• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Development of Pt substituted wood carbon cathode catalysts from cellulose for fuel cells

Research Project

Project/Area Number 24580244
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Wood science
Research InstitutionKyoto University

Principal Investigator

HATA TOSHIMITSU  京都大学, 生存圏研究所, 講師 (10243099)

Co-Investigator(Renkei-kenkyūsha) HONMA Sensho  地方独立行政法人北海道立総合研究機構, 森林研究本部林産試験場, 主査
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥5,330,000 (Direct Cost: ¥4,100,000、Indirect Cost: ¥1,230,000)
Fiscal Year 2014: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2013: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2012: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywordsセルロース / メラミン / 炭化 / 窒素官能基 / 酸素還元反応 / 燃料電池 / 酸素還元活性 / 固体高分子形燃料電池 / 窒素 / 細孔構造 / 木質炭素化物 / Py-GC-MS / レボグルコサン
Outline of Final Research Achievements

The development of the catalyst for fuel cells from unused biomass is important for the society to realize the sustainability. Elemental analysis, X-ray photoelectron spectroscopy (XPS), and high-resolution electron microscope (HR-TEM) were performed in order to reveal the influence of synthesis conditions on oxygen reduction activity. Quaternary nitrogen and oxygen component functional groups were found to be important in order to improve oxygen reduction activity of the catalysts. Nano-shell structure of carbons was formed by the catalytic action of the iron complex, which led to the improvement of the oxygen reduction activity. Multiple regression analysis give informative results for determining optimum conditions of the synthetic conditions.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (23 results)

All 2014 2013 2012 Other

All Journal Article (2 results) (of which Open Access: 1 results,  Peer Reviewed: 1 results) Presentation (16 results) Book (2 results) Remarks (3 results)

  • [Journal Article] 木材から燃料電池用材料をつくる2014

    • Author(s)
      畑 俊充
    • Journal Title

      生存圏研究

      Volume: 10 Pages: 17-21

    • NAID

      120005575257

    • Related Report
      2014 Annual Research Report
    • Open Access
  • [Journal Article] ウッドバイオリファイナリー2.スギ炭素化物からの機能性材料の開発2012

    • Author(s)
      畑 俊充
    • Journal Title

      材料

      Volume: 61(8) Pages: 742-747

    • NAID

      130002084919

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] 窒素ドープ木質炭素化物の空隙構造に及ぼす合成条件の影響2014

    • Author(s)
      畑 俊充, 内本善晴, R. Benoit, S. Bonnamy, P. Bronsveld
    • Organizer
      第41回炭素材料学会年会
    • Place of Presentation
      福岡
    • Year and Date
      2014-12-08 – 2014-12-10
    • Related Report
      2014 Annual Research Report
  • [Presentation] Effect of Synthesis Conditions on the Porosity, Microtexture, and Surface Chemistry of Nitrogen-doped Carbonized Wood2014

    • Author(s)
      Toshimitsu Hata, Yoshiharu Uchimoto, Roland Benoit, Sylvie Bonnamy, Paul Bronsveld
    • Organizer
      CARBON2014
    • Place of Presentation
      Korea
    • Year and Date
      2014-06-29 – 2014-07-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] 窒素ドープ木質系炭素化物の合成条件が細孔構造に与える影響2014

    • Author(s)
      畑 俊充, 内本 善晴, R.Benoit, S.Bonnamy, P.Bronsveld
    • Organizer
      第64回日本木材学会大会
    • Place of Presentation
      愛媛県, 松山市
    • Related Report
      2013 Research-status Report
  • [Presentation] セルロースからの白金代替燃料電池用カソード触媒合成条件の最適化2013

    • Author(s)
      畑 俊充, 本間千晶, 内本喜晴
    • Organizer
      第11回木質炭化学会発表会
    • Place of Presentation
      新潟市
    • Related Report
      2013 Research-status Report
  • [Presentation] Structural analysis of nitrogen contained in carbonized cellulose used as catalalytic cathode in fuel cells2013

    • Author(s)
      T. Hata, R. Asakura, Y. Uchimoto., R. Benoit, S. Bonnamy, P. Bronsveld
    • Organizer
      The annual World Conference on Carbon
    • Place of Presentation
      Rio de Janeiro, Brazil
    • Related Report
      2013 Research-status Report
  • [Presentation] Structural analysis of nitrogen contained carbonized cellulose used as catalytic cathode in fuel cells by electron energy loss spectroscopy2013

    • Author(s)
      Toshimitsu Hata, Ryohei Asakura, Yoshiharu Uchimoto, Roland Benoit, Sylvie Bonnamy
    • Organizer
      WOODCHEM 2013
    • Place of Presentation
      Porto, Portugal
    • Related Report
      2013 Research-status Report
  • [Presentation] 窒素ドープセルロース炭素化物の構造解析と熱分解-GCMSによる加熱発生ガス分析2013

    • Author(s)
      畑 俊充, 本間千晶, 内本喜晴
    • Organizer
      第40回炭素材料学会年会
    • Place of Presentation
      京都市
    • Related Report
      2013 Research-status Report
  • [Presentation] セルロースとメラミンを原料とした窒素含有炭素化物の構造解析2013

    • Author(s)
      畑 俊充、朝倉 良平、内本 喜晴、Roland Benoit、Sylvie Bonnamy、Paul Bronsveld
    • Organizer
      第63回日本木材学会大会
    • Place of Presentation
      岩手県、盛岡市
    • Related Report
      2012 Research-status Report
  • [Presentation] Characterization of carbonized cellulose as catalytic cathode in fuel cells2012

    • Author(s)
      T.Hata, R.Asakura, Y.Uchimoto, R.Benoit, S.Bonnamy, P.Bronsveld
    • Organizer
      Order/Disorder in Bulk Carbon Materials: Structure/texture,quantification,imaging,modeling,structure--‐propertyrelationships
    • Place of Presentation
      Krakow, Poland
    • Related Report
      2012 Research-status Report
  • [Presentation] Activation of Carbonized Cellulose for Improvement of Oxygen Reduction Reaction Activity of Catalytic Cathode in Fuel Cells2012

    • Author(s)
      T. Hata, R. Asakura, Y. Uchimoto., R. Benoit, S. Bonnamy, P. Bronsveld
    • Organizer
      Carbon2012
    • Place of Presentation
      Krakow, Poland
    • Related Report
      2012 Research-status Report
  • [Presentation] 原子状酸素照射による木質炭素化物1Si焼結体表面における構造変化の解明2012

    • Author(s)
      梶本武志, 畑俊充, 小嶋浩嗣, 田川雅人, 早川基
    • Organizer
      第10回木質炭化学会発表会
    • Place of Presentation
      岩手県、盛岡市
    • Related Report
      2012 Research-status Report
  • [Presentation] 木質熱処理物の化学構造および金属イオン処理における錯体の形成2012

    • Author(s)
      本間千晶, 畑俊充
    • Organizer
      第10回木質炭化学会発表会
    • Place of Presentation
      岩手県、盛岡市
    • Related Report
      2012 Research-status Report
  • [Presentation] 木質からの白金代替燃料電池用カソード触媒合成条件のPy-GC∠MSによる最適化2012

    • Author(s)
      畑俊充, 朝倉良平, 内本喜晴, 本間千晶
    • Organizer
      第10回木質炭化学会発表会
    • Place of Presentation
      岩手県、盛岡市
    • Related Report
      2012 Research-status Report
  • [Presentation] Synthesis and characterization of carbonized cellulose for eco fuel cells2012

    • Author(s)
      T. Hata, R. Asakura, Y. Uchimoto., R. Benoit, S. Bonnamy, P. Bronsveld
    • Organizer
      Ecowood 2012
    • Place of Presentation
      Porto, Portogal
    • Related Report
      2012 Research-status Report
  • [Presentation] セルロースとメラミンを原料とした窒素含有炭素化物の合成2012

    • Author(s)
      畑, 朝倉, 内本, R. Benoit, S. Bonnamy, P. Bronsveld
    • Organizer
      第39回炭素材料学会年会
    • Place of Presentation
      長野県、長野市
    • Related Report
      2012 Research-status Report
  • [Presentation] ヒドロキシエチルセルロース由来微粒子状炭素の調製2012

    • Author(s)
      島田 武, 木島正志, 畑 俊充
    • Organizer
      第39回炭素材料学会年会
    • Place of Presentation
      長野県、長野市
    • Related Report
      2012 Research-status Report
  • [Book] Resistance of Silicon-Containing Carbonized Lignin to Atomic Oxygen Erosion. Protection of Materials and Structures From the Space Environment; Jacob Kleiman, et al2013

    • Author(s)
      T.Kajimoto, T.Hata, M.Tagawa, H.Kojima, and H.Hayakawa
    • Total Pages
      617
    • Publisher
      Springer
    • Related Report
      2012 Research-status Report
  • [Book] 2-3-B08 炭, 持続型生存基盤論ハンドブック第6巻2012

    • Author(s)
      畑 俊充
    • Total Pages
      534
    • Publisher
      京都大学学術出版会
    • Related Report
      2012 Research-status Report
  • [Remarks] ミッション研究室-研究内容

    • URL

      http://www.rish.kyoto-u.ac.jp/L/hata/naiyo.html

    • Related Report
      2014 Annual Research Report
  • [Remarks] ミッション研究室

    • URL

      http://www.rish.kyoto-u.ac.jp/L/hata/index.html

    • Related Report
      2013 Research-status Report
  • [Remarks] ミッション研究室

    • URL

      http://www.rish.kyoto-u.ac.jp/L/hata/naiyo.html

    • Related Report
      2012 Research-status Report

URL: 

Published: 2013-05-31   Modified: 2019-07-29  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi