation: 青山学院大学 相模原キャンパス
• [Presentation] Fe2VAl系ホイスラー合金薄膜熱電材料の作製
  • Author(s): 古田幸大，竹内恒博
  • Organizer: 日本金属学会2014年春期(第154回)講演大会
  • Place of Presentation: 東京工業大学大岡山キャンパス
• [Presentation] 重元素置換を行ったAl基準結晶を利用した熱整流効果
  • Author(s): 中山隆介，竹内恒博
  • Organizer: 日本金属学会2014年春期(第154回)講演大会
  • Place of Presentation: 東京工業大学大岡山キャンパス
• [Presentation] Al-(Mn,X)-Si C40相 (X=Ta,W, Re)熱電材料の物性改質
  • Author(s): 山本晃生，竹内恒博
  • Organizer: 日本金属学会2014年春期(第154回)講演大会
  • Place of Presentation: 東京工業大学大岡山キャンパス
• [Presentation] Mnを重元素で部分置換したMnSiγ (γ=1.75)の熱電物性
  • Author(s): 広石尚也，竹内恒博
  • Organizer: 日本金属学会2014年春期(第154回)講演大会
  • Place of Presentation: 東京工業大学大岡山キャンパス
• [Presentation] 狭い擬ギャップと準周期性を利用した熱整流材料の開発
  • Author(s): 竹内恒博
  • Organizer: 日本物理学会第69回年次大会
  • Place of Presentation: 東海大学 湘南キャンパス
• [Book] CRC handbook "Thermoelectrics and its Energy Harvesting, Vol.1 Materials, Preparation, and Characterization in Thermoelectrics" Section 1-7 (2012)
  • Author(s): T. Takeuchi, 他
  • Publisher: CRC Press
• [Book] CRC Hand book Thermoelectrics and its Energy Harvesting Vol. Materials, Preparation, and Characterization in Thermoelectrics edited by D. Rowe” 1-7 “New thermoelectric materials with precisely determined electronic structure and phonon dispersion” (2012)
  • Author(s): T. Takeuchi
  • Total Pages: 25
  • Publisher: CRC Press
• [Book] 熱電変換技術の基礎と応用第2章 第5節 (2011)
  • Author(s): 竹内恒博, 他
  • Publisher: 株式会社 シーエムシー出版
• [Book] 熱電変換技術の基礎と応用-クリーンなエネルギー社会を目指して-第2章第5節フォノン分散の特徴から理解される格子熱伝導度低減機構 (2011)
  • Author(s): 竹内恒博, 他名
  • Publisher: 株式会社シーエムシー出版