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Demonstration test of laser isotope separation utilizing rotational coherence and its applicability evaluation for heavy isotopes

Research Project

Project/Area Number 23656594
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Nuclear engineering
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

AKAGI Hiroshi  独立行政法人日本原子力研究開発機構, 量子ビーム応用研究部門, 研究副主幹 (70354818)

Co-Investigator(Renkei-kenkyūsha) KUMADA Takayuki  独立行政法人日本原子力研究開発機構, 量子ビーム応用研究部門, 研究主幹 (00343939)
ITAKURA Ryuji  独立行政法人日本原子力研究開発機構, 量子ビーム応用研究部門, 研究副主幹 (80334241)
OHSHIMA Yasuhiro  分子科学研究所, 光分子科学研究領域, 教授 (60213708)
HASEGAWA Hirokazu  東京大学, 総合文化研究科, 准教授 (20373350)
Project Period (FY) 2011 – 2012
Project Status Completed (Fiscal Year 2012)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2012: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2011: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Keywords同位体分離 / 回転コヒーレンス / フェムト秒レーザーパルス / 非共鳴多光子イオン化 / 原子分子物理 / 分子制御
Research Abstract

We have demonstrated a new laser isotope separation method utilizing molecular rotational coherence. In the demonstration, isotope selective ionization for a gas mixture of nitrogen isotopologues (^<14>N_2 and ^<15>N_2) has been realized by two-pulse irradiation of femto second laser, indicating that the present method is applicable as an isotope separation method. Additionally, we have tested the following two subjects, to improve the isotope selectivity and to examine the possibility for heavy isotopes. (1) A pulse-train irradiation of femto-second laser pulses for the molecular alignment, and (2) optimization of the gas jet conditions.

Report

(3 results)
  • 2012 Annual Research Report   Final Research Report ( PDF )
  • 2011 Research-status Report
  • Research Products

    (16 results)

All 2013 2012 2011 Other

All Journal Article (1 results) (of which Peer Reviewed: 1 results) Presentation (12 results) Remarks (3 results)

  • [Journal Article] Isotope-selective ionization utilizing molecular alignment and non- resonant multiphoton ionization2012

    • Author(s)
      H. Akagi, T. Kasajima, T. Kumada, R. Itakura, A. Yokoyama, H. Hasegawa, and Y. Ohshima
    • Journal Title

      Appl. Phys. B

      Volume: 109 Issue: 1 Pages: 75-80

    • DOI

      10.1007/s00340-012-5222-3

    • Related Report
      2012 Annual Research Report 2012 Final Research Report
    • Peer Reviewed
  • [Presentation] Molecular laser isotope separation without tunable lasers ―Isotope-selective ionization utilizing molecular alignment and angular dependent ionization―2013

    • Author(s)
      H. Akagi, T. Kasajima, T. Kumada, R. Itakura, A. Yokoyama, H. Hasegawa, and Y. Ohshima
    • Organizer
      International Conference on Laser Applications in Nuclear Engineering (LANE'13)
    • Place of Presentation
      Yokohama, Japan
    • Year and Date
      2013-04-24
    • Related Report
      2012 Final Research Report
  • [Presentation] フェムト秒パルスレーザーによる分子回転制御を利用した同位体選択的イオン化2013

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      第11回同位体科学研究会
    • Place of Presentation
      東京・産総研臨海副都心センター
    • Year and Date
      2013-03-14
    • Related Report
      2012 Final Research Report
  • [Presentation] Isotope Selective Ionization of N2 Isotopologues utilizing Rotational Coherence and Angular Dependent Ionization2013

    • Author(s)
      H. Akagi, T. Kasajima, T. Kumada, R. Itakura, A. Yokoyama, H. Hasegawa, and Y. Ohshima
    • Organizer
      第72回岡崎コンファレンス"Ultimate control of coherence"
    • Place of Presentation
      岡崎市・岡崎カンファレンスセンター
    • Year and Date
      2013-01-08
    • Related Report
      2012 Final Research Report
  • [Presentation] Isotope-selective ionization using four-pulse alignment2012

    • Author(s)
      H. Akagi, T. Kasajima, T. Kumada, R. Itakura, A. Yokoyama, H. Hasegawa, and Y. Ohshima
    • Organizer
      28th Symposium on Chemical Kinetics and Dynamics (化学反応討論会)
    • Place of Presentation
      九州大学・筑紫キャンパス
    • Year and Date
      2012-06-07
    • Related Report
      2012 Final Research Report
  • [Presentation] 分子配列制御を利用した同位体選択的イオン化2011

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      分子科学討論会2011
    • Place of Presentation
      札幌・札幌コンベンションセンター
    • Year and Date
      2011-09-23
    • Related Report
      2012 Final Research Report
  • [Presentation] Isotope-selective ionization using laser molecular alignment2011

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島裕
    • Organizer
      第27回化学反応討論会
    • Place of Presentation
      東京工業大学・大岡山キャンパス
    • Year and Date
      2011-06-09
    • Related Report
      2012 Final Research Report
  • [Presentation] 分子配列制御を利用した同位体選択的イオン化2011

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      分子科学討論会
    • Place of Presentation
      札幌コンベンションセンター(北海道)
    • Related Report
      2011 Research-status Report
  • [Presentation] Isotope-selective ionization using laser molecular alignment2011

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      化学反応討論会
    • Place of Presentation
      東京工業大学(東京都)
    • Related Report
      2011 Research-status Report
  • [Presentation] フェムト秒パルスレーザーによる分子回転制御を利用した同位体選択的イオン化

    • Author(s)
      赤木 浩、笠島辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      第11回同位体科学研究会
    • Place of Presentation
      東京
    • Related Report
      2012 Annual Research Report
  • [Presentation] Molecular laser isotope separation without tunable lasers ―Isotope-selective ionization utilizing molecular alignment and angular dependent ionization―

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      International Conference on Laser Applications in Nuclear Engineering (LANE’13)
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2012 Annual Research Report
  • [Presentation] Isotope-selective ionization using four-pulse alignment

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      28th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      九州大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] Isotope Selective Ionization of N2 Isotopologues utilizing Rotational Coherence and Angular Dependent Ionization

    • Author(s)
      赤木 浩、笠嶋辰也、熊田高之、板倉隆二、横山 淳、長谷川宗良、大島康裕
    • Organizer
      第72回岡崎コンファレンス “Ultimate control of coherence”
    • Place of Presentation
      岡崎カンファレンスセンター(愛知県岡崎市)
    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://wwwapr.kansai.jaea.go.jp/aprc/app-ilms.html

    • Related Report
      2012 Final Research Report
  • [Remarks] 高強度場物質制御研究グループ

    • URL

      http://wwwapr.kansai.jaea.go.jp/aprc/app-ilms.html

    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://wwwapr.kansai.jaea.go.jp/aprc/app-ilms.html

    • Related Report
      2011 Research-status Report

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Published: 2011-08-05   Modified: 2019-07-29  

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