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Laser-field Fourier synthesis by quantum control of molecular tunneling ionization

Research Project

Project/Area Number 24340097
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Atomic/Molecular/Quantum electronics
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

OHMURA Hideki  独立行政法人産業技術総合研究所, 計測フロンティア研究部門, 主任研究員 (60356665)

Co-Investigator(Kenkyū-buntansha) SAITO Naoaki  (独)産業技術総合研究所, 計測フロンティア研究部門, 副研究部門長 (90357070)
MORISHITA Toru  電気通信大学, 情報理工学(系)研究科, 准教授 (20313405)
Co-Investigator(Renkei-kenkyūsha) MADSEN L. B.  Aarhus University, デンマーク, 教授
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥19,630,000 (Direct Cost: ¥15,100,000、Indirect Cost: ¥4,530,000)
Fiscal Year 2014: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2013: ¥7,020,000 (Direct Cost: ¥5,400,000、Indirect Cost: ¥1,620,000)
Fiscal Year 2012: ¥8,580,000 (Direct Cost: ¥6,600,000、Indirect Cost: ¥1,980,000)
Keywords量子制御 / コヒーレント制御 / トンネルイオン化 / フーリエ合成 / 原子・分子 / 位相制御レーザーパルス
Outline of Final Research Achievements

We have investigated intense phase-controlled two-color laser fields consisting of a fundamental light and a second harmonic light to achieve quantum control of molecular tunneling ionization (TI) in the space domain and the resultant orientation-selective molecular TI (OSMTI) in simple molecules.
Here, we have extended the quantum control of molecular tunneling ionization by using four-color Fourier-synthesized laser fields. The directionally asymmetric molecular TI induced by intense (~10^13 W/cm^2) Fourier-synthesized laser fields consisting of fundamental, second-, third-, and fourth-harmonic light achieves the OSMTI. We show that the OSMTI is very effective for measurement of the relative phase differences between the fundamental and each harmonic light. Our results promise not only lightwave engineering but also the control of matter, triggering the creation and establishment of usage of Fourier-synthesized laser fields.

Report

(5 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Products Report
  • Research Products

    (44 results)

All 2015 2014 2013 2012 Other

All Journal Article (21 results) (of which Peer Reviewed: 21 results,  Open Access: 1 results,  Acknowledgement Compliant: 7 results) Presentation (17 results) (of which Invited: 4 results) Book (1 results) Remarks (3 results) Patent(Industrial Property Rights) (2 results)

  • [Journal Article] Structure factors for tunneling ionization rates of diatomic molecules2015

    • Author(s)
      R. Saito, O. I. Tolstikhin, L. B. Madsen, and ,T. Morishita
    • Journal Title

      Atomic Data and Nuclear Data Tables

      Volume: 103-104 Pages: 4-49

    • DOI

      10.1016/j.adt.2015.02.001

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Weak-field asymptotic theory of tunneling ionization: benchmark2015

    • Author(s)
      V. H. Trinh, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Journal of Physics B: Atomic, Molecular and Optical Physics

      Volume: 48 Issue: 6 Pages: 061003-061003

    • DOI

      10.1088/0953-4075/48/6/061003

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Molecular tunnelling ionization of allyl halides induced by phase-controlled2014

    • Author(s)
      Hideki Ohmura and Naoaki Saito
    • Journal Title

      Journal of Physics B: Atomic, Molecular and Optical Physics

      Volume: 47 Issue: 20 Pages: 204007-204007

    • DOI

      10.1088/0953-4075/47/20/204007

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Application of the many-electron weak-field asymptotic theory of tunneling ionization to atoms2014

    • Author(s)
      I. Y. Tolstikhina,T. Morishita, and O. I. Tolstikhin
    • Journal Title

      Physical Review A

      Volume: 90 Issue: 5 Pages: 053413-053413

    • DOI

      10.1103/physreva.90.053413

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Rydberg states in the strong field ionization of hydrogen by 800, 12002014

    • Author(s)
      Q. Li, X.-M. Tong, T. Morishita, C. Jin, H. Wei and C. D. Lin
    • Journal Title

      Journal of Physics B: Atomic, Molecular and Optical Physics

      Volume: 47 Issue: 20 Pages: 204019-204019

    • DOI

      10.1088/0953-4075/47/20/204019

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Rescattering photoelectron spectroscopy of small molecules2014

    • Author(s)
      M. Okunishi,R.R. Lucchesse, T. Morishita, K. Ueda
    • Journal Title

      Journal of Electron Spectroscopy and Related Phenomena

      Volume: 195 Pages: 313-319

    • DOI

      10.1016/j.elspec.2013.12.002

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Universality of Returning Electron Wave Packet in High-Order Harmonic2014

    • Author(s)
      A.-T. Le, H. Wei, C. Jin, V. N. Tuoc, T. Morishita, and C. D. Lin
    • Journal Title

      Physical Review Letters

      Volume: 113 Issue: 3 Pages: 033001-033001

    • DOI

      10.1103/physrevlett.113.033001

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Molecular tunneling ionization of the carbonyl sulfide molecule by double-frequency phase-controlled laser fields2014

    • Author(s)
      H. Ohmura, N. Sato, and T. Morishita
    • Journal Title

      Phy. Rev. A

      Volume: 89 Issue: 1

    • DOI

      10.1103/physreva.89.013405

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Orientation-selective molecular tunneling ionization by phase-controlled laser fields2014

    • Author(s)
      Hideki Ohmura
    • Journal Title

      Advances in Multi-photon Processes and Spectroscopy(AMPS)

      Volume: 21 Pages: 55-103

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Probing dipole-forbidden autoionizing states by isolated attosecond pulses2014

    • Author(s)
      W.-C. Chu, T. Morishita, and C. D. Lin
    • Journal Title

      Phys. Rev. A

      Volume: 89 Issue: 3

    • DOI

      10.1103/physreva.89.033427

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular Siegert states in an electric field. II. Transverse momentum distribution of the ionized electrons2014

    • Author(s)
      V. N. T. Pham, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev

      Volume: A89 Issue: 3 Pages: 33426-33426

    • DOI

      10.1103/physreva.89.033426

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Application of the weak-field asymptotic theory to tunneling ionization of H2O2014

    • Author(s)
      L. B. Madsen, Frank Jensen, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 89 Issue: 3 Pages: 33412-33412

    • DOI

      10.1103/physreva.89.033412

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fine structures in the intensity dependence of excitation and ionization probabilities of hydrogen atoms in intense 800-nm laser pulses2014

    • Author(s)
      Q. Li, X.-M. Tong, T. Morishita, H. Wei, and C. D. Lin
    • Journal Title

      Phys. Rev. A

      Volume: 89 Issue: 2

    • DOI

      10.1103/physreva.89.023421

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Weak-field asymptotic theory of tunneling ionization in many-electron atomic and molecular systems2014

    • Author(s)
      O. I. Tolstikhin, L. B. Madsen, and T. Morishita
    • Journal Title

      Phys. Rev

      Volume: A89 Issue: 1 Pages: 13421-13421

    • DOI

      10.1103/physreva.89.013421

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoelectron spectra and high Rydberg states of lithium generated by intense lasers in the over-the-barrier ionization regime2013

    • Author(s)
      T. Morishita and C. D. Lin
    • Journal Title

      Phy. Rev. A

      Volume: 87 Issue: 6

    • DOI

      10.1103/physreva.87.063405

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] First-order correction terms in the weak-field asymptotic theory of tunneling ionization2013

    • Author(s)
      V. H. Trinh, O. I. Tolstikhin, L. B. Madsen, and T. Morishita
    • Journal Title

      Phys. Rev

      Volume: A87 Issue: 4 Pages: 43426-43426

    • DOI

      10.1103/physreva.87.043426

    • NAID

      110009754754

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] "Effect of nuclear motion on tunneling ionization rates of molecules"2013

    • Author(s)
      O. I. Tolstikhin, H. J. Worner, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 87, 041401(R) Issue: 4

    • DOI

      10.1103/physreva.87.041401

    • Related Report
      2013 Annual Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Orientation-selective molecular tunneling ionization by phase-controlled laser fields2013

    • Author(s)
      Hideki Ohmura
    • Journal Title

      Advances in Multi-photon Processes and Spectroscopy(AMPS)

      Volume: 21(掲載予定)

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] "Structure factors for tunneling ionization rates of molecules"2013

    • Author(s)
      L. B. Madsen, F. Jensen, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 87, 013406 Issue: 1 Pages: 13406-13406

    • DOI

      10.1103/physreva.87.013406

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Adiabatic theory of ionization by intense laser pulses : Finite-range potentials.2012

    • Author(s)
      0. I. Tolstikhin and T.Morishita
    • Journal Title

      Physical Review A

      Volume: 86

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular Siegert states in an electric field2012

    • Author(s)
      L. Hamonou, T. Morishita, and O. I. Tolstikhin
    • Journal Title

      Phys. Rev.

      Volume: A 86 Issue: 1 Pages: 13412-13412

    • DOI

      10.1103/physreva.86.013412

    • URL

      http://link.aps.org/doi/10.1103/PhysRevA.86.013412

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Presentation] Adiabatic Theory of ionization of atoms by intense laser pulses2014

    • Author(s)
      Toru Morishita
    • Organizer
      Seminor on Peking University
    • Place of Presentation
      Peking University, China
    • Year and Date
      2014-11-03
    • Related Report
      2014 Annual Research Report
  • [Presentation] Atomic and molecular tunneling ionization in a static electric field: From tunneling to over-the-barrier regiemes2014

    • Author(s)
      Toru Morishita
    • Organizer
      International Workshop on Strong Field Physics and Ultrafast Phenomena(SFPUP 2014)
    • Place of Presentation
      Zhangjiajie, China
    • Year and Date
      2014-10-31 – 2014-11-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] Laser induced rescattering electron spectroscopy for ultrafast atomic and molecular imaging2014

    • Author(s)
      Toru Morishita
    • Organizer
      Abbaye des Vaux de Cernay
    • Place of Presentation
      Cernay la Ville, France
    • Year and Date
      2014-07-21 – 2014-07-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] Atomic and molecular tunneling ionization in a static electric field: From tunneling to over-the-barrier regiemes2014

    • Author(s)
      Toru Morishita
    • Organizer
      LPHYS 14, 23 th International Laser Physics Workshop
    • Place of Presentation
      Sofia, Burgaria
    • Year and Date
      2014-07-14 – 2014-07-18
    • Related Report
      2014 Annual Research Report
  • [Presentation] 強いレーザー場による分子配向制御2013

    • Author(s)
      大村英樹
    • Organizer
      東北大学 多元物質科学研究所 量子電子科学研究分野 高橋研セミナー
    • Place of Presentation
      東北大学(招待講演)
    • Year and Date
      2013-01-24
    • Related Report
      2012 Annual Research Report
  • [Presentation] Ultra High-Resolution Imaging of Atoms and Molecules with Laser Induced Rescattering Electron Spectroscopy2012

    • Author(s)
      T. Morishita
    • Organizer
      10th Asian International Seminar on Atomic and Molecular Physics
    • Place of Presentation
      Taipei, Taiwan
    • Year and Date
      2012-10-23
    • Related Report
      2012 Annual Research Report
  • [Presentation] 分子トンネルイオン化の量子制御を利用したレーザー場フーリエ合成2012

    • Author(s)
      大村英樹
    • Organizer
      分子研研究会
    • Place of Presentation
      分子科学研究所(招待講演)
    • Year and Date
      2012-10-12
    • Related Report
      2012 Annual Research Report
  • [Presentation] 分子トンネルイオン化の量子制御を利用したレーザー場フーリエ合成2012

    • Author(s)
      大村英樹、斎藤直明、森下亨
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京大学
    • Year and Date
      2012-09-20
    • Related Report
      2012 Annual Research Report
  • [Presentation] 位相制御レーザーパルスによる分子トンネルイオン化の量子制御2012

    • Author(s)
      大村英樹
    • Organizer
      原子衝突学会第37回年回
    • Place of Presentation
      電気通信大学(招待講演)
    • Year and Date
      2012-07-28
    • Related Report
      2012 Annual Research Report
  • [Presentation] Laser induced rescattering electron spectroscopy for ultrafast atomic and molecular imaging2012

    • Author(s)
      T. Morishita
    • Organizer
      5th Asian Workshop on Generation and Application of Coherent XUV and X-ray Radiation (5th AWCXR) and the ISSP International Workshop on Coherent Soft X-ray Sciences
    • Place of Presentation
      Kasihwa, ISSP, Japan
    • Year and Date
      2012-06-27
    • Related Report
      2012 Annual Research Report
  • [Presentation] Molecular tunneling ionization by multi-color phase-controlled laser fields

    • Author(s)
      Hideki Ohmura
    • Organizer
      International workshop on theory for attosecond quantum dynamics (IWTAQD) 9
    • Place of Presentation
      電気通信大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 分子トンネルイオン化の量子制御を利用したレーザー場フーリエ合成 2

    • Author(s)
      大村英樹、斎藤直明、森下亨
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ
    • Related Report
      2013 Annual Research Report
  • [Presentation] 位相制御レーザーパルスによる分子トンネルイオン化の量子制御

    • Author(s)
      大村英樹
    • Organizer
      2013年鳩山サイエンスフォーラム第42回講演会
    • Place of Presentation
      東京電機大学理工学部物理学教室
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 強いレーザー場によって引き起こされる分子トンネルイオン化における最近の動向

    • Author(s)
      大村英樹
    • Organizer
      東北大学 多元物質科学研究所 量子電子科学研究分野 高橋研セミナー
    • Place of Presentation
      東北大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Atomic and Molecular Ionization by Intense Laser Fields: From Tunneling to Over-the-Barrier Regimes

    • Author(s)
      T. Morishita
    • Organizer
      Gordon Research Conference, Photoionization & Photodetachment, Probing Electronic and Nuclear Dynamics
    • Place of Presentation
      Galveston, TX
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Two-electron dynamics in nonlinear double excitation of helium by intense ultrashort extreme-ultraviolet pulses

    • Author(s)
      T. Morishita
    • Organizer
      International Symposium on (e,2e), Double Photoionization and Related Topics & 17th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions
    • Place of Presentation
      He Fei, China.
    • Related Report
      2013 Annual Research Report
  • [Presentation] Atomic and molecular ionization in a static electric field: From tunneling to over-the-barrier regimesAtomic and molecular ionization in a static electric field: From tunneling to over-the-barrier regimes

    • Author(s)
      T. Morishita
    • Organizer
      The workshop on Strong Laser Physics, Shang-tou university
    • Place of Presentation
      Shang-tou, China.
    • Related Report
      2013 Annual Research Report
  • [Book] 強光子場の化学 Part II 第二章 位相制御レーザーパルスによる配向選択分子イオン化2015

    • Author(s)
      大村英樹
    • Total Pages
      7
    • Publisher
      化学同人
    • Related Report
      2014 Annual Research Report
  • [Remarks] 計測フロンティア研究部門

    • URL

      http://unit.aist.go.jp/riif/ja/group/ionqm.html

    • Related Report
      2014 Annual Research Report
  • [Remarks] (独)産業技術総合研究所計測フロンティア研究部門

    • URL

      http://unit.aist.go.jp/riif/ja/group/ionqm.html

    • Related Report
      2013 Annual Research Report
  • [Remarks]

    • URL

      http://unit.aist.go.jp/riif/ja/group/ionqm.html

    • Related Report
      2012 Annual Research Report
  • [Patent(Industrial Property Rights)] レーザー光フーリエ合成法及び装置2013

    • Inventor(s)
      大村 英樹
    • Industrial Property Rights Holder
      大村 英樹
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2013-196982
    • Filing Date
      2013-09-24
    • Related Report
      2013 Annual Research Report
  • [Patent(Industrial Property Rights)] レーザー光フーリエ合成法及び装置2013

    • Inventor(s)
      大村 英樹, 齋藤 直昭
    • Industrial Property Rights Holder
      産業技術総合研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2013-196982
    • Filing Date
      2013-09-24
    • Acquisition Date
      2017-07-21
    • Related Report
      Products Report

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Published: 2012-04-24   Modified: 2019-07-29  

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