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Four-dimensional Mapping of Local Viscoelastic Functions: A Proposal for the Picture of Hierarchical Heterogeneity in Physical Properties of Polymers

Research Project

Project/Area Number 23655106
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Polymer chemistry
Research InstitutionKyushu University

Principal Investigator

TANAKA Keiji  九州大学, 大学院・工学研究院, 教授 (20325509)

Co-Investigator(Kenkyū-buntansha) SHUNDO Atsuomi  九州大学, 大学院・工学研究院, 助教 (40585915)
Project Period (FY) 2011 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2012: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2011: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywords光ピンセット / 粒子追跡法 / マイクロレオロジ- / ソフトマテリアル / 粘弾性関数 / 不均一性
Research Abstract

A novel methodology using optical tweezers for local rheological measurements in soft materials has been established. By using this, we have found that there exists a spatial heterogeneity in the viscoelastic properties of a supramolecular hydrogel, a lyotropic liquid crystal, etc. Notably, the heterogeneity in a worm-like micelle solution strongly depended on the measurement frequency. Also, it was found that a sol-to-gel transition process of a supramolecular polymer solution was accompanied by a homogenization of the physical properties.

Report

(3 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Research-status Report
  • Research Products

    (42 results)

All 2013 2012 2011 Other

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (33 results) (of which Invited: 3 results) Book (2 results) Remarks (1 results)

  • [Journal Article] Spatial Heterogeneity in the Sol-gel Transition of a Supramolecular System2013

    • Author(s)
      D. P. Penaloza Jr., A. Shundo, K. Matsumoto, M. Ohno, K. Miyaji, M. Goto, K. Tanaka
    • Journal Title

      Soft Matter

      Volume: Vol. 9 Issue: 21 Pages: 5127-5306

    • DOI

      10.1039/c3sm50225b

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Optical tweezers with fluorescence detection for temperature-dependent microrheological measurements2013

    • Author(s)
      Keiji Tanaka et al.
    • Journal Title

      Review of Scientific Instruments

      Volume: 84 Issue: 1

    • DOI

      10.1063/1.4789429

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Microscopic heterogeneity in viscoelastic properties of molecular assembled systems2013

    • Author(s)
      Keiji Tanaka et al.
    • Journal Title

      Chinese Journal of Polymer Science

      Volume: 31 Issue: 1 Pages: 1-11

    • DOI

      10.1007/s10118-013-1193-z

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Time-dependent heterogeneity in viscoelastic properties of worm-like micelle solutions2012

    • Author(s)
      Keiji Tanaka et al.
    • Journal Title

      Soft Matter

      Volume: 8 Issue: 28 Pages: 7361-7364

    • DOI

      10.1039/c2sm25549a

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Journal Article] Spatial Heterogeneity in A Lyotropic Liquid Crystal with Hexagonal Phase2012

    • Author(s)
      D. P. Penaloza Jr., K. Hori, A. Shundo, K. Tanaka
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: Vol. 14 Issue: 15 Pages: 5247-5250

    • DOI

      10.1039/c2cp40284j

    • Related Report
      2012 Final Research Report 2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Controllable heterogeneity in a supramolecular hydrogel2011

    • Author(s)
      Keiji Tanaka, et al
    • Journal Title

      Chemical Communications

      Volume: 47 Issue: 31 Pages: 8844-8846

    • DOI

      10.1039/c1cc12733k

    • Related Report
      2012 Final Research Report
    • Peer Reviewed
  • [Presentation] 温度制御型光ピンセットを用いたソフトマテリアルの局所物性解析2013

    • Author(s)
      春藤淳臣、堀耕一郎、David P. Penaloza Jr.、田中敬二
    • Organizer
      電子情報通信学会・有機エレクトロニクス研究会
    • Place of Presentation
      佐賀
    • Year and Date
      2013-03-05
    • Related Report
      2012 Final Research Report
  • [Presentation] ソフトマテリアルの粘弾特性におけるメゾスコピックな空間不均一性2013

    • Author(s)
      春藤淳臣
    • Organizer
      高分子学会九州支部・支部フォーラム
    • Place of Presentation
      福岡
    • Year and Date
      2013-02-23
    • Related Report
      2012 Final Research Report
  • [Presentation] Spatial Heterogeneity in Reological Properties of Soft Materials2013

    • Author(s)
      A. Shundo, K. Tanaka
    • Organizer
      Soft-interfaces Mini-symposium
    • Place of Presentation
      Fukuoka
    • Related Report
      2012 Final Research Report
  • [Presentation] Spatial Heterogeneity and Sol-gel Transition of Supramolecular Hydrogel by Particle Tracking2013

    • Author(s)
      Y . Matsumoto, A. Shundo, K. Matsumoto, M.Ohno, K. Miyaji, M. Goto, K. Tanaka
    • Organizer
      Soft-interfaces Mini-symposium 2013
    • Place of Presentation
      Fukuoka
    • Related Report
      2012 Final Research Report
  • [Presentation] Tunable Viscoelastic Properties and Heterogeneity in Supramolecular Hydrogel2012

    • Author(s)
      A. Shundo, K. Mizuguchi, K. Matsumoto, M.Ohno, K. Miyaji, M. Goto, K. Tanaka
    • Organizer
      The 9th SPSJ International Polymer Conference (IPC2012)
    • Place of Presentation
      Kobe
    • Year and Date
      2012-12-12
    • Related Report
      2012 Final Research Report
  • [Presentation] Direct Observation of Heterogeneity During Sol-to-Gel Transition of Supramolecular Hydrogel2012

    • Author(s)
      D. P. Penaloza Jr., A. Shundo, K. Matsumoto, M. Ohno, K. Miyaji, M. Goto, K. Tanaka
    • Organizer
      The 9th SPSJ International Polymer Conference (IPC2012)
    • Place of Presentation
      Kobe
    • Year and Date
      2012-12-12
    • Related Report
      2012 Final Research Report
  • [Presentation] 超分子ゲルのメゾスコピック不均一性とその制御2012

    • Author(s)
      春藤淳臣、David P. Penaloza、水口景子、松本圭吾、大野正司、宮地克明、後藤雅宏、田中敬二
    • Organizer
      第24回エラストマー討論会
    • Place of Presentation
      東京
    • Year and Date
      2012-11-29
    • Related Report
      2012 Final Research Report
  • [Presentation] Microscopic Rheological Properties in Supramolecular Systems2012

    • Author(s)
      A. Shundo, K. Hori, D. P. Penaloza Jr., K.Tanaka
    • Organizer
      Polymer Symposium
    • Place of Presentation
      Vietnam
    • Year and Date
      2012-11-04
    • Related Report
      2012 Final Research Report
  • [Presentation] Mesoscopic Heterogeneity in Supramolecular Hydrogel by Optical Tweezers2012

    • Author(s)
      A. Shundo, K. Matsumoto, M. Ohno, K. Miyaji, M. Goto, K. Tanaka
    • Organizer
      The 6th International Workshop on ADVANCED MATERIALS SCIENCE AND NANOTECHNOLOGY
    • Place of Presentation
      Vietnam
    • Year and Date
      2012-11-01
    • Related Report
      2012 Final Research Report
  • [Presentation] Analysis of Local Rheological Properties in Self-Assembled Molecular Systems2012

    • Author(s)
      D. P. Penaloza Jr., K. Hori, A. Shundo, K.Tanaka
    • Organizer
      Japan-Taiwan Bilateral Polymer Symposium
    • Place of Presentation
      Fukuoka
    • Year and Date
      2012-10-07
    • Related Report
      2012 Final Research Report
  • [Presentation] 粒子追跡法による超分子ゲルの不均一性評価2012

    • Author(s)
      春藤淳臣、David P. Penaloza、水口景子、松本圭吾、大野正司、宮地克明、後藤雅宏、田中敬二
    • Organizer
      第60回レオロジー討論会
    • Place of Presentation
      名古屋
    • Year and Date
      2012-09-27
    • Related Report
      2012 Final Research Report
  • [Presentation] 超分子ヒドロゲルの形成過程における空間不均一性2012

    • Author(s)
      春藤淳臣、David P. Penaloza、松本圭吾、大野正司、宮地克明、後藤雅宏、田中敬二
    • Organizer
      第61回高分子討論会
    • Place of Presentation
      名古屋
    • Year and Date
      2012-09-20
    • Related Report
      2012 Final Research Report
  • [Presentation] Heterogeneity Based on Supramolecular Nanospace2012

    • Author(s)
      David P. Penaloza、春藤淳臣、堀耕一郎、田中敬二
    • Organizer
      第61回高分子討論会
    • Place of Presentation
      名古屋
    • Year and Date
      2012-09-20
    • Related Report
      2012 Final Research Report
  • [Presentation] 局所粘弾特性から観た自己組織化材料の空間不均一性2012

    • Author(s)
      春藤淳臣
    • Organizer
      第49回化学関連支部合同九州大会
    • Place of Presentation
      福岡
    • Year and Date
      2012-06-30
    • Related Report
      2012 Final Research Report
  • [Presentation] Local Viscoelastic Properties in Molecular Assembled Systems by Optical Tweezers2012

    • Author(s)
      A. Shundo
    • Organizer
      The 17th International Workshop on Future Molecular Systems
    • Place of Presentation
      Fukuoka
    • Year and Date
      2012-02-06
    • Related Report
      2012 Final Research Report
  • [Presentation] Mesoscopic Heterogeneity in Supramolecular Systems2012

    • Author(s)
      A. Shundo, K. Tanaka
    • Organizer
      IUPAC World Polymer Congress
    • Place of Presentation
      USA
    • Related Report
      2012 Final Research Report
  • [Presentation] Analysis of Mesoscopic Heterogeneity in Polymer and Supramolecular Solutions by Optical Tweezers2012

    • Author(s)
      K. Hori, D. P. Penaloza, A. Shundo, K. Tanaka
    • Organizer
      第61回高分子学会年次大会
    • Place of Presentation
      神奈川
    • Related Report
      2012 Final Research Report
  • [Presentation] 光ピンセットによる紐状ミセルの動的不均一性の評価2012

    • Author(s)
      堀耕一郎、David P. Penaloza、春藤淳臣、田中敬二
    • Organizer
      日本ゴム協会 2012 年年次大会
    • Place of Presentation
      京都
    • Related Report
      2012 Final Research Report
  • [Presentation] 光ピンセットを用いたソフトマテリアルの局所粘弾特性評価2012

    • Author(s)
      春藤淳臣、堀耕一郎、David P. Penaloza、田中敬二
    • Organizer
      レオロジー学会第39 年会
    • Place of Presentation
      東京
    • Related Report
      2012 Final Research Report
  • [Presentation] 超分子ゲルの局所粘弾性における不均一性とその制御2012

    • Author(s)
      春藤淳臣、水口景子、宇野弘基、松本圭吾、大野正司、宮地克明、後藤雅宏、田中敬二
    • Organizer
      日本化学会第92 春季年会
    • Place of Presentation
      東京
    • Related Report
      2012 Final Research Report
  • [Presentation] 紐状ミセルの局所粘弾性における時空間不均一性2012

    • Author(s)
      堀耕一郎、春藤淳臣、田中敬二
    • Organizer
      日本化学会第92 春季年会
    • Place of Presentation
      東京
    • Related Report
      2012 Final Research Report
  • [Presentation] Structure-induced Dynamic Heterogeneity in Lyotropic Liquid Crystal2012

    • Author(s)
      David P. Penaloza Jr、春藤淳臣、田中敬二
    • Organizer
      日本化学会第92 春季年会
    • Place of Presentation
      東京
    • Related Report
      2012 Final Research Report
  • [Presentation] Spatial Heterogeneity in Lyotropc Liquid Crystal Solutions2012

    • Author(s)
      D. P. Penaloza Jr., A. Shundo, K. Tanaka
    • Organizer
      The 12th International Symposium on Biomimetic Materials Processing
    • Place of Presentation
      Nagoya
    • Related Report
      2012 Final Research Report
  • [Presentation] 光ピンセットによる紐状ミセルの動的不均一性の評価2012

    • Author(s)
      田中敬二
    • Organizer
      日本ゴム協会2012年年次大会
    • Place of Presentation
      京都市
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 異種相界面における高分子の構造・物性と機能化2012

    • Author(s)
      田中敬二
    • Organizer
      第61回高分子学会年次大会
    • Place of Presentation
      横浜市
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 異種相界面における高分子のナノキャラクタリゼーション2012

    • Author(s)
      田中敬二
    • Organizer
      日本接着学会関西支部 第8回若手の会
    • Place of Presentation
      福岡市
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Heterogeneity in Molecular Systems by Optical Tweezers2011

    • Author(s)
      A. Shundo, K. Mizuguchi, K. Hori, D. P. Penaloza Jr, K. Tanaka
    • Organizer
      Mini-Symposium on Soft Interfaces
    • Place of Presentation
      Fukuoka
    • Year and Date
      2011-09-23
    • Related Report
      2012 Final Research Report
  • [Presentation] Heterogeneity in Supramolecular Hydrogel2011

    • Author(s)
      A. Shundo, M. Miyamoto, M. Goto, K. Tanaka
    • Organizer
      The 12th Pacific Polymer Conference
    • Place of Presentation
      Korea
    • Related Report
      2012 Final Research Report
  • [Presentation] Dynamic Heterogeneity of Local Viscoelastic Propertiesin Worm-like Micelle Solution by Optical Tweezers2011

    • Author(s)
      K. Hori, A. Shundo, K. Tanaka
    • Organizer
      Pusan-Gyeongnam/Kyushu-Seibu Joint Symposium on High Polymers (15th) and Fibers (13th)
    • Place of Presentation
      Korea
    • Related Report
      2012 Final Research Report
  • [Presentation] 紐状ミセルの動的挙動とその空間不均一性2011

    • Author(s)
      堀耕一郎、春藤淳臣、田中敬二
    • Organizer
      第59回レオロジー討論会
    • Place of Presentation
      群馬
    • Related Report
      2012 Final Research Report
  • [Presentation] Microscopic Heterogeneity in Local Viscoelastic Properties of Aqueous Solution of Worm-like Micelles by Optical Tweezers2011

    • Author(s)
      K. Hori, A. Shundo, K. Tanaka
    • Organizer
      The 3rd Asian Symposium on Advanced Materials
    • Place of Presentation
      Fukuoka
    • Related Report
      2012 Final Research Report
  • [Presentation] Polymer Conformation at Inorganic Interface2011

    • Author(s)
      Keiji Tanaka
    • Organizer
      HyMap2011(招待講演)
    • Place of Presentation
      Pusan(Korea)
    • Related Report
      2011 Research-status Report
  • [Presentation] Thickness Dependence of Methanol Case II Diffusion in Thin Poly(methyl methacrylate) Films Studied by Optical Reflectivity2011

    • Author(s)
      Keiji Tanaka
    • Organizer
      The 12th Pacific Polymer Conference(招待講演)
    • Place of Presentation
      Jeju(Korea)
    • Related Report
      2011 Research-status Report
  • [Book] 電気情報通信学会技術研究報告 温度制御型光ピンセットを用いたソフトマテリアルの局所物性解析2013

    • Author(s)
      春藤淳臣、堀耕一郎、David P. Penaloza Jr.、田中敬二
    • Total Pages
      51
    • Related Report
      2012 Final Research Report
  • [Book] 超分子ヒドロゲルの物性制御による素材開発-光ピンセットによる局所粘弾性の評価2013

    • Author(s)
      春藤淳臣、田中敬二
    • Total Pages
      23
    • Publisher
      フレグランスジャーナル
    • Related Report
      2012 Final Research Report
  • [Remarks]

    • URL

      http://www.cstf.kyushu-u.ac.jp/~tanaka-lab/cgi-bin/research/index.html

    • Related Report
      2012 Final Research Report

URL: 

Published: 2011-08-05   Modified: 2019-07-29  

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