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Visualization of valence electron density distribution by quadrupole scattering measurement

Research Project

Project/Area Number 23654127
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Condensed matter physics II
Research InstitutionThe Institute of Physical and Chemical Research

Principal Investigator

OHSUMI Hiroyuki  独立行政法人理化学研究所, 高田構造科学研究室, 専任研究員 (90360825)

Project Period (FY) 2011 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2012: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2011: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
KeywordsX線回折 / 偏光依存性 / 消衰効果 / 多波回折 / 電荷整列 / 軌道整列 / X線回折 / 電子密度解析 / 放射線、X線、粒子線
Research Abstract

The aim of this study is to detect non-Thomson scattering, which plays a key role in selective measurement of scattered X-rays only from valence electrons, by utilizing polarization properties of synchrotron radiation and improving polarization control/measurement techniques. From the dependence of diffraction intensity on incident X-ray polarization, it has been found that the super-lattice reflection arising from orbital ordering in manganites is attributed to non-Thomson scattering. In addition, it has been demonstrated that the effect of extinction can be independently evaluated for every reflection.

Report

(3 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Research-status Report
  • Research Products

    (20 results)

All 2013 2012 Other

All Journal Article (8 results) (of which Peer Reviewed: 4 results) Presentation (12 results) (of which Invited: 1 results)

  • [Journal Article] Tetrahedral Magnetic Order and the Metal-Insulator Transition in the Pyrochlore Lattice of Cd_2Os_2O_72012

    • Author(s)
      J. Yamaura, K. Ohgushi, H. Ohsumi, T. Hasegawa, I. Yamauchi, K. Sugimoto, S. Takeshita, A. Tokuda, M. Takata, M. Udagawa, M. Takigawa, H. Harima, T. Arima, and Z. Hiroi
    • Journal Title

      Phys. Rev. Lett

      Volume: 108 Pages: 247205-247205

    • Related Report
      2012 Final Research Report
  • [Journal Article] Two-dimensional Heisenberg behavior of J_<eff>=1/2 isospins in the paramagnetic state of spin-orbit Mott insulator Sr_2IrO_42012

    • Author(s)
      S. Fujiyama, H. Ohsumi, T. Komesu, J. Matsuno, B. J. Kim, M. Takata, T. Arima, and H. Takagi
    • Journal Title

      Phys. Rev. Lett

      Volume: 108 Pages: 247212-247212

    • Related Report
      2012 Final Research Report
  • [Journal Article] Orbital structures in spinel vanadates AV_2O_4 (A=Fe, Mn)2012

    • Author(s)
      Y. Nii, H. Sagayama, T, Arima, S. Aoyagi, R. Sakai, S. Maki, E. Nishibori, H. Sawa, K. Sugimoto, H. Ohsumi, and M. Takata
    • Journal Title

      Phys. Rev

      Volume: B 86 Pages: 125142-125142

    • Related Report
      2012 Final Research Report
  • [Journal Article] Weak antiferromagnetism of J_<eff>=1/2 band in bilayer iridate Sr_3Ir_2O_72012

    • Author(s)
      S. Fujiyama, K. Ohashi, H. Ohsumi, K. Sugimoto, T. Takayama, T. Komesu, M. Takata, T. Arima, and H. Takagi
    • Journal Title

      Phys. Rev

      Volume: B 86 Pages: 174414-174414

    • Related Report
      2012 Final Research Report
  • [Journal Article] Tetrahedral Magnetic Order without Spatial Symmetry Breaking in the Pyrochlore Lattice of Cd2Os2O72012

    • Author(s)
      J. Yamaura, K. Ohgushi, H. Ohsumi, T. Hasegawa, I. Yamauchi, K. Sugimoto, S. Takeshita, A. Tokuda, M. Takata, M. Udagawa, M. Takigawa, H. Harima, T. Arima, and Z. Hiroi
    • Journal Title

      Phys. Rev. Lett.

      Volume: 108 Issue: 24 Pages: 247205-247205

    • DOI

      10.1103/physrevlett.108.247205

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Two-Dimensional Heisenberg Behavior of Jeff = 1/2 Isospins in the Paramagnetic State of the Spin-Orbital Mott Insulator Sr2IrO42012

    • Author(s)
      S. Fujiyama, H. Ohsumi, T. Komesu, J. Matsuno, B. J. Kim, M. Takata, T. Arima, and H. Takagi
    • Journal Title

      Physical Review Letters

      Volume: 108 Issue: 24 Pages: 247212-247212

    • DOI

      10.1103/physrevlett.108.247212

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Orbital structures in spinel vanadates AV_2O_4 (A=Fe, Mn)2012

    • Author(s)
      Y.Nii, H. Sagayama, T. Arima, S. Aoyagi, R. Sakai, S. Maki, E.Nishibori, H. Sawa, K. Sugimoto, H. Ohsumi, M. Takata
    • Journal Title

      Physical Review B

      Volume: 86 Issue: 12

    • DOI

      10.1103/physrevb.86.125142

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Weak antiferromagnetism of Jeff=1/2 band in bilayer iridate Sr3Ir2O72012

    • Author(s)
      S. Fujiyama,H. Ohsumi et al.
    • Journal Title

      Phys. Rev. B

      Volume: 86 Issue: 17

    • DOI

      10.1103/physrevb.86.174414

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Presentation] Magnetic domain imaging in the frustrated all-in/all-out pyrochlore Cd_2Os_2O_72013

    • Author(s)
      Samuel Tardif、竹下聡史、大隅寛幸、山浦淳一、有馬孝尚
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島
    • Year and Date
      2013-03-29
    • Related Report
      2012 Final Research Report
  • [Presentation] Pr_<0.5>Ca_<0.5>MnO_3/La_<0.5>Sr_<0.5>MnO_3超格子薄膜における電荷秩序ドメインと電気伝導2013

    • Author(s)
      竹下聡史、大隅寛幸、Samuel Tardif、有馬孝尚、高田昌樹、中村優男、久保田将司、川崎雅司、十倉好紀、湯本博勝、小山貴久、大橋治彦
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島
    • Year and Date
      2013-03-27
    • Related Report
      2012 Final Research Report
  • [Presentation] 放射光によるカイラリティドメインの可視化2012

    • Author(s)
      大隅寛幸
    • Organizer
      第3回「カイラル磁性体―起源と機能―」
    • Place of Presentation
      東海村
    • Year and Date
      2012-12-18
    • Related Report
      2012 Final Research Report
  • [Presentation] 非共鳴X線回折実験によるURu2Si2の隠れた秩序に伴う多重極秩序の検証2012

    • Author(s)
      高阪勇輔、大隅寛幸、竹下聡史、有馬孝尚、高田昌樹、網塚浩、田端千紘、椎名亮輔、秋光純
    • Organizer
      日本物理学会2012年秋季大会
    • Place of Presentation
      横浜
    • Year and Date
      2012-09-18
    • Related Report
      2012 Final Research Report
  • [Presentation] 偏光X線を活用したキラル磁性・マルチフェロイックス研究2012

    • Author(s)
      大隅寛幸
    • Organizer
      SPring-8シンポジウム2012
    • Place of Presentation
      吹田
    • Year and Date
      2012-08-25
    • Related Report
      2012 Final Research Report
  • [Presentation] "Simultaneous Investigation on Valence and Magnetic Orderings in Multiferroic LuFe_2O_42012

    • Author(s)
      H. Ohsumi
    • Organizer
      SAGAMORE XVII Conference on Electron Charge, Spin and Momentum Densities
    • Place of Presentation
      Kitayuzawa, Japan
    • Year and Date
      2012-07-17
    • Related Report
      2012 Final Research Report
  • [Presentation] Simultaneous Investigation on Valence and Magnetic Orderings in Multiferroic LuFe_2O_4

    • Author(s)
      H. Ohsumi
    • Organizer
      SAGAMORE XVII Conference on Electron Charge, Spin and Momentum Densities
    • Place of Presentation
      Kitayuzawa(Hokkaido)
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 偏光X線を活用したキラル磁性・マルチフェロイックス研究

    • Author(s)
      大隅寛幸
    • Organizer
      SPring-8シンポジウム2012
    • Place of Presentation
      吹田市
    • Related Report
      2012 Annual Research Report
  • [Presentation] 非共鳴X線回折実験によるURu_2Si_2の隠れた秩序に伴う多重極秩序の検証

    • Author(s)
      高阪勇輔
    • Organizer
      日本物理学会2012年秋季大会
    • Place of Presentation
      横浜市
    • Related Report
      2012 Annual Research Report
  • [Presentation] 放射光によるカイラリティドメインの可視化

    • Author(s)
      大隅寛幸
    • Organizer
      Workshop: CROSSroads of Users and J-PARC 第3回 「カイラル磁性体-起源と機能-」
    • Place of Presentation
      東海村
    • Related Report
      2012 Annual Research Report
  • [Presentation] Pr_<0.5>Ca_<0.5>MnO_3/La_<0.5>Sr_<0.5>MnO_3超格子薄膜における電荷秩序ドメインと電気伝導

    • Author(s)
      竹下聡史
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      東広島市
    • Related Report
      2012 Annual Research Report
  • [Presentation] Magnetic domain imaging in the frustrated all-in/all-out pyrochlore Cd_2Os_2O_7

    • Author(s)
      S. Tardif
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      東広島市
    • Related Report
      2012 Annual Research Report

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Published: 2011-08-05   Modified: 2020-05-15  

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