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Control of molecular vibrations by double impulsive resonance Raman excitation

Research Project

Project/Area Number 24550004
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Physical chemistry
Research InstitutionHokkaido University

Principal Investigator

Sato Shin-ichiro  北海道大学, 工学(系)研究科(研究院), 准教授 (10262601)

Co-Investigator(Kenkyū-buntansha) 木場 隆之  北見工業大学, 工学部, 助教 (40567236)
Project Period (FY) 2012-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2014: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2013: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2012: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywords脱位相緩和抑制 / 量子制御 / シクロデキストリン / 分子動力学 / 高分子 / 熱運動 / 脱位相抑制 / 量子化学 / RIKES / ラマン誘起カー効果 / 二硫化炭素 / アルコール / libration / デコヒーレンス / 分子振動 / 制御
Outline of Final Research Achievements

In the last decade, the direct control of quantum wave functions of molecular electronic and vibrational states has been developed in the areas pf coherent control of chemical reactions and quantum computing by using ultrafast femtosecond laser. For the achievment of quantum control, the suppression of decohrence of wavefunctions are obviously important. Therefore, we studied the decohrence process of molecular wavefunctions of polycondensed aromatic molecules in the cyclodextrin nanocavity in aqueous/alcohol or aqueous/keton solvents with the deconvolution method by using Voigt function fitting. We also studied fluctuation of polymers motions in aqueous solution by using molecular dynamics simulations.

Report

(5 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (26 results)

All 2016 2015 2014 2013 2012 Other

All Journal Article (15 results) (of which Peer Reviewed: 15 results,  Acknowledgement Compliant: 3 results,  Open Access: 1 results) Presentation (10 results) (of which Int'l Joint Research: 2 results,  Invited: 4 results) Remarks (1 results)

  • [Journal Article] B(C6F5)3-Catalyzed Group Transfer Polymerization of N,N-Disubstituted Acrylamide Using Hydrosilane: Effect of Hydrosilane and Monomer Structures, Polymerization Mechanism, and Synthesis of α-End-Functionalized Polyacrylamides2016

    • Author(s)
      Kikuchi, S., Chen, Y., Kitano, K., Sato, S.-i., Satoh, T.,Kakuchi, T.
    • Journal Title

      Macromolecules

      Volume: in press Issue: 8 Pages: 3049-3060

    • DOI

      10.1021/acs.macromol.6b00190

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] OFF-ON-OFF fluorescent response of N,N,N′,N′-tetrakis(1-isoquinolylmethyl)-2-hydroxy-1,3-propanediamine (1-isoHTQHPN) toward Zn2+2016

    • Author(s)
      Yuji Mikata, Risa Ohnishi, Anna Ugai, Hideo Konno, Yasushi Nakata, Ikuko Hamagamie, Shin-ichiro Sato
    • Journal Title

      Dalton Transactions

      Volume: 45 Issue: 17 Pages: 7250-7257

    • DOI

      10.1039/c6dt00506c

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Synthesis of AB block and A2B2 and A3B3 miktoarm star-shaped copolymers using ω-end-functionalized poly(methyl methacrylate) with a hydroxyl group prepared by organocatalyzed group transfer polymerization2015

    • Author(s)
      Eric, O.-T., Chen, Y., Takada, K., Sato, S.-i., Satoh, T.,Kakuchi, T
    • Journal Title

      Polymer Chemistry

      Volume: 6 Issue: 45 Pages: 7841-7850

    • DOI

      10.1039/c5py01112d

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Zinc-specific intramolecular excimer formation in TQEN derivatives: fluorescence and zinc binding properties of TPEN-based hexadentate ligands2014

    • Author(s)
      Y. Mikata, S. Takeuchi, E. Higuchi, A. Ochi, H. Konno, K. Yanai, S.-i. Sato
    • Journal Title

      Dalton Transactions

      Volume: 43 Issue: 43 Pages: 16377-16386

    • DOI

      10.1039/c4dt01847h

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Stereoblock-like Brush Copolymers Consisting of Poly(l-lactide) and Poly(d-lactide) Side Chains along Poly(norbornene) Backbone: Synthesis, Stereocomplex Formation, and Structure-Property Relationship2014

    • Author(s)
      T. Isono, Y. Kondo, S. Ozawa, Y. Chen, R. Sakai, S.-i. Sato, K. Tajima, T. Kakuchi, T. Satoh
    • Journal Title

      Macromolecules

      Volume: 47 Issue: 20 Pages: 7118-7128

    • DOI

      10.1021/ma501647m

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Thermoresponsive properties of 3-, 4-, 6-, and 12-armed star-shaped poly[2-(dimethylamino)ethyl methacrylate]s prepared by core-first group transfer polymerization2014

    • Author(s)
      Seiya Kikuchi, Chen, Yougen, Keita Fuchise, Kenji Takada, Junsuke Kitakado, Shin-ichiro Sato, Toshifumi Satoh, Toyoji Kakuchi
    • Journal Title

      Polymer Chemistry

      Volume: 5 Issue: 16 Pages: 4701-4709

    • DOI

      10.1039/c4py00290c

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Synthesis of Linear, Cyclic, Figure-Eight-Shaped, and Tadpole-Shaped Amphiphilic Block Copolyethers via t-Bu-P4-Catalyzed Ring-Opening Polymerization of Hydrophilic and Hydrophobic Glycidyl Ethers2014

    • Author(s)
      Isono, T.; Satoh, Y.; Miyachi, K.; Chen, Y.; Sato, S.-i.; Tajima, K.; Satoh, T.; Kakuchi, T.
    • Journal Title

      Macromolecules

      Volume: 47 Issue: 9 Pages: 2853-2863

    • DOI

      10.1021/ma500494e

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Diphenyl Phosphate/4-Dimethylaminopyridine as an Efficient Binary Organocatalyst System for Controlled/Living Ring-Opening Polymerization of L-Lactide Leading to Diblock and End-Functionalized Poly(L-lactide)s2014

    • Author(s)
      牧口 孝祐、菊地 誠也、屋内 一馬、小笠原 啓孝、佐藤 信一郎、佐藤 敏文、覚知 豊次
    • Journal Title

      Journal of Polymer Science Part A : Polymer Chemistry

      Volume: 52 Issue: 7 Pages: 1047-1054

    • DOI

      10.1002/pola.27089

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Theoretical Study of Intramolecular Charge Transfer Turn-off Switching of N-(4-Dimethylaminobenzoyl) Thiourea Induced by Anion Recognition2013

    • Author(s)
      KAZUMA YANAI,SHIN-ICHIRO SATO
    • Journal Title

      Mol. Cryst. Liq. Cryst.

      Volume: 580 Issue: 1 Pages: 15-21

    • DOI

      10.1080/15421406.2013.803893

    • NAID

      120005472203

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Structure and Intermolecular Dynamics of Carbon Disulfide/Alcohols Binary Solution2013

    • Author(s)
      Takayuki Kiba, Takashi Hirota, Akihiro Murayama, Shin-Ichiro Sato
    • Journal Title

      Mol. Cryst. Liq. Cryst.

      Volume: 579 Issue: 1 Pages: 103-109

    • DOI

      10.1080/15421406.2013.802966

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Photophysical Properties of Self-assembled Cyanine-dye Dimmer Formation Assisted by Cyclodextrin Inclusion Complexation2013

    • Author(s)
      Shigeaki Abe, Takashi Hirota, Takayuki Kiba, Naoyuki Miyakawa, Fumio Watari, Akihiro Murayama, Shin-Ichiro Sato
    • Journal Title

      Mol. Cryst. Liq. Cryst.

      Volume: 579 Issue: 1 Pages: 22-29

    • DOI

      10.1080/15421406.2013.804799

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Spectral Narrowing of UV-Visible Absorption and Emission Spectra of Anthracene-Derivatives in -Cyclodextrin Nanocavity: Effects of Host/Guest Stoichiometry2012

    • Author(s)
      Shin-Ichiro Sato, Yuuki Yoshizumi, Takayuki Kiba, Akihiro Murayama, Shigeaki Abe
    • Journal Title

      Molecular Crystals and Liquid Crystals

      Volume: 568 Issue: 1 Pages: 60-65

    • DOI

      10.1080/15421406.2012.710176

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Morphology and Photophysical Properties of One-Dimensional Arrayed Porphyrin Aggregates Assisted by Cyclodextrin Inclusion Complexation2012

    • Author(s)
      Shigeaki Abe, Hirohisa Kobayashi, Takayuki Kiba, Fumio Watari, Shin-ichiro Sato
    • Journal Title

      Molecular Crystals and Liquid Crystals

      Volume: 566 Issue: 1 Pages: 151-157

    • DOI

      10.1080/15421406.2012.701879

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fluorescence Turn-On Sensing of Anions Based on Disassembly Process of Urea-Functionalized Poly(phenylenebutadiynylene) Aggregates2012

    • Author(s)
      R. Sakai, A. Nagai, Y. Tago, S. Sato, Y. Nishimura, T. Arai, T. Satoh and T. Kakuchi
    • Journal Title

      Macromolecules

      Volume: 45 Issue: 10 Pages: 4122-4127

    • DOI

      10.1021/ma300481j

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Biodistribution of water-soluble Carbon Nanotubes in mice and its biocompatibility2012

    • Author(s)
      S.Abe, S.Itoh, D.Hayashi, T.Kobayashi, T.i Kiba, T.Akasaka, M.Uo, Y.Yawaka, S.Sato, F.Watari, T.Takada
    • Journal Title

      J.Nanoscience and Nanotechnology

      Volume: 12 Issue: 1 Pages: 700-706

    • DOI

      10.1166/jnn.2012.5391

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] Molecular dynamics study on star-shaped thermoresponsive polymers in aqueous solution2015

    • Author(s)
      Shin-ichiro Sato
    • Organizer
      Pacifichem 2015
    • Place of Presentation
      Hawaii Convention Center, Honolulu, USA
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Molecular Dynamics Simulation on Phase-transition dynamics for aqueous solution of thermoresponsive polyisocyanate with oligoethyleneoxide sidechains2015

    • Author(s)
      Shin-ichiro Satto
    • Organizer
      The 4th Joint Symposium between Hokkaido University and Harbin Engineering University
    • Place of Presentation
      Suzuki Hall, Hokkaido University, Sapporo
    • Year and Date
      2015-09-01
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Computational study of fluorescent anion-sensing molecules: effects of conformational change in the electronic excited state2014

    • Author(s)
      Shin-ichiro Sato
    • Organizer
      SNU-HU Joint Symposium 2014
    • Place of Presentation
      Sapporo
    • Year and Date
      2014-11-27 – 2014-11-29
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] In silico study of fluorescent anion-sensing molecules: effects of conformational change in the electronic excited state2014

    • Author(s)
      Shin-ichiro Sato
    • Organizer
      HU-AGH Joint Symposium 2014
    • Place of Presentation
      Krakow
    • Year and Date
      2014-09-03 – 2014-09-06
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Theoretical study of intramolecular charge transfer turn-off switching of N-(4-Dimethylaminobenzoyl) thiourea induced by anion recognition2012

    • Author(s)
      Kazuma Yanai, Shin-ichiro Sato
    • Organizer
      KJF International Conference on Organic Materials for Electronics and Photonics 2012
    • Place of Presentation
      仙台 東北大学 さくらホール
    • Related Report
      2012 Research-status Report
  • [Presentation] Structure and intermolecular dynamics of carbon disulfide/alcohols binary solution2012

    • Author(s)
      akayuki Kiba1, Takashi Hirota, Akihiro Murayama, Shin-ichiro Sato
    • Organizer
      KJF International Conference on Organic Materials for Electronics and Photonics 2012
    • Place of Presentation
      仙台 東北大学 さくらホール
    • Related Report
      2012 Research-status Report
  • [Presentation] Morphology and photophysical properties of one-dimensional arrayed porphyrin aggregates assisted by cyclodextrin inclusion complexation2012

    • Author(s)
      Shigeaki Abe, Hirohisa Kobayashi, Takayuki Kiba, Fumio Watari, Shin-ichiro Sato
    • Organizer
      KJF International Conference on Organic Materials for Electronics and Photonics 2012
    • Place of Presentation
      仙台 東北大学 さくらホール
    • Related Report
      2012 Research-status Report
  • [Presentation] Extension of Redfield theory: Inclusion of non-elastic collisions

    • Author(s)
      Shin-ichiro Sato
    • Organizer
      245th ACS National Meeting, COMP division
    • Place of Presentation
      New Orleans, LA, United States
    • Related Report
      2013 Research-status Report
  • [Presentation] Vibronic switching of fluorescence output from urea-functionalized poly (p-phenylene) receptor by fluoride-anion recognition

    • Author(s)
      Kazuma Yanai, Shin-ichiro Sato
    • Organizer
      245th ACS National Meeting, COMP division
    • Place of Presentation
      New Orleans, LA, United States
    • Related Report
      2013 Research-status Report
  • [Presentation] Selective vibronic switching of fluorescence output from urea-functionalized poly (p-phenylene) induced by anion recognition

    • Author(s)
      Shin-ichiro Sato
    • Organizer
      20th International SPACC Symposium
    • Place of Presentation
      Changchun, China
    • Related Report
      2013 Research-status Report
    • Invited
  • [Remarks] Understanding of Cutting Edge Chemistry

    • URL

      http://kkyoka.oeic.hokudai.ac.jp/frontier/en/researcher/18/050

    • Related Report
      2014 Research-status Report

URL: 

Published: 2013-05-31   Modified: 2019-07-29  

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