• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Investigation of Preferential Source Generation Mechanism for the Realization of Bulk Crystal Growth of Indium Nitride

Research Project

Project/Area Number 23760006
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Applied materials science/Crystal engineering
Research InstitutionTokyo University of Agriculture and Technology

Principal Investigator

TOGASHI Rie  東京農工大学, 工学(系)研究科(研究院), 助教 (50444112)

Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2013: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2012: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2011: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywordsエピタキシャル / 結晶成長 / 窒化インジウム / HVPE / 熱力学解析
Research Abstract

In order to realize high-crystalline quality and thick InN layers, following studies were performed: (1) investigation of the influence of growth rate and grown thickness on InN crystalline quality using a conventional hydride vapor phase epitaxy (HVPE) system, (2) thermodynamic analysis of the In source zone for appreciable generation of InCl3, (3) design and development of a new HVPE system with a two-stage source generation for the generation of InCl3, and (4) investigation of high-speed InN growth in both In- and N-polarities using the new HVPE system.
The same growth rate of InN grown by new HVPE system was achieved only using around 1/40 times the total Cl2 input partial pressure of InN grown by conventional HVPE system. Thus, efficiency for the generation of InCl3 gas was significantly improved compared with conventional HVPE system. In and N polarity InN can be grown at high growth rates at high temperature, owing to the preferential formation of InCl3.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (40 results)

All 2013 2012 2011 Other

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (33 results) (of which Invited: 3 results) Remarks (5 results)

  • [Journal Article] Effect of High NH_3 Input Partial Pressure on Hydride Vapor Phase Epitaxy of InN Using Nitrided (0001) Sapphire Substrates2013

    • Author(s)
      Rie Togashi, Sho Yamamoto, K. Fredrik Karlsson, Hisashi Murakami, Yoshinao Kumagai, Per-Olof Holtz, and Akinori Koukitu
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: Vol. 52

    • URL

      http://jjap.jsap.jp/cgi-bin/getarticle?magazine=JJAP&volume=52&page=08JD05

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effect of High NH3 Input Partial Pressure on Hydride Vapor Phase Epitaxy of InN Using Nitrided (0001) Sapphire Substrates2013

    • Author(s)
      Rie Togashi, Sho Yamamoto, K. Fredrik Karlsson, Hisashi Murakami, Yoshinao Kumagai, Per-Olof Holtz, and Akinori Koukitu
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 52

    • NAID

      210000142640

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] High-Speed InN Growth Using a Novel Two-Stage Source Generation Hydride Vapor Phase Epitaxy System2013

    • Author(s)
      Rie Togashi, Naoto Fujita, Ryota Imai, Hisashi Murakami, Yoshinao Kumagai, and Akinori Koukitu
    • Organizer
      8th International Workshop on Bulk Nitride Semiconductors (IWBNS-VIII)
    • Place of Presentation
      Kloster Seeon, Seeon, Germany
    • Year and Date
      2013-10-03
    • Related Report
      2013 Final Research Report
  • [Presentation] Demonstration of high-speed growth of InN by HVPE with a two-step precursor generation scheme2013

    • Author(s)
      Naoto Fujita, Ryota Imai, Rie Togashi, Hisashi Murakami, Yoshinao Kumagai, and Akinori Koukitu
    • Organizer
      2013 JSAP-MRS Joint Symposia
    • Place of Presentation
      Doshisha University, Kyoto, Japan(17p-M6-3.)
    • Year and Date
      2013-09-17
    • Related Report
      2013 Final Research Report
  • [Presentation] Temperature Dependence of InN Growth by a Novel HVPE System with Two-Step Generation of InCl_32013

    • Author(s)
      Naoto Fujita, Ryota Imai, Rie Togashi, Hisashi Murakami, Yoshinao Kumagai and Akinori Koukitu
    • Organizer
      10th International Conference on Nitride Semiconductors (ICNS-10)
    • Place of Presentation
      Gaylord National Resort & Convention Center, Washington, D.C., U.S.A.(A1.05.)
    • Year and Date
      2013-08-26
    • Related Report
      2013 Final Research Report
  • [Presentation] Comparative Study on High-Speed InN Growth in Both In- and N-Polarities Using a Two-Stage Source Generation Hydride Vapor Phase Epitaxy System2013

    • Author(s)
      Rie Togashi, Naoto Fujita, Ryota Imai, Hisashi Murakami, Yoshinao Kumagai and Akinori Koukitu
    • Organizer
      10th International Conference on Nitride Semiconductors (ICNS-10)
    • Place of Presentation
      Gaylord National Resort & Convention Center, Washington, D.C., U.S.A.(A1.04.)
    • Year and Date
      2013-08-26
    • Related Report
      2013 Final Research Report
  • [Presentation] High-Speed Growth of In- and N-polarity InN Using a Two-Stage Source Generation Hydride Vapor Phase Epitaxy System2013

    • Author(s)
      Rie Togashi, Naoto Fujita, Ryota Imai, Hisashi Murakami, Yoshinao Kumagai, and Akinori Koukitu
    • Organizer
      Conference on LED and its industrial application '13 (LEDIA '13)
    • Place of Presentation
      Pacifico Yokohama, Yokohama, Japan(LEDp3-15.)
    • Year and Date
      2013-04-24
    • Related Report
      2013 Final Research Report
  • [Presentation] High-Speed Growth of InN Using a Two-Stage Source Generation HVPE System2012

    • Author(s)
      Rie Togashi, Ryota Imai, Sho Yamamoto, Hisashi Murakami, Yoshinao Kumagai, and Akinori Koukitu
    • Organizer
      Intensive Discussion on Growth of Nitride Semiconductors
    • Place of Presentation
      Tohoku University, Sendai, Japan
    • Year and Date
      2012-10-22
    • Related Report
      2013 Final Research Report
  • [Presentation] HVPE growth of InN on InN/sapphire (0001) templates prepared by MBE2012

    • Author(s)
      Ryota Imai, Sho Yamamoto, Rie Togashi, Hisashi Murakami, Yoshinao Kumagai, Tomohiro Yamaguchi, Tsutomu Araki, Yasushi Nanishi, and Akinori Koukitu
    • Organizer
      International Workshop on Nitride Semiconductors 2012 (IWN2012)
    • Place of Presentation
      Sapporo Convention Center, Sapporo, Japan(TuP-GR-60.)
    • Year and Date
      2012-10-16
    • Related Report
      2013 Final Research Report
  • [Presentation] Effect of high NH_3 input partial pressure on hydride vapor phase epitaxy of InN using nitrided (0001) sapphire substrates2012

    • Author(s)
      Rie Togashi, Sho Yamamoto, Fredrik Karlsson, Hisashi Murakami, Yoshinao Kumagai, Per-Olof Holtz, and Akinori Koukitu
    • Organizer
      International Workshop on Nitride Semiconductors 2012 (IWN2012)
    • Place of Presentation
      Sapporo Convention Center, Sapporo, Japan(TuP-GR-55.)
    • Year and Date
      2012-10-16
    • Related Report
      2013 Final Research Report
  • [Presentation] InN/sapphire(0001)MBEテンプレート上へのInN HVPEにおける成長速度の影響2011

    • Author(s)
      山本翔,東川義弘,富樫理恵,村上尚,熊谷義直,山口智弘,荒木努,名西やすし,纐纈明伯
    • Organizer
      第72回応用物理学会学術講演会
    • Place of Presentation
      山形大学小白川キャンパス(30a-ZE-12.)
    • Year and Date
      2011-08-30
    • Related Report
      2013 Final Research Report
  • [Presentation] HVPE法によるInN/sapphire(0001)テンプレート上InN高速成長の検討2011

    • Author(s)
      山本翔, 東川義弘, 富樫理恵, 村上尚, 熊谷義直, 山口智弘, 荒木努, 名西やすし, 纐纈明伯
    • Organizer
      第3回 窒化物半導体結晶成長講演会
    • Place of Presentation
      九州大学 筑紫キャンパス
    • Related Report
      2011 Research-status Report
  • [Presentation] InN/sapphire(0001)MBEテンプレート上へのInN HVPEにおける成長速度の影響2011

    • Author(s)
      山本翔, 東川義弘, 富樫理恵, 村上尚, 熊谷義直, 山口智弘, 荒木努, 名西やすし, 纐纈明伯
    • Organizer
      第72回応用物理学会学術講演会
    • Place of Presentation
      山形大学 小白川キャンパス
    • Related Report
      2011 Research-status Report
  • [Presentation] HVPE法によるInN/sapphire(0001)MBEテンプレート上へのInN成長の検討2011

    • Author(s)
      山本翔, 東川義弘, 富樫理恵, 村上尚, 熊谷義直, 山口智弘, 荒木努, 名西やすし, 纐纈明伯
    • Organizer
      第41回結晶成長国内会議(NCCG-41)
    • Place of Presentation
      つくば国際会議場
    • Related Report
      2011 Research-status Report
  • [Presentation] Comparative Study on High-Speed InN Growth in Both In- and N-Polarities Using a Two-Stage Source Generation Hydride Vapor Phase Epitaxy System

    • Author(s)
      Rie Togashi, Naoto Fujita, Ryota Imai, Hisashi Murakami, Yoshinao Kumagai and Akinori Koukitu
    • Organizer
      10th International Conference on Nitride Semiconductors (ICNS-10)
    • Place of Presentation
      Gaylord National Resort & Convention Center, Washington, D.C., U.S.A.
    • Related Report
      2013 Annual Research Report
  • [Presentation] Temperature Dependence of InN Growth by a Novel HVPE System with Two-Step Generation of InCl3

    • Author(s)
      Naoto Fujita, Ryota Imai, Rie Togashi, Hisashi Murakami, Yoshinao Kumagai and Akinori Koukitu
    • Organizer
      10th International Conference on Nitride Semiconductors (ICNS-10)
    • Place of Presentation
      Gaylord National Resort & Convention Center, Washington, D.C., U.S.A.
    • Related Report
      2013 Annual Research Report
  • [Presentation] Demonstration of high-speed growth of InN by HVPE with a two-step precursor generation scheme

    • Author(s)
      Naoto Fujita, R. Imai, R. Togashi, H. Murakami, Y. Kumagai, and A. Koukitu
    • Organizer
      2013 JSAP-MRS Joint Symposia
    • Place of Presentation
      Doshisha University, Kyoto, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] High-Speed InN Growth Using a Novel Two-Stage Source Generation Hydride Vapor Phase Epitaxy System

    • Author(s)
      R. Togashi, N. Fujita, R. Imai, H. Murakami, Y. Kumagai, and A. Koukitu
    • Organizer
      8th International Workshop on Bulk Nitride Semiconductors (IWBNS-VIII)
    • Place of Presentation
      Kloster Seeon, Seeon, Germany
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] High-Speed InN Growth on Yttria-Stabilized Zirconia (111) Substrates by a Two-Step Precursor Generation HVPE System

    • Author(s)
      C. Kojima, R. Togashi, R. Imai, N. Fujita, H. Saito, H. Murakami, Y. Kumagai, and A. Koukitu
    • Organizer
      Conference on LED and its industrial application '14 (LEDIA ’14)
    • Place of Presentation
      Pacifico Yokohama, Yokohama, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] 前駆体二段階生成HVPE法によるInNの高速成長の実現

    • Author(s)
      藤田直人,斉藤広伸,今井亮太,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      日本結晶成長学会ナノ構造・エピタキシャル成長分科会 第5回窒化物半導体結晶成長講演会
    • Place of Presentation
      大阪大学銀杏会館
    • Related Report
      2013 Annual Research Report
  • [Presentation] 前駆体二段階生成HVPE装置を用いたIn極性およびN極性InN成長の比較検討

    • Author(s)
      斉藤広伸,藤田直人,今井亮太,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      日本結晶成長学会ナノ構造・エピタキシャル成長分科会 第5回窒化物半導体結晶成長講演会
    • Place of Presentation
      大阪大学銀杏会館
    • Related Report
      2013 Annual Research Report
  • [Presentation] 前駆体二段階生成HVPE法によるIn極性およびN極性InNの高速成長

    • Author(s)
      斉藤広伸, 藤田直人,今井亮太,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      第74回応用物理学会学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] 前駆体二段階生成HVPE法によるInN成長の温度依存性

    • Author(s)
      藤田直人, 斉藤広伸,今井亮太,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      第43回結晶成長国内会議(NCCG-43)
    • Place of Presentation
      長野市生涯学習センター
    • Related Report
      2013 Annual Research Report
  • [Presentation] 前駆体二段階生成HVPE法によるIn, N各極性InN高速成長の比較検討

    • Author(s)
      斉藤広伸, 藤田直人,今井亮太,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      第43回結晶成長国内会議(NCCG-43)
    • Place of Presentation
      長野市生涯学習センター
    • Related Report
      2013 Annual Research Report
  • [Presentation] 前駆体二段階生成HVPE法により作製したInN成長層の特性評価

    • Author(s)
      富樫理恵, 斉藤広伸,藤田直人,今井亮太,村上尚,熊谷義直,纐纈明伯
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学相模原キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] Effect of high NH3 input partial pressure on hydride vapor phase epitaxy of InN using nitrided (0001) sapphire substrates

    • Author(s)
      Rie Togashi, Sho Yamamoto, Fredrik Karlsson, Hisashi Murakami, Yoshinao Kumagai, Per-Olof Holtz, and Akinori Koukitu
    • Organizer
      International Workshop on Nitride Semiconductors 2012 (IWN2012)
    • Place of Presentation
      Sapporo Convention Center, Sapporo, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] HVPE growth of InN on InN/sapphire (0001) templates prepared by MBE

    • Author(s)
      Ryota Imai, Sho Yamamoto, Rie Togashi, Hisashi Murakami, Yoshinao Kumagai, Tomohiro Yamaguchi, Tsutomu Araki, Yasushi Nanishi, and Akinori Koukitu
    • Organizer
      International Workshop on Nitride Semiconductors 2012 (IWN2012)
    • Place of Presentation
      Sapporo Convention Center, Sapporo, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] High-Speed Growth of InN Using a Two-Stage Source Generation HVPE System

    • Author(s)
      R. Togashi, R. Imai, S. Yamamoto, H. Murakami, Y. Kumagai, A. Koukitu
    • Organizer
      Intensive Discussion on Growth of Nitride Semiconductors
    • Place of Presentation
      Tohoku University, Sendai, Japan
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] High-Speed Growth of In- and N-polarity InN Using a Two-Stage Source Generation Hydride Vapor Phase Epitaxy System

    • Author(s)
      R. Togashi, N. Fujita, R. Imai, H. Murakami, Y. Kumagai, and A. Koukitu
    • Organizer
      Conference on LED and its industrial application '13 (LEDIA ’13)
    • Place of Presentation
      Pacifico Yokohama, Yokohama, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] High-speed growth of InN over 10 μm/h by a novel HVPE system

    • Author(s)
      N. Fujita, R. Imai, H. Saito, R. Togashi, H. Murakami, Y. Kumagai, and A. Koukitu
    • Organizer
      Conference on LED and its industrial application '13 (LEDIA ’13)
    • Place of Presentation
      Pacifico Yokohama, Yokohama, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] GaN自立基板上InNハイドライド気相成長における基板極性の影響

    • Author(s)
      富樫理恵, 村上尚, 熊谷義直, 纐纈明伯
    • Organizer
      第4回窒化物半導体結晶成長講演会(プレIWN2012講演会)
    • Place of Presentation
      東京大学生産技術研究所 An棟 コンベンションホール
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Improvement of crystalline and optical properties of InN grown on nitrided (0001) sapphire with high NH3 input partial pressures by HVPE

    • Author(s)
      R. Togashi, S. Yamamoto, K. F. Karlsson, H. Murakami, Y. Kumagai, P. O. Holtz, A. Koukitu
    • Organizer
      第73回応用物理学会学術講演会
    • Place of Presentation
      松山大学文京キャンパス
    • Related Report
      2012 Research-status Report
  • [Presentation] 2段階原料生成機構を有する新規HVPE法によるInNの高速成長の検討

    • Author(s)
      今井亮太,山本翔,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      第73回応用物理学会学術講演会
    • Place of Presentation
      松山大学文京キャンパス
    • Related Report
      2012 Research-status Report
  • [Presentation] HVPE法を用いたsapphire(0001)基板上InN成長におけるNH3供給分圧依存性

    • Author(s)
      富樫理恵,山本翔,K. F. Karlsson,村上尚,熊谷義直,P. O. Holtz,纐纈明伯
    • Organizer
      第42回結晶成長国内会議(NCCG-42)
    • Place of Presentation
      九州大学筑紫キャンパス
    • Related Report
      2012 Research-status Report
  • [Presentation] 2段階原料生成HVPE法によるGaN/sapphire(0001)テンプレート上InN成長

    • Author(s)
      今井亮太,山本翔,富樫理恵,村上尚,熊谷義直,纐纈明伯
    • Organizer
      第42回結晶成長国内会議(NCCG-42)
    • Place of Presentation
      九州大学筑紫キャンパス
    • Related Report
      2012 Research-status Report
  • [Remarks] 所属研究室HPの成果発信欄

    • URL

      http://www.tuat.ac.jp/~kumagai/

    • Related Report
      2013 Final Research Report
  • [Remarks] 熊谷研究室ホームページの研究成果発信欄

    • URL

      http://www.tuat.ac.jp/~kumagai/gakkai_H25.html

    • Related Report
      2013 Annual Research Report
  • [Remarks] 熊谷研究室ホームページの研究成果発信欄

    • URL

      http://www.tuat.ac.jp/̃kumagai/gakkai_H23.html

    • Related Report
      2012 Research-status Report
  • [Remarks] 研究成果について、研究室ホームページの成果発信欄(

    • URL

      http://www.tuat.ac.jp/~kumagai/gakkai_H23.html

    • Related Report
      2011 Research-status Report
  • [Remarks] )を利用して公開している。

    • Related Report
      2011 Research-status Report

URL: 

Published: 2011-08-05   Modified: 2019-07-29  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi