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Study on anisotropy and optimization of thermoelectric properties of thermoelectric materials by a Seebeck micro-probe method

Research Project

Project/Area Number 23560363
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionEhime University (2013)
Japan Advanced Institute of Science and Technology (2011-2012)

Principal Investigator

NAKAMOTO Go  愛媛大学, 教育学部, 准教授 (10283152)

Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2013: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2012: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2011: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords熱電変換材料 / マイクロプローブ法 / ゼーベック係数 / マイクロプローブ / サーマルプローブ / 熱電材料
Research Abstract

In this study, a two-dimensional Seebeck coefficient measurement system has been developed by a micro-probe method and two-dimensional distribution of Seebeck coefficient has evaluated for various thermoelectric materials. It is revealed that the anisotropic Seebeck coefficient reflecting the grain distribution in the zinc-antimonide system. In the bismuth-terullide system, it is found that the sign inversion of the Seebeck coefficient from p- to n-type occurs originating from the gradient of the excess Te content along the crystal growth direction. As a result, the evaluation method of microscopic thermoelectric properties has been established by using the Seebeck micro-probe method. It is expected that the Seebeck micro-probe method becomes one of the new and powerful ways for measurement of microscopic physical properties for various functional materials.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (21 results)

All 2013 2012 2011 Other

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (18 results)

  • [Journal Article] Development of a two dimensional scanning Seebeck coefficient measurement system by a micro-probe method2013

    • Author(s)
      G. Nakamoto, Y. Nakabayashi
    • Journal Title

      Intermetallics

      Volume: vol. 32 Pages: 233-238

    • DOI

      10.1016/j.intermet.2012.08.012

    • Related Report
      2013 Final Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Development of a measurement system for the figure of merit in the high-temperature region2013

    • Author(s)
      H. Iwasaki, T. Yamamoto, H. Kim, G. Nakamoto
    • Journal Title

      Journal of Electronic Materials

      Volume: vol. 42 Issue: 7 Pages: 1840-1845

    • DOI

      10.1007/s11664-012-2448-0

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Preparation of the crack-free single phase (Zn_<1-x>Cd_x)_<13>Sb_<10> by a gradient freeze method and their structural and thermoelectric properties2012

    • Author(s)
      G. Nakamoto, Y. Tajima, M. Kurisu
    • Journal Title

      Intermetallics

      Volume: vol. 23 Pages: 163-168

    • DOI

      10.1016/j.intermet.2011.11.021

    • Related Report
      2013 Final Research Report 2011 Research-status Report
    • Peer Reviewed
  • [Presentation] Effects of chemical composition and crystal texture on local Seebeck coefficient for various thermoelectric materials investigated by the Seebeck micro-probe method2013

    • Author(s)
      G. Nakamoto, Y. Nakabayashi
    • Organizer
      International Conference on Thermoelectrics
    • Place of Presentation
      神戸
    • Year and Date
      2013-07-01
    • Related Report
      2013 Final Research Report
  • [Presentation] コールドプローブ法を用いた走査型ゼーベック係数測定装置の開発2013

    • Author(s)
      仲林裕司, 中本剛
    • Organizer
      日本熱電学会
    • Place of Presentation
      名古屋大学
    • Related Report
      2013 Final Research Report
  • [Presentation] コールドプローブ法を用いた走査型ゼーベック係数測定装置の開発2013

    • Author(s)
      仲林裕司、中本剛
    • Organizer
      日本熱電学会
    • Place of Presentation
      名古屋大学(愛知県)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 走査型ゼーベック係数測定装置に用いる微小プローブの開発2012

    • Author(s)
      中本剛, 仲林裕司
    • Organizer
      応用物理学会
    • Place of Presentation
      愛媛大学
    • Year and Date
      2012-09-12
    • Related Report
      2013 Final Research Report
  • [Presentation] Fabrication of probe tips for a Seebeck micro-probe measurement system2012

    • Author(s)
      G. Nakamoto, Y. Nakabayashi
    • Organizer
      International Conference on Thermoelectrics
    • Place of Presentation
      Aalborg, Denmark
    • Year and Date
      2012-07-10
    • Related Report
      2013 Final Research Report
  • [Presentation] Development of measurement system for the figure of merit in high temperature region2012

    • Author(s)
      H. Iwasaki, T. Yamamoto, H. Kim, G. Nakamoto
    • Organizer
      International Conference on Thermoelectrics
    • Place of Presentation
      Aalborg, Denmark
    • Year and Date
      2012-07-10
    • Related Report
      2013 Final Research Report
  • [Presentation] ハーマン法による中温度領域における性能指数評価装置開発2012

    • Author(s)
      山本哲生, Hosung Kim, 鈴木聡, 中本剛, 岩崎秀夫
    • Organizer
      応用物理学会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2012-03-17
    • Related Report
      2013 Final Research Report
  • [Presentation] 走査型ゼーベック係数測定装置に用いる微小サーマルプローブの検討2012

    • Author(s)
      仲林裕司, 中本剛
    • Organizer
      第18回分子科学研究所技術研究会
    • Place of Presentation
      分子科学研究所
    • Year and Date
      2012-03-09
    • Related Report
      2013 Final Research Report
  • [Presentation] 二次元走査型ゼーベック係数評価装置に搭載する微小サーマルプローブの作製2012

    • Author(s)
      仲林裕司, 中本剛
    • Organizer
      日本熱電学会
    • Place of Presentation
      東京工業大学
    • Related Report
      2013 Final Research Report
  • [Presentation] 二次元走査型ゼーベック係数評価装置に搭載する微小サーマルプローブの作製2012

    • Author(s)
      仲林 裕司、中本 剛
    • Organizer
      日本熱電学会
    • Place of Presentation
      東京工業大学(東京都)
    • Related Report
      2012 Research-status Report
  • [Presentation] 走査型ゼーベック係数測定装置に用いる微小サーマルプローブの検討2012

    • Author(s)
      仲林 裕司
    • Organizer
      第18回分子科学研究所技術研究会
    • Place of Presentation
      分子科学研究所 (愛知県)
    • Related Report
      2011 Research-status Report
  • [Presentation] ハーマン法による中温度領域における性能指数評価装置開発2012

    • Author(s)
      岩崎 秀夫
    • Organizer
      応用物理学会
    • Place of Presentation
      早稲田大学 (東京都)
    • Related Report
      2011 Research-status Report
  • [Presentation] 微小プローブを用いた走査型ゼーベック係数評価装置の開発2011

    • Author(s)
      中本剛, 仲林裕司
    • Organizer
      日本熱電学会
    • Place of Presentation
      北海道大学
    • Related Report
      2013 Final Research Report
  • [Presentation] 微小プローブを用いた走査型ゼーベック係数評価装置の開発2011

    • Author(s)
      中本 剛
    • Organizer
      日本熱電学会
    • Place of Presentation
      北海道大学 (北海道)
    • Related Report
      2011 Research-status Report
  • [Presentation] Effects of chemical composition and crystal texture on local Seebeck coefficient for various thermoelectric materials investigated by the Seebeck micro-probe method

    • Author(s)
      G. Nakamoto, Y. Nakabayashi
    • Organizer
      International Conference on Thermoelectrics
    • Place of Presentation
      Kobe (Japan)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Fabrication of probe tips for a Seebeck micro-probe measurement system

    • Author(s)
      Go Nakamoto, Yuuji Nakabayashi
    • Organizer
      International conference on thermoelectrics
    • Place of Presentation
      Aalborg (Denmark)
    • Related Report
      2012 Research-status Report
  • [Presentation] Development of Measurement System for the Figure of Merit in High Temperature Region

    • Author(s)
      Hideo Iwasaki, Ttsuo Yamamoto, Ho-sung Kim, Go Nakamoto
    • Organizer
      International conference on thermoelectrics
    • Place of Presentation
      Aalborg (Denmark)
    • Related Report
      2012 Research-status Report
  • [Presentation] 走査型ゼーベック係数測定装置に用いる微小プローブの開発

    • Author(s)
      中本 剛、仲林 裕司
    • Organizer
      応用物理学会
    • Place of Presentation
      愛媛大学(愛媛県)
    • Related Report
      2012 Research-status Report

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Published: 2011-08-05   Modified: 2019-07-29  

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