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Investigation of mechanism of electrical conduction via functionalized dislocation networks in atomically-bonded metal-oxide crystals

Research Project

Project/Area Number 24360017
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionOsaka University

Principal Investigator

SAKAI Akira  大阪大学, 基礎工学研究科, 教授 (20314031)

Co-Investigator(Renkei-kenkyūsha) NAKAMURA Yoshiaki  大阪大学, 大学院基礎工学研究科, 教授 (60345105)
KIKKAWA Jun  物質材料研究機構, 先端的共通技術部門表界面構造物性ユニット, 主任研究員 (20435754)
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥18,330,000 (Direct Cost: ¥14,100,000、Indirect Cost: ¥4,230,000)
Fiscal Year 2014: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Fiscal Year 2013: ¥10,010,000 (Direct Cost: ¥7,700,000、Indirect Cost: ¥2,310,000)
Fiscal Year 2012: ¥5,980,000 (Direct Cost: ¥4,600,000、Indirect Cost: ¥1,380,000)
Keywords転位 / 抵抗スイッチング / 金属酸化物結晶 / 電気伝導 / ヒステリシス / 空間電荷制限電流 / 酸素空孔 / 欠陥準位 / 金属酸化物 / 還元 / フォーミング / 集束イオンビーム加工 / 走査透過電子顕微鏡 / 電子エネルギー損失分光 / 抵抗遷移 / 透過電子顕微鏡 / バーガースベクトル
Outline of Final Research Achievements

We have controlled dislocation structure and morphology in SrTiO3 crystals by using the atomic bonding method (ABM) and investigated electrical conduction mechanisms via dislocation networks in the crystals formed by ABM. Although resistive switching phenomena have been observed for both Nb-doped SrTiO3 and reduction-annealed non-doped SrTiO3 (RSTO), their mechanisms are different from each other: the former can be explained by carrier emission and capture at metal/SrTiO3 interfacial traps accompanied by the space charge limited current conduction, and the latter by the drift motion of oxygen vacancies in the crystal. In particular, by measuring electrical properties of micrometer-scaled devices made from the atomically bonded RSTO, it was found that the dislocation network can effectively be functionalized as an electrical conduction site having the ability of resistive switching.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (3 results)

All 2014 2012

All Journal Article (1 results) Presentation (2 results)

  • [Journal Article] 貼り合わせ直接接合SrtiO_3(001)基板の抵抗スイッチング特製評価2012

    • Author(s)
      浅田遼大, Pham Phu Than Son, Kokate Nishad Vasant, 吉川純, 竹内政太郎, 中村芳明, 酒井朗
    • Journal Title

      信学技報(IEICE Tschnical Report)

      Volume: 112 Pages: 7-12

    • Related Report
      2012 Annual Research Report
  • [Presentation] Electrical conduction characteristics of single crystal and directly-bonded Nb-doped SrTiO32014

    • Author(s)
      R. Asada, S. Kondo, S. Takeuchi, Y. Sugi, Y. Nakamura, A. Sakai
    • Organizer
      The 15th IUMRS-International Conference in Asia (IUMRS-ICA 2014)
    • Place of Presentation
      Fukuoka University, Fukuoka, Japan
    • Year and Date
      2014-08-24 – 2014-08-30
    • Related Report
      2014 Annual Research Report 2013 Annual Research Report
  • [Presentation] 貼り合わせ直接接合SrT103(001)基板の抵抗スイッチング特性評価2012

    • Author(s)
      浅田遼太、Pham Phu Than Son、Kokate Nishad Vasant、吉川純、竹内正太郎、中村芳明、酒井朗
    • Organizer
      シリコン材料・デバイス研究会(SDM)
    • Place of Presentation
      名古屋大学VBL(愛知県)
    • Year and Date
      2012-06-21
    • Related Report
      2012 Annual Research Report

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Published: 2012-04-24   Modified: 2019-07-29  

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