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Spatiotemporal structures of dynamic heterogeneities in glass-forming liquids

Research Project

Project/Area Number 23684037
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Biophysics/Chemical physics
Research InstitutionNiigata University (2013)
Institute for Molecular Science (2011-2012)

Principal Investigator

KIM Kang  新潟大学, 自然科学系, 准教授 (20442527)

Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2013: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2012: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2011: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Keywordsガラス転移 / 過冷却液体 / 分子シミュレーション / 動的不均一性 / 動的相関長 / 多点相関 / 多時間相関 / フラジリティ / 動的相関
Research Abstract

We study the multi-point and multi-time correlation functions to reveal the spatio-temporal structures of dynamic heterogeneities in glass-forming liquids. Molecular dynamics simulations are carried out for the supercooled states of various prototype models of glass-forming. First, we quantify the length scale of the dynamic heterogeneities utilizing the four-point correlation function. The growth of the dynamic length scale with decreasing temperature is characterized by various scaling relations that are analogous to the critical phenomena. Second, the four-point correlation function is extended to a three-time correlation function to characterize the temporal structures of the dynamic heterogeneities. We provide comprehensive numerical results obtained from the three-time correlation function for the above models. From these calculations, we examine the time scale of the dynamic heterogeneities and determine the associated lifetime in a consistent and systematic way.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (49 results)

All 2014 2013 2012 Other

All Journal Article (8 results) (of which Peer Reviewed: 6 results) Presentation (39 results) (of which Invited: 3 results) Remarks (2 results)

  • [Journal Article] ガラス転移のフラジリティと動的不均一性 : モデル依存性の系統的な解析2014

    • Author(s)
      金鋼, 斉藤真司
    • Journal Title

      分子シミュレーション研究会会誌「アンサンブル」

      Volume: (印刷中)

    • NAID

      130005075259

    • Related Report
      2013 Final Research Report
  • [Journal Article] Dynamics in a tetrahedral network glassformer : Vibrations, network rearrangements, and diffusion2014

    • Author(s)
      川崎猛史, 金鋼, 小貫明
    • Journal Title

      Journal of Chemical Physics

      Volume: 140 Issue: 18 Pages: 184502-184502

    • DOI

      10.1063/1.4873346

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] ガラス転移のフラジリティと動的不均一性:モデル依存性の系統的な解析2014

    • Author(s)
      金鋼, 斉藤真司
    • Journal Title

      分子シミュレーション研究会会誌「アンサンブル」

      Volume: 印刷中

    • NAID

      130005075259

    • Related Report
      2013 Annual Research Report
  • [Journal Article] Dynamics in a tetrahedral network glassformer: Vibrations, network rearrangements, and diffusion2014

    • Author(s)
      川崎猛史, 金鋼, 小貫明
    • Journal Title

      Journal of Chemical Physics

      Volume: 印刷中

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dynamic Length Scales in Glass-Forming Liquids : An Inhomogeneous Molecular Dynamics Simulation Approach2013

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Journal Title

      Journal of Physical Chemistry B

      Volume: 113 Issue: 42 Pages: 13259-13267

    • DOI

      10.1021/jp4035419

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Slow dynamics of supercooled liquids confined in random pinning fields : Type A-B relaxations and reentrant transition2013

    • Author(s)
      金鋼, 宮崎州正, 斉藤真司
    • Journal Title

      AIP Conference Proceedings

      Volume: 1518 Pages: 227-231

    • DOI

      10.1063/1.4794572

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Multiple Length and Time Scales of Dynamic Heterogeneities in Model Glass-Forming Liquids: A Systematic Analysis of Multi-Point and Multi-Time Correlations2013

    • Author(s)
      K. Kim S. Saito
    • Journal Title

      J. Chem. Phys.

      Volume: 138 Issue: 12 Pages: 1-12

    • DOI

      10.1063/1.4769256

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Slow dynamics, dynamic heterogeneities, and fragility of super cooled liquids confined in random media2012

    • Author(s)
      K. Kim, K. Miyazaki, S. Saito
    • Journal Title

      Journal of Physics : Condensed Matter

      Volume: 23 Issue: 23 Pages: 234123-234123

    • DOI

      10.1088/0953-8984/23/23/234123

    • NAID

      120007137306

    • Related Report
      2013 Final Research Report 2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] Dynamic length scales identified by three-point correlations in supercooled liquids : MD and IMCT or MD vs IMCT?2014

    • Author(s)
      金鋼
    • Organizer
      Soft Matter Seminars on Glass Physics
    • Place of Presentation
      韓国・昌原大学
    • Year and Date
      2014-04-12
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラス転移の計算シミュレーション : 動的不均一性とフラジリティ2013

    • Author(s)
      金鋼
    • Organizer
      名古屋大学理学部物理学教室R研コロキウム
    • Place of Presentation
      名古屋大学
    • Year and Date
      2013-10-09
    • Related Report
      2013 Final Research Report
  • [Presentation] 過冷却液体のフラジリティと動的不均一性の時空間構造に関する考察2013

    • Author(s)
      金鋼,斉藤真司
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学
    • Year and Date
      2013-09-26
    • Related Report
      2013 Final Research Report
  • [Presentation] Role of length and time scales of dynamic heterogeneities on fragility in various model glasses2013

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      STATPHYS25 sattelite meeting"Physics of glassy and granular materials"
    • Place of Presentation
      京都大学
    • Year and Date
      2013-07-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Role of dynamic heterogeneities on fragility of model glasses2012

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      Workshop on the Open Problems of the Glass Transition and Related Topics
    • Place of Presentation
      九州大学
    • Year and Date
      2012-12-19
    • Related Report
      2013 Final Research Report
  • [Presentation] Slow dynamics of supercooled liquids confined in random pinning fields : Type A-B relaxations and reentrant transition2012

    • Author(s)
      金鋼, 宮崎州正, 斉藤真司
    • Organizer
      The 4th International Symposium on Slow Dynamics in Complex Systems
    • Place of Presentation
      東北大学
    • Year and Date
      2012-12-06
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラスのフラジリティと動的不均一性に関する考察2012

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      第26回分子シミュレーション討論会
    • Place of Presentation
      九州大学
    • Year and Date
      2012-11-26
    • Related Report
      2013 Final Research Report
  • [Presentation] Multiple spatio-temporal structures of dynamic heterogeneities in glasses : Probing multi-point and multi-time correlations2012

    • Author(s)
      金鋼
    • Organizer
      Seminar of Théorie et Simulation
    • Place of Presentation
      フランス・モンペリエ大学第2シャルル・クーロン研究所
    • Year and Date
      2012-11-15
    • Related Report
      2013 Final Research Report
  • [Presentation] Multiple spatiotemporal structures of dynamic heterogeneities in glass-forming liquids : Probing multi-point and multi-time correlations2012

    • Author(s)
      金鋼
    • Organizer
      The 3rd Workshop on Computational and Statistical Physics
    • Place of Presentation
      京都リサーチパーク
    • Year and Date
      2012-10-19
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラス転移における動的不均一性の時空間構造 : 多点・多時間相関関数による解析2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Organizer
      第2回ソフトマター研究会
    • Place of Presentation
      九州大学
    • Year and Date
      2012-09-25
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラス系における不均一ダイナミクスの多点相関関数による解析2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京大学
    • Year and Date
      2012-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Multi-point and multi-time density correlations for probing dynamic heterogeneities in glasses : On the analogy of multi-dimensional spectroscopies2012

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      6th International Conference on Coherent Multidimensional Spectroscopy
    • Place of Presentation
      ドイツ・ベルリン
    • Year and Date
      2012-07-16
    • Related Report
      2013 Final Research Report
  • [Presentation] Slow dynamics of fluids confined in random media : Crossover from glass to Lorentz gas2012

    • Author(s)
      金鋼
    • Organizer
      Soft Matter Seminars on Glass Physics
    • Place of Presentation
      韓国・昌原大学
    • Year and Date
      2012-04-13
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラス転移および荷電コロイド分散系のダイナミクスに対する計算シミュレーション2012

    • Author(s)
      金鋼
    • Organizer
      日本物理学会第67回年次大会日本物理学会第5回若手奨励賞(領域12)
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-25
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラス転移および荷電コロイド分散系のダイナミクスに対する計算シミュレーション2012

    • Author(s)
      金鋼
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学(兵庫県)(招待講演)
    • Year and Date
      2012-03-25
    • Related Report
      2011 Annual Research Report
  • [Presentation] ガラス転移における多点相関関数と動的相関長 : NEMD and IMCT or NEMD vs IMCT?2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学
    • Year and Date
      2012-03-24
    • Related Report
      2013 Final Research Report
  • [Presentation] ガラス転移における多点相関関数と動的相関長:NEMD and IMCT? or NEMD vs IMCT?2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R.Reichman
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学(兵庫県)
    • Year and Date
      2012-03-24
    • Related Report
      2011 Annual Research Report
  • [Presentation] Dynamic length scales identified by three-point correlations in glass-forming liquids : MD and IMCT or MD vs IMCT?2012

    • Author(s)
      Kang Kim, Shiji Saito, Kunimasa Miyazaki, Giulio Biroli, David R.Reichman
    • Organizer
      The International Conference on Statistical Mechanics of Liquids : From Water to Biomolecules
    • Place of Presentation
      分子科学研究所(愛知県)
    • Year and Date
      2012-03-13
    • Related Report
      2011 Annual Research Report
  • [Presentation] Lifetime of dynamical heterogeneity in glass-forming liquids : Unveiling by multi-time correlations2012

    • Author(s)
      Kang Kim, Shinji Saito
    • Organizer
      The International Conference on Statistical Mechanics of Liquids : From Water to Biomolecules
    • Place of Presentation
      分子科学研究所(愛知県)
    • Year and Date
      2012-03-13
    • Related Report
      2011 Annual Research Report
  • [Presentation] Dynamic length scales identified by three-point correlations : MD and IMCT or MD vs IMCT?2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Organizer
      The 5th Discussion Meeting on Glass Transition
    • Place of Presentation
      東北大学
    • Year and Date
      2012-02-28
    • Related Report
      2013 Final Research Report
  • [Presentation] Lifetime of dynamical heterogeneity in Supercooled liquids : Unveiling by multi-time correlation functions2012

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      The 5th Discussion Meeting on Glass Transition
    • Place of Presentation
      東北大学
    • Year and Date
      2012-02-28
    • Related Report
      2013 Final Research Report
  • [Presentation] Dynamic length scales identified by three-point correlations : MD and IMCT or MD vs IMCT?2012

    • Author(s)
      Kang Kim, Shiji Saito, Kunimasa Miyazaki, Giulio Biroli, David R.Reichman
    • Organizer
      The 5th Discussion Meeting on Glass Transition
    • Place of Presentation
      東北大学(宮城県)
    • Year and Date
      2012-02-28
    • Related Report
      2011 Annual Research Report
  • [Presentation] Lifetime of dynamical heterogeneity in Supercooled liquids : Unveiling by multi-time correlation functions2012

    • Author(s)
      Kang Kim, Shinji Saito
    • Organizer
      The 5th Discussion Meeting on Glass Transition
    • Place of Presentation
      東北大学(宮城県)
    • Year and Date
      2012-02-28
    • Related Report
      2011 Annual Research Report
  • [Presentation] Dynamic length scales identified by three-point correlations in glasses : MD and IMCT or MD vs IMCT?2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Organizer
      Phase Transition Dynamics in Soft Matter : Bridging Microscale and Mesoscale
    • Place of Presentation
      京都大学
    • Year and Date
      2012-02-21
    • Related Report
      2013 Final Research Report
  • [Presentation] Dynamic length scales identified by three-point correlations in glasses : MD and IMCT or MD vs IMCT?2012

    • Author(s)
      Kang Kim, Shiji Saito, Kunimasa Miyazaki, Giulio Biroli, David R.Reichman
    • Organizer
      Phase Transition Dynamics in Soft Matter : Bridging Microscale and Mesoscale
    • Place of Presentation
      京都大学(京都県)
    • Year and Date
      2012-02-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] Dynamic length scales identified by three-point correlations in glass-forming liquids : MD and IMCT or MD vs IMCT?2012

    • Author(s)
      金鋼, 斉藤真司, 宮崎州正, Giulio Biroli, David R. Reichman
    • Organizer
      The International Conference on Statistical Mechanics of Liquids : From Water to Biomolecules
    • Place of Presentation
      分子科学研究所
    • Year and Date
      2012-02-13
    • Related Report
      2013 Final Research Report
  • [Presentation] Lifetime of dynamical heterogeneity in glass-forming liquids : Unveiling by multi-time correlations2012

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      The International Conference on Statistical Mechanics of Liquids : From Water to Biomolecules
    • Place of Presentation
      分子科学研究所
    • Year and Date
      2012-02-13
    • Related Report
      2013 Final Research Report
  • [Presentation] 過冷却液体のフラジリティと動的不均一性の時空間構造に関する考察

    • Author(s)
      金鋼, 斉藤真司
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] Role of length and time scales of dynamic heterogeneities on fragility in various model glasses

    • Author(s)
      Kang Kim and Shinji Saito
    • Organizer
      STATPHYS25 sattelite meeting "Physics of glassy and granular materials"
    • Place of Presentation
      YITP, Kyoto University
    • Related Report
      2013 Annual Research Report
  • [Presentation] Role of dynamic heterogeneities on fragility of model glasses

    • Author(s)
      Kang Kim
    • Organizer
      Workshop on the Open Problems of the Glass Transition and Related Topics
    • Place of Presentation
      九州大学(福岡県)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Slow dynamics of supercooled liquids confined in random pinning fields: Type A-B relaxations and reentrant transition

    • Author(s)
      Kang Kim, Kunimasa Miyazaki, Shinji Saito
    • Organizer
      The 4th International Symposium on Slow Dynamics in Complex Systems
    • Place of Presentation
      東北大学(宮城県)
    • Related Report
      2012 Annual Research Report
  • [Presentation] ガラスのフラジリティと動的不均一性に関する考察

    • Author(s)
      金 鋼, 斉藤 真司
    • Organizer
      第26回分子シミュレーション討論会
    • Place of Presentation
      九州大学(福岡県)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Multiple spatio-temporal structures of dynamic heterogeneities in glasses: Probing multi-point and multi-time correlations

    • Author(s)
      Kang Kim
    • Organizer
      Seminar of Theorie et Simulation, Laboratoire Charles Coulomb
    • Place of Presentation
      Montpellier University II, France
    • Related Report
      2012 Annual Research Report
  • [Presentation] Multiple spatiotemporal structures of dynamic heterogeneities in glass-forming liquids: Probing multi-point and multi-time correlations

    • Author(s)
      Kang Kim
    • Organizer
      The 3rd Workshop on Computational and Statistical Physics
    • Place of Presentation
      京都リサーチパーク(京都府)
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] ガラス転移における動的不均一性の時空間構造: 多点・多時間相関関数による解析

    • Author(s)
      金 鋼, 斉藤 真司, 宮崎 州正, Giulio Biroli, David R. Reichman
    • Organizer
      第2回ソフトマター研究会
    • Place of Presentation
      九州大学(福岡県)
    • Related Report
      2012 Annual Research Report
  • [Presentation] ガラス系における不均一ダイナミクスの多点相関関数による解析

    • Author(s)
      金 鋼, 斉藤 真司
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京大学(東京都)
    • Related Report
      2012 Annual Research Report
  • [Presentation] Multi-point and multi-time density correlations for probing dynamic heterogeneities in glasses: On the analogy of multi-dimensional spectroscopies

    • Author(s)
      Kang Kim, Shinji Saito
    • Organizer
      6th International Conference on Coherent Multidimensional Spectroscopy
    • Place of Presentation
      Berlin, Germany
    • Related Report
      2012 Annual Research Report
  • [Presentation] Slow dynamics of fluids confined in random media: Crossover from glass to Lorentz gas

    • Author(s)
      Kang Kim
    • Organizer
      Soft Matter Seminars on Glass Physics
    • Place of Presentation
      Changwon University, Korea
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Dynamic length scales identified by three-point correlations in supercooled liquids: MD and IMCT or MD vs IMCT?

    • Author(s)
      Kang Kim
    • Organizer
      Soft Matter Seminars on Glass Physics
    • Place of Presentation
      Changwon University, Korea
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Remarks] ホームページ

    • URL

      http://bussei.gs.niigata-u.ac.jp/~kk/

    • Related Report
      2013 Final Research Report
  • [Remarks]

    • URL

      http://dyna.ims.ac.jp/kin/

    • Related Report
      2011 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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