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Photoluminescene decay time of the exciton-exciton scattering in a semiconductor thin film

Research Project

Project/Area Number 24560011
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Applied materials science/Crystal engineering
Research InstitutionNippon Bunri University (2014)
Osaka University (2012-2013)

Principal Investigator

ICHIDA Hideki  日本文理大学, 工学部, 特任准教授 (50379129)

Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2014: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2013: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2012: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Keywords励起子ポラリトン / 励起子ー励起子散乱 / 時間分解発光スペクトル / 時間分解発光ダイナミクス / 励起子 / ポラリトン / 発光寿命 / 励起子-励起子散乱
Outline of Final Research Achievements

We have investigated the mechanism of the photoluminescence-decay time of the exciton-exciton scattering so-called P emission in semiconductor thin films from the viewpoint of the photon-like polariton state which is created by the exciton-exciton scattering process, and located the lower energy region of the bottle neck in the exciton-polariton picture. From the analysis of the time-resolved photoluminescence spectra observed in the ZnO thin files under the high-density excitation conditions, we have obtained the results that the decay time of the PL band of the exciton-exciton scattering becomes faster with decreasing film thickness. From the analysis of the experimental results, we find that the decay time of the photoluminescence of the exciton-exciton scattering is governed by the conversion time from the exciton state to the polariton state.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (10 results)

All 2014 2013 2012 Other

All Journal Article (4 results) (of which Peer Reviewed: 4 results,  Acknowledgement Compliant: 1 results) Presentation (6 results)

  • [Journal Article] Emission-energy dependence of ultrafast P-emission decay in ZnO from bulk to nanofilm2014

    • Author(s)
      Shuji Wakaikia, Hideki Ichida, Motoaki Bamba, Toshiki Kawase, Masaki Kawakami, Kohji Mizoguchi, DaeGwi Kim, Masaaki Nakayama, Yasuo Kanematsu
    • Journal Title

      Journal of Luminescence

      Volume: 152 Pages: 250-253

    • DOI

      10.1016/j.jlumin.2013.12.024

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Slow propagation of photon-like polaritons generated by exciton-exciton scattering in ZnO thin films2013

    • Author(s)
      H. Ichida, S. Wakaiki, K. Mizoguchi, D. Kim, Y. Kanematsu, M. Nakayama
    • Journal Title

      The European Physical Journal Web of Conferences

      Volume: 41 Pages: 04014-04014

    • DOI

      10.1051/epjconf/20134104014

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Thickness dependence of photoluminescence-decay profiles of exciton-exciton scattering in ZnO thin films2013

    • Author(s)
      S. Wakaiki, H. Ichida, T. Kawase, K. Mizoguchi, D. Kim, M. Nakayama, and Y. Kanematsu
    • Journal Title

      The European Physical Journal B

      Volume: 86 Issue: 9

    • DOI

      10.1140/epjb/e2013-30631-5

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Photoluminescence Dynamics from Exciton-exciton Scattering and Exciton-electron Scattering in GaN Thin Film2012

    • Author(s)
      S. Wakaiki, H. Tokumaru, H. Ichida, K. Mizoguchi, D. G. Kim, Y. Kanematsu, M. Nakayama
    • Journal Title

      physica status solidi (c)

      Volume: 9 Issue: 12 Pages: 2497-2500

    • DOI

      10.1002/pssc.201200316

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] P-emission decay in ZnO from bulk to nanofilm2014

    • Author(s)
      Motoaki Bamba, Shuji Wakaikia, Hideki Ichida, Masaki Kawakami, Kohji Mizoguchi, DaeGwi Kim, Masaaki Nakayama, Yasuo Kanematsu
    • Organizer
      ICSCE-7, The 7th International Conference on Spontaneous Coherence in Excitonic Systems
    • Place of Presentation
      Hakone, Japan
    • Year and Date
      2014-08-21 – 2014-08-25
    • Related Report
      2014 Annual Research Report
  • [Presentation] ZnO 薄膜における励起子-励起子散乱発光ダイナミクスの膜厚依存性2014

    • Author(s)
      若生周治,市田秀樹,馬場基彰、川瀬稔貴、川上将輝、溝口幸司,金大貴,中山正昭、兼松泰男
    • Organizer
      日本物理学会 第69回年次大会
    • Place of Presentation
      東海大学
    • Related Report
      2013 Research-status Report
  • [Presentation] Peculiar thickness-dependent behavior of the ultrafast P-emission dynamics for ZnO thin films. I2013

    • Author(s)
      Shuji Wakaiki, Hideki Ichida, Toshiki Kawase, Masaki Kawakami, Motoaki Bamba, Kohji Mizoguchi, DaeGwi Kim, Masaaki Nakayama, and Yasuo Kanematsu
    • Organizer
      18th International Conference on Dynamical Processes in Excited States of Solids (DPC'13)
    • Place of Presentation
      Fuzhou, China
    • Related Report
      2013 Research-status Report
  • [Presentation] Photoluminescence dynamics originating from exciton-exciton and exciton-electron scattering in a GaN thin film

    • Author(s)
      Shuji Wakaiki,Hitoshi Tokumaru, Hideki Ichida, Kohji Mizoguchi, DaeGwi Kim, Yasuo Kanematsu, Masaaki Nakayama
    • Organizer
      Fifth International Conference on Optical, Optoelectronic and Photonic Materials and Applications
    • Place of Presentation
      Nara, Japan
    • Related Report
      2012 Research-status Report
  • [Presentation] Thickness dependence of photoluminescence-decay profiles of exciton-exciton scattering in ZnO thin films

    • Author(s)
      Shuji Wakaiki, Hideki Ichida, Toshiki Kawase, Kohji Mizoguchi, DaeGwi Kim, Masaaki Nakayama, and Yasuo Kanematsu
    • Organizer
      The 10th International Conference on Excitonic Processes in Condensed Matter, Nanostructured and Molecular Materials
    • Place of Presentation
      Groningen, Netherlands
    • Related Report
      2012 Research-status Report
  • [Presentation] ZnO 薄膜における励起子-励起子散乱発光の時間分解発光特性

    • Author(s)
      若生周治,市田秀樹,川瀬稔貴,川上将輝,溝口幸司,金大貴,中山正昭,兼松泰男
    • Organizer
      日本物理学会,第68回年次大会
    • Place of Presentation
      広島大学(広島県)
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2019-07-29  

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