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In-situ observation of molecules in intense laser fields by ultrafast photoelectron spectroscopy

Research Project

Project/Area Number 24350006
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Physical chemistry
Research InstitutionNagoya University

Principal Investigator

HISHIKAWA Akiyoshi  名古屋大学, 理学(系)研究科(研究院), 教授 (50262100)

Co-Investigator(Renkei-kenkyūsha) FUSHITANI Mizuho  名古屋大学, 大学院理学研究科, 助教 (50446259)
YASUIKE Tomokazu  放送大学, 准教授 (10419856)
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥18,330,000 (Direct Cost: ¥14,100,000、Indirect Cost: ¥4,230,000)
Fiscal Year 2014: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2013: ¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2012: ¥11,180,000 (Direct Cost: ¥8,600,000、Indirect Cost: ¥2,580,000)
Keywords強レーザー場科学 / 超高速分光 / 光電子分光 / 分子ダイナミクス / 電子ダイナミクス / 強レーザー場 / NO / ポンプープローブ計測 / 反応動力学 / 反応コントロール
Outline of Final Research Achievements

A system for ultrafast photoelectron spectroscopy was constructed using laser high-order harmonics in extreme ultraviolet, which was successfully applied to femtosecond pump-probe real-time tracking of ultrafast electron wavepacket dynamics. The effect of electronic excitation in molecular dynamics in intense laser fields was studied by momentum imaging of dissociative ionization of UV-excited molecules. Based on the finding, a novel method to visualize electron dynamics in molecules in real time was proposed. Photoelectron spectroscopy of molecules before and after the irradiation of an intense laser pulse was performed, revealing selective excitation of specific electronic states in the laser field.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (22 results)

All 2015 2014 2013 2012 Other

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (18 results) (of which Invited: 15 results) Remarks (1 results)

  • [Journal Article] Time-resolved laser Coulomb explosion imaging using few-cycle intense laser pulses: Application to exploding CS2 in highly charged states2014

    • Author(s)
      A. Matsuda, E. J. Takahashi and A. Hishikawa
    • Journal Title

      J. Electron. Spectrosc. Relat. Phenom.

      Volume: 195 Pages: 327-331

    • DOI

      10.1016/j.elspec.2013.12.011

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Non-resonant EUV-UV two-color two-photon ionization of He studied by single-shot photoelectron spectroscopy2013

    • Author(s)
      M. Fushitani, Y. Hikosaka, A. Matsuda, T. Endo, E. Shigemasa, M. Nagasono, T. Sato, T. Togashi, M. Yabashi, T. Ishikawa and A. Hishikawa
    • Journal Title

      Phys. Rev. A

      Volume: 88 Pages: 63422-63422

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Resonances in three-photon double ionization of Ar in intense extreme ultraviolet free-electron laser fields studied by shot-by-shot photoelectron spectroscopy2013

    • Author(s)
      Y. Hikosaka, M. Fushitani, A. Matsuda, T. Endo, Y. Toida, E. Shigemasa, M. Nagasono, K. Tono, T. Togashi, M. Yabashi, T. Ishikawa and A. Hishikawa
    • Journal Title

      Phys. Rev. A

      Volume: 88 Issue: 2 Pages: 0234211-6

    • DOI

      10.1103/physreva.88.023421

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] EUV-NIR two-color photoelectron spectroscopy on isolated atoms and molecules in highly excited states2015

    • Author(s)
      A. Hishikawa
    • Organizer
      Soft X-ray in Energy and Time Workshop (SXET)
    • Place of Presentation
      Berlin
    • Year and Date
      2015-08-20 – 2015-08-21
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Visualizing ultrafast chemical reactions by few-cycle intense laser pulses2014

    • Author(s)
      A. Hishikawa
    • Organizer
      ndo-Japan Joint Workshop on “Frontiers in Molecular Spectroscopy: Fundamentals and Applications to Material and Biology”
    • Place of Presentation
      Nara
    • Year and Date
      2014-11-25 – 2014-11-28
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 近赤外強レーザー場におけるHe原子の超高速2光子ラビ振動過程2014

    • Author(s)
      菱川明栄
    • Organizer
      「新しい光科学の創成とナノ情報デバイスへの展開Ⅱ」研究会
    • Place of Presentation
      東北大学
    • Year and Date
      2014-10-30 – 2014-10-31
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Visualizing ultrafast chemical reactions by few-cycle intense laser pulses2014

    • Author(s)
      A. Hishikawa
    • Organizer
      P. N. Lebedev Physical Institute seminar
    • Place of Presentation
      Moscow
    • Year and Date
      2014-09-25
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 強レーザーパルスによる超高速反応イメージング2014

    • Author(s)
      菱川明栄
    • Organizer
      第1回森野ディスカッション
    • Place of Presentation
      東京大学
    • Year and Date
      2014-08-29
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Ultrafast two-photon Rabi oscillations in excited He atoms in strong laser fields2014

    • Author(s)
      A. Hishikawa
    • Organizer
      International workshop on theory for attosecond quantum dynamics (IWTAQD) 11
    • Place of Presentation
      電気通信大学
    • Year and Date
      2014-06-30 – 2014-07-01
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Multiphoton ionization of He studied by time-resolved single-shot spectroscopy2014

    • Author(s)
      Mizuho Fushitani
    • Organizer
      International workshop on theory for attosecond quantum dynamics (IWTAQD) 10
    • Place of Presentation
      Chofu, Japan
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Anisotropic dissociative ionization of electronically excited NO in few-cycle intense laser fields2014

    • Author(s)
      Akiyoshi Hishikawa
    • Organizer
      International workshop on theory for attosecond quantum dynamics (IWTAQD) 10
    • Place of Presentation
      Chofu, Japan
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 単一次数レーザー高次高調波による実時間光電子分光2013

    • Author(s)
      伏谷瑞穂
    • Organizer
      日本分光学会平成24年度中部支部東海・信州ブロック講演会
    • Place of Presentation
      分子科学研究所(招待講演)
    • Year and Date
      2013-03-21
    • Related Report
      2012 Annual Research Report
  • [Presentation] Ultrafast dissociative ionization of molecules in few-cycle intense laser fields2013

    • Author(s)
      Akiyoshi Hishikawa
    • Organizer
      Workshop on "Fundamentals and applications of laser filaments"
    • Place of Presentation
      Okazaki, Japan
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 極短レーザーパルスによる超高速反応イメージング2013

    • Author(s)
      菱川明栄
    • Organizer
      日本顕微鏡学会第69回学術講演会
    • Place of Presentation
      ホテル阪急エキスポパーク
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 数サイクル強レーザーパルスによる超高速反応イメージング2013

    • Author(s)
      菱川明栄
    • Organizer
      分子研シンポジウム2013
    • Place of Presentation
      岡崎コンファレンスセンター
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Time-resolved photoelectron spectroscopy by single-order laser high harmonics in VUV2013

    • Author(s)
      Mizuho Fushitani
    • Organizer
      The 38th International conference on Vacuum Ultraviolet and X-ray Physics (VUVX2013)
    • Place of Presentation
      Hefei, China
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Non-linear atomic ionization of He in EUV and NIR intense laser fields2013

    • Author(s)
      Akiyoshi Hishikawa
    • Organizer
      International Symposium on Ultrafast Intense Laser Science (ISUILS12)
    • Place of Presentation
      Salamanca, Spain
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 強レーザー場におけるNO分子の解離性イオン化:π-σ軌道遷移の効果2013

    • Author(s)
      菱川明栄
    • Organizer
      新しい光科学の創成とナノ情報デバイスへの展開」研究会
    • Place of Presentation
      東北大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 数サイクル強レーザーパルスによる超高速反応イメージング2013

    • Author(s)
      菱川明栄
    • Organizer
      第4回統合物質シンポジウム
    • Place of Presentation
      北海道大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Time-Resolved Photoelectron Spectroscopy of N_2 Rydberg Wavepackets2012

    • Author(s)
      M.Fushitani, Y. Toida, F. Legare, and A. Hishikawa
    • Organizer
      The 2nd International Conference on MEXT Project of Integrated Research on Chemical Synthesis
    • Place of Presentation
      名古屋大学
    • Year and Date
      2012-12-10
    • Related Report
      2012 Annual Research Report
  • [Presentation] EUV領域レーザー高調波を用いたN_2リュードベリ波束の超高速光電子分光2012

    • Author(s)
      伏谷瑞穂, 樋田裕斗, Francois Legare,菱川明栄
    • Organizer
      第6回分子科学討論会2012
    • Place of Presentation
      東京大学
    • Related Report
      2012 Annual Research Report
  • [Remarks] 名古屋大学光物理化学研究室

    • URL

      http://photon.chem.nagoya-u.ac.jp/HOME/HOME.html

    • Related Report
      2013 Annual Research Report

URL: 

Published: 2012-04-24   Modified: 2019-07-29  

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