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Development of grain oriented multilayer ceramic actuator using bismuth based lead-free perovskites

Research Project

Project/Area Number 23760643
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Inorganic materials/Physical properties
Research InstitutionTokyo University of Science

Principal Investigator

NAGATA Hajime  東京理科大学, 理工学部, 准教授 (70339117)

Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2013: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2012: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2011: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywords非鉛圧電セラミックス / チタン酸ビスマスカリウム / 積層セラミックアクチュエータ / 粒子配向セラミックス / 圧電特性 / 非鉛強誘電体セラミックス / ペロブスカイト化合物 / 粒子配向技術
Research Abstract

Lead-based piezoelectric ceramics of Pb(Zr,Ti)O3 (PZT) are widely used in piezoelectric devices such as ultrasonic generators, sensors, resonators, and actuators. Recently, there has been a strong demand to develop environmentally friendly, that is, lead-free ferroelectric and piezoelectric ceramics. (Bi1/2K1/2)TiO3 [BKT] is one of bismuth based perovskite materials and showing high Curie temperature at approximately 400 oC and relatively large piezoelectric strain constant d33 about 100 pC/N. Therefore, BKT ceramics have been paid attention as one of candidates for lead-free piezoelectric actuator materials. In this study, we demonstrated multilayer piezoelectric actuators by using lead-free BKT ceramics and showing good electrical properties as compared with bulk BKT ceramics.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (42 results)

All 2014 2013 2012 2011 Other

All Journal Article (19 results) (of which Peer Reviewed: 19 results) Presentation (23 results) (of which Invited: 2 results)

  • [Journal Article] Key Engineering Materials, Piezoelectric Properties and Electric Field- Induced-Strains of Textured (Bi_<1/2>K_<1/2>)TiO_3- BaTiO_3 Ceramics2013

    • Author(s)
      Fumiaki Kawada, Yuji Hiruma, Hajime Nagata, and Tadashi Takenaka
    • Journal Title

      Electroceramics in Japan XIIV

      Volume: Vol. 566 Pages: 50-53

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication and electrical properties of potassium excess and poor (Bi_<1/2>K_<1/2>)TiO_3 ceramics2013

    • Author(s)
      Kazuya TABUCHI, Hajime NAGATA, Tadashi TAKENAKA
    • Journal Title

      Journal of The Ceramic Society of Japan

      Volume: Vol. 121 Pages: 623-626

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication and Electrical Properties of Multilayer Ceramic Actuator Using Lead-Free (Bi_<1/2>K_<1/2>)TiO_32013

    • Author(s)
      Hajime Nagata, Kazuya Tabuchi, and Tadashi Takenaka
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: Vol. 52

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Effects of Starting Raw Materials for Fabricating Dense (Bi_<1/2>K_<1/2>)TiO_3 Ceramics2013

    • Author(s)
      Kazuya Tabuchi, Yuta Inoue, Hajime Nagata and Tadashi Takenaka
    • Journal Title

      Ferroelectrics

      Volume: Vol. 457 Pages: 124-130

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication and Electrical Properties of Multilayer Ceramic Actuator Using Lead-Free (Bi1/2K1/2)TiO32013

    • Author(s)
      Hajime. Nagata, Kazuya. Tabuchi, and Tadashi. Takenaka
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 52

    • NAID

      210000142844

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication and electrical properties of potassium excess and poor (Bi1/2K1/2)TiO3 ceramics2013

    • Author(s)
      Kazuya TABUCHI, Hajime NAGATA, Tadashi TAKENAKA
    • Journal Title

      Journal of The Ceramic Society of Japan

      Volume: 121 Pages: 623-626

    • NAID

      130004480198

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effects of Starting Raw Materials for Fabricating Dense (Bi1/2K1/2)TiO3 Ceramics2013

    • Author(s)
      Kazuya Tabuchi, Yuta Inoue, Hajime Nagata and Tadashi Takenaka
    • Journal Title

      Ferroelectrics

      Volume: 457 Pages: 124-130

    • Related Report
      2013 Annual Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Piezoelectric Properties and Electric Field-Induced-Strains of Textured (Bi1/2K1/2)TiO3- BaTiO3 Ceramics,2013

    • Author(s)
      Fumiaki Kawada, Yuji Hiruma, Hajime Nagata, and Tadashi Takenaka,
    • Journal Title

      Key Engineering Materials, “Electroceramics in Japan XIIV

      Volume: 566 Pages: 50-53

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dielectric and Piezoelectric Properties of Mn-doped KNbO3 Ceramics2013

    • Author(s)
      Nobutaka Yawata, Hajime Nagata and Tadashi Takenaka
    • Journal Title

      Ferroelectrics

      Volume: 458 Pages: 158-162

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electrical Properties of Grain Oriented Bi4Ti3O12-based Ceramics for High Temperature Sensors2013

    • Author(s)
      Koji Shiga, Shogo Yasuda, Yuji Hiruma, Hajime Nagata, and Tadashi Takenaka,
    • Journal Title

      Key Engineering Materials, “Electroceramics in Japan XIIV”

      Volume: 566 Pages: 237-240

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Piezoelectric Properties and Electric Field-Induced-Strains of Textured (Bi1/2K1/2)TiO3- BaTiO3 Ceramics2013

    • Author(s)
      Fumiaki Kawada, Yuji Hiruma, Hajime Nagata, and Tadashi Takenaka
    • Journal Title

      Key Engineering Materials, “Electroceramics in Japan XIIV”

      Volume: in press

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fabrication and Electrical Properties of Potassium Excess and poor (Bi1/2K1/2)TiO3 ceramics2013

    • Author(s)
      Kazuya Tabuchi, Yuta Inoue, Hajime Nagata and Tadashi Takenaka
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: in press

    • NAID

      130004480198

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Excess Potassium and Microstructure Control for Producing Dense KNbO_3 Ceramics2012

    • Author(s)
      Shigeki. Sato, Yuji Hiruma, Hajime Nagata and Tadashi Takenaka
    • Journal Title

      Transactions of the Materials Research Society of Japan

      Volume: Vol. 37 Pages: 65-68

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication and Electrical Properties of Mn-Doped KNbO_3 Ceramics Synthesized from KHCO_3 as a Starting Material2012

    • Author(s)
      Hajime Nagata, Nobutaka Yawata, Shigeki Sato and Tadashi Takenaka
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: Vol. 51

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Piezoelectric Properties and Electric Field-Induced-Strains of Textured (Bi1/2K1/2)TiO3-BaTiO3 Ceramics2012

    • Author(s)
      Fumiaki Kawada, Yuji Hiruma, Hajime Nagata, and Tadashi Takenaka
    • Journal Title

      Key Engineering Materials

      Volume: in press

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Excess Potassium and Microstructure Control for Producing Dense KNbO3 Ceramics2012

    • Author(s)
      Shigeki. Sato, Yuji Hiruma, Hajime Nagata and Tadashi Takenaka
    • Journal Title

      Transactions of the Materials Research Society of Japan

      Volume: 37 Pages: 65-68

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fabrication of Dense KNbO_3 Ceramics Derived from KHCO_3 as a Starting Material2011

    • Author(s)
      Hajime Nagata, Shigeki Sato, Yuji Hiruma, and Tadashi Takenaka
    • Journal Title

      Applied Physics Express

      Volume: Vol. 5 Pages: 11502-11502

    • NAID

      10030154610

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication of Dense KNbO3 Ceramics Derived from KHCO3 as a Starting Material2011

    • Author(s)
      Hajime Nagata, Shigeki Sato, Yuji Hiruma, and Tadashi Takenaka
    • Journal Title

      Applied Physics Express

      Volume: 5 Pages: 11502-11502

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] High-temperature and High-power Piezoelectric Characteristics for (Bi_<0.5>Na_<0.5>)TiO_3- based Lead-Free Piezo- electric Ceramics

    • Author(s)
      Shinya Someno, Hajime Nagata, and Tadashi Takenaka
    • Journal Title

      Journal of The Ceramic Society of Japan

      Volume: (in press)

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Presentation] (Bi_<1/2>K_<1/2>)TiO_3セラミックスの焼結性及び電気的諸特性に及ぼす添加物効果2014

    • Author(s)
      染谷拓巳、田渕量也、永田肇、竹中正
    • Organizer
      日本セラミックス協会2014年年会
    • Place of Presentation
      慶応大学(東京)
    • Related Report
      2013 Final Research Report
  • [Presentation] (Bi1/2K1/2)TiO3セラミックスの焼結性及び電気的諸特性に及ぼす添加物効果2014

    • Author(s)
      染谷 拓巳・田渕 量也・永田 肇・竹中 正
    • Organizer
      日本セラミックス協会 2014年 年会
    • Place of Presentation
      慶応大学、東京
    • Related Report
      2013 Annual Research Report
  • [Presentation] (Bi_<1/2>K_<1/2>)TiO_3セラミックスのカリウム量の変化による電気的諸特性2013

    • Author(s)
      田渕量也,永田肇,竹中正
    • Organizer
      日本セラミックス協会2013年年会
    • Place of Presentation
      東京工業大学(東京)
    • Related Report
      2013 Final Research Report
  • [Presentation] Historical Overview and Current Developments of Lead-free Piezoelectric Ceramics2013

    • Author(s)
      Hajime Nagata, and Tadashi Takenaka
    • Organizer
      10th Pacific Rim Conference on Ceramic and Glass Technology (PACRIM 10)
    • Place of Presentation
      Coronado, USA
    • Related Report
      2013 Final Research Report
  • [Presentation] Fabrication and Electrical Properties of Dense (Bi_<1/2>K_<1/2>)TiO_3 Ceramics and Their Multilayer Actuator2013

    • Author(s)
      H. Nagata, K. Tabuchi, T. Takenaka
    • Organizer
      The 2nd International Conference on Advanced Electromaterials
    • Place of Presentation
      Jeju, Korea
    • Related Report
      2013 Final Research Report
  • [Presentation] (Bi_<1/2>K_<1/2>)TiO_3セラミックスの焼結性と電気的諸特性2013

    • Author(s)
      田渕量也,永田肇,竹中正
    • Organizer
      第23回日本MRS年次大会
    • Place of Presentation
      横浜(神奈川)
    • Related Report
      2013 Final Research Report
  • [Presentation] Historical Overview and Current Developments of Lead-free Piezoelectric Ceramics2013

    • Author(s)
      Tadashi Takenaka, and Hajime Nagata
    • Organizer
      Tadashi Takenaka, and Hajime Nagata, 10th Pacific Rim Conference on Ceramic and Glass Technology (PACRIM 10)
    • Place of Presentation
      Coronado, USA
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Fabrication and Electrical Properties of Dense (Bi1/2K1/2)TiO3 Ceramics and Their Multilayer Actuator2013

    • Author(s)
      Hajime Nagata, Kazuya Tabuchi, and Tadashi Takenaka
    • Organizer
      The 2nd International Conference on Advanced Electromaterials (ICAE2013)
    • Place of Presentation
      Jeju, Korea
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 非鉛(Bi1/2K1/2)TiO3積層セラミックアクチュエータの試作と電気的諸特性2013

    • Author(s)
      永田 肇 ・ 坂本遼太 ・ 竹中 正
    • Organizer
      第30回 強誘電体応用会議(FMA)
    • Place of Presentation
      コープイン京都
    • Related Report
      2013 Annual Research Report
  • [Presentation] KHCO_3を用いた(Bi_<1/2>K_<1/2>)TiO_3の作製と電気的諸特性2012

    • Author(s)
      田渕量也,井上雄太,永田肇,竹中正
    • Organizer
      第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学(東京)
    • Related Report
      2013 Final Research Report
  • [Presentation] Fabrication and Electrical Properties of dense (Bi_<1/2>K_<1/2>)TiO_3 Ceramics Synthesized from KHCO_3 as a Starting Material2012

    • Author(s)
      Kazuya Tabuchi, Hajime Nagata, Tadashi Takenaka
    • Organizer
      The 6th International Conference on the Science and Technology for Advanced Ceramics
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] Fabrication and Electrical Properties of Dense (Bi_<1/2>K_<1/2>)TiO_3 Ceramic2012

    • Author(s)
      Hajime Nagata, Kazuya Tabuchi, Tadashi Takenaka
    • Organizer
      ISAF ECPAD PFM 2012
    • Place of Presentation
      Aveiro, Portugal
    • Related Report
      2013 Final Research Report
  • [Presentation] Excess Potassium Effects for Fabricating Dense KNbO_3 and (Bi_<1/2>K_<1/2>)TiO_3 Ceramics2012

    • Author(s)
      Hajime Nagata, Kazuya Tabuchi, Nobutaka Yawata, Tadashi Takenaka
    • Organizer
      IUMRS-International Conference on Electronic Materials
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] (Bi_<1/2>K_<1/2>)TiO_3セラミックスの焼結性に及ぼす出発原料の粒子径効果2012

    • Author(s)
      井上雄太,田渕量也,永田肇,竹中正
    • Organizer
      第32回エレクトロセラミックス研究討論会
    • Place of Presentation
      東京工業大学(東京)
    • Related Report
      2013 Final Research Report
  • [Presentation] Fabrication and Electrical Properties of Potassium Excess or Poor (Bi_<1/2>K_<1/2>)TiO_3 Ceramics2012

    • Author(s)
      Kazuya Tabuchi, Hajime Nagata, Tadashi Takenaka
    • Organizer
      The 8th Asian Meeting on Ferroelectrics
    • Place of Presentation
      Pataya, Thailand
    • Related Report
      2013 Final Research Report
  • [Presentation] FABRICATION AND ELECTRICAL PROPERTIES OF DENSE (Bi1/2K1/2)TiO3 CERAMIC2012

    • Author(s)
      Hajime Nagata, Kazuya Tabuchi, and Tadashi Takenaka
    • Organizer
      IEEE International Symposium on the Applications of Ferroelectrics 2013
    • Place of Presentation
      Aveiro, Portugal
    • Related Report
      2012 Research-status Report
  • [Presentation] Excess Potassium Effects for Fabricating Dense KNbO3 and (Bi1/2K1/2)TiO3 Ceramics2012

    • Author(s)
      Hajime Nagata, K. Tabuchi, N. Yawata and Tadashi Takenaka
    • Organizer
      IUMRS International Conference on Electronic Materials 2012
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] Kazuya Tabuchi, Hajime Nagata and Tadashi Takenaka2012

    • Author(s)
      Fabrication and Electrical Properties of dense (Bi1/2K1/2)TiO3 Ceramics Synthesized from KHCO3 as a Starting Material
    • Organizer
      The 6th International Conference on the Science and Technology for Advanced Ceramics
    • Place of Presentation
      Yokohama, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] Kazuya Tabuchi, Hajime Nagata and Tadashi Takenaka2012

    • Author(s)
      Fabrication and Electrical Properties of Potassium Excess and Poor (Bi1/2K1/2)TiO3 Ceramics
    • Organizer
      The 8th Asian Meeting on Ferroelectrics
    • Place of Presentation
      Pataya, Thailand
    • Related Report
      2012 Research-status Report
  • [Presentation] 井上 雄太、田渕 量也、永田 肇、竹中 正2012

    • Author(s)
      (Bi1/2K1/2)TiO3セラミックスの焼結性に及ぼす出発原料の粒子径効果
    • Organizer
      日本セラミックス協会 エレクトロセラミックス研究討論会 2012
    • Place of Presentation
      東京
    • Related Report
      2012 Research-status Report
  • [Presentation] 坂本 遼太・永田 肇・竹中 正2012

    • Author(s)
      (Bi1/2K1/2)TiO3積層セラミックアクチュエータの試作と電気的諸特性
    • Organizer
      日本セラミックス協会 第25回秋季シンポジウム
    • Place of Presentation
      名古屋
    • Related Report
      2012 Research-status Report
  • [Presentation] 出発原料にKHCO3を用いた(Bi1/2K1/2)TiO3セラミックスの作製と電気的諸特性2012

    • Author(s)
      田渕量也 ・ 井上雄太 ・ 永 田 肇 ・ 竹 中 正
    • Organizer
      応用物理学会 2012年春季講演会
    • Place of Presentation
      早稲田大学 早稲田キャンパス(東京都)
    • Related Report
      2011 Research-status Report
  • [Presentation] 粒子配向型(Bi1/2K1/2)TiO3- BaTiO3系強誘電体セラミックスの電界誘起歪み特性2011

    • Author(s)
      川田 文亮 ・ 晝間 裕二・ 永 田 肇 ・ 竹 中 正
    • Organizer
      日本セラミックス協会・第31回エレクトロセラミックス研究討論会
    • Place of Presentation
      東京大学駒場II リサーチキャンパス(東京都)
    • Related Report
      2011 Research-status Report

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Published: 2011-08-05   Modified: 2019-07-29  

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