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Development of the novel liquid processing by combining an atmospheric-pressure microplasma with microbubbles

Research Project

Project/Area Number 23540582
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Plasma science
Research InstitutionTsuruoka National College of Technology

Principal Investigator

YOSHIKI Hiroyuki  鶴岡工業高等専門学校, その他部局等, その他 (00300525)

Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Fiscal Year 2013: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2012: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2011: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords大気圧プラズマ / 酸素ラジカル / 微細気泡 / 有機物分解 / 殺菌処理 / OHラジカル / プラズマ化学 / マイクロバブル / 気液界面反応 / 滅菌処理 / 水処理 / 液中プロセス / ラジカル反応 / 水浄化
Research Abstract

Atmospheric-pressure microplasma flow was generated between a surgical needle electrode and GND by a pulsed high voltage. Decolorization of an indigo carmine solution, sterilization of E-coil and bacteria and synthesis of graphite oxide were studied using microbubbles of the plasma gas. Since ozone production efficiency is low and the ozone concentration dissolved in water is less than 0.25 ppm, it suggests the possibility of water treatment without using dense ozone. In O2 plasma bubbling, rapid oxidation occurs due to O radicals. On the other hand, N2/O2 plasma bubbling shows organic compounds were decomposed slowly via introducing nitroso groups with NO2 ions under weak acidity. Furthermore, ESR measurement and chemical probe method using terephthalic acid showed OH radicals generated in water by the O2 plasma bubbling.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (27 results)

All 2014 2013 2012 2011

All Journal Article (5 results) (of which Peer Reviewed: 3 results) Presentation (19 results) Book (2 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] 大気圧高周波プラズマによるガラス細管内壁の二酸化チタンコーティング2014

    • Author(s)
      吉木宏之, 乙坂佳輝
    • Journal Title

      J. Vac. Soc. Jpn

      Volume: 57(4) Pages: 163-166

    • NAID

      130004952512

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] 大気圧高周波プラズマによるガラス細管内壁の二酸化チタンコーティング2014

    • Author(s)
      吉木宏之、乙坂佳輝
    • Journal Title

      J. Vac. Soc. Jpn. (真空)

      Volume: 57 Pages: 163-166

    • NAID

      130004952512

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 特集 : 排水処理・汚泥除去技術"大気圧プラズマとマイクロバブルの融合による水処理技術の試み"2013

    • Author(s)
      吉木宏之
    • Journal Title

      食品工業

      Volume: 第 56巻 第14号 Pages: 59-65

    • Related Report
      2013 Final Research Report
  • [Journal Article] 大気圧プラズマとマイクロバブルの融合による水処理技術の試み2013

    • Author(s)
      吉木宏之
    • Journal Title

      食品工業

      Volume: 56 Pages: 59-65

    • Related Report
      2013 Annual Research Report
  • [Journal Article] パルスマイクロ放電を用いたプラスチック製マイクロ流路チップ内壁処理2012

    • Author(s)
      吉木宏之
    • Journal Title

      J. Vac. Soc. Jpn. (真空)

      Volume: 55(3) Pages: 121-124

    • NAID

      10030337415

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Presentation] Water Treatment by Bubbling of Atmospheric- Pressure Plasma Radical Flow2014

    • Author(s)
      H. Yoshiki, K. Sato, Syafiq and T. Sugawara
    • Organizer
      8th Inter- national Conference on Reactive Plasmas/ 31st Symposium on Plasma Processing
    • Place of Presentation
      Fukuoka, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] プラズマラジカル流のバブリングによる水処理の研究[2]2014

    • Author(s)
      吉木宏之, 板垣 伸, 五十嵐 侑
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学
    • Related Report
      2013 Final Research Report
  • [Presentation] Water Treatment by Bubbling of Atmospheric-Pressure Plasma Radical Flow2014

    • Author(s)
      H. Yoshiki, K. Sato, Syafiq and T. Sugawara
    • Organizer
      8th International Conference on Reactive Plasmas/ 31st Symposium on Plasma Processing (ICRP-8/SPP-31)
    • Place of Presentation
      福岡国際会議場
    • Related Report
      2013 Annual Research Report
  • [Presentation] プラズマラジカル流のバブリングによる水処理の研究 [2]2014

    • Author(s)
      吉木宏之、板垣 伸、五十嵐 侑
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] Modification of inner walls of a commercial microfluidic chip by pulsed micro plasma treatment2013

    • Author(s)
      H. Yoshiki
    • Organizer
      21th Inter- national Symposium on Plasma Chemistry
    • URL

      http://www.ispc-conference.org/ProceedingsID527

    • Place of Presentation
      Cairns, Australia
    • Related Report
      2013 Final Research Report
  • [Presentation] プラズマラジカル流のバブリングによる大腸菌群の殺菌処理2013

    • Author(s)
      吉木宏之
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学
    • Related Report
      2013 Annual Research Report 2013 Final Research Report
  • [Presentation] プラズマラジカル流のバブリングによる水処理の研究2013

    • Author(s)
      吉木宏之, 佐藤航平
    • Organizer
      第60回応用物理学会春季学術講演会
    • Place of Presentation
      神奈川工科大学
    • Related Report
      2013 Final Research Report 2012 Research-status Report
  • [Presentation] プラズマガスのバブリングによる水処理の研究2013

    • Author(s)
      佐藤航平, シャフィック, 吉木宏之
    • Organizer
      第18回高専シンポジウムin仙台
    • Place of Presentation
      仙台高専
    • Related Report
      2013 Final Research Report
  • [Presentation] Modification of inner walls of a commercial microfluidic chip by pulsed micro plasma treatment2013

    • Author(s)
      H. Yoshiki
    • Organizer
      21th International Symposium on Plasma Chemistry (ISPC 21)
    • Place of Presentation
      オーストラリア、ケアンズ
    • Related Report
      2013 Annual Research Report
  • [Presentation] Study on Water Treatment by Atmospheric-Pressure Plasma Gas Bubbling2013

    • Author(s)
      H. Yoshiki、K. Sato、Syafiq
    • Organizer
      The 30th Symposium on Plasma Processing (SPP-30)
    • Place of Presentation
      アクトシティ、浜松市
    • Related Report
      2012 Research-status Report
  • [Presentation] プラズマガスのバブリングによる水処理の研究2013

    • Author(s)
      佐藤航平、シャフィック、吉木宏之
    • Organizer
      第18回高専シンポジウムin仙台
    • Place of Presentation
      仙台高専名取キャンパス
    • Related Report
      2012 Research-status Report
  • [Presentation] Plasma- Microbubble Generator for Water Purification2012

    • Author(s)
      H. Yoshiki, K. Okuda and K. Sato
    • Organizer
      4th International Conference on Plasma Medicine
    • Place of Presentation
      Orleans, France
    • Year and Date
      2012-06-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Decolorization of Indigo Carmine Solution Using Plasma- Microbubbles2012

    • Author(s)
      H. Yoshiki and S. Ishikawa
    • Organizer
      The 5th International Conference on Plasma-Nanotechnology & Science
    • Place of Presentation
      Aichi, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] プラズマ・マイクロバブルを用いたインジゴカルミン水溶液の脱色2012

    • Author(s)
      吉木宏之, 奥田航紀, 佐藤一誠, 石川修一, 矢作友弘, 瀬川透
    • Organizer
      第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学
    • Related Report
      2013 Final Research Report 2011 Research-status Report
  • [Presentation] Plasma-Microbubble Generator for Water Purification2012

    • Author(s)
      H. Yoshiki, K. Okuda and K. Sato
    • Organizer
      4th International Conference on Plasma Medicine
    • Place of Presentation
      Orleans, France
    • Related Report
      2012 Research-status Report
  • [Presentation] Decolorization of Indigo Carmine Solution Using Plasma-Microbubbles2012

    • Author(s)
      H. Yoshiki and S. Ishikawa
    • Organizer
      The 5th International Conference on Plasma-Nanotechnology & Science (IC-PLANTS 2012)
    • Place of Presentation
      愛知県犬山市
    • Related Report
      2011 Research-status Report
  • [Presentation] パルスマイクロ放電を用いたプラスチック製マイクロ流路チップ内壁処理2011

    • Author(s)
      吉木宏之
    • Organizer
      第52回真空に関する連合講演会
    • Place of Presentation
      学習院大学
    • Related Report
      2013 Final Research Report
  • [Presentation] Water purification technology by combining an atmospheric- pressure μplasma with microbubbles2011

    • Author(s)
      H. Yoshiki, S. Ishikawa
    • Organizer
      第24回プラズマ材料科学シンポジウム(SPSM-24)
    • Place of Presentation
      大阪大学
    • Related Report
      2013 Final Research Report
  • [Presentation] Water purification technology by combining an atmospheric-pressure μplasma with microbubbles2011

    • Author(s)
      H. Yoshiki and S. Ishikawa
    • Organizer
      第24回プラズマ材料科学シンポジウム (SPSM-24)
    • Place of Presentation
      大阪大学
    • Related Report
      2011 Research-status Report
  • [Book] 排水・汚水処理技術集成, 分筆部"プラズマラジカル流のバブリングを用いた水処理技術"2013

    • Author(s)
      吉木宏之, 他
    • Publisher
      (株)エヌ・ティー・エス出版
    • Related Report
      2013 Final Research Report
  • [Book] 排水・汚水処理技術集成 Vol. 22013

    • Author(s)
      吉木宏之、田中宏明 他 56名
    • Total Pages
      397
    • Publisher
      ㈱エヌ・ティー・エス
    • Related Report
      2013 Annual Research Report
  • [Patent(Industrial Property Rights)] 液体処理装置2012

    • Inventor(s)
      吉木宏之, 石川修一
    • Industrial Property Rights Holder
      独立行政法人 国立高等専門学校機構, 石川修一
    • Industrial Property Rights Type
      特許
    • Acquisition Date
      2012-10-05
    • Related Report
      2013 Final Research Report

URL: 

Published: 2011-08-05   Modified: 2019-07-29  

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