Determination of geometrical structures of molecules by ultrafast gas electron diffraction and gas X ray diffraction
Project/Area Number |
24245003
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Research Category |
Grant-in-Aid for Scientific Research (A)
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Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Physical chemistry
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Research Institution | The University of Tokyo |
Principal Investigator |
YAMANOUCHI Kaoru 東京大学, 理学(系)研究科(研究院), 教授 (40182597)
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Co-Investigator(Renkei-kenkyūsha) |
KATO Tsuyoshi 東京大学, 理学系研究科, 准教授 (10321986)
IWASAKI Atsushi 東京大学, 理学系研究科, 准教授 (30447073)
KANYA Reika 東京大学, 理学系研究科, 助教 (10401168)
SATO Takahiro 東京大学, 理学系研究科, 助教 (30599113)
|
Project Period (FY) |
2012-04-01 – 2015-03-31
|
Project Status |
Completed (Fiscal Year 2014)
|
Budget Amount *help |
¥45,110,000 (Direct Cost: ¥34,700,000、Indirect Cost: ¥10,410,000)
Fiscal Year 2014: ¥10,400,000 (Direct Cost: ¥8,000,000、Indirect Cost: ¥2,400,000)
Fiscal Year 2013: ¥15,600,000 (Direct Cost: ¥12,000,000、Indirect Cost: ¥3,600,000)
Fiscal Year 2012: ¥19,110,000 (Direct Cost: ¥14,700,000、Indirect Cost: ¥4,410,000)
|
Keywords | 分子構造 / 電子回折 / X線回折 / 量子動力学計算 / 時間分解 |
Outline of Final Research Achievements |
We developed laser-assisted electron diffraction (LAED) method by which geometrical structures of molecules can be determined with femtosecond temporal resolution. In addition, by recording the diffraction patterns, we demonstrated for the first time that the effect of the creation of light-dressed atoms appears in the scattering angle distributions of the LAED signals. We developed a time-resolved X-ray diffraction (XRD) apparatus for time resolved measurements of geometrical structure of molecules in the gas phase using the XFEL light source, and confirmed that XRD patterns of molecules can be recorded in the wide scattering angle range by using synchrotron radiation of SPring-8. Furthermore, in order to analyze the effect of the electron-nucleus correlation appearing in the LAED and XRD signals, we developed the time-dependent effective potential method based on the extended time-dependent multi-configuration theory, and applied it to the hydrogen molecular model.
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Report
(4 results)
Research Products
(112 results)
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[Journal Article] Selective control over fragmentation reactions in polyatomic molecules using impulsive laser alignment2014
Author(s)
X. Xie, K. Doblhoff-Dier, H. Xu, S. Roither, M. Schoffler, D. Kartashov, S. Erattupzha, T. Rathje, G. Paulus, K. Yamanouchi, A. Baltuska, S. Graefe, M. Kitzler
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Journal Title
Physical Review Letters
Volume: 112
Issue: 16
DOI
Related Report
Peer Reviewed
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[Journal Article] Lasing action induced by femtosecond laser filamentation in ethanol flame for combustion diagnosis2014
Author(s)
W. Chu, H. Li, J. Ni, B. Zeng, J. Yao, H. Zhang, G. Li, C. Jing, H. Xie, H. Xu, K. Yamanouchi, Y. Cheng
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Journal Title
Appled Physics Letters
Volume: 104
Issue: 9
Pages: 091106-091106
DOI
Related Report
Peer Reviewed
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[Journal Article] Carrier-envelope-phase dependence of asymmetric C-D bond breaking in C2D2 in an intense few-cycle laser field2014
Author(s)
S. Miura, T. Ando, K. Ootaka, A. Iwasaki, H. Xu, T. Okino, K. Yamanouchi, D. Hoff, T. Rathje, G. G. Paulus, M. Kitzler, A. Baltuska, G. Sansone, M, Nisoli
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Journal Title
Chemical Physics Letters
Volume: 595-596C
Pages: 61-66
DOI
Related Report
Peer Reviewed / Acknowledgement Compliant
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[Journal Article] Electronic pre-determination of ethylene fragmentation dynamics2014
Author(s)
X. Xie, S. Roither, M. Schoffler, E. Lotstedt, D. Kartashov, L. Zhang, G. G. Paulus, A. Iwasaki, A. Baltuska, K. Yamanouchi, M. Kitzler
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Journal Title
Physical Review X
Volume: 4
Issue: 2
DOI
Related Report
Peer Reviewed
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[Journal Article] Strong and coherent forward emissions from molecules driven by femtosecond infrared laser pulses2014
Author(s)
H. Xu, J. Yao, W. Chu, B. Zeng, J. Ni, G. Li, Y. Cheng, Z. Xu, D. Kartashov, S. Alisauskas, A. Pugzlys, A. Baltuska, K. Yamanouchi, S. L. Chin
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Journal Title
Progress in Ultrafast Intense Laser Science
Volume: 10
Pages: 95-109
DOI
ISBN
9783319005201, 9783319005218
Related Report
Peer Reviewed
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[Journal Article] XUV interferometry of attosecond pulses2012
Author(s)
Y. Nabekawa, E. J. Takahashi, Y. Furukawa, T. Okino, K. Yamanouchi, K. Midorikawa
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Journal Title
Multiphoton Processes and Attosecond Physics: Proceedings of the 12th International Conference on Multiphoton Processes (ICOMP12) and the 3rd International Conference on Attosecond Physics (ATTO3)
Volume: 125
Pages: 127-135
DOI
ISBN
9783642289477, 9783642289484
Related Report
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[Journal Article] Enormous amplification of full-coherent radiation in the extreme ultraviolet region with a free-electron laser2012
Author(s)
E. J. Takahashi, T. Togashi, M. Aoyama, K. Yamakawa, T. Sato, A. Iwasaki, S. Owada, K. Yamanouchi, T. Hara, S. Matsubara, T. Ohshima, Y. Otake, H. Tanaka, T. Tanaka, H. Tomizawa, T. Watanabe, M. Yabashi, K. Midorikawa, T. Ishikawa
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Journal Title
Multiphoton Processes and Attosecond Physics: Proceedings of the 12th International Conference on Multiphoton Processes (ICOMP12) and the 3rd International Conference on Attosecond Physics (ATTO3)
Volume: 125
Pages: 155-161
DOI
ISBN
9783642289477, 9783642289484
Related Report
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[Journal Article] Classical models of H3+ interacting with intense laser fields2012
Author(s)
E. Loetstedt, T. Kato, K. Yamanouchi
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Journal Title
Multiphoton Processes and Attosecond Physics: Proceedings of the 12th International Conference on Multiphoton Processes (ICOMP12) and the 3rd International Conference on Attosecond Physics (ATTO3)
Volume: 125
Pages: 233-237
DOI
ISBN
9783642289477, 9783642289484
Related Report
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[Journal Article] High energy proton ejection from hydrocarbon molecules driven by highly efficient field ionization2012
Author(s)
S. Roither, X. Xie, D. Kartashov, L. Zhang, M. Shöffler, H. Xu, A. Iwasaki, T. Okino, K. Yamanouchi, A. Baltuška, M. Kitzler
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Journal Title
Multiphoton Processes and Attosecond Physics: Proceedings of the 12th International Conference on Multiphoton Processes (ICOMP12) and the 3rd International Conference on Attosecond Physics (ATTO3)
Volume: 125
Pages: 341-346
DOI
ISBN
9783642289477, 9783642289484
Related Report
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[Journal Article] Efficient ionization of acetylene in intense laser fields2012
Author(s)
E. Loetstedt, T. Kato, K. Yamanouchi
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Journal Title
Multiphoton Processes and Attosecond Physics: Proceedings of the 12th International Conference on Multiphoton Processes (ICOMP12) and the 3rd International Conference on Attosecond Physics (ATTO3)
Volume: 125
Pages: 347-350
DOI
ISBN
9783642289477, 9783642289484
Related Report
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[Presentation] Improvement for HHG-seeded EUV free electron laser with timing measurement system by EO sampling2014
Author(s)
K. Ogawa, T. Sato, S. Owada, S. Matsubara, Y. Okayasu, T. Togashi, T. Watanabe, E. J. Takahashi, K. Midorikawa, M. Aoyama, K. Yamakawa, A. Iwasaki, K. Yamanouchi, T. Oshima, Y. Otake, T. Hara, T. Tanaka, H. Tanaka, H. Tomizawa, M. Yabashi, T. Ishikawa
Organizer
19th International Conference on Ultrafast Phenomena
Place of Presentation
Okinawa Convention Center, Okinawa, Japan
Year and Date
2014-07-07 – 2014-07-11
Related Report
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[Presentation] Stable operation of HHG-seeded EUV-FEL at the SCSS test accelerator2013
Author(s)
H. Tomizawa, T. Hara, T. Ishikawa, K. Ogawa, H. Tanaka, T. Tanaka, T. Togashi, K. Togawa, M. Yabashi, M. Aoyama, K. Yamakawa, A. Iwasaki, S. Owada, T. Sato, K. Yamanouchi, S. Matsubara, Y. Okayasu, T. Watanabe, K. Midorikawa, E. Takahashi
Organizer
35th International Free-Electron Laser Conference (FEL2013)
Place of Presentation
New York Marriott Marquis Hotel, Manhattan, USA
Year and Date
2013-08-25 – 2013-08-30
Related Report
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[Presentation] Full-coherent HHG-seeded EUV-FEL locked by EOS timing feedback2013
Author(s)
K. Ogawa, T. Sato, S. Matsubara, Y. Okayasu, T. Togashi, T. Watanabe, E. J. Takahashi, K. Midorikawa, M. Aoyama, K. Yamakawa, A. Iwasaki, S. Owada, K. Yamanouchi, T. Ohshima, Y. Otake, T. Hara, T. Tanaka, H. Tanaka, H. Tomizawa, M. Yabashi, T. Ishikawa
Organizer
Conference on Lasers and Electro-Optics/Pacific Rim
Place of Presentation
Kyoto, Japan
Year and Date
2013-06-30 – 2013-07-04
Related Report
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[Presentation] A few tens of microjoule full-coherent EUV-FEL seeded by high-order harmonic beam2013
Author(s)
E. J. Takahashi, T. Togashi, M. Aoyama, K. Yamakawa, T. Sato, A. Iwasaki, S. Owada, K. Yamanouchi, T. Hara, S. Matsubara, K. Ogawa, H. Ohshima, Y. Okayasu, Y. Otake, H. Tanaka, T. Tanaka, H. Tomizawa, T. Watanabe, M. Yabashi, K. Midorikawa, T. Ishikawa
Organizer
CLEO: QELS_Fundamental Science
Place of Presentation
San Jose, California, United States
Year and Date
2013-06-09 – 2013-06-14
Related Report
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[Presentation] Full-coherent free electron laser seeded by high-order harmonics of near-infrared femtosecond laser pulses2013
Author(s)
A. Iwasaki, S. Owada, S. Ogami, T. Sato, T. Togashi, E. J. Takahashi, K. Midorikawa, M. Aoyama, K. Yamakawa, S. Matsubara, K. Ogawa, Y. Okayasu, H. Tomizawa, T. Watanabe, M. Nagasono, M. Yabashi, T. Ishikawa, K. Yamanouchi
Organizer
第29回化学反応討論会
Place of Presentation
東北大学 片平キャンパス,仙台市,宮城県
Year and Date
2013-06-05 – 2013-06-07
Related Report
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[Presentation] Temporal overlapping for HHG- seeded EUV-FEL operation by using EOS-based timing-drift controlling system2013
Author(s)
S. Matsubara, T. Togashi , E. J. Takahashi , K. Midorikawa, M. Aoyama, .K. Yamakawa, T. Sato, A. Iwasaki, S. Owada, K. Yamanouchi, K. Togawa, T. Hara, K. Ogawa, T. Ohshima, Y. Okayasu, Y. Otake , H. Tanaka, T. Tanaka, H. Tomizawa, T. Watanabe, M. Yabashi, T. Ishikawa
Organizer
The European Conference on Lasers and Electro-Optics
Place of Presentation
Munich, Germany
Year and Date
2013-05-12 – 2013-05-16
Related Report
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