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Development and Functional Exploration of Special Molecular Space based on Conjugated Porous Polymers

Research Project

Project/Area Number 24245030
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Functional materials chemistry
Research InstitutionInstitute for Molecular Science

Principal Investigator

Jiang Donglin  分子科学研究所, 物質分子科学研究領域, 教授(兼任) (40302765)

Project Period (FY) 2012-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥46,800,000 (Direct Cost: ¥36,000,000、Indirect Cost: ¥10,800,000)
Fiscal Year 2014: ¥9,750,000 (Direct Cost: ¥7,500,000、Indirect Cost: ¥2,250,000)
Fiscal Year 2013: ¥10,530,000 (Direct Cost: ¥8,100,000、Indirect Cost: ¥2,430,000)
Fiscal Year 2012: ¥26,520,000 (Direct Cost: ¥20,400,000、Indirect Cost: ¥6,120,000)
Keywords共役多孔性高分子 / 分子設計 / 合成 / 構造制御 / エネルギー貯蔵 / 有機触媒 / 不斉反応 / ガス吸着 / 機能 / 不斉合成 / 触媒再利用 / 共役高分子 / 多孔高分子 / 機能性材料 / 分子空間 / 多孔性高分子 / 触媒 / 再利用
Outline of Final Research Achievements

In this study, we designed molecular structures of conjugated porous polymers, explored the methodology to control their frameworks and pores, synthesised a series of polymers with special nano space, and succeeded in developing novel functions. Especially, we have developed a series of novel convo;end organic frameworks by elucidating their special interactions with molecules. Ind details, we developed materials for energy storage, materials for organic catalysis, and materials for gas storages. Among these advanced materials, we explored materials that exhibited high capacity and high energy density and powder density for energy storage,recyclable materials for organic catalysis with high activity for asymmetric organic transformations, and materials for gas storages such as carbon dioxide and amines.

Report

(4 results)
  • 2015 Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (42 results)

All 2016 2015 2014 2013 Other

All Int'l Joint Research (3 results) Journal Article (23 results) (of which Int'l Joint Research: 10 results,  Peer Reviewed: 23 results,  Open Access: 13 results,  Acknowledgement Compliant: 9 results) Presentation (14 results) (of which Int'l Joint Research: 8 results,  Invited: 12 results) Book (2 results)

  • [Int'l Joint Research] University of Amsterdam(オランダ)

    • Related Report
      2014 Annual Research Report
  • [Int'l Joint Research] Jilin University/Sun Yat-sen University/South China University of Technology(中国)

    • Related Report
      2014 Annual Research Report
  • [Int'l Joint Research] KAIST(韓国)

    • Related Report
      2014 Annual Research Report
  • [Journal Article] Covalent Organic Frameworks with Spatially Confined Guest Molecules in Nanochannels and Their Impacts on Crystalline Structures2016

    • Author(s)
      Jia Guo, Donglin Jiang
    • Journal Title

      Chem. Commun.

      Volume: 52 Issue: 7 Pages: 1498-1500

    • DOI

      10.1039/c5cc09225f

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Porous Organic Polymers with Tunable Work Functions and Selective Hole and Electron Conductions for Energy Conversions2016

    • Author(s)
      Cheng Gu, Ning Huang, Youchun Chen, Huanhuan Zhang, Shitong Zhang, Fenghong Li, Yuguang Ma, and Donglin Jiang
    • Journal Title

      Angew. Chem., Int. Ed.

      Volume: 55 Issue: 9 Pages: 3049-3053

    • DOI

      10.1002/anie.201510723

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Two-Dimensional Covalent Organic Frameworks for Carbon Dioxide Capture via Channel-Wall Functionalization2015

    • Author(s)
      Ning Huang, Xiong Chen, Rajamani Krishna, Donglin Jiang
    • Journal Title

      Angew. Chem., Int. Ed.

      Volume: 54 Issue: 10 Pages: 2986-2990

    • DOI

      10.1002/anie.201411262

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Electrochemically Active, Crystalline, Mesoporous Covalent Organic Frameworks on Carbon Nanotubes for Synergistic Lithium Battery Energy Storage2015

    • Author(s)
      Fei Xu, Shangbin Jin, Hui Zhong, Dingcai Wu, Xiaoqing Yang, Xiong Chen, Hao Wei, Ruowen Fu, Donglin Jiang
    • Journal Title

      Scientific Reports

      Volume: 1 Issue: 1 Pages: 1-8

    • DOI

      10.1038/srep08225

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Cascade Exciton-Pumping Engines with Manipulated Speed and Efficiency in Light-Harvesting Porous π-Network Films2015

    • Author(s)
      Cheng Gu, Ning Huang, Fei Xu, Jia Gao, Donglin Jiang
    • Journal Title

      Scientific Reports

      Volume: 1 Issue: 1 Pages: 1-9

    • DOI

      10.1038/srep08867

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Locking Covalent Organic Frameworks with Hydrogen Bonds: General and Remarkable Effects on Crystalline Structure, Physical Properties, and Photochemical Activities2015

    • Author(s)
      X. Chen, M. Addicoat, E. Jin, L. Zhai, H. Xu, N. Huang, Z. Guo, L. Liu, S. Irle, D. Jiang
    • Journal Title

      J. Am. Chem. Soc. (Communication)

      Volume: 137 Issue: 9 Pages: 3241-3247

    • DOI

      10.1021/ja509602c

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Radical Covalent Organic Frameworks: A General Strategy to Immobilize Open-Accessible Polyradicals and High-Performance Capacitive Energy Storage2015

    • Author(s)
      Fei Xu , Hong Xu, Xiong Chen, Dingcai Wu, Yang Wu, Hao Liu, Cheng Gu, Ruowen Fu, Donglin Jiang
    • Journal Title

      Angew. Chem., Int. Ed.

      Volume: 48 Issue: 23 Pages: 6814-6818

    • DOI

      10.1002/anie.201501706

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] π-Electronic Covalent Organic Framework Catalyst: π-Walls as Catalytic Beds for Diels-Alder Reactions Under Ambient Conditions2015

    • Author(s)
      Yang Wu, Jia Gao, Donglin Jiang
    • Journal Title

      Chem. Commun.

      Volume: 51 Issue: 50 Pages: 10096-10098

    • DOI

      10.1039/c5cc03457d

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A Photoresponsive Smart Covalent Organic Framework2015

    • Author(s)
      Ning Huang, Xuesong Ding, Jangbae Kim, Hyotcherl Ihee, Donglin Jiang
    • Journal Title

      Angew. Chem., Int. Ed.

      Volume: 54 Issue: 30 Pages: 8704-8707

    • DOI

      10.1002/anie.201503902

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Creation of Superheterojunction Polymers via Direct Polycondensation: Segregated and Bicontinuous Donor-Acceptor π-Columnar Arrays in Covalent Organic Frameworks for Long-Lived Charge Separation2015

    • Author(s)
      Shangbin Jin, Mustafa Supur, Matthew Addicoat, Ko Furukawa, Long Chen, Toshikazu Nakamura, Shunichi Fukuzumi, Stephan Irle, Donglin Jiang
    • Journal Title

      J. Am. Chem. Soc.

      Volume: 137 Pages: 7817-7827

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Tailor-Made Pore Surface Engineering in Covalent Organic Frameworks: Systematic Functionalization for Performance Screening2015

    • Author(s)
      Ning Huang, Rajamani Krishna, Donglin Jiang
    • Journal Title

      J. Am. Chem. Soc.

      Volume: 137 Pages: 7079-7082

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Rational Design of Crystalline Supermicroporous Covalent Organic Frameworks with Triangular Topologies2015

    • Author(s)
      Sasanka Dalapati, Matthew Addicoat, Shangbin Jin, Tsuneaki Sakurai, Jia Gao, Hong Xu, Stephan Irle, Shu Seki, Donglin Jiang
    • Journal Title

      Nature Communications

      Volume: 6 Issue: 1 Pages: 1-9

    • DOI

      10.1038/ncomms8786

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Design of AIE-Based Highly Photofunctional Porous Polymer Films with Controlled Thickness and Prominent Microporosity2015

    • Author(s)
      Cheng Gu, Ning Huang, Yang Wu, Hong Xu, Donglin Jiang
    • Journal Title

      Angew. Chem., Int. Ed.

      Volume: 54 Issue: 39 Pages: 11540-11544

    • DOI

      10.1002/anie.201504786

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Stable, Crystalline, Porous, Covalent Organic Frameworks As A Platform for Chiral Organocatalysis2015

    • Author(s)
      Hong Xu, Jia Gao, Donglin Jiang
    • Journal Title

      Nature Chemistry

      Volume: 7 Pages: 905-912

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Designed Synthesis of Double-Stage Two-Dimensional Covalent Organic Frameworks2015

    • Author(s)
      Xiong Chen, Matthew Addicoat, Enquan Jin, Hong Xu, Taku Hayashi, Fei Xu, Ning Huang, Stephan Irle, Donglin Jiang
    • Journal Title

      Scientific Reports

      Volume: 1 Pages: 1-12

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] π-Conjugated Microporous Polymer Films: Designed Synthesis, Conducting Properties and Photoenergy Conversions2015

    • Author(s)
      Cheng Gu, Ning Huang, Youchun Chen, Leiqiang Qin, Hong Xu, Shitong Zhang, Fenghong Li, Yuguang Ma, Donglin Jiang
    • Journal Title

      Angew. Chem., Int. Ed.

      Volume: 54 Issue: 46 Pages: 13594-13598

    • DOI

      10.1002/anie.201506570

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Catalytic Covalent Organic Frameworks via Pore Surface Engineering2014

    • Author(s)
      Hong Xu, Xiong Chen, Jia Gao, Jianbin Lin, Matthew Addicoat, Stephan Irle and Donglin Jiang
    • Journal Title

      Chem. Commun.

      Volume: 50 Issue: 11 Pages: 1292-1294

    • DOI

      10.1039/c3cc48813f

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Large Pore Donor-Acceptor Covalent Organic Frameworks2013

    • Author(s)
      S. Jin, K. Furukawa, M. Addicoat, L. Chen, T. Seiya, S. Irle, T. Nakamura and D. Jiang
    • Journal Title

      Chem. Sci

      Volume: 4 Issue: 12 Pages: 4505-4511

    • DOI

      10.1039/c3sc52034j

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Conjugated organic framework with three-dimensionally ordered stable polymer with delocalized π clouds2013

    • Author(s)
      Jia Guo, Yanhong Xu, Shangbin Jin, Long Chen, Toshihiko Kaji, Yoshihito Honsho, Matthew A. Addicoat, Jangbae Ki, Akinori Saeki, Hyotcherl Ihee, Shu Seki, Stephan Irle, Masahiro Hiramoto, Jia Gao and Donglin Jiang
    • Journal Title

      Nature Communications

      Volume: 4 Issue: 1 Pages: 1-8

    • DOI

      10.1038/ncomms3736

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] An Azine-Linked Covalent Organic Framework2013

    • Author(s)
      Sasanka Dalapati, Shangbin Jin, Jiao Gao, Yanhong Xu, Atsushi Nagai and Donglin Jiang
    • Journal Title

      J. Am. Chem. Soc.

      Volume: 135 Issue: 46 Pages: 17310-17313

    • DOI

      10.1021/ja4103293

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Conjugated Microporous Polymers: Design, Synthesis and Application2013

    • Author(s)
      Yanhong Xu, Shangbin Jin, Hong Xu, Atsushi Nagai, and Donglin Jiang
    • Journal Title

      Chem. Soc. Rev.

      Volume: 42 Issue: 20 Pages: 8012-8031

    • DOI

      10.1039/c3cs60160a

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Super Absorbent Conjugated Microporous Polymers: A Synergistic Structural Effect on Exceptional Uptake of Amines2013

    • Author(s)
      Xiaoming Liu, Yanhong Xu, Zhaoqi Guo, Atsushi Nagai, and Donglin Jiang
    • Journal Title

      Chem. Commun.

      Volume: 49 Issue: 31 Pages: 3233-3235

    • DOI

      10.1039/c3cc41082j

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Core-Shell Conjugated Microporous Polymers: A New Strategy for Exploring Color-Tunable and -Controllable Light Emissions2013

    • Author(s)
      Yanhong Xu, Atsushi Nagai, and Donglin Jiang
    • Journal Title

      Chem. Commun.

      Volume: 49 Issue: 16 Pages: 1591-1593

    • DOI

      10.1039/c2cc38211c

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] Two-Dimensional Covalent Organic Frameworks2015

    • Author(s)
      Donglin Jiang
    • Organizer
      Pacifichem 2015
    • Place of Presentation
      Honolulu, USA
    • Year and Date
      2015-12-15
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Covalent Organic Frameworks: A Platform for Crystalline Organic Optoelectronics2015

    • Author(s)
      Donglin Jiang
    • Organizer
      1st European Conference on Metal Organic Frameworks and Porous Polymers
    • Place of Presentation
      Potsdam, Germany
    • Year and Date
      2015-10-11
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Covalent Organic Frameworks for Battery Energy Storage2015

    • Author(s)
      Donglin Jiang
    • Organizer
      250th ACS Meeting
    • Place of Presentation
      Boston, USA
    • Year and Date
      2015-08-16
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Covalent Organic Frameworks2015

    • Author(s)
      Donglin Jiang
    • Organizer
      Commemorative Golden Jubilee Chemistry Conference
    • Place of Presentation
      Singapore
    • Year and Date
      2015-08-06
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Two-Dimensional Polymers and Covalent Organic Frameworks2015

    • Author(s)
      Donglin Jiang
    • Organizer
      8th International Conference on Materials for Advanced Technologies (ICMAT2015)
    • Place of Presentation
      Singapore
    • Year and Date
      2015-06-28
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Conjugated Microporous Polymers2015

    • Author(s)
      Donglin Jiang
    • Organizer
      8th International Conference on Materials for Advanced Technologies (ICMAT2015)
    • Place of Presentation
      Singapore
    • Year and Date
      2015-06-28
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Two-Dimensional Polymers and Covalent Organic Frameworks2015

    • Author(s)
      Donglin Jiang
    • Organizer
      The 13th International Conference on Polymer Advanced Technologies (PAT2015)
    • Place of Presentation
      Hangzhou
    • Year and Date
      2015-06-25
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Porous Polymer Nanofilms with AIE Skeletons2015

    • Author(s)
      Donglin Jiang
    • Organizer
      The 2nd International Symposium on Aggregation-Induced Emission
    • Place of Presentation
      Guangzhou
    • Year and Date
      2015-05-15
    • Related Report
      2014 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Two-Dimensional Polymers and Covalent Organic Frameworks2013

    • Author(s)
      Donglin Jiang
    • Organizer
      The 9th IUPAC International Symposium on Novel Materials and Their Synthesis
    • Place of Presentation
      Shanghai, China
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Two-Dimensional Polymers as a Novel Functional Material Platform2013

    • Author(s)
      Donglin Jiang
    • Organizer
      The 6th China-Japan Joint Symposium on Functional Supramolecular Architecture
    • Place of Presentation
      Suzhou, China
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Covalent Organic Frameworks: A Class of Polymers with Periodic Built-in Intra- and Inter-molecular Orderings for Functional Exploration2013

    • Author(s)
      Donglin Jiang
    • Organizer
      The 15th Asian Chemical Congress
    • Place of Presentation
      Singapore
    • Related Report
      2013 Annual Research Report
  • [Presentation] Two-Dimensional Polymers and Covalent Organic Frameworks2013

    • Author(s)
      Donglin Jiang
    • Organizer
      The 11th China-Japan Joint Symposium on Conduction and Photoconduction in Organic Solids and Related Phenomena
    • Place of Presentation
      Changchun, China
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Exploring Two-Dimensional Polymers and Framework for the Construction of Segregated Donor-Acceptor System2013

    • Author(s)
      Donglin Jiang
    • Organizer
      The 11th International Symposium on Functional π-electron systems
    • Place of Presentation
      Arcachon, France
    • Related Report
      2013 Annual Research Report
  • [Presentation] Two-Dimensional Polymers and Covalent Organic Frameworks2013

    • Author(s)
      Donglin Jiang
    • Organizer
      The 11th China-Japan Joint Symposium on Conduction and Photoconduction in Organic Solids and Related Phenomena
    • Place of Presentation
      Changchun Institute of Applied Chemistry, Changchun, China
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Book] 太陽光と光電変換機能2016

    • Author(s)
      江 東林
    • Total Pages
      307
    • Publisher
      シーエムシー
    • Related Report
      2014 Annual Research Report
  • [Book] Nanoporous Materials: Synthesis and Applications2013

    • Author(s)
      Donglin Jiang, Shangbin Jin, Yanhong Xu, Xiaoming Liu
    • Total Pages
      384
    • Publisher
      Taylor & Francis Books
    • Related Report
      2013 Annual Research Report

URL: 

Published: 2013-05-15   Modified: 2019-07-29  

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