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SHG studies of multi-ferroelectricity of hexagonal rare-earth ferrite thin films

Research Project

Project/Area Number 23540379
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics I
Research InstitutionWaseda University

Principal Investigator

UESU Yoshiaki  早稲田大学, 理工学術院, 名誉教授 (10063744)

Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2013: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2012: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2011: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywords強誘電体 / マルチフェロ物質 / 強弾性体 / SHG顕微鏡 / 薄膜 / 希土類フェライト / 錫ペロブスカイト酸化物 / チタン酸カルシウム / ドメイン / ドメイン境界 / 国際情報交流、フランス / 国際情報交流、イギリス / 国際情報交流、アメリカ
Research Abstract

Under this research project, the following three results were attained. (1)The coexistence of ferroelectricity and magnetic order in epitaxial hexagonal YbFeO3 thin films fabricated by the PLD method was experimentally found for the first time (published in J.Phys.Soc.Jpn. 2012) (2) Sn doped PbTiO3 thin films were successfully synthesized using a newly developed PLD method with three different ceramic targets. It was revealed that the films is a mixed state of SnTiO3, PbSnO3, and PbTiO3 and ferroelectrics with Tc of 277C. (3) The polar nature of twin boundaries (TBs) of inherently non-polar ferroelastic CaTiO3 was examined by the confocal SHG microscope. Three-dimensional SHG images confirmed that both crystallographically prominent TB and non-prominent TB are SHG active and consequently polar. The point group symmetries of the TBs and directions of the electric polarization are determined from the anisotropy of SHG intensities (published in Phys.Rev.B 2014).

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (37 results)

All 2014 2013 2012 2011 Other

All Journal Article (11 results) (of which Peer Reviewed: 11 results) Presentation (23 results) (of which Invited: 16 results) Book (1 results) Remarks (2 results)

  • [Journal Article] Direct evidence of polar nature of ferroelastic twin boundaries in CaTiO3 obtained by second harmonic generation microscope2014

    • Author(s)
      H. Yokota, H. Usami, R. Haumont, P. Hicher, J. Kaneshiro, E. K. H. Salje, and Y. Uesu
    • Journal Title

      Physical Review. B

      Volume: 89 Pages: 144109-144109

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Direct evidence of polar nature of ferroelastic twin boundaries in CaTiO3 obtained by second harmonic generation microscope2014

    • Author(s)
      H. Yokota, H. Usami, R. Haumont, P. Hicher, J. Kaneshiro, E. K. H. Salje, and Y. Uesu
    • Journal Title

      Physical Review B

      Volume: 89 Issue: 14 Pages: 144109-144109

    • DOI

      10.1103/physrevb.89.144109

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Identification of LiNbO3, LiNb3O8 and Li3NbO4 phases in thin films synthesized with different deposition techniques by means of XRD and Raman spectroscopy2013

    • Author(s)
      A. Bartasyte, V. Plausinaitiene, A. Abrutis, S. Stanionyte, S. Margueron, P. Boulet, T. Kobata, Y. Uesu, and J. Gleize
    • Journal Title

      Journal of Physics, Condensed Matter

      Volume: 25 Pages: 20590-20590

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Identification of LiNbO3, LiNb3O8 and Li3NbO4 phases in thin films synthesized with different deposition techniques by means of XRD and Raman spectroscopy2013

    • Author(s)
      A. Bartasyte, V. Plausinaitiene, A. Abrutis, S .Stanionyte, S. Margueron, P. Boulet, T. Kobata, Y. Uesu, J. Gleize
    • Journal Title

      J. Phys. Cond. Mat.

      Volume: -

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ferroelectricity and Ferrimagnetism of Hexagonal YbFeO3 Thin Films2012

    • Author(s)
      H. Iida, T. Koizumi, Y. Uesu, K. Kohn, N. Ikeda, S. Mori, R. Haumont, P.-E. Janolin, J. M. Kiat, M. Fukunaga, and Y. Noda
    • Journal Title

      Journal of Physical Society of Japan

      Volume: 81 Pages: 24719-24719

    • NAID

      210000109412

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Optical Second Harmonic Generation Microscopy as a Tool of Material Diagnosis2012

    • Author(s)
      H. Yokota, J. Kaneshiro, Y. Uesu
    • Journal Title

      Physics Research International, Invited Review paper

      Volume: 2012 Pages: 704634-12

    • DOI

      10.1155/2012/704634

    • Related Report
      2013 Final Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ferroelectricity and ferromagnetism of BaTiO3/BaFeO3 super-lattice thin films2012

    • Author(s)
      J. Fukatani, H. Yokota, Y. Uesu, M. Fukunaga, Y. Noda
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 51

    • NAID

      210000141238

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Polarization properties of bismuth strontium tantalate ceramic films deposited by aerosol deposition method2012

    • Author(s)
      M. Suzuki, Y. Nishihara, Y. Uesu, J. Akedo
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 51

    • NAID

      210000141235

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Ferroelectricity and ferromagnetism of BatiO3/BaFeO3 super-lattice thin films2012

    • Author(s)
      J. Fukatani, H. Yokota, Y. Uesu, M. Fukunaga, Y. Noda
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 51

    • NAID

      210000141238

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Polarization properties of bismuth strontium tantalate ceramic films deposited by aerosol deposition method2012

    • Author(s)
      M. Suzuki, Y. Nishihara, Y. Uesu, J. Akedo
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 51

    • NAID

      210000141235

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ferroelectricity and ferrimagnetism of hexagonal YbFeO3 thin films2012

    • Author(s)
      H.Iida
    • Journal Title

      J.Phys.Soc.Jpn

      Volume: 81 Issue: 2 Pages: 024719-024719

    • DOI

      10.1143/jpsj.81.024719

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Presentation] Polar nature of twin boundaries of inherently non-polar ferroelastic CaTiO3 evidenced by SHG microscope2014

    • Author(s)
      Y. Uesu
    • Organizer
      Electroceramics XIV
    • Place of Presentation
      ブカレスト, ルーマニア
    • Year and Date
      2014-06-17
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Sn-substituted perovskite oxide films - newly featured ferroelectrics -2013

    • Author(s)
      Y. Uesu
    • Organizer
      International Meeting of Ferroelectrics
    • Place of Presentation
      クラコフ, ポーランド
    • Year and Date
      2013-09-03
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] SHG microscope and its application to domain structure analyses of PZN/PT at the MPB2013

    • Author(s)
      Y. Uesu
    • Organizer
      International WS on relaxors
    • Place of Presentation
      Ioffe Physco-Technical Institute, サンクトペテルスブルグ, ロシア
    • Year and Date
      2013-07-05
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] SHG microscope revisited2012

    • Author(s)
      Y. Uesu
    • Organizer
      9th Korean-Japan Conference of Ferroelectricity
    • Place of Presentation
      蔚山, 韓国
    • Year and Date
      2012-08-12
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 光第2高調波顕微鏡でドメインを観る2012

    • Author(s)
      上江洲由晃
    • Organizer
      強誘電体応用会議
    • Place of Presentation
      京都コープホテル
    • Year and Date
      2012-05-24
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] SHGを利用した分域構造解析2012

    • Author(s)
      上江洲由晃
    • Organizer
      第67回日本物理学会年次大会
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-25
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] シンポジウム「分極反転が拓く光制御の未来」イントロダクトリートーク2012

    • Author(s)
      上江洲由晃
    • Organizer
      応用物理学会春季講演会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2012-03-15
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Ferroelectric (PbSnTi)O3 thin films synthesized by nucleation-mixture depositions and their structural and dielectric properties2012

    • Author(s)
      Y.Uesu
    • Organizer
      WS of fundamental physics of ferroelectricity
    • Place of Presentation
      Argonne National Laboratory, 米国
    • Year and Date
      2012-01-29
    • Related Report
      2013 Final Research Report
  • [Presentation] Ferroelectric (PbSnTi)O3 thin films synthesized by nucleation-mixture depositions and their structural and dielectric properties2012

    • Author(s)
      上江洲由晃
    • Organizer
      WS of fundamental physics of ferroelectricity
    • Place of Presentation
      米国、Argonne National Lboratory
    • Related Report
      2011 Research-status Report
  • [Presentation] Ferroelectricity and ferrimagnetism of thin-film stabilized hexagonal YbFeO32011

    • Author(s)
      Y.Uesu
    • Organizer
      強誘電体応用国際会議(ISAF2011)
    • Place of Presentation
      カナダ
    • Year and Date
      2011-07-27
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Ferroelectricity and ferrimagnetism of thin-film stabilized hexagonal YbFeO32011

    • Author(s)
      Yoshiaki UESU
    • Organizer
      ISAF2011(招待講演)
    • Place of Presentation
      カナダ、バンクーバー
    • Related Report
      2011 Research-status Report
  • [Presentation] SHG microscopy and its application to domain structure analyses of PZN/PT at the MPB

    • Author(s)
      上江洲由晃
    • Organizer
      International WS of relaxor ferroielectrics
    • Place of Presentation
      Ioffe Physico-Technical Institute, St. Petersburg, Russia
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Sn-substituted perovskite oxide films – newly featured ferroelectrics -

    • Author(s)
      上江洲由晃
    • Organizer
      International meeting of ferroelectrics and related materials
    • Place of Presentation
      Krakow, Poland
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Polar nature of twin boundaries of inherently non-polar ferroelastic CaTiO3 evidenced by SHG microscope

    • Author(s)
      上江洲由晃
    • Organizer
      Electronic Ceramics XIV
    • Place of Presentation
      Bucharest, Romani
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] SHG microscope revisited

    • Author(s)
      Y. Uesu
    • Organizer
      9th Korean-Japan Conference of Ferroelectricity
    • Place of Presentation
      Ulsan, Korea
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] SHGを利用した分域構造解析

    • Author(s)
      上江洲由晃
    • Organizer
      第67回日本物理学会年次大会
    • Place of Presentation
      関西学院大学
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] シンポジウム「分極反転が拓く 光制御の未来」イントロダクトリートーク

    • Author(s)
      上江洲由晃
    • Organizer
      応用物理学会春季講演会
    • Place of Presentation
      早稲田大学
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] 光第2高調波顕微鏡でドメインを観る

    • Author(s)
      上江洲由晃
    • Organizer
      強誘電体応用会議
    • Place of Presentation
      京都コープホテル
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] New approach to fabricate thin films using pulse laser deposition method

    • Author(s)
      H. Yokota, K. Ono, J. Iwasaki, Y. Uesu, P. E. Janolin, J. M. Kiat, R. Haumont
    • Organizer
      Joint International Workshop of WFF&WFSO
    • Place of Presentation
      北海道大学
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] 混合核形成法による強誘電(Pb-Sn-Ti)O3薄膜の作成、構造と誘電物性

    • Author(s)
      岩崎隼司, 上江洲由晃, 横田紘子, P. E. Janolin, J. M. Kiat, R. Haumont
    • Organizer
      第67回日本物理学会年次大会
    • Place of Presentation
      関西学院大学
    • Related Report
      2012 Research-status Report
  • [Presentation] SYMMETRY LOWERING OF LiNbO3/LiTaO3 SUPER-LATTICE THIN FILMS

    • Author(s)
      H. Yokota, T. Kobata, Y. Uesu, S. Huband, P. Thomas, A. M. Glazer, A. Bartasyte
    • Organizer
      International Symposium on Applications of Ferroelectrics
    • Place of Presentation
      Aveiro, Portugal
    • Related Report
      2012 Research-status Report
  • [Presentation] New ferroelectric phases induced by magnetic orderings in hexagonal YbFeO3 thin films

    • Author(s)
      Y. Uesu, H. Iida, T. Koizumi, K. Kohn, H. Yokota, M. Fukunaga, Y. Noda, R. Haumont, J. M. Kiat
    • Organizer
      15th EUROPEAN CONFERENCE ON COMPOSITE MATERIALS (ECCM-15)
    • Place of Presentation
      Venice, Italia
    • Related Report
      2012 Research-status Report
  • [Presentation] Designed multiferroics: BaTiO3/BaFeO3 super-lattice films

    • Author(s)
      H. Yokota, K. Fukatani, Y. Uesu, M. Fukunaga, Y. Noda
    • Organizer
      15th EUROPEAN CONFERENCE ON COMPOSITE MATERIALS (ECCM-15)
    • Place of Presentation
      Venice, Italia
    • Related Report
      2012 Research-status Report
  • [Book] 「物性物理学ハンドブック」リラクサー

    • Author(s)
      上江洲由晃
    • Total Pages
      11
    • Publisher
      朝倉書店
    • Related Report
      2013 Final Research Report 2012 Research-status Report
  • [Remarks] 上江洲研究室

    • URL

      http://www.uesu.phys.waseda.ac.jp

    • Related Report
      2012 Research-status Report
  • [Remarks] 現在成果をアップロード中。

    • Related Report
      2011 Research-status Report

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Published: 2011-08-05   Modified: 2020-05-15  

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