Development of Metal/Semiconductor Cluster Sources Dedicated for Free Electron Laser Experiments

• Project/Area Number: 23600006
• Research Category: Grant-in-Aid for Scientific Research (C)
• Allocation Type: Multi-year Fund
• Section: 一般
• Research Field: Quantum beam science
• Research Institution: Kyoto University
• Principal Investigator: NAGAYA Kiyonobu 京都大学, 理学(系)研究科(研究院), 助教 (30273436)
• Project Period (FY): 2011 – 2013
• Project Status: Completed (Fiscal Year 2013)
• Budget Amount: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000); Fiscal Year 2013: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000); Fiscal Year 2012: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000); Fiscal Year 2011: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
• Keywords: 自由電子レーザー / クラスター

Research Abstract

We have constructed pulsed beam sources for producing giant rare-gas cluster and metal/semiconductor clusters dedicated for free electron laser (FEL) experiments. For giant rare-gas cluster, we have adopted supersonic jet type cluster source which has specially designed expansion nozzle. For metal/semiconductor elements, laser ablation type cluster source and liquid jet type source have been developed. Laser ablation source consists of intense pulse YAG laser, rotating sample disk and pulsed gas jet valve, that can produce relatively small cluster of non-volatile elements. High temperature liquid jet source has been designed to produce droplet of high temperature (up to 200 oC) liquid by modifying solenoid valve source. We are testing performance of apparatus for the use of FEL experiments such as electron spectroscopy, pump-probe measurements, x-ray scattering experiment, etc.

Research Products

• [Journal Article] Pulse delay effect in angular distribution of near-threshold EUV+IR two-photon ionization of Ne (2014)
  • Author(s): S. Mondal, H. Fukuzawa, K. Motomura, T. Tachibana, K. Nagaya, T. Sakai, K. Matsunami, S. Yase, M. Yao, S. Wada, H. Hayashita, N. Saito, C. Callegari, K. Prince, C. Miron, M. Nagasono, K. L. Ishikawa, A. K. Kazansky, N. M. Kabachnik and K. Ueda.
  • Journal Title: Phys. Rev. Volume: A 89 Pages: 13415-13415
  • Peer Reviewed
• [Journal Article] Pulse delay effect in angular distribution of near-threshold EUV+IR two-photon ionization of Ne (2014)
  • Author(s): S. Mondal, H. Fukuzawa, K. Motomura, T. Tachibana, K. Nagaya, T. Sakai, K. Matsunami, S. Yase, M. Yao, S. Wada, H. Hayashita, N. Saito, C. Callegari, K. C. Prince, C. Miron, M. Nagasono, T. Togashi, M. Yabashi, K. L. Ishikawa, A. K. Kazansky, N. M. Kabachnik, and K. Ueda
  • Journal Title: Phys. Rev. A Volume: 89 Issue: 1
  • DOI: 10.1103/physreva.89.013415
  • Peer Reviewed
• [Journal Article] Deep inner-shell multiphoton absorption by intense x-ray free-electron laser pulses (2013)
  • Author(s): H. Fukuzawa, S.-K. Son, K. Motomura, S. Mondal, K. Nagaya, S. Wada, X.-J. Liu, R. Feifel, T. Tachibana, Y. Ito, M. Kimura, T. Sakai, K. Matsunami, H. Hayashita, J. Kajikawa, P. Johnsson, M. Siano, E. Kukk, B. Rudek, B. Erk, L. Foucar, E. Robert, C. Miron, K. Tono, T. Togashi, Y. Inubushi, T. Sato, T. Katayama, T. Hatsui, T. Kameshima, M. Yabashi, M. Yao, R. Santra, and K. Ueda.
  • Journal Title: Phys. Rev. Lett. Volume: 110 Pages: 173005-173005
  • Peer Reviewed
• [Journal Article] Photoelectron Angular Distributions for Two-photon Ionization of Helium by Ultrashort Extreme Ultraviolet Free Electron Laser Pulses (2013)
  • Author(s): R. Ma, K. Motomura, K.L. Ishikawa, S. Mondal, H. Fukuzawa, A. Yamada, K. Ueda, K. Nagaya, S. Yase, Y. Mizoguchi, M. Yao, A. Rouz´ee, A. Hundermark, M.J.J. Vrakking, P. Johnsson, M. Nagasono, K. Tono, T. Togashi, Y. Senba, H. Ohashi, M. Yabashi, and T. Ishikawa.
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 46 Pages: 164018-164018
  • Peer Reviewed
• [Journal Article] Frustration of photoionization of Ar nanoplasma produced by extreme ultraviolet FEL pulses (2013)
  • Author(s): H Iwayama, K Nagaya, M Yao, H Fukuzawa, X-J Liu, G Pruemper, K Ueda, K Motomura, K. Ueda, N Saito, A Rudenko, L Foucar, M Nagasono, A Higashiya, M Yabashi, T Ishikawa, H Ohashi and H Kimura.
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 46 Pages: 164019-164019
  • Peer Reviewed
• [Journal Article] Photoelectron angular distributions for two-photon sequential double ionization of xenon by ultrashort extreme ultraviolet free electron laser pulses (2013)
  • Author(s): S Mondal, R Ma, K Motomura, H Fukuzawa, A Yamada, K Nagaya, S Yase, Y Mizoguchi, M Yao, A Rouz´ee, A Hundertmark, M J J Vrakking, P Johnsson, M Nagasono, K Tono, T Togashi, Y Senba, H Ohashi, M Yabashi, T Ishikawa, I P Sazhina, S Fritzsche, N M Kabachnik and K Ueda.
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 46 Pages: 164022-164022
  • Peer Reviewed
• [Journal Article] Unusual Under-threshold Ionization of Neon Clusters Studied by Ion Spectroscopy (2013)
  • Author(s): K. Nagaya, A. Sugishima, H. Iwayama, H. Murakami, M. Yao, H. Fukuzawa, X.-J. Liu, K. Motomura, K. Ueda, N. Saito, L. Foucar, A. Rudenko, M. Kurka, K.-U. Kühne, J. Ullrich, A. Czasch, R. Dörner, R. Feifel, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, T. Togashi, H. Kimura, and H. Ohashi.
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 46 Pages: 164023-164023
  • Peer Reviewed
• [Journal Article] Sequential multiphoton multiple ionization of atomic argon and xenon irradiated by x-ray free-electron laser pulses from SACLA (2013)
  • Author(s): K. Motomura, H. Fukuzawa, S-K. Son, S. Mondal, T. Tachibana, Y. Ito, M. Kimura, K. Nagaya, T. Sakai, K. Matsunami, S. Wada, H. Hayashita, J. Kajikawa, X-J. Liu, R. Feifel, P. Johnsson, M. Siano, E. Kukk, B. Rudek, B. Erk, L. Foucar, E. Robert, C. Miron, K. Tono, Y. Inubushi, T. Hatsui, M. Yabashi, M. Yao, R. Santra, K. Ueda.
  • Journal Title: J. Phys. B : At. Mol. Opt. Phys. Volume: 46 Pages: 164024-164024
  • Peer Reviewed
• [Journal Article] Crossover in the Photo-ionization Processes of Ne Clusters with Increasing EUV-FEL Intensity (2013)
  • Author(s): S. Yase, K. Nagaya, Y. Mizoguchi, M. Yao, H. Fukuzawa, K. Motomura, A. Yamada, Ri Ma, K. Ueda, N. Saito, M. Nagasono, T. Togashi, K. Tono, M. Yabashi, T. Ishikawa, H. Ohashi, and Y. Senba.
  • Journal Title: Phys. Rev. Volume: A 88 Pages: 43203-43203
  • Peer Reviewed
• [Journal Article] Unusual Under-threshold Ionization of Neon Clusters Studied by Ion Spectroscopy (2013)
  • Author(s): K.Nagaya, A. Sugishima, H. Iwayama, H. Murakami, M. Yao, H. Fukuzawa, X.-J. Liu, K. Motomura, K. Ueda, N. Saito, L. Foucar, A. Rudenko, M. Kurka, K.-U. Kuehnel, J. Ullrich, A. Czasch, R. Doerner, R. Feifel, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, T. Togashi, H. Kimura, and H. Ohashi
  • Journal Title: J. Phys. B: At. Mol. Opt. Phy Volume: 46 Issue: 16 Pages: 164023-164023
  • DOI: 10.1088/0953-4075/46/16/164023
  • Peer Reviewed
• [Journal Article] Frustration of photoionization in Ar nanoplasma produced by extreme ultraviolet FEL pulses (2013)
  • Author(s): H. Iwayama, K. Nagaya, M. Yao, H. Fukuzawa, X.-J. Liu, G. Prümper, K. Motomura, K. Ueda, N. Saito, A. Rudenko, L. Foucar, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, H. Ohashi, H. Kimura
  • Journal Title: J. Phys. B: At. Mol. Opt. Phys. Volume: 46 Issue: 16 Pages: 1640191-6
  • DOI: 10.1088/0953-4075/46/16/164019
  • Peer Reviewed
• [Journal Article] Deep inner-shell multiphoton ionization by intense x-ray free-electron laser pulses (2013)
  • Author(s): H. Fukuzawa, S.-K. Son, K. Motomura, S. Mondal, K. Nagaya, (23名 ) M. Yao, R. Santra, and K. Ueda
  • Journal Title: Phys. Rev. Letts. Volume: 110 Issue: 17
  • DOI: 10.1103/physrevlett.110.173005
  • Peer Reviewed
• [Journal Article] Crossover in the Photo-ionization Processes of Ne Clusters with Increasing EUV-FEL Intensity (2013)
  • Author(s): S. Yase, K. Nagaya, Y. Mizoguchi, M. Yao, H. Fukuzawa, K. Motomura, A. Yamada, R. Ma, K. Ueda, N. Saito, A. Rouzee, A. Hundermark, M. Vrakking, P. Johnsson , M. Nagasono, T. Togashi, K. Tono, M. Yabashi, T. Ishikawa, H. Ohashi , Y. Senba
  • Journal Title: Phys. Rev. A Volume: 88 Issue: 4
  • DOI: 10.1103/physreva.88.043203
  • Peer Reviewed
• [Journal Article] Anomalous signal from sulphur atoms in protein crystallographic data from an X-ray free-electron laser (2013)
  • Author(s): T. Barends, L. Foucar, R. Shoeman, S. Bari, S. Epp, R. Hartmann, G. Hauser, M. Huth, C. Kieser, L. Lomb, K. Motomura, K. Nagaya, C. Schmidt, R. Strecker, D. Anielski, R. Boll, B. Erk, H. Fukuzawa, S. Wada, I. Schlichting 他25名
  • Journal Title: Acta Crystallographica Section D Volume: 69 Issue: 5 Pages: 838-842
  • DOI: 10.1107/s0907444913002448
  • Peer Reviewed
• [Journal Article] Charge and Energy Transfer in Ar core-Ne shell clusters irradiated by Free Electron Laser Pulses at 62 nm (2012)
  • Author(s): A. Sugishima, H. Iwayama, H. Murakami, K. Nagaya, M. Yao, H. Fukuzawa, X.-J. Liu, K. Motomura, K. Ueda, N. Saito, L. Foucar, A. Rudenko, M. Kurka, K.-U. Kuehnel, J. Ullrich, A. Czasch, R. Doerner, R. Feifel, M. Nagasono, A. Higashiya, M. Yabashi, T. Ishikawa, T. Togashi, H. Kimura, and H. Ohashi.
  • Journal Title: Phys. Rev. Volume: A 86 Pages: 33203-33203
  • Peer Reviewed
• [Journal Article] Charge and Energy Transfer in Ar core-Ne shell clusters irradiated by Free Electron Laser Pulses at 62 nm (2012)
  • Author(s): A. Sugishima, H. Iwayama, H. Murakami, K. Nagaya, M. Yao 他20名
  • Journal Title: Phys. Rev. A Volume: 86 Issue: 3 Pages: 33203-33203
  • DOI: 10.1103/physreva.86.033203
  • Peer Reviewed
• [Journal Article] Ultra-Efficient Ionization of Heavy Atoms by Intense X-Ray Free-Electron Laser Pulses (2012)
  • Author(s): Benedikt Rudek, Kiyonobu Nagaya 他54名
  • Journal Title: Nature Photonics Volume: 6 Issue: 12 Pages: 858-865
  • DOI: 10.1038/nphoton.2012.261
  • Peer Reviewed
• [Journal Article] Doubly resonant three-photon double ionization of Ar atoms induced by an EUV free-electron laser (2011)
  • Author(s): E. V. Gryzlova, Ri Ma, H. Fukuzawa, K. Motomura, A. Yamada, K. Ueda, A. N. Grum-Grzhimailo, N. M. Kabachnik, S. I. Strakhova, A. Rouz´ee, A. Hundertmark, M. J. J. Vrakking, P. Johnsson, K. Nagaya, S. Yase, Y. Mizoguchi, M. Yao, M. Nagasono, K. Tono, T. Togashi, Y. Senba, H. Ohashi, M. Yabashi, and T. Ishikawa.
  • Journal Title: Phys. Rev. Volume: A84 Pages: 63405-63405
  • Peer Reviewed
• [Journal Article] Doubly resonant three-photon double ionization of Ar atoms induced by an EUV free-electron laser (2011)
  • Author(s): E. V. Gryzlova, K. Nagaya, 他22名
  • Journal Title: Phys Rev A Volume: 84 Pages: 63405-63405
  • Peer Reviewed
• [Journal Article] Second-order autocorrelation of XUV FEL pulses via time resolved two-photon single ionization of He (2011)
  • Author(s): R. Moshammer, M.Nagaya 他30名
  • Journal Title: OPTICS EXPRESS Volume: 19 Pages: 21698-21706
  • Peer Reviewed
• [Journal Article] Metallic-like droplets produced by irradiating rare-gas clusters with free electron laser pulses (2011)
  • Author(s): M.Yao , K Nagaya 他5名
  • Journal Title: Eur. Phys. J. Special Topics Volume: 196 Pages: 175-180
  • Peer Reviewed
• [Presentation] SCSS試験加速器による希ガスクラスターからのナノプラズマ生成とダイナミクス (2014)
  • Author(s): 永谷清信、酒井司、西山俊幸、松波健司、八瀬哲志、八尾誠、福澤宏宣、本村幸治、立花哲也、上田潔、和田真一、林下弘憲、齋藤則生、永園充、富樫格、登野健介、矢橋牧名、石川哲也、大橋治彦、仙波泰徳
  • Organizer: 軟X線光化学研究会
  • Place of Presentation: SPring8上坪講堂(兵庫県佐用郡)
  • Year and Date: 2014-02-01
• [Presentation] SACLAのフェムト秒XFELパルスによる原子・分子・クラスターの多光子吸収ダイナミクス (2014)
  • Author(s): 永谷清信
  • Organizer: SPring-8利用ワークショップ--SPring-8とユーザーのさらなる連携を目指して
  • Place of Presentation: SPring8上坪講堂(兵庫県佐用郡)
  • Year and Date: 2014-02-01
• [Presentation] EUV-FELパルス照射によるネオン・クラスターのナノプラズマ化とダイナミクス計測 (2014)
  • Author(s): 永谷清信、西山俊幸、八尾誠、松波健司、酒井司、福澤宏宣、本村幸治、立花哲也、上田潔、和田真一、富樫格
  • Organizer: 第27回放射光学会年会・放射光化学合同シンポジウム
  • Place of Presentation: 広島国際会議場(広島県広島市)
  • Year and Date: 2014-01-11
• [Presentation] EUV-FELパルス照射によるネオン・クラスターのナノプラズマ化とダイナミクス計測 (2014)
  • Author(s): 永谷清信
  • Organizer: 第27回放射光学会年会・放射光化学合同シンポジウム
  • Place of Presentation: 広島国際会議場 （広島県広島市）
• [Presentation] SCSS試験加速器による希ガスクラスターからのナノプラズマ生成とダイナミクス (2014)
  • Author(s): 永谷清信
  • Organizer: 軟X線光化学研究会
  • Place of Presentation: SPring8 上坪講堂 （兵庫県佐用郡）
  • Invited
• [Presentation] SACLAのフェムト秒XFELパルスによる原子・分子・クラスターの 多光子吸収ダイナミクス (2014)
  • Author(s): 永谷清信
  • Organizer: SPring-8利用ワークショップ --SPring-8とユーザーのさらなる連携を目指して
  • Place of Presentation: SPring8 上坪講堂 （兵庫県佐用郡）
  • Invited
• [Presentation] EUV-FEL光励起により誘起されるネオンクラスターでのresonant ICDとナノプラズマ形成 (2013)
  • Author(s): 永谷清信、八尾誠、松波健司、酒井司、福澤宏宣、本村幸治、立花哲也、Subhend Mondal、上田潔、和田真一、齋藤則生、Kevin Prince、Carlo Callegari、Catalin Miron、永園充
  • Organizer: 物理学会第68回年次大会
  • Place of Presentation: 広島大学東広島キャンパス
• [Presentation] EUV-FEL照射によるXeクラスターの多価イオン化とナノプラズマ生成のダイナミクス (2013)
  • Author(s): 永谷清信,酒井司,松波健司,八瀬哲志,八尾誠,福澤宏宣,本村幸治,上田潔,和田真一,林下弘憲,斎藤則生,永園充,富樫格,登野健介,矢橋牧名,石川哲也,大橋治彦,仙波泰徳
  • Organizer: 第26回放射光学会年会・放射光化学合同シンポジウム
  • Place of Presentation: 名古屋大学(名古屋市千種区不老町)
• [Presentation] Nano-plasma Formation and Thermal Electron Emission of Neon Clusters Induced by Extreme Ultraviolet Free Electron Laser Pulses (2013)
  • Author(s): K. Nagaya, S. Yase, Y. Mizoguchi, M. Yao, H. Fukuzawa, K. Motomura, A. Yamada, R. Ma, K. Ueda, N. Saito, A. Rouzee , A. Hundertmark, M. Vrakking , P. Johnsson, M. Nagasono, T. Togashi, K. Tono, M. Yabashi, T. Ishikawa, H. Ohashi, Y. Senba.
  • Organizer: XXVIII International Conference on Photonic, Electronic and Atomic Collisions
  • Place of Presentation: Lanzhou, China
• [Presentation] Electron Spectroscopic Study of Multiple Photoionization Processes of Xe Clusters by Intense EUV-FEL Pulses (2013)
  • Author(s): K. Nagaya, K. Matsunami, T. Sakai, S. Yase, M. Yao, H. Fukuzawa, K. Motomura, K. Ueda, S. Wada, H. Hayashita,, N. Saito, M. Nagasono, T. Togashi, K. Tono , M. Yabashi, T. Ishikawa, H. Ohashi , Y. Senba.
  • Organizer: XXVIII International Conference on Photonic, Electronic and Atomic Collisions
  • Place of Presentation: Lanzhou, China
• [Presentation] Dynamics of multiple photoionization of rare-gas clusters caused by intense EUV-FEL pulses (2013)
  • Author(s): K. Nagaya.
  • Organizer: VI International Symposium on Atomic Cluster Collisions (ISACC 2013)
  • Place of Presentation: Wuhan-Chongqing, China
• [Presentation] EUV-pump - NIR-probe experiments of xenon cluster (2013)
  • Author(s): T. Sakai, K. Matsunami, K. Nagaya, S. Yase, M. Yao, H. Fukuzawa, K. Motomura, K. Ueda, S. Wada, H. Hayashita, N. Saito, M. Nagasono.
  • Organizer: 38th International conference on Vacuum Ultraviolet and X-ray Physics
  • Place of Presentation: Hefei, China
• [Presentation] EUV-FEL照射によるXe クラスターの多価イオン化とナノプラズマ生成のダイナミクス (2013)
  • Author(s): 永谷清信
  • Organizer: 第26回放射光学会年会・放射光化学合同シンポジウム
  • Place of Presentation: 名古屋大学
• [Presentation] Multiple ionization, electronic decay and charge migration in clusters (2012)
  • Author(s): K. Nagaya.
  • Organizer: Satellite workshop of 2nd Japanese-German Presidents'Conference
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2012-03-28
• [Presentation] 極紫外自由電子レーザー照射により誘起される希ガスクラスターの励起子モット転移II (2012)
  • Author(s): 永谷清信、八尾誠、八瀬哲志、酒井司、松波健司、溝口悠里、福澤宏宣、本村幸治、立花哲也、Subhend Mondal、山田綾子、Ri Ma、上田潔、齋藤則生、Arnaud Rouzee、Axel Hundermark、Marc Vrakking、Per Johnsson、和田真一、Kevin Prince、Carlo Callegari、Catalin Miron、永園充、登野健介,富樫格、矢橋牧名、石川哲也、大橋治彦、仙波泰徳
  • Organizer: 物理学会秋季大会
  • Place of Presentation: 横浜国立大
• [Presentation] ネオン・クラスターのEUV-FEL誘起イオン化のクロスオーバー (2012)
  • Author(s): 八瀬哲志、八尾誠他20名
  • Organizer: 第25回放射光学会年会・放射光化学合同シンポジウム
  • Place of Presentation: 佐賀県 鳥栖市民文化会館・中央公民館
• [Presentation] Cluster experiments at SCSS : present status and perspective (2011)
  • Author(s): K. Nagaya.
  • Organizer: JSPS-DFG Bilateral Seminar
  • Place of Presentation: Kyoto, Japan
  • Year and Date: 2011-10-10
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 物理学会秋季大会
  • Place of Presentation: 富山大学
  • Year and Date: 2011-09-24
• [Presentation] Dynamics of multiple photoionization of rare-gas clusters caused by intense EUV-FEL pulses (2011)
  • Author(s): K. Nagaya.
  • Organizer: International workshop DyNano2011"Structure and Dynamics of Nano-objects using short wavelength radiation"
  • Place of Presentation: Kyoto, Japan
• [Presentation] Dynamics of multiple photoionization of rare-gas clusters caused by intense EUV-FEL pulses (2011)
  • Author(s): Kiyonobu Nagaya
  • Organizer: International workshop DyNano2011(招待講演)
  • Place of Presentation: Kyoto, Japan
• [Presentation] EUV-FELによるクラスターの多重イオン化とダイナミクス (2011)
  • Author(s): 永谷清信
  • Organizer: 日本物理学会 秋季大会(招待講演)
  • Place of Presentation: 富山大学
• [Presentation] 極紫外自由電子レーザー照射により誘起される希ガスクラスターの励起子モット転移II
  • Author(s): 永谷清信
  • Organizer: 日本物理学会 秋季大会
  • Place of Presentation: 横浜国立大学
• [Presentation] EUV-FEL光励起により誘起されるネオンクラスターでのresonant ICDとナノプラズマ形成
  • Author(s): 永谷清信
  • Organizer: 日本物理学会第68回年次大会
  • Place of Presentation: 広島大学 東広島キャンパス