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Development of clean coal technology by using the feature of oxy-fuel combustion

Research Project

Project/Area Number 24686027
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypePartial Multi-year Fund
Research Field Thermal engineering
Research InstitutionTokyo Institute of Technology

Principal Investigator

Watanabe Hirotatsu  東京工業大学, 工学院, 助教 (40551825)

Project Period (FY) 2012-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥16,380,000 (Direct Cost: ¥12,600,000、Indirect Cost: ¥3,780,000)
Fiscal Year 2015: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2014: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2013: ¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2012: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
KeywordsCO2回収型燃焼 / 石炭 / 二酸化炭素 / クリーンコールテクノロジー / O2/CO2/H2O燃焼 / O2/CO2燃焼 / O_2/CO_2燃焼
Outline of Final Research Achievements

Oxy-fuel combustion technology is an emerging approach to capture post combustion CO2. In this technique, fuel is burned using a mixture of high-purity oxygen and recycled flue gas. In this study, clean coal technologies using the feature of oxy-fuel combustion were developed. It was shown that O2/CO2 environments were suited to reduce soot due to the CO2 reactivity (CO2 + H → CO + OH). Moreover, Char gasification in mixtures of O2 and CO2 was also discussed. A sufficient active site, mainly consisting of catalyst in this study, was important not only to enhance char gasification reactions but also to prevent competitive reactions between char-O2 and CO2 gasification.

Report

(6 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Annual Research Report
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • Research Products

    (42 results)

All 2017 2016 2015 2014 2013 2012 Other

All Int'l Joint Research (2 results) Journal Article (11 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 8 results,  Open Access: 3 results,  Acknowledgement Compliant: 5 results) Presentation (24 results) Remarks (5 results)

  • [Int'l Joint Research] Massachusetts Institute of Technology(米国)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] Massachusetts Institute of Technology(米国)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] On the characteristic flow and flame times for scaling oxy and air flame stabilization modes in premixed swirl combustion2017

    • Author(s)
      Soufien Taamallah, Nadim W Chakroun, Hirotatsu Watanabe, Santosh J. Shanbhogue, Ahmed F. Ghoniem
    • Journal Title

      Proceedings of the Combustio Institute

      Volume: 36 Issue: 3 Pages: 3799-3807

    • DOI

      10.1016/j.proci.2016.07.022

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] The structure of swirl-stabilized turbulent premixed CH4/air and CH4/O2/CO2 flames and mechanisms of intense burning of oxy-flames2016

    • Author(s)
      Hirotatsu Watanabe, Santosh J. Shanbhogue, Soufien Taamallah, Nadim W. Chakroun, Ahmed F. Ghoniem
    • Journal Title

      Combustion and Flame

      Volume: 174 Pages: 111-119

    • DOI

      10.1016/j.combustflame.2016.09.015

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Effect of minerals on surface morphologies and competitive reactions during char gasification in mixtures of O2 and CO22015

    • Author(s)
      Hirotatsu Watanabe, Ken Okazaki
    • Journal Title

      Proceedings of the Combustion Institute

      Volume: 35 Issue: 2 Pages: 2363-2371

    • DOI

      10.1016/j.proci.2014.06.119

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Carbonate formation during lignin pyrolysis under CO2 and its effect on char oxidation2015

    • Author(s)
      Hirotatsu Watanabe, Kiyomi Shimomura, Ken Okazaki
    • Journal Title

      Proceedings of the Combustion Institute

      Volume: 35 Issue: 2 Pages: 2423-2430

    • DOI

      10.1016/j.proci.2014.06.014

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Oxy-fuel combustionとクリーンコールテクノロジー2015

    • Author(s)
      渡部弘達, 岡崎健
    • Journal Title

      日本燃焼学会誌

      Volume: 57 Pages: 8-15

    • Related Report
      2014 Annual Research Report
    • Acknowledgement Compliant
  • [Journal Article] Experimental Investigation of Carbonate Formation Characteristics during Coal and Biomass Pyrolysis under CO22014

    • Author(s)
      Hirotatsu Watanabe, Kiyomi Shimomura, Ken Okazaki
    • Journal Title

      Energy and Fuels

      Volume: 28 Issue: 7 Pages: 4795-4800

    • DOI

      10.1021/ef500832t

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Oxy-fuel combustionと石炭火力2014

    • Author(s)
      渡部弘達, 岡崎健
    • Journal Title

      日本ガスタービン学会誌

      Volume: 42 Pages: 297-302

    • Related Report
      2014 Annual Research Report
    • Acknowledgement Compliant
  • [Journal Article] Experimental and Kinetic Studies of Chemical Role of CO<sub>2</sub> in Hydrocarbon Oxidation during Fuel-Rich O<sub>2</sub>/CO<sub>2</sub> Combustion2013

    • Author(s)
      Hirotatsu Watanabe, Dejudom Kiatpanachart, Ken Okazaki
    • Journal Title

      Journal of Thermal Science and Technology

      Volume: 8 Issue: 3 Pages: 504-516

    • DOI

      10.1299/jtst.8.504

    • NAID

      130004699329

    • ISSN
      1880-5566
    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Role of CO2 in the CH4 oxidation and H2 formation during fuel-rich combustion in O2/CO2 environments2013

    • Author(s)
      Hirotatsu Watanabe, Fumiya Arai, Ken Okazaki
    • Journal Title

      Combustion and Flame

      Volume: 160 Issue: 11 Pages: 2375-2385

    • DOI

      10.1016/j.combustflame.2013.05.022

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] O2/CO2燃焼における Fuel-NO および Recycled-NO の還元メカニズム(CO2の反応性の影響解明)2013

    • Author(s)
      渡部弘達,Dejudom Kiatpanachart, Ken Okazaki
    • Journal Title

      日本機械学会論文集B編

      Volume: 79 Pages: 1703-1713

    • NAID

      130003374894

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] CO2の反応性を活用したOxy-fuel combustion (O2/CO2 combustion)の高度化2013

    • Author(s)
      渡部弘達
    • Journal Title

      日本機械学会熱工学部門ニュースレター

      Volume: 69 Pages: 8-12

    • Related Report
      2013 Annual Research Report
  • [Presentation] O2/CO2/H2O雰囲気における炭化水素の反応メカニズム2016

    • Author(s)
      渡部弘達,米野孝
    • Organizer
      第54回燃焼シンポジウム
    • Place of Presentation
      仙台国際センター(仙台)
    • Year and Date
      2016-11-23
    • Related Report
      2016 Annual Research Report
  • [Presentation] The structures of premixed CH4/air and CH4/O2/CO2 flames in swirl stabilized combustor2015

    • Author(s)
      Hirotatsu Watanabe, Santosh J. Shanbhogue, Soufien Taamallah, Ahmed F. Ghoniem
    • Organizer
      第53回燃焼シンポジウム
    • Place of Presentation
      つくば国際会議場(つくば)
    • Year and Date
      2015-11-16
    • Related Report
      2015 Annual Research Report
  • [Presentation] CO2の反応性を活用したO2/CO2燃焼における未燃炭化水素の排出抑制2014

    • Author(s)
      菅井俊輔, 渡部 弘達, 岡崎健
    • Organizer
      第52回燃焼シンポジウム
    • Place of Presentation
      岡山コンベンションセンター(岡山県岡山市)
    • Year and Date
      2014-12-03 – 2014-12-05
    • Related Report
      2014 Annual Research Report
  • [Presentation] Hydrocarbon formation and oxidation characteristics in CH4 flat flame doped with toluene under air and O2/CO2 environments2014

    • Author(s)
      Shunsuke Sugai, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      The 25th International Symposium on Transport Phenomena
    • Place of Presentation
      Aonang Villa Resort, Krabi, Thailand
    • Year and Date
      2014-11-05 – 2014-11-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] ROLE OF CO2 IN THE SOOT FORMATION AND REDUCTION MECHANISMS IN CH4 FLAT FLAME DOPED WITH TOLUENE UNDER O2/CO2 ENVIRONMENTS2014

    • Author(s)
      Hirotatsu Watanabe, Shunsuke Sugai, Ken Okazaki
    • Organizer
      15th International Heat Transfer Conference
    • Place of Presentation
      Kyoto International Conference Center, Kyoto, Japan
    • Year and Date
      2014-08-10 – 2014-08-15
    • Related Report
      2014 Annual Research Report
  • [Presentation] A role of CO2 in volatile matter reaction and soot formation in oxy-fuel combustion2013

    • Author(s)
      Shunsuke Sugai, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      International Symposium on EcoTopia Science 2013
    • Place of Presentation
      Nagoya University (Nagoya)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Char Gasification Behavior Focusing on Surface Morphology Change during O2/CO2 Gasification2013

    • Author(s)
      Kei Yoshikawa, Kiyomi Shimomura, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      International Symposium on EcoTopia Science 2013
    • Place of Presentation
      Nagoya University (Nagoya)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Effect of CO2 during Solid Fuel pyrolysis in oxy-fuel combustion2013

    • Author(s)
      Kiyomi Shimomura, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      International Symposium on EcoTopia Science 2013
    • Place of Presentation
      Nagoya University (Nagoya)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Clarification of gasification behavior of solid fuel char prepared under CO2 atmosphere2013

    • Author(s)
      Kiyomi Shimomura, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      3rd Oxyfuel Combustion Conference
    • Place of Presentation
      Templar castle (Ponferrada, Spain)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Coal Char Gasification in O2/Ar, Ar/CO2 and O2/CO2 Environments2013

    • Author(s)
      Hirotatsu Watanabe, Li Xiaofan, Ken Okazaki
    • Organizer
      3rd Oxyfuel Combustion Conference
    • Place of Presentation
      Templar castle (Ponferrada, Spain)
    • Related Report
      2013 Annual Research Report
  • [Presentation] CO2回収型石炭燃焼におけるすすの生成特性2013

    • Author(s)
      菅井俊輔,渡部弘達,岡崎健
    • Organizer
      第51回燃焼シンポジウム
    • Place of Presentation
      大田区産業プラザPio(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] CO2 雰囲気下で生成される固体燃料のチャーガス化特性 - 灰組成の影響解明 -2013

    • Author(s)
      下村聖実,渡部弘達,岡崎健
    • Organizer
      第51回燃焼シンポジウム
    • Place of Presentation
      大田区産業プラザPio(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] CO2と灰分の反応に着目した固体燃料の熱分解およびガス化プロセスの解明2013

    • Author(s)
      渡部弘達,下村聖実,岡崎健
    • Organizer
      第50回石炭科学会議
    • Place of Presentation
      九州大学(福岡市)
    • Related Report
      2013 Annual Research Report
  • [Presentation] O2/CO2燃焼のすす生成メカニズムにおけるCO2の反応性の影響2013

    • Author(s)
      渡部弘達,菅井俊輔,岡崎健
    • Organizer
      日本機械学会熱工学コンファレンス2013
    • Place of Presentation
      弘前大学(弘前市)
    • Related Report
      2013 Annual Research Report
  • [Presentation] O2/CO2雰囲気におけるチャーのガス化挙動と表面形状変化の特異性2013

    • Author(s)
      渡部弘達,吉川恵,岡崎健
    • Organizer
      第22回日本エネルギー学会大会
    • Place of Presentation
      工学院大学(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] CO2回収型石炭燃焼における揮発分の反応メカニズムの解明2013

    • Author(s)
      菅井俊輔,Dejudom Kiatpanachart, 渡部弘達,岡崎健
    • Organizer
      第50回日本伝熱シンポジウム
    • Place of Presentation
      ウェスティンホテル仙台(仙台市)
    • Related Report
      2013 Annual Research Report
  • [Presentation] O2/CO2雰囲気におけるFuel-NOの生成およびRecycled-NOの還元メカニズム2013

    • Author(s)
      渡部弘達,Dejudom Kiatpanachart, 岡崎健
    • Organizer
      第50回日本伝熱シンポジウム
    • Place of Presentation
      ウェスティンホテル仙台(仙台市)
    • Related Report
      2013 Annual Research Report
  • [Presentation] An experimental and kinetic modeling study of CH4 decomposition in air and O2/CO2 fuel-rich combustion2013

    • Author(s)
      Hirotatsu Watanabe, Dejudom Kiatpanachart, Ken Okazaki
    • Organizer
      The 9th Asia-Pacific Conference on Combustion
    • Place of Presentation
      Gyeongju Hilton Hotel(Gyeongju, Korea)
    • Related Report
      2013 Annual Research Report
  • [Presentation] O_2/CO_2雰囲気におけるチャーの細孔発達挙動の解明2012

    • Author(s)
      渡部弘達, Li Xiaofan, 下村聖実, 岡崎健
    • Organizer
      第50回燃焼シンポジウム
    • Place of Presentation
      愛知県産業労働センターウインクあいち(愛知県)
    • Year and Date
      2012-12-07
    • Related Report
      2012 Annual Research Report
  • [Presentation] 燃料過濃条件下の0_2/C0_2石炭燃焼における炭化水素分解メカニズム2012

    • Author(s)
      Kiatpanachart Dejudom, 菅井俊輔, 渡部弘達, 岡崎健
    • Organizer
      第50回燃焼シンポジウム
    • Place of Presentation
      愛知県産業労働センターウインクあいち(愛知県)
    • Year and Date
      2012-12-06
    • Related Report
      2012 Annual Research Report
  • [Presentation] C0_2雰囲気下での熱分解特性に着目したチャーガス化メカニズムの解明2012

    • Author(s)
      下村聖実, 渡部弘達, 岡崎健
    • Organizer
      第50回燃焼シンポジウム
    • Place of Presentation
      愛知県産業労働センターウインクあいち(愛知県)
    • Year and Date
      2012-12-05
    • Related Report
      2012 Annual Research Report
  • [Presentation] Effect of fuel-N concentration on NO_x emission during air and O_2/CO_2 coal combustion2012

    • Author(s)
      Dejudom Kiatpanachart, Fumiya Arai, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      The third international forum on heat transfer
    • Place of Presentation
      長崎ブリックホール(長崎)
    • Year and Date
      2012-11-14
    • Related Report
      2012 Annual Research Report
  • [Presentation] Characteristics of volatile reactions and char gasification in O_2/CO_2 coal combustion2012

    • Author(s)
      Li xiaofan. Kumiya Arai, Kiatpanachart Dejudom, Hirotatsu Watanabe, Ken Okazaki
    • Organizer
      化学工学会 第44回秋季大会
    • Place of Presentation
      東北大学 川内北キャンパス(宮城)
    • Year and Date
      2012-09-19
    • Related Report
      2012 Annual Research Report
  • [Presentation] H_2およびCO生成に及ぼすO_2/CO_2ガス化の特異性2012

    • Author(s)
      渡部弘達, Kiatpanachart Dejudom, 荒井郁也, 岡崎健
    • Organizer
      化学工学会 第44回秋季大会
    • Place of Presentation
      東北大学 川内北キャンパス(宮城)
    • Year and Date
      2012-09-19
    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://www.mech.titech.ac.jp/~epl/

    • Related Report
      2016 Annual Research Report
  • [Remarks] http://www.mech.titech.ac.jp/~epl/

    • Related Report
      2015 Annual Research Report
  • [Remarks] 東京工業大学大学院理工学研究科機械制御システム専攻エネルギー事象分野

    • URL

      http://www.mech.titech.ac.jp/~epl

    • Related Report
      2014 Annual Research Report
  • [Remarks] エネルギー事象分野 岡崎研究室

    • URL

      http://www.mech.titech.ac.jp/~epl

    • Related Report
      2013 Annual Research Report
  • [Remarks]

    • URL

      http://www.mech.titcch.ac.jp/~epl

    • Related Report
      2012 Annual Research Report

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Published: 2012-04-24   Modified: 2022-01-27  

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