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Investigation of the electron dynamics in expanded fluid metals through the observation of plasmons

Research Project

Project/Area Number 24540401
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Mathematical physics/Fundamental condensed matter physics
Research InstitutionKyoto University

Principal Investigator

MATSUDA Kazuhiro  京都大学, 理学(系)研究科(研究院), 准教授 (50362447)

Research Collaborator HIRAOKA Nozomu  台湾NSRRC, SPring-8 Office, Assistant Scientist
KIMURA Koji  京都大学, 理学研究科
INUI Masanori  広島大学, 総合科学研究科, 教授 (40213136)
KAJIHARA Yukio  広島大学, 総合科学研究科, 助教 (20402654)
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2014: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2013: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2012: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords液体金属 / 非弾性散乱 / 電子状態
Outline of Final Research Achievements

Experimental investigations for the electronic states in fluid alkali metals were carried out through the observation of the plasmon excitation. Plasmon energies and the line widths were measured by inelastic x-ray scattering experiments using synchrotron radiation. It was found that plasmon behaviors in liquid Rb near the melting point, which become a reference for characterizing plasmon behaviors in fluid Rb, exhibit characteristics more close to those of the electron gas model than solid Rb. This finding indicates that the liquid state is quite effective to get insight into behaviors of the electron gas. Furthermore, by using techniques for the experiments at high temperature regions developed in this study, inelastic x-ray measurements up to 1000 C were successfully carried out. The observation reveals that the plasmon energy decreases with increasing temperature, which reflects the reduction of the average electron density with volume expansion of the fluid.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (26 results)

All 2015 2014 2013 2012

All Journal Article (5 results) (of which Peer Reviewed: 5 results) Presentation (21 results) (of which Invited: 3 results)

  • [Journal Article] Inelastic x-ray scattering study of plasmon dispersions in solid and liquid Rb2014

    • Author(s)
      K. Kimura, K. Matsuda, N. Hiraoka, T. Fukumaru, Y. Kajihara, M. Inui, M. Yao
    • Journal Title

      Phys. Rev. B

      Volume: 89 Issue: 1 Pages: 14206-14206

    • DOI

      10.1103/physrevb.89.014206

    • NAID

      120005530936

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Plasmon line width in liquid metals2013

    • Author(s)
      K. Kimura, K. Matsuda and M. Yao
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 82 Issue: 11 Pages: 115001-115001

    • DOI

      10.7566/jpsj.82.115001

    • NAID

      210000132848

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Electron Momentum Density in Liquid Silicon2013

    • Author(s)
      K. Matsuda, T. Nagao, Y. Kajihara, M. Inui, K. Tamura, J. Nakamura, K. Kimura, M. Yao, M. Itou, and Y. Sakurai
    • Journal Title

      Phys. Rev. B

      Volume: 88 Issue: 11 Pages: 115125-115125

    • DOI

      10.1103/physrevb.88.115125

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Chemical order in liquid As2Se3 at high temperatures obtained by X-ray scattering and reverse Monte Carlo modeling2013

    • Author(s)
      Masanori Inui, Yukio Kajihara, Koji Kimura, Takayuki Fukumaru, Kazuhiro Matsuda, Makoto Yao
    • Journal Title

      Journal of Non-Crystalline Solids

      Volume: 366 Pages: 22-29

    • DOI

      10.1016/j.jnoncrysol.2013.01.035

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Density fluctuations at the continuous liquid-liquid phase transition in chalcogen systems2012

    • Author(s)
      Y. Kajihara, M. Inui, K. Matsuda, T. Nagao, and K. Ohara
    • Journal Title

      Physical Review B

      Volume: 86 Issue: 21

    • DOI

      10.1103/physrevb.86.214202

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] 高温領域における液体Rbのプラズモン測定2015

    • Author(s)
      萩谷透,木村耕治,松田和博,平岡望,宮武至,石黒陽太郎,梶原行夫,乾雅祝,八尾誠
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] 低密度アルカリ金属流体における電子励起観測のためのNb製試料容器の開発2015

    • Author(s)
      木村耕治,萩谷透,松田和博,平岡望,宮武至,石黒陽太郎,梶原行夫,乾雅祝,八尾誠
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] 非弾性X線散乱による液体Siのプラズモン観測2015

    • Author(s)
      石黒陽太郎,松田和博,木村耕治,平岡望,梶原行夫,萩谷透,宮武至,乾雅祝,八尾誠
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] 液体カルシウムの非弾性X線散乱測定2015

    • Author(s)
      乾雅祝,梶原行夫,細川伸也,千葉文野,木村耕治,松田和博,宮武至,筒井智嗣,AQR. Baron
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] 液体ナトリウムのコンプトン散乱測定2015

    • Author(s)
      松田和博,宮武至,木村耕治,石黒陽太郎,萩谷透,梶原行夫,乾雅祝,田村剛三郎,八尾誠,伊藤 真義,櫻井吉晴
    • Organizer
      第28回放射光学会年会・放射光化学合同シンポジウム
    • Place of Presentation
      立命館大学びわこ・くさつキャンパス
    • Year and Date
      2015-01-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] 低密度アルカリ金属液体の電子状態研究 ―高温・高圧下における非弾性X線散乱測定―2015

    • Author(s)
      木村耕治,松田和博,平岡望,萩谷透,宮武至,石黒陽太郎,八尾誠
    • Organizer
      第28回放射光学会年会・ 放射光化学合同シンポジウム
    • Place of Presentation
      立命館大学びわこ・くさつキャンパス
    • Year and Date
      2015-01-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] 膨張金属流体の電子状態観測2014

    • Author(s)
      松田和博,木村耕治,宮武至,石黒陽太郎,萩谷透,梶原行夫,乾雅祝、平岡望,田村 剛三郎,八尾 誠,伊藤 真義,櫻井 吉晴
    • Organizer
      第55回高圧討論会
    • Place of Presentation
      徳島大学常三島キャンパス
    • Year and Date
      2014-11-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] コンプトン散乱実験による液体Naの電子物性研究2014

    • Author(s)
      宮武至,木村耕治,松田和博,石黒陽太郎,梶原行夫,田村剛三郎,八尾誠,伊藤真義,櫻井吉晴
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学
    • Year and Date
      2014-09-09
    • Related Report
      2014 Annual Research Report
  • [Presentation] Plasmons in liquid alkali metals: An inelastic x-ray scattering study2014

    • Author(s)
      K. Kimura
    • Organizer
      2nd International Symposium on Kumamoto Synchrotron Radiation
    • Place of Presentation
      Kumamoto, Japan
    • Year and Date
      2014-05-16
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 液体Csにおけるプラズモン分散:非弾性X線散乱による研究2014

    • Author(s)
      木村耕治,宮武至,松田和博,平岡望,梶原行夫,石黒陽太郎,乾雅祝,八尾誠
    • Organizer
      日本物理学会年次大会
    • Place of Presentation
      東海大学湘南キャンパス,平塚市
    • Related Report
      2013 Research-status Report
  • [Presentation] 液体Rbにおけるプラズモン線幅:非弾性X線散乱による研究2014

    • Author(s)
      木村耕治,松田和博,平岡望,乾雅祝,梶原行夫,八尾誠
    • Organizer
      第27回放射光学会年会・放射光化学合同シンポジウム
    • Place of Presentation
      広島国際会議場,広島市
    • Related Report
      2013 Research-status Report
  • [Presentation] The electronic states in fluid alkali metals: inelastic X-ray scattering study2013

    • Author(s)
      K. Matsuda
    • Organizer
      8th International Conference on Inelastic X-ray Scattering (IXS 2013)
    • Place of Presentation
      Menlo Park, California, USA
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Plasmon Line Width in Liquid Alkali Metal Studied by Inelastic X-ray Scattering2013

    • Author(s)
      K. Kimura, K. Matsuda, N. Hiraoka, T. Fukumaru, M. Inui, Y. Kajihara, M. Yao
    • Organizer
      8th International Conference on Inelastic X-ray Scattering (IXS 2013)
    • Place of Presentation
      Menlo Park, California, USA
    • Related Report
      2013 Research-status Report
  • [Presentation] Electronic states in expanded fluid alkali metals investigated by inelastic X-ray Compton scattering2013

    • Author(s)
      K. Matsuda, T. Fukumaru, K. Kimura, Y. Kajihara, M. Inui, K. Tamura, M. Yao, M. Ito and Y. Sakurai
    • Organizer
      15th international conference on liquid and amorphous metals (LAM15)
    • Place of Presentation
      Beijing, China
    • Related Report
      2013 Research-status Report
  • [Presentation] Plasmon damping in liquid Rb: An inelastic x-ray scattering study2013

    • Author(s)
      K. Kimura, K. Matsuda, N. Hiraoka, Y. Kajihara, M. Inui, M. Yao
    • Organizer
      15th international conference on liquid and amorphous metals (LAM15)
    • Place of Presentation
      Beijing, China
    • Related Report
      2013 Research-status Report
  • [Presentation] アルカリ金属流体のX線コンプトン散乱測定 II2013

    • Author(s)
      松田和博,木村耕治,梶原行夫,乾雅祝,田村剛三郎,八尾誠,伊藤真義,櫻井吉晴
    • Organizer
      第54回高圧討論会
    • Place of Presentation
      朱鷺メッセ,新潟市
    • Related Report
      2013 Research-status Report
  • [Presentation] アルカリ金属液体におけるプラズモン線幅2013

    • Author(s)
      木村耕治,松田和博,平岡望,梶原行夫,乾雅祝,八尾誠
    • Organizer
      日本物理学会秋季大会
    • Place of Presentation
      徳島大学 常三島キャンパス,徳島市
    • Related Report
      2013 Research-status Report
  • [Presentation] X-ray Compton Scattering Measurements of Expanded Fluid Alkali Metals2012

    • Author(s)
      K. Matsuda
    • Organizer
      Sagamore XVII Conference on Electron Charge, Spin and Momentum Densities
    • Place of Presentation
      Hokkaido, Japan
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Compton scattering study of expanded fluid alkali metals2012

    • Author(s)
      K. Matsuda
    • Organizer
      14th International Conference on the Physics of Non-ideal Plasmas
    • Place of Presentation
      Rostock, Germany
    • Related Report
      2012 Research-status Report
  • [Presentation] アルカリ金属流体のX線コンプトン散乱測定2012

    • Author(s)
      松田 和博
    • Organizer
      第53回高圧討論会
    • Place of Presentation
      大阪大学会館
    • Related Report
      2012 Research-status Report
  • [Presentation] Inelastic X-ray Scattering Study of Plasmons in Solid and Liquid Rb2012

    • Author(s)
      K. Kimura
    • Organizer
      14th International Conference on the Physics of Non-ideal Plasmas
    • Place of Presentation
      Rostock, Germany
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2019-07-29  

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