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Basic process of lower-order organic compound synthesis via carbon dioxide reduction induced by low temperature plasma radical reactions

Research Project

Project/Area Number 23654198
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Plasma science
Research InstitutionTohoku University

Principal Investigator

IIZUKA Satoru  東北大学, 工学(系)研究科(研究院), 准教授 (20151227)

Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2013: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2012: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2011: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywords二酸化炭素還元 / ラジカル照射 / 低温プラズマ / メタン / メタノール / 二酸化炭素削減 / インパルス放電 / 重合反応 / 炭酸ガス還元 / ラジカル / CO2削減
Research Abstract

Suppression of carbon dioxide emission into the environment, which has been thought as a cause of global warming, is an urgent issue. Moreover, lower order organic compounds containing fewer carbons such as methane or methanol were important reusable energy source as alternative energy materials, as well as the raw material of chemical industry. In this study, basic physical and chemical mechanisms of radical reactions of carbon monoxide and hydrogen, generated in plasma-free space or cold plasma by decomposing water vapor and carbon dioxide, were investigated for synthesizing reusable lower order organic compounds such as methane and methanol.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (33 results)

All 2013 2012 2011

All Journal Article (16 results) (of which Peer Reviewed: 10 results) Presentation (17 results)

  • [Journal Article] Conversion of methane to methanol by a low-pressure steam plasma2013

    • Author(s)
      土屋貴之, 飯塚哲
    • Journal Title

      Journal of Environmental Engineering and Technology

      Volume: 2 , No.3 Pages: 35-39

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Plasma-assisted conversion of carbon dioxide to methane by low-pressure pulse discharges2013

    • Author(s)
      有田圭介, 飯 塚 哲
    • Journal Title

      31th International Conference on Phenomena of Ionized Gases

      Volume: P1-104-1-6

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Conversion of carbondioxide to methane by low-pressure pulse discharge2013

    • Author(s)
      Keisuke Arita, Satoru Iizuka
    • Journal Title

      30th Symposium on Plasma Processing

      Pages: 203-204

    • Related Report
      2013 Final Research Report
  • [Journal Article] Conversion of methane to methanol by a low-pressure steam plasma2013

    • Author(s)
      Takayuki Tsuchiya, Satoru Iizuka
    • Journal Title

      Journal of Environmental Engineering and Technology

      Volume: 2 Pages: 35-39

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Plasma-assisted conversion of carbon dioxide to methane by low-pressure pulse discharges2013

    • Author(s)
      Keisuke Arita, Satoru Iizuka
    • Journal Title

      31th International Conference on Phenomena of Ionized Gases

      Volume: 31

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Conversion of carbon dioxide to methane by low-pressure pulse discharge2013

    • Author(s)
      Keisuke Arita
    • Journal Title

      30th Simposium on Plasma Processing

      Volume: 30 Pages: 203-204

    • Related Report
      2012 Research-status Report
  • [Journal Article] 水素プラズマ改質による二酸化炭素のメタンへの変換2012

    • Author(s)
      有田圭介, 飯塚哲
    • Journal Title

      化学工業

      Volume: 63 , No.12 Pages: 41-45

    • Related Report
      2013 Final Research Report
  • [Journal Article] Diamond particle deposited among nickel/cupper particles in energy controlled CH_4/H_2 rf discharge plasma2012

    • Author(s)
      Junichi Emi, Satoru Iizuka
    • Journal Title

      Journal of Surface Engineered Materials and Advanced Technology

      Volume: 2 Pages: 158-162

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Conversion of CO_2 to methane by a low-pressure hollow-cathode discharge2012

    • Author(s)
      Toshitsugu Gunji, Satoru Iizuka
    • Journal Title

      Europhysics Conference on the Atomic and Molecular Physics of Ionized Gases (ESCAMPIG 2012)

      Volume: P1.1.2.1-2

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] 水素プラズマ改質による二酸化炭素のメタンへの変換2012

    • Author(s)
      有田圭介
    • Journal Title

      化学工業

      Volume: 63 Pages: 41-45

    • Related Report
      2012 Research-status Report
  • [Journal Article] , Diamond particles deposited among nickel/cupper particles in energy controlled CH4/H2 RF discharge plasmas2012

    • Author(s)
      Junichi Emi
    • Journal Title

      Journal of Surface Engineered Materials and Advanced Technology

      Volume: 2 Pages: 158-162

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Conversion of CO2 to methane by a low-pressure hollow-cathode discharge2012

    • Author(s)
      Toshitsugu Gunji
    • Journal Title

      Europhysics Conference on the Atomic and Molecular Physics of Ionized Gases (ESCAMPIG 2012)

      Volume: 1

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Reforming of carbon dioxide to methane and methanol by electric impulse low-pressure discharge with hydrogen2011

    • Author(s)
      Masaki Kano, Genki Satoh, Satoru Iizuka
    • Journal Title

      Plasma Chemistry and Plasma Processing

      Volume: non Issue: 2 Pages: 1-9

    • DOI

      10.1007/s11090-011-9333-0

    • Related Report
      2013 Final Research Report 2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Conversion of methane to gaseous and/or solid carbon materials by control of plasma reaction in RF discharge2011

    • Author(s)
      Takayuki Tsuchiya, Satoru Iizuka
    • Journal Title

      30th International Conference on Phenomena of Ionized Gases

      Volume: D13-061-1-6

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Reforming of Methane to Methanol by a Low-Pressure Steam Plasma2011

    • Author(s)
      Takayuki Tsuchiya, and Satoru Iizuka
    • Journal Title

      Plasma Conference 2011

      Volume: 22G6-1-2

    • Related Report
      2013 Final Research Report
  • [Journal Article] Conversion of CH4 to gaseous and/or solid....2011

    • Author(s)
      Takayuki Tsuchiya, Satoru Iizuka
    • Journal Title

      30th Int. Conf. Phenomena of Ionized Gases

      Volume: non

    • Related Report
      2011 Research-status Report
  • [Presentation] 水素プラズマと二酸化炭素の接触によるメタンの生成2013

    • Author(s)
      有田圭佑, 飯塚哲
    • Organizer
      第30回プラズマ・核融合学会年会
    • Place of Presentation
      東京工業大学
    • Year and Date
      2013-12-04
    • Related Report
      2013 Final Research Report
  • [Presentation] 水素プラズマによる二酸化炭素分解とメタンへの変換2013

    • Author(s)
      有田圭佑, 飯塚哲
    • Organizer
      第74回応用物理学会秋季学術講演会
    • Place of Presentation
      同志社大学
    • Year and Date
      2013-09-17
    • Related Report
      2013 Final Research Report
  • [Presentation] 低圧矩形波パルス放電による二酸化炭素のメタンへの変換2013

    • Author(s)
      有田圭佑, 飯塚哲
    • Organizer
      第60回応用物理学会学術講演会
    • Place of Presentation
      神奈川工業大学
    • Year and Date
      2013-03-27
    • Related Report
      2013 Final Research Report
  • [Presentation] Conversion of carbon dioxide to methane by low-pressure pulse discharge2013

    • Author(s)
      有田圭佑, 飯塚哲
    • Organizer
      30th Symposium on Plasma Processing
    • Place of Presentation
      アクトシティ浜松研修交流センター
    • Year and Date
      2013-01-21
    • Related Report
      2013 Final Research Report
  • [Presentation] Plasma-assisted conversion of carbon dioxide to methane by low-pressure pulse discharges2013

    • Author(s)
      有田圭介, 飯塚哲
    • Organizer
      31th International Conference on Phenomena of Ionized Gases
    • Place of Presentation
      Granada, Spain
    • Related Report
      2013 Final Research Report
  • [Presentation] 水素プラズマと二酸化炭素の接触によるメタンの生成2013

    • Author(s)
      有田圭介、飯塚哲
    • Organizer
      プラズマ・核融合学会
    • Place of Presentation
      東京工業大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] 水素プラズマによる二酸化炭素分解とメタンへの変換2013

    • Author(s)
      有田圭介、飯塚哲
    • Organizer
      応用物理学会
    • Place of Presentation
      同志社大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] 低圧矩形波パルス放電による二酸化炭素のメタンへの変換2013

    • Author(s)
      有田圭介
    • Organizer
      第60回応用物理学会学術講演会
    • Place of Presentation
      神奈川工科大学
    • Related Report
      2012 Research-status Report
  • [Presentation] Conversion of carbon dioxide to methane by low-pressure pulse discharge2013

    • Author(s)
      Keisuke Arita
    • Organizer
      30th Simposium on Plasma Processing
    • Place of Presentation
      アクトシティ浜松
    • Related Report
      2012 Research-status Report
  • [Presentation] 水素プラズマ改質による二酸化炭素のメタンへの変換2012

    • Author(s)
      有田圭佑, 飯塚哲
    • Organizer
      第73回応用物理学会学術講演会
    • Place of Presentation
      愛媛大学
    • Year and Date
      2012-09-13
    • Related Report
      2013 Final Research Report 2012 Research-status Report
  • [Presentation] Conversion of CO_2 to methane by a low-pressure hollow-cathode discharge2012

    • Author(s)
      Toshitsugu Gunji, Satoru Iizuka
    • Organizer
      Europhysics Conference on the Atomic and Molecular Physics of Ionized Gases ( ESCAMPIG 2012 )
    • Place of Presentation
      Viana do Castelo, Portugal
    • Related Report
      2013 Final Research Report
  • [Presentation] Synthesis of methanol by a low-pressure steam-methane plasma2012

    • Author(s)
      Takayuki Tsuchiya, Satoru Iizuka
    • Organizer
      International Symposium on Non-Thermal/Thermal Plasma Pollution Control Technology & Sustainable Energy ( ISNTP-8 )
    • Place of Presentation
      Camaret Sur Mer, France
    • Related Report
      2013 Final Research Report
  • [Presentation] Conversion of CO2 to methane by a low-pressure hollow-cathode discharge2012

    • Author(s)
      Toshitsugu Gunji
    • Organizer
      Europhysics Conference on the Atomic and Molecular Physics of Ionized Gases (ESCAMPIG 2012)
    • Place of Presentation
      Viana do Castelo, Portugal
    • Related Report
      2012 Research-status Report
  • [Presentation] Synthesis of Methanol by a Low-Pressure Steam-Methane Plasma2012

    • Author(s)
      Takayuki Tsuchiya
    • Organizer
      International Symposium on Non-Thermal/Thermal Plasma Pollution Control Technology & Sustainable Energy (ISNTP-8)
    • Place of Presentation
      Camaret Sur Mer, France
    • Related Report
      2012 Research-status Report
  • [Presentation] 低圧水蒸気プラズマを用いたメタンガスのメタノールへの変換2011

    • Author(s)
      土屋貴之, 飯塚哲
    • Organizer
      Plasma Conference 2011
    • Place of Presentation
      石川県立音楽堂
    • Year and Date
      2011-11-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Conversion of methane to gaseous and/or solid carbon materials by control of plasma reaction in RF discharge2011

    • Author(s)
      Takayuki Tsuchiya, Satoru Iizuka
    • Organizer
      30th International Conference on Phenomena of Ionized Gases
    • Place of Presentation
      Belfast, Great Briton
    • Related Report
      2013 Final Research Report
  • [Presentation] Reforming of CH4 to CH3OH by a Low-Pressure..2011

    • Author(s)
      Takayuki Tsuchiya, Satoru  Iizuka
    • Organizer
      Plasma Conference 2011
    • Place of Presentation
      Ishikawa Ongakudo, Kanazawa
    • Related Report
      2011 Research-status Report

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Published: 2011-08-05   Modified: 2019-07-29  

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