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Ionization of molecules irradiated by intense laser fields

Research Project

Project/Area Number 23685001
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Physical chemistry
Research InstitutionThe University of Tokyo

Principal Investigator

HASEGAWA Hirokazu3  東京大学, 総合文化研究科, 准教授 (20373350)

Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥29,770,000 (Direct Cost: ¥22,900,000、Indirect Cost: ¥6,870,000)
Fiscal Year 2013: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2012: ¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2011: ¥23,790,000 (Direct Cost: ¥18,300,000、Indirect Cost: ¥5,490,000)
Keywords高強度レーザー光 / イオン化過程 / 分子配列 / 強レーザー場 / 光イオン化 / クーロン爆発 / イオン化 / 状態分布
Research Abstract

We studied the ionization processes of molecules irradiated by intense laser fields. In the case of acetylene, the ion yield of singly charged and doubly charged acetylene ions is larger when molecular axis is perpendicular to laser polarization direction than parallel to that. We revealed that this behavior reflects the shape of the highest occupied molecular orbital (HOMO). As a result, electrons in acetylene are ionized by tunnel ionization or over barrier ionization of the laser electric fields. In addition, in the case of oxygen molecule, the ion yield of singly charged ion behaves like acetylene. On the other hand, we found that the ion yield of the doubly charged oxygen molecule is different from acetylene and singly charged oxygen molecule.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (13 results)

All 2014 2013 2011

All Presentation (13 results)

  • [Presentation] Molecular alignment in laser fields2014

    • Author(s)
      H. Hasegawa
    • Organizer
      International symposium on ultrafast intense laser science 13th
    • Place of Presentation
      Taj Hari Hahal (Jodhpur, India)
    • Related Report
      2013 Final Research Report
  • [Presentation] Reconstruction of a rotational wave packet created in the X2Pi1/2 state of the NO radical by a nonresonant intense ultrashort laser pulse2014

    • Author(s)
      H. Hasegawa and Y. Ohshima
    • Organizer
      19^<th> international conference on ultrafast phenomena
    • Place of Presentation
      Okinawa convention center (Okinawa)
    • Related Report
      2013 Final Research Report
  • [Presentation] Ionization of aligned O2 by intense laser pulse2014

    • Author(s)
      K. Sonoda, H. Hasegawa,T. Sato, A. Iwasaki, and K. Yamanouchi
    • Organizer
      19^<th> international conference on ultrafast phenomena
    • Place of Presentation
      Okinawa convention center (Okinawa)
    • Related Report
      2013 Final Research Report
  • [Presentation] Intense field ionization of C2H2 and ^<12>C^<13>CH2 aligned in field-free space2014

    • Author(s)
      H. Hasegawa,Y. Ikeda, K. Sonoda, T. Sato, A. Iwasaki, and K. Yamanouchi
    • Organizer
      19^<th> international conference on ultrafast phenomena
    • Place of Presentation
      Okinawa convention center (Okinawa)
    • Related Report
      2013 Final Research Report
  • [Presentation] ionization of aligned O2 by intense laser pulse2014

    • Author(s)
      K. Sonoda, H. Hasegawa, T. Sato, A. Iwasaki, K. Yamanouchi
    • Organizer
      19th international conference on ultrafast phenomena
    • Place of Presentation
      Okinawa convention center(Okinawa)
    • Related Report
      2013 Annual Research Report
  • [Presentation] intense field ionization of C2H2 and 12C13CH2 aligned in field-free space2014

    • Author(s)
      H. Hasegawa, Y. Ikeda, K. Sonoda, T. Sato, A. Iwasaki, K. Yamanouchi
    • Organizer
      19th international conference on ultrafast phenomena
    • Place of Presentation
      Okinawa convention center(Okinawa)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Reconstruction of a Rotational Wave Packet Created in the X2Π1/2 State of the NO Radical by a Nonresonant Intense Ultrashort Laser Pulse2014

    • Author(s)
      H. Hasegawa, Y. Ohshima
    • Organizer
      19th international conference on ultrafast phenomena
    • Place of Presentation
      Okinawa convention center(Okinawa)
    • Related Report
      2013 Annual Research Report
  • [Presentation] フェムト秒レーザーの複数パルス瀟洒による同位体選択的回転励起学会名2013

    • Author(s)
      赤城浩,笠嶋辰也,熊田高之,板倉隆二,横山淳,長谷川宗良,大島康裕
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ(京都府)
    • Related Report
      2013 Final Research Report
  • [Presentation] 窒素分子の回転波束への振動回転相互作用の影響2013

    • Author(s)
      横山淳,赤城浩,熊田高之,板倉隆二,長谷川宗良,大島康裕
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ(京都府)
    • Related Report
      2013 Final Research Report
  • [Presentation] 窒素分子の回転波束への振動回転相互作用の影響2013

    • Author(s)
      横山淳,赤木浩,熊田高之,板倉隆二,長谷川宗良,大島康裕
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ(京都府)
    • Related Report
      2013 Annual Research Report
  • [Presentation] フェムト秒レーザーの複数パルス照射による同位体選択的回転励起2013

    • Author(s)
      赤木浩,笠嶋辰也,熊田高之,板倉隆二,横山淳,長谷川宗良,大島康裕
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ(京都府)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 波束干渉を用いた電子基底状態におけるNO分子の回転状態分布制御2011

    • Author(s)
      長谷川宗良,大島康裕
    • Organizer
      第5回分子科学討論会
    • Place of Presentation
      札幌コンベンションセンター(北海道)
    • Year and Date
      2011-09-23
    • Related Report
      2013 Final Research Report
  • [Presentation] 波束干渉を用いた電子基底状態におけるNO分子の回転状態分布制御2011

    • Author(s)
      長谷川宗良, 大島康裕
    • Organizer
      第5回分子科学討論会
    • Place of Presentation
      札幌(北海道)
    • Year and Date
      2011-09-23
    • Related Report
      2011 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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