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Diagenetic change of residual gas in mudstones

Research Project

Project/Area Number 24540484
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Geology
Research InstitutionHokkaido University

Principal Investigator

SUZUKI Noriyuki  北海道大学, 理学(系)研究科(研究院), 教授 (00144692)

Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2014: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2013: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2012: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywordsシェールガス / 残留ガス / メタン / 天然ガス / 四万十帯 / 続成作用 / 変成作用 / 基礎試錐 / 変成
Outline of Final Research Achievements

Concentration and compositional changes of hydrocarbon gases in shale rocks and metapelites during diagenesis and metamorphism were revealed by this study. The shale rocks and metapelites were collected from borehole MITI-Mishima and outcrops in Shimanto belt, Chichibu belt, and Sanbagawa metamorphic belt in Shikoku region. Concentration of residual methane begins to increase when shale rock porosity reaches about 5%, suggesting a significant retention of methane in shale rocks. The highest concentration of residual methane corresponds to maturity levels of vitrinite refrectance (VR)=2 to 3 % (maximum heated temperature=200 to 250ºC). Residual methane concentration significantly decreases in the stage of metamorphism suggesting the graphitization of methane. The maturity level of VR=2 to 3 % is the main maturation stage for the formation of shale gas deposit. Several gas seepages observed in Shimanto belt suggest the formation of shale gas deposits in accretionary prism.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (31 results)

All 2014 2013 Other

All Journal Article (6 results) (of which Peer Reviewed: 6 results,  Acknowledgement Compliant: 1 results) Presentation (24 results) Remarks (1 results)

  • [Journal Article] In-reservoir fractionation and the accumulation of oil and condensates in the Surma basin, NE Bangladish.2014

    • Author(s)
      Hossain, Md. A., Suzuki, N., Matsumoto, K., Sakamoto, R., Takeda, N.
    • Journal Title

      Journal of Petroleum Geology

      Volume: 37 Issue: 3 Pages: 269-286

    • DOI

      10.1111/jpg.12583

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 古第三紀石炭の炭化水素ガス排出タイミングを推定するための開放系・閉鎖系熱分解実験.2014

    • Author(s)
      高橋幸士, 鈴木德行, 齋藤裕之
    • Journal Title

      石油技術協会誌

      Volume: 79 Pages: 353-354

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Compositional and isotopic changes in expelled and residual gases during anhydrous closed system pyrolysis of hydrogen-rich Eocene subbituminous coal.2014

    • Author(s)
      Takahashi,K.U.,Suzuki,N.,Saito,H.,
    • Journal Title

      International Journal of Coal Geology

      Volume: 127 Pages: 14-23

    • DOI

      10.1016/j.coal.2014.02.009

    • NAID

      120005457023

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Origin of crude oil and condensates from Surma basin, north-eastern Bangladesh.2013

    • Author(s)
      Hossain,Md.A.,Suzuki,N.,Matsumoto,K.,Sato,N.,Takeda.
    • Journal Title

      石油技術協会誌

      Volume: 78(5) Pages: 421-422

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] 続成作用・変成作用における泥岩残留炭化水素ガスの変化と四万十帯付加体のシェールガスポテンシャル2013

    • Author(s)
      鈴木德行 前本健太 星野太一
    • Journal Title

      石油技術協会誌

      Volume: 78(1) Pages: 16-27

    • NAID

      10031139710

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] A petroleum system in the Gulf of Mannar Basin, Offshore, Sri Lanka.2013

    • Author(s)
      Premarathne, D.M.U.A.K., Suzuki、N., Ratnayake.N.P., Kularathne,E.K.C.W.
    • Journal Title

      Proceedings of 30th Technical Sessions of Geological Society of Sri Lanka

      Volume: 9-12 Pages: 75-78

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] 地下深部の有機物起源の水素.2014

    • Author(s)
      鈴木德行
    • Organizer
      第32回日本有機地球化学シンポジウム
    • Place of Presentation
      ニューウェルシティ湯河原(静岡県熱海市)
    • Year and Date
      2014-11-07
    • Related Report
      2014 Annual Research Report
  • [Presentation] 熱熟成に伴う石炭起源炭化水素ガスの水素同位体組成の変化.2014

    • Author(s)
      高橋幸士, 鈴木德行, 齋藤裕之
    • Organizer
      第32回日本有機地球化学シンポジウム
    • Place of Presentation
      ニューウェルシティ湯河原(静岡県熱海市)
    • Year and Date
      2014-11-06 – 2014-11-08
    • Related Report
      2014 Annual Research Report
  • [Presentation] テルペン類の加水熱分解で生成するナフタレン類の特徴.2014

    • Author(s)
      朝比奈健太, 鈴木德行
    • Organizer
      第32回日本有機地球化学シンポジウム
    • Place of Presentation
      ニューウェルシティ湯河原(静岡県熱海市)
    • Year and Date
      2014-11-06
    • Related Report
      2014 Annual Research Report
  • [Presentation] Closed and semi-open system pyrolysis for estimating the timing of hydrocarbon gas expulsion from Paleogene coal.2014

    • Author(s)
      Takahashi, K., Suzuki, N., Saito, H.
    • Organizer
      31st TSOP ANNUAL MEETING
    • Place of Presentation
      シドニー(オーストラリア)
    • Year and Date
      2014-09-27 – 2014-10-03
    • Related Report
      2014 Annual Research Report
  • [Presentation] 北海道新生代コールベッドメタンの炭素同位体組成.2014

    • Author(s)
      齋藤裕之, 鈴木德行
    • Organizer
      日本地球化学会第61回年会
    • Place of Presentation
      富山大学五福キャンパス(富山県富山市)
    • Year and Date
      2014-09-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] 頁岩と泥質変成岩中の水素の同位体組成と起源.2014

    • Author(s)
      鈴木德行, 星野太一,齋藤裕之
    • Organizer
      日本地球化学会第61回年会
    • Place of Presentation
      富山大学五福キャンパス(富山県富山市)
    • Year and Date
      2014-09-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] 閉鎖系・準開放系熱分解実験による石炭起源ガスの排出温度推定.2014

    • Author(s)
      高橋幸士, 鈴木德行, 齋藤裕之
    • Organizer
      日本地球化学会第61回年会
    • Place of Presentation
      富山大学五福キャンパス(富山県富山市)
    • Year and Date
      2014-09-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] 石狩層群泥質岩の高等植物ワックス水素同位体組成 から見た始新世の海水準変動.2014

    • Author(s)
      佐藤光, 鈴木德行
    • Organizer
      日本地質学会第121年学術大会
    • Place of Presentation
      鹿児島大学郡元キャンパス(鹿児島県鹿児島市)
    • Year and Date
      2014-09-14
    • Related Report
      2014 Annual Research Report
  • [Presentation] Carbon and hydrogen isotope compositions of individual n-alkanes in oil and condensate from the Surma basin, Bangladesh, showing source and evaporative fractionation.2014

    • Author(s)
      Hossain, Md. A., 鈴木德行, 齋藤裕之, 坂本亮, 武田信從
    • Organizer
      平成26年度石油技術協会春季講演会
    • Place of Presentation
      朱鷺メッセ(新潟県新潟市)
    • Year and Date
      2014-06-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] 古第三紀石炭の炭化水素ガス排出タイミングを推定するための開放系・閉鎖系熱分解実験.2014

    • Author(s)
      高橋幸士, 鈴木德行, 齋藤裕之
    • Organizer
      平成26年度石油技術協会春季講演会
    • Place of Presentation
      朱鷺メッセ(新潟県新潟市)
    • Year and Date
      2014-06-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] Origin of crude oil and condensates from Surma basin, north-eastern Bangladesh.2013

    • Author(s)
      Hossain,MD.A.,Suzuki,N.,Matsumoto,K.,Sato,N.,Takeda,N.
    • Organizer
      平成25年度石油技術協会春季講演会
    • Place of Presentation
      国立オリンピック記念青少年総合センター(東京都)
    • Related Report
      2013 Research-status Report
  • [Presentation] The diversity of n-alkane distribution and possible migration fractionation of oils in Kutei Basin, Indonesia.2013

    • Author(s)
      Murwani,R.T.,Suzuki,N.,Sosrowidjojo,I.B.
    • Organizer
      平成25年度石油技術協会春季講演会
    • Place of Presentation
      国立オリンピック記念青少年総合センター(東京都)
    • Related Report
      2013 Research-status Report
  • [Presentation] Source rock potential of some Mesozoic sediments from Gulf of Mannar Basin, offshore Sri Lanka.2013

    • Author(s)
      Premarathne,D.M.U.K.,Suzuki,N.,Ratenayake,N.P.
    • Organizer
      平成25年度石油技術協会春季講演会
    • Place of Presentation
      国立オリンピック記念青少年総合センター(東京都)
    • Related Report
      2013 Research-status Report
  • [Presentation] Origin of desorbed coalbed gas from middle to late Miocene coals in Kutei Basin, Indonesia.2013

    • Author(s)
      Wicaksono, A.B.,Suzuki,N.,Saito,H.,Takahashi,K.,Sosrowidjojo,I.B.
    • Organizer
      平成25年度石油技術協会春季講演会
    • Place of Presentation
      国立オリンピック記念青少年総合センター(東京都)
    • Related Report
      2013 Research-status Report
  • [Presentation] 石狩層群幌加別層の有機地球化学的特徴と始新世の巨大湖沼2013

    • Author(s)
      角勇樹、鈴木德行
    • Organizer
      第31回日本有機地球化学シンポジウム
    • Place of Presentation
      倉敷市芸文館 (岡山県)
    • Related Report
      2013 Research-status Report
  • [Presentation] 地下深部での泥岩残留メタン・水素の炭素水素同位体組成の変化2013

    • Author(s)
      星野太一、鈴木德行、齋藤裕之
    • Organizer
      第31回日本有機地球化学シンポジウム
    • Place of Presentation
      倉敷市芸文館 (岡山県)
    • Related Report
      2013 Research-status Report
  • [Presentation] 北海道新生代露頭炭のコールベッドガスの地球化学的特徴2013

    • Author(s)
      齋藤裕之、鈴木德行
    • Organizer
      第31回日本有機地球化学シンポジウム
    • Place of Presentation
      倉敷市芸文館 (岡山県)
    • Related Report
      2013 Research-status Report
  • [Presentation] 陸生堆積物の高等直物ワックス水素同位体比から見た始新世海水準変動。2013

    • Author(s)
      佐藤光、鈴木德行
    • Organizer
      第31回日本有機地球化学シンポジウム
    • Place of Presentation
      倉敷市芸文館 (岡山県)
    • Related Report
      2013 Research-status Report
  • [Presentation] 新生代石炭から排出される熱分解起源炭化水素ガスの同位体組成の変化2013

    • Author(s)
      高橋幸士、鈴木德行、齋藤裕之
    • Organizer
      第31回日本有機地球化学シンポジウム
    • Place of Presentation
      倉敷市芸文館 (岡山県)
    • Related Report
      2013 Research-status Report
  • [Presentation] セスキテルペンの加水熱分解に由来するナフタレン類の特徴。2013

    • Author(s)
      朝比奈健太、鈴木德行
    • Organizer
      日本地球化学会第60回年会
    • Place of Presentation
      筑波大学(つくば市)
    • Related Report
      2013 Research-status Report
  • [Presentation] Isotopic and compositional changes of expelled and residual gases during laboratory maturation of Eocene sub-bituminous coal.2013

    • Author(s)
      Takahashi,K.,Suzuki,N.,Saito,H.
    • Organizer
      International Conference on Gas Geochemistry 2013.
    • Place of Presentation
      Conference&Cultural Center of the University of Patras (ギリシャ)
    • Related Report
      2013 Research-status Report
  • [Presentation] Biogenic coalbed methane from Miocene crop coals,Hokkaido, Japan.2013

    • Author(s)
      Saito,H.,Suzuki,N.
    • Organizer
      26th International Meeting on Organic Geochemistry
    • Place of Presentation
      Magma Arte & Congresos(スペイン)
    • Related Report
      2013 Research-status Report
  • [Presentation] Change of residual gas in shale and metamorphic rocks during diagenesis and metamorphism.2013

    • Author(s)
      Suzuki,N.,Saito,H.,Maemoto,Hoshino,T., Takahashi, K.U.
    • Organizer
      26th International Meeting on Organic Geochemistry
    • Place of Presentation
      Magma Arte & Congresos(スペイン)
    • Related Report
      2013 Research-status Report
  • [Presentation] 化石燃料や堆積岩中のナフタレン類の起源と生成機構

    • Author(s)
      朝比奈健太、鈴木德行
    • Organizer
      日本化学会北海道支部2013年夏季研究発表会
    • Place of Presentation
      北見工業大学(北見市)
    • Related Report
      2013 Research-status Report
  • [Remarks] N.Suzuki's Home Page

    • URL

      http://www.hucc.hokudai.ac.jp/~k15507/

    • Related Report
      2013 Research-status Report

URL: 

Published: 2013-05-31   Modified: 2019-07-29  

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