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Research on ultrashort-wavelength vacuum ultraviolet generation by using stimulated Raman scattering

Research Project

Project/Area Number 24656048
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeSingle-year Grants
Research Field Applied optics/Quantum optical engineering
Research InstitutionOsaka University

Principal Investigator

YOSHIMURA Masashi  大阪大学, 工学(系)研究科(研究院), 准教授 (60314382)

Co-Investigator(Kenkyū-buntansha) MORI Yusuke  大阪大学, 大学院工学研究科, 教授 (90252618)
Project Period (FY) 2012-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2013: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2012: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Keywordsセシウム・リチウム・ボレート / 非線形光学 / 真空紫外光 / 波長変換 / 誘導ラマン散乱 / アンチストークス光 / 応用光学・量子工学 / 光源技術 / 先端機能デバイス / 量子エレクトロニクス
Research Abstract

We have improved laser-induced damage tolerance of CsLiB6O10 (CLBO), and attempted to construct vacuum-ultraviolet (VUV) laser source below 190 nm as a new pump source of anti-Stokes (AS) stimulated Raman scattering (SRS). By using an Nd:YAG laser, the fifth harmonic and infrared (IR) OPO at 1697.9 nm were generated via several frequency conversion stages. At the final stage, VUV light below 190 nm was generated by sum-frequency generation with the fifth-harmonic and IR in a CLBO. A 189 nm output was produced with a conversion efficiency of 7.3% from the 213 nm input. Based on the experimental result, we have newly designed VUV laser system at 185 nm using a 20-W Nd:YAG laser with high-peak power density. Although we are currently constructing the final stage in the system, we estimate the average power over 100 mW at 185 nm and expect ultrashort-wavelength VUV radiation by SRS in H2 such as 1st, 3rd, and 8th AS lines at 172, 150, and 115 nm.

Report

(3 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • Research Products

    (51 results)

All 2014 2013 2012 Other

All Journal Article (9 results) (of which Peer Reviewed: 9 results) Presentation (40 results) (of which Invited: 5 results) Book (2 results)

  • [Journal Article] Sub-180 nm generation with borate crystal2014

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Journal Title

      Optical Materials

      Volume: (In Press) Issue: 12 Pages: 1970-1972

    • DOI

      10.1016/j.optmat.2014.01.021

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Ultraviolet laser-induced degradation of CsLiB_6O_<10> andβ-BaB_2O_42014

    • Author(s)
      K. Takachiho, M. Yoshimura, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Journal Title

      Optical Materials Express

      Volume: Vol.4, Issue 3 Pages: 559-567

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Ultraviolet laser-induced degradation of CsLiB6O10 and β-BaB2O42014

    • Author(s)
      K. Takachiho et al.
    • Journal Title

      Optical Materials Express

      Volume: Vol.4, Issue3 Issue: 3 Pages: 559-567

    • DOI

      10.1364/ome.4.000559

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 不純物・欠陥制御を用いた非線形光学結晶CsLiB_6O_<10>の紫外レーザー損傷耐性向上2013

    • Author(s)
      高千穂慧, 吉村政志, 増田一稀, 高橋義, 今出完, 佐々木孝友, 森勇介
    • Journal Title

      レーザー研究

      Volume: Vol.41, No.10 Pages: 830-834

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Al doping of CsLiB_6O_<10> for high resistance to ultraviolet-induced degradation2013

    • Author(s)
      K. Takachiho, M. Yoshimura, Y. Fukushima, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Journal Title

      Applied Physics Express

      Volume: Vol.6, No.2

    • NAID

      10031152690

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] 不純物・欠陥制御を用いた非線形光学結晶CsLiB6O10の紫外レーザー損傷耐性向上2013

    • Author(s)
      高千穂 慧 他
    • Journal Title

      レーザー研究

      Volume: Vol.41, No.10 Pages: 830-834

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Al Doping of CsLiB6O10 for High Resistance to Ultraviolet-Induced Degradation2013

    • Author(s)
      K. Takachiho, M. Yoshimura, Y. Fukushima, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Journal Title

      Applied Physics Express

      Volume: 6 Issue: 2 Pages: 022701-022701

    • DOI

      10.7567/apex.6.022701

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Phase-matching properties at around 190 nm of various borate crystals2012

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, K. Zhang, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Journal Title

      Applied Physics Express

      Volume: Vol.5, No.6

    • NAID

      10030769833

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Phase-Matching Properties at around 190nm of Various Borate Crystals2012

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, K. Zhang, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Journal Title

      Applied Physics Express

      Volume: 5 Issue: 6 Pages: 062601-062601

    • DOI

      10.1143/apex.5.062601

    • NAID

      10030769833

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] 非線形光学結晶CLBO, BBOの紫外光誘起経時劣化特性2014

    • Author(s)
      高千穂慧, 吉村政志, 高橋義典, 今出完, 佐々木孝友, 森勇介
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学相模原キャンパ
    • Year and Date
      2014-03-18
    • Related Report
      2013 Final Research Report
  • [Presentation] 波長変換結晶CLBO, BBOの紫外光誘起経時劣化特性2014

    • Author(s)
      高千穂慧, 高橋義典, 今出完, 吉村政志, 佐々木孝友, 森勇介
    • Organizer
      レーザー学会学術講演会第34回年次大会
    • Place of Presentation
      北九州国際会議
    • Year and Date
      2014-01-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Recent progress in nonlinear optical crystal CsLiB_6O_<10>2014

    • Author(s)
      Y. Mori, M. Yoshimura, T. Sasaki, and Y. Takahashi
    • Organizer
      International Symposium on Nanophotonics and Nanomaterials 2014 (ISONP2014)
    • Place of Presentation
      Beijing, China
    • Year and Date
      2014-01-16
    • Related Report
      2013 Final Research Report
  • [Presentation] Improvement of UV laser-induced degradation resistance of CsLiB_6O_<10>2013

    • Author(s)
      K. Masuda, M. Yoshimura, K. Takachiho, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      The 6th International Symposium on Lasers Scintillators and Non-Linear Optical Materials (ISLNOM-6)
    • Place of Presentation
      Shanghai, China
    • Year and Date
      2013-10-22
    • Related Report
      2013 Final Research Report
  • [Presentation] VUV generation below 200 nm with borate crystals2013

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      The 6th International Symposium on Lasers Scintillators and Non-Linear Optical Materials (ISLNOM-6)
    • Place of Presentation
      Shanghai, China
    • Year and Date
      2013-10-22
    • Related Report
      2013 Final Research Report
  • [Presentation] Recent progress in nonlinear optical crystal CsLiB_6O_<10>2013

    • Author(s)
      Y. Mori, M. Yoshimura, T. Sasaki, Y. Takahashi
    • Organizer
      The 6th International Symposium on Lasers Scintillators and Non-Linear Optical Materials (ISLNOM-6)
    • Place of Presentation
      Shanghai, China
    • Year and Date
      2013-10-21
    • Related Report
      2013 Final Research Report
  • [Presentation] VUV Light Generation with CsLiB6O10 and LiB_3O_52013

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      JSAP-OSA Joint Symposia 2013
    • Place of Presentation
      Doshisha University
    • Year and Date
      2013-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] The correlation between optical properties and electrical properties of CsLiB_6O_<10> crystal2013

    • Author(s)
      Z. Lu, M. Yoshimura, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      JSAP-OSA Joint Symposia 2013
    • Place of Presentation
      Doshisha University
    • Year and Date
      2013-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] The correlation of point defects and UV induced degradation of CsLiB_6O_<10>2013

    • Author(s)
      K. Masuda, M. Yoshimura, K. Takachiho, Y. Takahashi, M. Imade, T. Sasaki and Y. Mori
    • Organizer
      JSAP-OSA Joint Symposia 2013
    • Place of Presentation
      Doshisha University
    • Year and Date
      2013-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Impurity control of CsLiB_6O_<10> for improving UV-induced damage tolerance2013

    • Author(s)
      K. Takachiho, M. Yoshimura, K. Masuda, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      17th International Conference on Crystal Growth and Epitaxy - ICCGE-17
    • Place of Presentation
      Warsaw, Poland
    • Year and Date
      2013-08-15
    • Related Report
      2013 Final Research Report
  • [Presentation] 波長変換結晶CLBO, BBOの266nm紫外光損傷に関する研究2013

    • Author(s)
      吉村政志, 高千穂慧, 増田一稀, 高橋義典, 佐々木孝友, 森勇介
    • Organizer
      レーザー学会第445回研究会「高機能固体レーザーとその応用」
    • Place of Presentation
      大阪
    • Year and Date
      2013-07-16
    • Related Report
      2013 Final Research Report
  • [Presentation] 179 nm generation with borate crystal2013

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      The 10th Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR&OECC/PS) 2013
    • Place of Presentation
      Kyoto, Japan
    • Year and Date
      2013-07-06
    • Related Report
      2013 Final Research Report
  • [Presentation] UV laser-induced degradation in CsLiB_6O_<10>2013

    • Author(s)
      K. Takachiho, M. Yoshimura, K. Masuda, Y. Takahashi, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      The 10th Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR&OECC/PS) 2013
    • Place of Presentation
      Kyoto, Japan
    • Year and Date
      2013-07-03
    • Related Report
      2013 Final Research Report
  • [Presentation] Ultraviolet laser-induced degradation in CsLiB_6O_<10>2013

    • Author(s)
      M. Yoshimura, K. Takachiho, Y. Takahashi, T. Sasaki, and Y. Mori
    • Organizer
      The 2nd Advance Lasers and Photon Sources (ALPS'13)
    • Place of Presentation
      Yokohama, Kanagawa
    • Year and Date
      2013-04-25
    • Related Report
      2013 Final Research Report
  • [Presentation] VUV light generation with borate crystals2013

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      The 2nd Advance Lasers and Photon Sources (ALPS'13)
    • Place of Presentation
      Yokohama, Kanagawa
    • Year and Date
      2013-04-24
    • Related Report
      2013 Final Research Report
  • [Presentation] 非線形光学結晶CLBOの不純物制御と紫外光発生応用2013

    • Author(s)
      吉村政志, 高橋義典, 佐々木孝友, 森勇介
    • Organizer
      レーザー学会学術講演会第33回年次大会
    • Place of Presentation
      姫路商工会議所, 兵庫
    • Year and Date
      2013-01-28
    • Related Report
      2013 Final Research Report
  • [Presentation] 非線形光学結晶CLBOの不純物制御と紫外光発生応用2013

    • Author(s)
      吉村政志, 高橋義典, 佐々木孝友, 森勇介
    • Organizer
      レーザー学会学術講演会第33回年次大会
    • Place of Presentation
      姫路, 兵庫
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Development of CsLiB_6O_<10> for vacuum-UV light generation2012

    • Author(s)
      M. Yoshimura, Y. Takahashi, T. Sasaki, and Y. Mori
    • Organizer
      The Third China-Japan Crystal Growth and Technology Symposium
    • Place of Presentation
      Hefei, China
    • Year and Date
      2012-10-20
    • Related Report
      2013 Final Research Report
  • [Presentation] ボレート系結晶を用いた深紫外・真空紫外光発生2012

    • Author(s)
      吉村政志, 森勇介, 佐々木孝友
    • Organizer
      日本結晶成長学会バルク成長分科会第85回研究会
    • Place of Presentation
      大阪
    • Year and Date
      2012-05-25
    • Related Report
      2013 Final Research Report
  • [Presentation] 189-nm wavelength generation with borate crystals2012

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      Conference on Laser and Electro-Optics 2012 (CLEO2012)
    • Place of Presentation
      San Jose, USA
    • Year and Date
      2012-05-11
    • Related Report
      2013 Final Research Report
  • [Presentation] Al-doping in CsLiB_6O_<10> for high resistance against UV laser-induced damage2012

    • Author(s)
      K. Takachiho, M. Yoshimura, Y. Fukushima, Z. Lu, Y. Takahashi, T. Sasaki, and Y. Mori
    • Organizer
      Conference on Laser and Electro-Optics 2012 (CLEO2012)
    • Place of Presentation
      San Jose, USA
    • Year and Date
      2012-05-10
    • Related Report
      2013 Final Research Report
  • [Presentation] Development of CsLiB6O10 for Vacuum-UV Light Generation2012

    • Author(s)
      M. Yoshimura, Y. Takahashi, T. Sasaki, and Y. Mori
    • Organizer
      The Third China-Japan Crystal Growth and Technology Symposium
    • Place of Presentation
      Hefei, China
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] 189-nm Wavelength Generation with Borate Crystals2012

    • Author(s)
      C. Qu, M. Yoshimura, J. Tsunoda, Y. Kaneda, M. Imade, T. Sasaki, and Y. Mori
    • Organizer
      Conference on Laser and electro-Optics 2012 (CLEO2012)
    • Place of Presentation
      San Jose, USA
    • Related Report
      2012 Research-status Report
  • [Presentation] Al-doping in CsLiB6O10 for high resistance against UV laser-induced damage2012

    • Author(s)
      K. Takachiho, M. Yoshimura, Y. Fukushima, Z. Lu, Y. Takahashi, T. Sasaki, and Y. Mori
    • Organizer
      Conference on Laser and electro-Optics 2012 (CLEO2012)
    • Place of Presentation
      San Jose, USA
    • Related Report
      2012 Research-status Report
  • [Presentation] VUV light generation with borate crystals

    • Author(s)
      C. Qu et al.
    • Organizer
      The 2nd Advance Lasers and Photon Sources (ALPS’13)
    • Place of Presentation
      Yokohama, Kanagawa
    • Related Report
      2013 Annual Research Report
  • [Presentation] Ultraviolet laser-induced degradation in CsLiB6O10

    • Author(s)
      M. Yoshimura et al.
    • Organizer
      The 2nd Advance Lasers and Photon Sources (ALPS’13)
    • Place of Presentation
      Yokohama, Kanagawa
    • Related Report
      2013 Annual Research Report
  • [Presentation] 179 nm generation with borate crystal

    • Author(s)
      C. Qu et al.
    • Organizer
      The 10th Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR & OECC/PS) 2013
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] UV laser-induced degradation in CsLiB6O10

    • Author(s)
      K. Takachiho et al.
    • Organizer
      The 10th Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR & OECC/PS) 2013
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] 波長変換結晶CLBO, BBO の266nm紫外光損傷に関する研究

    • Author(s)
      吉村 政志 他
    • Organizer
      レーザー学会第445回研究会「高機能固体レーザーとその応用」
    • Place of Presentation
      大阪
    • Related Report
      2013 Annual Research Report
  • [Presentation] Impurity control of CsLiB6O10 for improving UV-induced damage tolerance

    • Author(s)
      K. Takachiho et al.
    • Organizer
      17th International Conference on Crystal Growth and Epitaxy (ICCGE-17)
    • Place of Presentation
      Warsaw, Poland
    • Related Report
      2013 Annual Research Report
  • [Presentation] The correlation of point defects and UV induced degradation of CsLiB6O10

    • Author(s)
      K. Masuda et al.
    • Organizer
      JSAP-OSA Joint Symposia 2013
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] The correlation between optical properties and electrical properties of CsLiB6O10 crystal

    • Author(s)
      Z. Lu et al.
    • Organizer
      JSAP-OSA Joint Symposia 2013
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] VUV light generation with CLB6O10 and LiB3O5

    • Author(s)
      C. Qu et al.
    • Organizer
      JSAP-OSA Joint Symposia 2013
    • Place of Presentation
      Kyoto, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Recent Progress in Nonlinear Optical Crystal CsLiB6O10

    • Author(s)
      Y. Mori et al.
    • Organizer
      The 6th International Symposium on Lasers, Scintillators and Non-Linear Optical Materials (ISLNOM-6)
    • Place of Presentation
      Shanghai, China
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] VUV generation below 200 nm with borate crystals

    • Author(s)
      C. Qu et al.
    • Organizer
      The 6th International Symposium on Lasers, Scintillators and Non-Linear Optical Materials (ISLNOM-6)
    • Place of Presentation
      Shanghai, China
    • Related Report
      2013 Annual Research Report
  • [Presentation] Improvement of UV laser-induced degradation resistance of CsLiB6O10

    • Author(s)
      K. Masuda et al.
    • Organizer
      The 6th International Symposium on Lasers, Scintillators and Non-Linear Optical Materials (ISLNOM-6)
    • Place of Presentation
      Shanghai, China
    • Related Report
      2013 Annual Research Report
  • [Presentation] Recent Progress in Nonlinear Optical Crystal CsLiB6O10

    • Author(s)
      Y. Mori et al.
    • Organizer
      International Symposium on Nanophotonics and Nanomaterials 2014 (ISONP2014)
    • Place of Presentation
      Beijing, China
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 波長変換結晶CLBO, BBOの紫外光誘起経時劣化特性

    • Author(s)
      高千穂 慧 他
    • Organizer
      レーザー学会学術講演会第34回年次大会
    • Place of Presentation
      北九州国際会議場, 福岡
    • Related Report
      2013 Annual Research Report
  • [Presentation] 非線形光学結晶CLBO,BBOの紫外光誘起経時劣化特性

    • Author(s)
      高千穂 慧 他
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学相模原キャンパス, 神奈川
    • Related Report
      2013 Annual Research Report
  • [Presentation] ボレート結晶を用いた深紫外・真空紫外光発生

    • Author(s)
      吉村政志、森勇介、佐々木孝友
    • Organizer
      日本結晶成長学会バルク成長分科会第85回研究会
    • Place of Presentation
      大阪, 大阪
    • Related Report
      2012 Research-status Report
    • Invited
  • [Book] Nonlinear Optical Borate Crystals2012

    • Author(s)
      M. Yoshimura, T. Sasaki, and Y. Mori
    • Publisher
      Wiley-VCH
    • Related Report
      2013 Final Research Report
  • [Book] Nonlinear Optical Borate Crystals, Ch.3.2.3 CsLiB6O10 (pp.161-178)2012

    • Author(s)
      M. Yoshimura et al.
    • Total Pages
      387
    • Publisher
      Wiley-VCG
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2019-07-29  

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