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Solid-phase crystallization of oxide thin films on nanoscale-controlled substrates via post-annealing under uniaxial compression for exploring the novel functionalities

Research Project

Project/Area Number 24360269
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionTokyo Institute of Technology

Principal Investigator

Yoshimoto Mamoru  東京工業大学, 総合理工学研究科(研究院), 教授 (20174998)

Co-Investigator(Kenkyū-buntansha) YODO Tokuo  大阪工業大学, 工学部, 教授 (70288752)
Co-Investigator(Renkei-kenkyūsha) MATSUDA Akifumi  東京工業大学, 大学院総合理工学研究科, 講師 (80621698)
Project Period (FY) 2012-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥14,950,000 (Direct Cost: ¥11,500,000、Indirect Cost: ¥3,450,000)
Fiscal Year 2014: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2013: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2012: ¥8,190,000 (Direct Cost: ¥6,300,000、Indirect Cost: ¥1,890,000)
Keywords結晶構造制御 / 一軸圧縮 / 酸化物薄膜 / 固相結晶化 / エピタキシャル成長 / 酸化バナジウム / 酸化モリブデン / 固相結晶成長 / 層状構造 / 酸化物 / 結晶構造 / 組織制御 / 超機能創出 / 表面ナノ修飾基板 / ナノインプリント
Outline of Final Research Achievements

In this study, the influence of thermal annealing under uniaxial compression on solid-state crystallization of electronic functional oxide thin films such as VOx or MoOx was investigated for exploring the novel functionalities. As a result, it was found that the epitaxial VO2 and epitaxial V2O3 thin films were obtained through annealing under uniaxial compression of 1 MPa and 10-30 MPa, respectively. Diffusion of oxygen atoms along the layered structure of VOx film under uniaxial compression was thought to have an important role for phase-selective solid state crystallization in this process.

Report

(5 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (25 results)

All 2016 2015 2014 2013 2012 Other

All Journal Article (11 results) (of which Peer Reviewed: 11 results,  Acknowledgement Compliant: 4 results) Presentation (13 results) (of which Int'l Joint Research: 2 results,  Invited: 1 results) Remarks (1 results)

  • [Journal Article] Atomic-scale Thermal Behavior of Nanoimprinted 0.3-nm-High Step Patterns on PMMA Polymer Sheets2016

    • Author(s)
      G. Tan, Y. Nozawa, T. Funabasama, K. Koyama, M. Mita, S. Kaneko, M. Komura, A. Matsuda and M. Yoshimoto
    • Journal Title

      Polymer Journal

      Volume: 48 Issue: 2 Pages: 225-227

    • DOI

      10.1038/pj.2015.99

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Subnano-scale nanoimprint fabrication of atomically stepped glassy substrates of silicate glass and acryl polymer2015

    • Author(s)
      Mamoru Yoshimoto
    • Journal Title

      Physics A

      Volume: 121 Issue: 2 Pages: 321-326

    • DOI

      10.1007/s00339-015-9247-4

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Atomic Step Patterning on Quartz Glass via Thermal Nanoimprinting2015

    • Author(s)
      Osamu Suga, Mamoru Yoshimoto, Chieko Okuyama, Akifumi Matsuda, Hiroshi Hiroshima, and Masaharu Takahashi
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 54 Issue: 9 Pages: 098001-098001

    • DOI

      10.7567/jjap.54.098001

    • NAID

      210000145692

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Formation of 0.3-nm-High Stepped Polymer Surface by Thermal Nanoimprinting2014

    • Author(s)
      Geng Tan, Naoya Inoue, Tomoyuki Funabasama, Masahiro Mita, Norimichi Okuda, Junichi Mori, Koji Koyama, Satoru Kaneko, Masaru Nakagawa, Akifumi Matsuda and Mamoru Yoshimoto
    • Journal Title

      Appl. Phys. Exp. (APEX)

      Volume: 7(5) Issue: 5 Pages: 055202-055202

    • DOI

      10.7567/apex.7.055202

    • NAID

      210000137094

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Formation of 0.3-nm-High Stepped Polymer Surface by Thermal Nanoimprinting2014

    • Author(s)
      Geng Tan, Naoya Inoue, Tomoyuki Funabasama, Masahiro Mita, Norimichi Okuda, Junichi Mori, Koji Koyama, Satoru Kaneko, Masaru Nakagawa, Akifumi Matsuda and Mamoru Yoshimoto
    • Journal Title

      Appl. Phys. Exp.

      Volume: 7

    • NAID

      210000137094

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Homoepitaxial growth of α-Al2O3 thin films on atomically stepped sapphire substrates by pulsed laser deposition at room-temperature2013

    • Author(s)
      Daishi Shiojiri, Ryosuke Yamauchi, Satoru Kaneko, Akifumi Matsuda, and Mamoru Yoshimoto
    • Journal Title

      J. Ceram. Soc. Japan

      Volume: 121

    • NAID

      130004480132

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of Momentary Annealing on Surface Morphology of Room Temperature Pulsed Laser Deposited NiO(111) Epitaxial Thin Film grown on Atomically Stepped Sapphire (0001) Substrates2013

    • Author(s)
      Ryosuke Yamauchi, Geng Tan, Daishi Shiojiri, Koji Koyama, Satoru Kaneko, Akifumi Matsuda, and Mamoru Yoshimoto
    • Journal Title

      Mater. Res. Soc. Symp. Proc.

      Volume: 1507

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Room-temperature synthesis of epitaxial oxide thin films for development of unequilibrium structure and novel electronic functionalization2013

    • Author(s)
      Mamoru YOSHIMOTO, Ryosuke YAMAUCHI, Daishi SHIOJIRI, Geng TAN, Satoru KANEKO and Akifumi MATSUDA
    • Journal Title

      J. Ceram. Soc. Japan

      Volume: 121

    • NAID

      130004950790

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Room-temperature synthesis of epitaxial oxide thin films for development of unequilibrium structure and novel electronic functionalization2013

    • Author(s)
      M. YOSHIMOTO, R. YAMAUCHI, D. SHIOJIRI, G. TAN, S. KANEKO and A. MATSUDA
    • Journal Title

      J. Ceram. Soc. Japan,

      Volume: 121 Pages: 1-9

    • NAID

      130004950790

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of Rapid Thermal Annealing and Substrate Terrace Width on Self-Organizing Formation of Periodic Straight Nanogroove Array on Ni0(111) Epitaxial Thin Film2012

    • Author(s)
      R. Yamauchi, G. Tan, D. Shiojiri, K. Koyama, S. Kaneko, A. Matsuda, and M. Yoshimoto
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 51

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropic magnetization of epitaxial Ni nanogroove-arrays prepared by reduction of self-organized oxides2012

    • Author(s)
      A. Matsuda, R. Yamauchi, G. Tan, H. Nakai, K. Koyama, K. Sunakawa, S. Kaneko and M. Yoshimoto
    • Journal Title

      Appl. Sur£Sci.

      Volume: 259 Pages: 208-212

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Presentation] 一軸加圧下熱処理による非晶質酸化モリブデン薄膜の固相結晶化2016

    • Author(s)
      難波 諒太郎, 野沢 靖久, 譚 ゴオン,土嶺信男, 金子 智,松田 晃史,吉本 護
    • Organizer
      応用物理学会 2016年春季年会
    • Place of Presentation
      東京工業大学
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Preparation of ultra-flat transparent conductive films on atomic step-and-terrace structured flexible polymer sheets2015

    • Author(s)
      Akifumi Matsuda, Goon Tan, Yasuhisa Nozawa, Daishi Shiojiri, Tatsuhiro Urakami, Satoru Kaneko, and Mamoru Yoshimoto
    • Organizer
      MRS 2015 Fall Meeting
    • Place of Presentation
      Boston, USA
    • Year and Date
      2015-11-29
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 一軸加圧下の熱処理による非晶質VOx 薄膜の相選択的エピタキシャル結晶化2015

    • Author(s)
      松田晃史、野沢靖久、難波諒太郎、吉本護、金子智
    • Organizer
      日本セラミックス協会2015年秋季年会
    • Place of Presentation
      富山大学
    • Year and Date
      2015-09-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] 一軸加圧熱処理による非晶質VOx薄膜の相選択的固相結晶化と配向制御2015

    • Author(s)
      野沢 靖久, 難波 諒太郎, 譚 ゴオン,金子 智,松田 晃史,吉本 護
    • Organizer
      応用物理学会 秋季年会
    • Place of Presentation
      名古屋国際会議場
    • Year and Date
      2015-09-13
    • Related Report
      2015 Annual Research Report
  • [Presentation] Nanoimprint fabrication of atomic step-and-terrace structured polymer sheets towards developing the novel flexible substrates2015

    • Author(s)
      Goon Tan, Yasuhisa Nozawa, Tomoyuki Funabasama, Satoru Kaneko, Akifumi Matsuda and Mamoru Yoshimoto
    • Organizer
      57th Electronic Materials Conference (EMC)
    • Place of Presentation
      The Ohio State University in Columbus, Ohio, USA
    • Year and Date
      2015-06-24
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 一軸圧縮下の熱処理による機能性酸化物薄膜の固相結晶挙動2015

    • Author(s)
      野沢 靖久,譚 ゴオン,船迫 友之,金子 智,松田 晃史,吉本 護
    • Organizer
      応用物理学会 春季年会
    • Place of Presentation
      東海大学湘南キャンパス
    • Year and Date
      2015-03-12 – 2015-03-13
    • Related Report
      2014 Annual Research Report
  • [Presentation] Nanoimprint Fabrication and Application of Subnano-Scale Surface-Patterned Glassy Substrates2014

    • Author(s)
      Geng Tan, Yasuhisa Nozawa, Tomoyuki Funabasama, Satoru Kaneko, Akifumi Matsuda and Mamoru Yoshimoto
    • Organizer
      13th International Conference on Nanoimprint and Nanoprint Technology (NNT 2014)
    • Place of Presentation
      Kyoto ANACrown Plaza Hotel
    • Year and Date
      2014-10-23 – 2014-10-24
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 透明導電性酸化物薄膜の固相結晶化における熱処理中の一軸圧縮応力印加の影響2013

    • Author(s)
      譚ゴオン・井上直哉・松田晃史・吉本護・大井秀雄・三田正弘・奥田徳路
    • Organizer
      日本セラミックス協会春季年会
    • Place of Presentation
      東京工業大学
    • Year and Date
      2013-03-17
    • Related Report
      2012 Annual Research Report
  • [Presentation] Nanoimprinting of self-organized atomic scale patterns of minerals onto the oxide glass surface2013

    • Author(s)
      N. Inoue, A. Matsuda, and M. Yoshimoto
    • Organizer
      第26回マイクロプロセス・ナノテクノロジー国際会議(MNC 2013)
    • Place of Presentation
      ロイトン札幌ホテル
    • Related Report
      2013 Annual Research Report
  • [Presentation] 室温レーザーMBE による酸化コバルト薄膜の相制御と評価2013

    • Author(s)
      松田晃史、吉本 護
    • Organizer
      第74回 応用物理学会 秋季学術講演会
    • Place of Presentation
      同志社大学 京田辺キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] 室温合成エピタキシャル酸化物薄膜の水素還元による磁気抵抗型積層薄膜の作製2013

    • Author(s)
      松田晃史、吉本 護
    • Organizer
      日本セラミックス協会 第26回秋季シンポジウム
    • Place of Presentation
      信州大学 長野キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] Solid-phase Crystallization of Transparent Conducting Oxide Thin Films Under Uniaxial Compression2012

    • Author(s)
      Geng Tan, Tsubasa Yamanoi, Hideo Oi, Masahiro Mita, Satoru Kaneko, Norimichi Okuda, Naoya Inoue, Noriko Kumagai, Ryosuke Yamauchi, Akifumi Matsuda, Mamoru Yoshimoto
    • Organizer
      MRS Fall Meetin, Symp.F: Oxide Thin Films for Renewable Energy Applications,
    • Place of Presentation
      Boston, USA
    • Year and Date
      2012-11-26
    • Related Report
      2012 Annual Research Report
  • [Presentation] Surface nanostructure control of indium tin oxide films on nanopatterne d glass substrates toward advanced thin film solar cells2012

    • Author(s)
      Geng Tan, Ryosuke Yamauchi, Satoru Kaneko, Akifumi Matsuda, Mamoru Yoshimoto
    • Organizer
      European Material Research Society (E-MRS 2012) Spring Meeting, Symposium Y (Advanced materials and characterization techniques for solar cells)
    • Place of Presentation
      the Congress Center in Strasbourg, France
    • Year and Date
      2012-05-14
    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://www.yoshimoto.iem.titech.ac.jp/

    • Related Report
      2012 Annual Research Report

URL: 

Published: 2012-04-24   Modified: 2019-07-29  

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