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Preparation of metal nanowires by high-energy-ion-beam technology and their applications to fuel-cell catalyst materials

Research Project

Project/Area Number 24561047
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Nuclear engineering
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

YAMAKI Tetsuya  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 量子ビーム応用研究センター, 研究主幹 (10354937)

Co-Investigator(Renkei-kenkyūsha) YAMAMOTO Shunya  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 量子ビーム応用研究センター, 研究主幹 (70354941)
HAKODA Teruyuki  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 量子ビーム応用研究センター, 研究主幹 (70354933)
YURI Yosuke  独立行政法人日本原子力研究開発機構, 原子力科学研究部門高崎量子応用研究所 放射線高度利用施設部, 研究副主幹 (90414565)
Research Collaborator TERAI Takayuki  東京大学, 工学系研究科, 教授
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2014: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2013: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2012: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Keywordsイオンビーム / 潜在飛跡 / 電子励起効果 / 放射線還元 / 金属ナノ細線 / 電極触媒 / 固体高分子形燃料電池
Outline of Final Research Achievements

We prepared metal nanowires by a radiation-reduction reaction occurring very locally in cylindrical heavy-ion tracks and then pursued the possibility of their applications to the oxygen reduction reaction catalyst in polymer electrolyte membrane fuel cells. According to the analysis of elemental chemical states and microscopic observations, the reduction of metal ions efficiently took place in each track, probably leading to the formation of metal nanowires whose morphology depended on the track structures.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (38 results)

All 2015 2014 2013 2012 Other

All Journal Article (12 results) (of which Peer Reviewed: 12 results) Presentation (19 results) (of which Invited: 6 results) Patent(Industrial Property Rights) (7 results) (of which Overseas: 2 results)

  • [Journal Article] Imidazolium Cation Based Anion-Conducting Electrolyte Membranes Prepared by Radiation Induced Grafting for Direct Hydrazine Hydrate Fuel Cells2014

    • Author(s)
      K. Yoshimura, H. Koshikawa, T. Yamaki, H. Shishitani, K. Yamamoto, S. Yamaguchi, H. Tanaka, Y. Maekawa
    • Journal Title

      Journal of The Electrochemical Society

      Volume: 161 Issue: 9 Pages: F889-F893

    • DOI

      10.1149/2.0511409jes

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Affinity of ion-exchange membranes for HI-I2-H2O mixture2014

    • Author(s)
      N. Tanaka, T. Yamaki, M. Asano, T. Terai, K. Onuki
    • Journal Title

      Journal of Membrane Science

      Volume: 456 Pages: 31-41

    • DOI

      10.1016/j.memsci.2014.01.012

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Preparation of Tungsten Carbide Nanoparticles by Ion Implantation and Electrochemical Etching2013

    • Author(s)
      S. Kato, T. Yamaki, S. Yamamoto, T. Hakoda, K. Kawaguchi, T. Kobayashi, A. Suzuki, T. Terai
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 314 Pages: 149-152

    • DOI

      10.1016/j.nimb.2013.05.052

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ion-Track Membranes of Fluoropolymers: Toward Controlling the Pore Size and Shape2013

    • Author(s)
      T. Yamaki, N. Nuryanthi, H. Koshikawa, M. Asano, S. Sawada, T. Hakoda, Y. Maekawa, K.-O. Voss, D. Severin, T. Seidl, C. Trautmann, R. Neumann
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 314 Pages: 77-81

    • DOI

      10.1016/j.nimb.2013.05.028

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Counter Anion Effect on the Properties of Anion-Conducting Polymer Electrolyte Membranes Prepared by Radiation-Induced Graft Polymerization2013

    • Author(s)
      H. Koshikawa, K. Yoshimura, W. Sinnananchi, T. Yamaki, M. Asano, K. Yamamoto, S. Yamaguchi, H. Tanaka, Y. Maekawa
    • Journal Title

      Macromolecular Chemistry and Physics

      Volume: 214 Issue: 15 Pages: 1756-1762

    • DOI

      10.1002/macp.201300225

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Applied-Voltage Dependence on Conductometric Track Etching of Poly(vinylidene fluoride) Films2013

    • Author(s)
      N. Nuryanthi, T. Yamaki, H. Koshikawa, M. Asano, S. Sawada, S. Hasegawa, Y. Maekawa, Y. Katsumura
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 314 Pages: 95-98

    • DOI

      10.1016/j.nimb.2013.05.035

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Microscopic Evaluation of the Absolute Fluence Distribution of a Large-Area Uniform Ion Beam Using the Track-Etching Technique2013

    • Author(s)
      A. Kitamura (Ogawa), T. Yamaki, Y. Yuri, S. Sawada, T. Yuyama
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 314 Pages: 47-50

    • DOI

      10.1016/j.nimb.2013.05.027

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Nanoparticle Formation by Tungsten Ion Implantation into Glassy Carbon2013

    • Author(s)
      S. Kato, T. Yamaki, S. Yamamoto, T. Hakoda, K. Kawaguchi, T. Kobayashi, A. Suzuki, T. Terai
    • Journal Title

      Transactions of the Materials Research Society of Japan

      Volume: 38 Pages: 81-84

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Hierarchical Structure Analysis of Graft-Type Polymer Electrolyte Membranes Consisting of Cross-Linked Polytetrafluoroethylene by Small-Angle Scattering in a Wide-Q Range2012

    • Author(s)
      H. Iwase, S. Sawada, T. Yamaki, S. Koizumi, M. Ohnuma, Y. Maekawa
    • Journal Title

      Macromolecules

      Volume: 45 Issue: 22 Pages: 9121-9127

    • DOI

      10.1021/ma301415r

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Investigation of Nanopore Evolution in Track-Etched Poly(vinylidene fluoride) Membranes2012

    • Author(s)
      T. Yamaki, N. Nuryanthi, H. Koshikawa, M. Asano, S. Sawada, S. Hasegawa, Y. Maekawa, K.-O. Voss, C. Trautmann, R. Neumann
    • Journal Title

      Transactions of the Materials Research Society of Japan

      Volume: 37 Pages: 223-226

    • NAID

      130003399088

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Alkaline Durable Anion Exchange Membranes Based on Graft-Type Fluoropolymer Films for Hydrazine Hydrate Fuel Cell2012

    • Author(s)
      K. Yoshimura, H. Koshikawa, T. Yamaki, Y. Maekawa, K. Yamamoto, H. Shishitani, K. Asazawa, S. Yamaguchi, H. Tanaka
    • Journal Title

      ECS Transactions

      Volume: 50 Issue: 2 Pages: 2075-2081

    • DOI

      10.1149/05002.2075ecst

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] In-Situ Analysis of Ion-Beam-Induced Degradation and Post-Irradiation Oxidation in Poly(vinylidene fluoride)2012

    • Author(s)
      T. Yamaki, M. Asano, H. Koshikawa, Y. Maekawa, D. Severin, T. Seidl, C. Trautmann
    • Journal Title

      GSI Scientific Report

      Volume: 2011 Pages: 420-420

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] Ar イオン照射によるグラッシーカーボン担持Pt ナノ微粒子触媒の高性能化2015

    • Author(s)
      木全哲也、加藤翔、八巻徹也、山本春也、箱田照幸、小林知洋、鈴木晶大、寺井隆幸
    • Organizer
      日本原子力学会2015年春の年会
    • Place of Presentation
      茨城大学日立キャンパス(茨城県・日立市)
    • Year and Date
      2015-03-20 – 2015-03-22
    • Related Report
      2014 Annual Research Report
  • [Presentation] Quantum Beam Technology: Catalytic Materials Prepared by Ion Beam Irradiation for Electrochemical Device Applications2015

    • Author(s)
      20.T. Yamaki, S. Kato, T. Kimata, S. Yamamoto, T. Hakoda, T. Kobayashi, A. Suzuki, T. Terai
    • Organizer
      The 10th Workshop on Reactive Metal Processing (RMW10)
    • Place of Presentation
      Cambridge (USA)
    • Year and Date
      2015-03-20 – 2015-03-21
    • Related Report
      2014 Annual Research Report
  • [Presentation] Fluoropolymer-Based Nanostructures Created by Swift-Heavy-Ion Irradiation2015

    • Author(s)
      T. Yamaki
    • Organizer
      6th Asian Forum for Accelerators and Detectors (AFAD 2015)
    • Place of Presentation
      Hsinchu (Taiwan)
    • Year and Date
      2015-01-26 – 2015-01-27
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] イオンビームによる燃料電池用Pt ナノ微粒子触媒の高性能化 -グラッシーカーボン基板へのAr イオン照射が及ぼす影響-2014

    • Author(s)
      木全哲也、加藤翔、八巻徹也、山本春也、箱田照幸、小林知洋、鈴木晶大、寺井隆幸
    • Organizer
      日本化学会関東支部群馬地区地域懇談会2014
    • Place of Presentation
      群馬大学桐生キャンパス(群馬県・桐生市)
    • Year and Date
      2014-12-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Ar イオン照射されたグラッシーカーボン基板におけるPt ナノ微粒子触媒の担持状態2014

    • Author(s)
      木全哲也、加藤翔、八巻徹也、山本春也、箱田照幸、小林知洋、鈴木晶大、寺井隆幸
    • Organizer
      第24回日本MRS 年次大会
    • Place of Presentation
      横浜市開港記念会館(神奈川県・横浜市)
    • Year and Date
      2014-12-10 – 2014-12-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Creation of Fluoropolymer-Based Nanostructures by Swift-Heavy-Ion Irradiation2014

    • Author(s)
      T. Yamaki
    • Organizer
      International Conference on Swift Heavy Ions in Materials and Engineering and Characterization (SHIMEC 2014)
    • Place of Presentation
      New Delhi (India)
    • Year and Date
      2014-10-14 – 2014-10-17
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Chemical Interaction of Energetic Metal Ions with Glassy Carbon Substrate: Comparison between Implanted Tungsten and Platinum Ions2014

    • Author(s)
      T. Yamaki, S. Kato, S. Yamamoto, T. Hakoda, K. Kawaguchi, T. Kobayashi, A.Suzuki, T. Terai
    • Organizer
      International Conference on Swift Heavy Ions in Materials and Engineering and Characterization (SHIMEC 2014)
    • Place of Presentation
      New Delhi (India)
    • Year and Date
      2014-10-14 – 2014-10-17
    • Related Report
      2014 Annual Research Report
  • [Presentation] Nanostructured Proton-Conductive Membranes Prepared by Swift Heavy Ion Irradiation for Fuel Cell Applications2014

    • Author(s)
      T. Yamaki
    • Organizer
      The 15th IUMRS International Conference in Asia (IUMRS-ICA 2014)
    • Place of Presentation
      福岡大学(福岡県・福岡市)
    • Year and Date
      2014-08-24 – 2014-08-30
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Chemical Interaction in Tungsten-Implanted Glassy Carbon2013

    • Author(s)
      T. Yamaki, S. Kato, S. Yamamoto, T. Hakoda, K. Kawaguchi, T. Kobayashi, A. Suzuki, T. Terai
    • Organizer
      The 17th International Conference on Radiation Effects in insulators (REI-2013)
    • Place of Presentation
      University of Helsinki (Finland)
    • Related Report
      2013 Research-status Report
  • [Presentation] 高エネルギー重イオンビームによる燃料電池用ナノ構造制御電解質膜の開発:プロトン伝導性の照射イオン依存性2013

    • Author(s)
      八巻徹也、関根敏彦、澤田真一、越川 博、鈴木晶大、寺井隆幸、浅野雅春、前川康成
    • Organizer
      日本膜学会第35年会
    • Place of Presentation
      早稲田大学西早稲田キャンパス(東京)
    • Related Report
      2013 Research-status Report
  • [Presentation] ケミルミネッセンス法による放射線グラフト膜の熱劣化特性解析2013

    • Author(s)
      澤田真一、八巻徹也、浅野雅春、前川康成、佐藤 哲、山田理恵
    • Organizer
      マテリアルライフ学会第24回研究発表会
    • Place of Presentation
      京都工芸繊維大学松ヶ崎キャンパス(京都)
    • Related Report
      2013 Research-status Report
  • [Presentation] イオン注入法による Pt ナノ微粒子の作製(1):作製方法と形態2013

    • Author(s)
      加藤 翔、八巻徹也、山本春也、箱田照幸、川口和弘、小林知洋、鈴木晶大、寺井隆幸
    • Organizer
      2013年電気化学会秋季大会
    • Place of Presentation
      東京工業大学大岡山キャンパス(東京)
    • Related Report
      2013 Research-status Report
  • [Presentation] イオン注入法による Pt ナノ微粒子の作製(2):電気化学特性2013

    • Author(s)
      加藤 翔、八巻徹也、山本春也、箱田照幸、川口和弘、小林知洋、鈴木晶大、寺井隆幸
    • Organizer
      2013年電気化学会秋季大会
    • Place of Presentation
      東京工業大学大岡山キャンパス(東京)
    • Related Report
      2013 Research-status Report
  • [Presentation] Ion-Track Membranes of Fluoropolymers: Toward Control of Pore Size and Shape2013

    • Author(s)
      T. Yamaki, N. Nuryanthi, H. Koshikawa, M. Asano, S. Sawada, T. Hakoda, Y. Maekawa, K.-O. Voss, D. Severin, T. Seidl, C. Trautmann and R. Neumann
    • Organizer
      第23回日本MRS年次大会(国際シンポジウム)
    • Place of Presentation
      横浜市開港記念会館(神奈川)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] フッ素系高分子からなるイオン穿孔膜の作製 -潜在飛跡の構造と前処理効果-

    • Author(s)
      八巻徹也、ヌリヤンティ ヌヌン、越川博、澤田真一、箱田照幸、浅野雅春、前川康成、フォス カイ-オッベ、ゼヴァリン ダニエル、ゼイドル ティム、トラウトマン クリスティーナ
    • Organizer
      膜シンポジウム2012
    • Place of Presentation
      神戸大学(兵庫)
    • Related Report
      2012 Research-status Report
  • [Presentation] Preparation of Tungsten Carbide Nanoparticles by Ion Implantation and Electrochemical Etching

    • Author(s)
      S. Kato, T. Yamaki, S. Yamamoto, T. Hakoda, K. Kawaguchi, T. Kobayashi, A. Suzuki, T. Terai
    • Organizer
      8th International Symposium on Swift Heavy Ions in Matter (SHIM2012)
    • Place of Presentation
      Kyoto University (Japan)
    • Related Report
      2012 Research-status Report
  • [Presentation] 放射線グラフト重合法と燃料電池用高分子電解質膜の開発:経緯と新しい展開

    • Author(s)
      八巻徹也
    • Organizer
      第55回放射線化学討論会
    • Place of Presentation
      モンタナリゾート岩沼(宮城)
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Nanoparticles of Tungsten Carbides Prepared by Tungsten-Ion Implantation in Glassy Carbon

    • Author(s)
      T. Yamaki, S. Kato, S. Yamamoto, T. Hakoda, K. Kawaguchi, T. Kobayashi, A. Suzuki, T. Terai
    • Organizer
      18th International Conference on Ion Beam Modifications of Materials (IBMM 2012)
    • Place of Presentation
      InterContinental Qingdao (China)
    • Related Report
      2012 Research-status Report
  • [Presentation] 「量子ビーム」を利用した有機機能薄膜の創製

    • Author(s)
      八巻徹也
    • Organizer
      第6 回自己組織化討論会
    • Place of Presentation
      つくばセミナーハウス(茨城)
    • Related Report
      2012 Research-status Report
    • Invited
  • [Patent(Industrial Property Rights)] 微量白金担持セリアナノワイヤ及びその製造方法2015

    • Inventor(s)
      森 利之、鈴木彰、小林知洋、山本春也、箱田照幸、八巻徹也
    • Industrial Property Rights Holder
      物質・材料研究機構、理化学研究所、日本原子力研究開発機構
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2015-009968
    • Filing Date
      2015-01-22
    • Related Report
      2014 Annual Research Report
  • [Patent(Industrial Property Rights)] 多孔性高分子フィルムの製造方法および多孔性高分子フィルム2014

    • Inventor(s)
      村木勇三、越川博、八巻徹也、百合庸介、湯山貴裕、石坂和久
    • Industrial Property Rights Holder
      日東電工株式会社、日本原子力研究開発機構
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2014-194358
    • Filing Date
      2014-09-24
    • Related Report
      2014 Annual Research Report
  • [Patent(Industrial Property Rights)] アニオン伝導電解質膜及びその製造方法2013

    • Inventor(s)
      吉村公男、越川博、八巻徹也、前川康成、猪谷秀幸、田中裕久ら
    • Industrial Property Rights Holder
      吉村公男、越川博、八巻徹也、前川康成、猪谷秀幸、田中裕久ら
    • Industrial Property Rights Type
      特許
    • Filing Date
      2013-12-26
    • Related Report
      2013 Research-status Report
  • [Patent(Industrial Property Rights)] Anion Exchange Membrane and Producing Method Thereof2013

    • Inventor(s)
      K. Yoshimura, T. Yamaki et al.
    • Industrial Property Rights Holder
      K. Yoshimura, T. Yamaki et al.
    • Industrial Property Rights Type
      特許
    • Filing Date
      2013-08-28
    • Related Report
      2013 Research-status Report
    • Overseas
  • [Patent(Industrial Property Rights)] 多孔性高分子フィルムの製造方法および多孔性高分子フィルム2013

    • Inventor(s)
      古山了、森山順一、長井陽三、百合庸介、湯山貴裕、八巻徹也ら
    • Industrial Property Rights Holder
      日東電工株式会社、日本原子力開発機構
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2013-067306
    • Filing Date
      2013-03-27
    • Related Report
      2012 Research-status Report
  • [Patent(Industrial Property Rights)] Anion Conducting Electrolyte Membrane and Manufacturing Method Thereof2013

    • Inventor(s)
      K. Yoshimura, T. Yamaki et al.
    • Industrial Property Rights Holder
      日本原子力開発機構、ダイハツ工業株式会社
    • Industrial Property Rights Type
      特許
    • Filing Date
      2013-03-05
    • Related Report
      2012 Research-status Report
    • Overseas
  • [Patent(Industrial Property Rights)] アニオン伝導電解質膜およびその製造方法2012

    • Inventor(s)
      吉村公男、越川博、八巻徹也、浅野雅春、前川康成、猪谷秀幸ら
    • Industrial Property Rights Holder
      日本原子力開発機構、ダイハツ工業株式会社
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2012-192620
    • Filing Date
      2012-08-31
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2019-07-29  

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