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NMR study of aging process of self-radiation damage in minor actinide dioxides

Research Project

Project/Area Number 23686137
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Nuclear engineering
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

TOKUNAGA Yo  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 先端基礎研究センター, 研究主幹 (00354902)

Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥25,610,000 (Direct Cost: ¥19,700,000、Indirect Cost: ¥5,910,000)
Fiscal Year 2013: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2012: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2011: ¥23,010,000 (Direct Cost: ¥17,700,000、Indirect Cost: ¥5,310,000)
Keywordsマイナーアクチニド酸化物 / 核磁気共鳴 / 自己照射損傷 / 磁気相転移 / アメリシウム酸化物 / 自己照射損傷効果 / 格子欠陥 / 酸化物燃料
Research Abstract

Aging process of self-radiation damage in minor actinide dioxides has been investigated microscopically by means of 17O NMR. In 243AmO2, we have observed a rapid change of the NMR line shape over the short time interval of one month. The result demonstrates that the self-radiation damage rapidly increases the numbers of defect at low temperatures, and further, that the electronic ground state of the system is highly sensitive to the disorder. The NMR data have also revealed short-range, spin-glass-like character for the magnetic transition in this system.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (16 results)

All 2014 2013 2012 2011

All Journal Article (6 results) (of which Peer Reviewed: 6 results) Presentation (10 results) (of which Invited: 6 results)

  • [Journal Article] NMR Studies of Actinide Oxides-a Review2014

    • Author(s)
      Russell E.Walstedt, Yo Tokunaga, Shinsaku Kambe
    • Journal Title

      Comptes rendus Physique

      Volume: (in press)

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Self-radiation effects and glassy nature of magnetic transitionin AmO_2 revealed by ^<17>O-NMR2014

    • Author(s)
      Yo Tokunaga,Tuyoshi Nishi, Masami Nakada, Akinori Itoh, Hironori Sakai, Shinsaku Kambe,Yoshiya Homma,Fuminori Honda, Dai Aoki, and Russell E. Walstedt
    • Journal Title

      Physical Review B

      Volume: (in press)

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Spin Fluctuation, Orbital States and Non-Conventional Superconductivity in Actinides Compounds2012

    • Author(s)
      S.Kambe
    • Journal Title

      Material Research Society Symposium Proceedings

      Volume: 1444 Issue: 9 Pages: 165-174

    • DOI

      10.1103/physrevb.86.094402

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] NMR Study on AmO_2: Comparison with UO_2 and NpO_22011

    • Author(s)
      Y.Tokunaga,T.Nishi,S.Kambe,M.Nakada, Y.Homma,H.Sakai and H.Chudo
    • Journal Title

      Journal of Physical Society of Japan

      Volume: Suppl. A 80

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Solid-State NMR Study on Actinide Dioxides2011

    • Author(s)
      Y.Tokunaga, H.Sakai, S.Kambe, H. Chudo, M.Osaka, S.Miwa, T.Nishi, M.Nakada, A.Itoh and Y.Homma
    • Journal Title

      Mater. Res. Soc. Symp. Proc

      Volume: 1444 Pages: 149-158

    • DOI

      10.1557/opl.2012.1001

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] NMR Study on AmO2 : Comparison with UO2 and NpO22011

    • Author(s)
      Y.Tokunaga, S.Kambe, 他7名
    • Journal Title

      J.Phys.Soc.Jpn.supplement A

      Volume: 80 Issue: Suppl.A Pages: SA110-SA110

    • DOI

      10.1143/jpsjs.80sa.sa110

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] AmO_2における磁気相転移と自己照射損傷効果のNMRによる研究2014

    • Author(s)
      徳永陽
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学(平塚)
    • Related Report
      2013 Final Research Report
  • [Presentation] AmO2における磁気相転移と自己照射損傷効果のNMRによる研究2014

    • Author(s)
      徳永陽、西剛史、中田正美、酒井宏典、神戸振作、本間佳哉、本多史憲、青木大
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学、平塚
    • Related Report
      2013 Annual Research Report
  • [Presentation] Low temperature electronic properties of actinide dioxides probed by ^<17>O-NMR2013

    • Author(s)
      Yo TOKUNAGA
    • Organizer
      EURACT-NMR Workshop 2013
    • Place of Presentation
      カールスルーエ(ドイツ)
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Low temperature electronic properties of actinide dioxides probed by 17O-NMR2013

    • Author(s)
      YO TOKUNAGA
    • Organizer
      EURACT-NMR Workshop 2013
    • Place of Presentation
      Karlsruhe, Germany
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Solid-State NMR Study on Actinide Dioxides2012

    • Author(s)
      Yo TOKUNAGA
    • Organizer
      2012 MRS Spring Meeting
    • Place of Presentation
      サンフランシスコ(米国)
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Solid-State NMR Study on Actinide Dioxides2012

    • Author(s)
      Yo Tokunaga
    • Organizer
      2012 MRS Spring Meeting
    • Place of Presentation
      サンフランシスコ アメリカ
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] NMRによる多極子秩序の観測2011

    • Author(s)
      徳永陽
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学(富山県)(招待講演)
    • Year and Date
      2011-09-22
    • Related Report
      2011 Annual Research Report
  • [Presentation] NMR study of various actinide system2011

    • Author(s)
      Y.Tokunaga
    • Organizer
      International workshop "J-Actinite meeting 2011
    • Place of Presentation
      東北大学東京分室(東京都)(招待講演)
    • Year and Date
      2011-09-01
    • Related Report
      2011 Annual Research Report
  • [Presentation] NMR study of various actinide system2011

    • Author(s)
      Yo TOKUNAGA、NMR study of various actinide system
    • Organizer
      J-Actinite meeting 2011
    • Place of Presentation
      東北大学東京分室(東京)
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] NMRによる多極子秩序の観測2011

    • Author(s)
      徳永陽
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学(富山)
    • Related Report
      2013 Final Research Report
    • Invited

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Published: 2011-04-06   Modified: 2019-07-29  

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