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Theoretical research on novel quantum states and phenomena induced by magnetic monopoles in pyrochlore materials

Research Project

Project/Area Number 24740253
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Condensed matter physics II
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

Onoda Shigeki  国立研究開発法人理化学研究所, 古崎物性理論研究室, 専任研究員 (70455335)

Project Period (FY) 2012-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2014: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2013: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2012: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywords磁性 / 物性理論 / スピン液体 / スピンアイス / トポロジカル絶縁体 / 量子スピンアイス / 量子スピン液体 / ゲージ場 / イリジウム酸化物
Outline of Final Research Achievements

Novel phases and phenomena induced by emergent fictitious monopoles in pyrochlore oxides have been revealed.
For quantum spin ice systems where the quantum magentism originates from rare-earth magnetic moments, we have provided theoretical evidence of a continuous crossover from a classical spin ice characterized by localized monopoles to a quantum spin liquid showing quantum dynamics of monopoles. Through analyses of extensive experimental results on a basis of a quantum spin ice model, we have uncovered that Yb2Ti2O7 and Tb2Ti2O7 are located in Higgs-confining ordered phases with Bose-condensed monopoles.
Our first-principles calculations have clarified the electronic structures of the paramagnetic semimetal Pr2Ir2O7 and the antiferromagnetic insulator Y2Ir2O7, and shown the conditions of the emergence of Weyl points acting as monopoles in the reciprocal lattice space.

Report

(5 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (51 results)

All 2016 2015 2014 2013 2012 Other

All Int'l Joint Research (3 results) Journal Article (10 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 8 results,  Acknowledgement Compliant: 5 results) Presentation (33 results) (of which Int'l Joint Research: 3 results,  Invited: 19 results) Remarks (5 results)

  • [Int'l Joint Research] NIST/Georgia Regents University(米国)

    • Related Report
      2015 Annual Research Report
  • [Int'l Joint Research] Institute Laue Langevin(France)

    • Related Report
      2015 Annual Research Report
  • [Int'l Joint Research] Chinese Academy of Sciences(China)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Quadrupole Order in the Frustrated Pyrochlore Tb2+xTi2-xO7+y2016

    • Author(s)
      H. Takatsu, S. Onoda, H. Takatsu, S. Kittaka, A. Kasahara, Y. Kono, T. Sakakibara, Y. Kato, B. Fak, J. Ollivier, J. W. Lynn, T. Taniguchi, M. Wakita, H. Kadowaki
    • Journal Title

      Physical Review Letters

      Volume: 未定

    • NAID

      120005848239

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] First-principles study on cubic pyrochlore iridates Y2Ir2O7 and Pr2Ir2O72015

    • Author(s)
      F. Ishii, Y.P. Mizuta, T. Kato, T. Ozaki, H. Weng, and S. Onoda
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 84 Issue: 7 Pages: 073703-073703

    • DOI

      10.7566/jpsj.84.073703

    • NAID

      210000133609

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Numerical evidence of quantum melting of spin ice: quantum-classical crossover2015

    • Author(s)
      Yasuyuki Kato, Shigeki Onoda
    • Journal Title

      Physical Review Letters

      Volume: 115 Issue: 7 Pages: 077202-077202

    • DOI

      10.1103/physrevlett.115.077202

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Static magnetic moments revealed by muon spin relaxation and thermodynamic measurements in the quantum spin ice Yb2Ti2O72014

    • Author(s)
      Lieh-Jeng Chang, Martin R. Lees, Isao Watanabe, Adrian D. Hillier, Yukio Yasui, and Shigeki Onoda,
    • Journal Title

      Physical Review B

      Volume: 89 Issue: 18

    • DOI

      10.1103/physrevb.89.184416

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Symmetry-protected topological phases and transition in a frustrated spin-1/2 XXZ chain2014

    • Author(s)
      Hiroshi Ueda, Shigeki Onoda
    • Journal Title

      Physical Review B

      Volume: 90 Issue: 21 Pages: 2144251-6

    • DOI

      10.1103/physrevb.90.214425

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] 物質中のモノポールとそのダイナミクス2014

    • Author(s)
      小野田繁樹
    • Journal Title

      数理科学

      Volume: 613

    • Related Report
      2013 Research-status Report
  • [Journal Article] Pushing bits through a spin wire2012

    • Author(s)
      Shigeki Onoda
    • Journal Title

      Physics

      Volume: 5 Pages: 53-53

    • DOI

      10.1103/physics.5.53

    • Related Report
      2012 Research-status Report
  • [Journal Article] Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O72012

    • Author(s)
      Lieh-Jeng Chang, Shigeki Onoda, Yixi Su, Ying-Jer Kao, Ku-Ding Tsuei, Yukio Yasui, Kazuhisa Kakurai, Martin Richard Lees
    • Journal Title

      Nature Communications

      Volume: 3 Issue: 1

    • DOI

      10.1038/ncomms1989

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Generic quantum spin ice2012

    • Author(s)
      SungBin Lee, Shigeki Onoda, Leon Balents
    • Journal Title

      Physical Review B

      Volume: 86 Issue: 10

    • DOI

      10.1103/physrevb.86.104412

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Ground-state phase diagram of a spin-1/2 frustrated ferromagnetic XXZ chain: Haldane dimer phase and gapped/gapless chiral phases2012

    • Author(s)
      Shunsuke Furukawa, Masahiro Sato, Shigeki Onoda, and Akira Furusaki
    • Journal Title

      Physical Review B

      Volume: 86 Issue: 9 Pages: 94417-94417

    • DOI

      10.1103/physrevb.86.094417

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] スピネル型Ir酸化物の第一原理計算2016

    • Author(s)
      石井史之、小野田繁樹
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学, 仙台市, 宮城県
    • Year and Date
      2016-03-21
    • Related Report
      2015 Annual Research Report
  • [Presentation] パイロクロア量子スピンアイス系のスピンダイナミクスの理論2016

    • Author(s)
      小野田繁樹, Trinanjan Datta
    • Organizer
      日本物理学会第71回年次大会
    • Place of Presentation
      東北学院大学, 仙台市, 宮城県
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Theory for magnetic excitations in quantum spin ice2016

    • Author(s)
      Shigeki Onoda, Trinanjan Datta
    • Organizer
      American Physical Society March Meeting 2016
    • Place of Presentation
      Baltimore, MD, USA
    • Year and Date
      2016-03-15
    • Related Report
      2015 Annual Research Report
  • [Presentation] Quantum spin ice: current issues and beyond2016

    • Author(s)
      Shigeki Onoda
    • Organizer
      2016 Quantum Materials Symposium
    • Place of Presentation
      Muui Island, Korea
    • Year and Date
      2016-02-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] パイロクロアU(1)量子スピン液体・秩序相における励起:フォトン、量子スピンアイスモノポール、ヒッグスモード2015

    • Author(s)
      小野田 繁樹
    • Organizer
      物性研短期研究会「スピン系物理の深化と最前線」
    • Place of Presentation
      東京大学物性研究所、柏市、千葉県
    • Year and Date
      2015-11-17
    • Related Report
      2015 Annual Research Report
    • Invited
  • [Presentation] Theory for electronic properties of oxide pyrochlores: quantum spin ice and iridates2015

    • Author(s)
      Shigeki Onoda
    • Organizer
      TMU International Symposium on “New Quantum Phases Emerging from Novel Crystal Structure”
    • Place of Presentation
      首都大学東京、八王子市、東京都
    • Year and Date
      2015-09-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] パイロクロア型Ir酸化物における磁気秩序と電子状態の第一原理計算2015

    • Author(s)
      石井史之, 水田耀ピエール, 加藤毅大, 尾崎泰助, Hongming Weng, 小野田繁樹
    • Organizer
      日本物理学会2015年秋季大会
    • Place of Presentation
      関西大学、吹田市、大阪府
    • Year and Date
      2015-09-18
    • Related Report
      2015 Annual Research Report
  • [Presentation] Thermal, transport, and spectral properties of generic quantum spin ice beyond the mean-field theory2015

    • Author(s)
      Shigeki Onoda
    • Organizer
      The 20th International Conference on Magnetism
    • Place of Presentation
      Barcelona, Spain
    • Year and Date
      2015-07-06
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] パイロクロア型Ir酸化物における熱電効果の第一原理計算2015

    • Author(s)
      水田耀ピエール、石井史之、小野田繁樹
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 (東京都新宿区)
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] 量子スピンアイス系Yb2Ti2O7のμSR測定2015

    • Author(s)
      濱地紀彰,安井幸夫,河野洋平,橘高俊一郎,榊原俊郎,L.J.Chang,小野田繁樹,渡邊功雄
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      早稲田大学 (東京都新宿区)
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] Numerical evidence of quantum melting of spin ice: quantum-classical crossover2015

    • Author(s)
      Yasuyuki Kato, Shigeki Onoda
    • Organizer
      American Physical Society March Meeting 2015
    • Place of Presentation
      Convention Center, San Antonio, TX, USA
    • Year and Date
      2015-03-02 – 2015-03-06
    • Related Report
      2014 Research-status Report
  • [Presentation] Two crossovers, deconfined spinons, and Higgs transition in quantum spin ice2014

    • Author(s)
      Shigeki Onoda
    • Organizer
      The long-term workshop "Nove Quantum States in Condensed Matter 2014"
    • Place of Presentation
      京都大学基礎物理学研究所 (京都府京都市)
    • Year and Date
      2014-11-04 – 2014-12-05
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] フラストレートしたスピン1/2鎖におけるSPT相とトポロジカル相転移2014

    • Author(s)
      小野田繁樹
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学 (愛知県春日井市)
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] パイロクロア型Ir酸化物とRh酸化物の第一原理計算:金属絶縁体転移、磁性とトポロジー2014

    • Author(s)
      石井史之,水田耀ピエール,加藤毅大,尾崎泰助,Hongming Weng,小野田繁樹
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学 (愛知県春日井市)
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] 量子スピンアイス模型の量子モンテカルロシミュレーション:非閉じ込めスピノン,ヒッグス閉じ込め転移,二つのクロスオーバー2014

    • Author(s)
      加藤康之、小野田繁樹
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学 (愛知県春日井市)
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] スピン1/2フラストレート交替鎖に現れる対称性に守られたトポロジカル相2014

    • Author(s)
      上田宏、小野田繁樹
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学 (愛知県春日井市)
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] Quantum spin ice2014

    • Author(s)
      Shigeki Onoda
    • Organizer
      Nordita programme: "Novel Directions in Frustrated and Critical Magnetism"
    • Place of Presentation
      Nordita, Nordic Institute of Theoretical Physics, KTH Royal Institute of Technology, Stockholm, Sweden
    • Year and Date
      2014-07-14 – 2014-08-08
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Phase transitions, crossovers, and extiations in quantum spin ice2014

    • Author(s)
      Shigeki Onoda, Yasuyuki Kato
    • Organizer
      International Conference on Highly Frustrated Magnetism 2014
    • Place of Presentation
      Cambridge University, Cambrkdge, UK
    • Year and Date
      2014-07-07 – 2014-07-11
    • Related Report
      2014 Research-status Report
  • [Presentation] Crossovers, deconfined spinons, and Higgs-confining transition in quantum spin ice2014

    • Author(s)
      Shigeki Onoda
    • Organizer
      2014 Aspen Summer Program "Modern Trends in Quantum Magnetism"
    • Place of Presentation
      Aspen Center for Physics, Aspen, CO, USA
    • Year and Date
      2014-05-25 – 2014-06-22
    • Related Report
      2014 Research-status Report
    • Invited
  • [Presentation] Quantum-classical crossover and Higgs confining transitions in quantum spin ice2014

    • Author(s)
      Shigeki Onoda
    • Organizer
      2014 Aspen Winter Program "Beyond Quasiparticles: New Paradigms for Quantum Fluids"
    • Place of Presentation
      Aspen Center for Physics, Aspen, CO (USA)
    • Related Report
      2013 Research-status Report
  • [Presentation] Classical and Quantum Coulomb Spin Liquids and Anderson-Higgs mechanism in quantum spin ice2014

    • Author(s)
      Shigeki Onoda
    • Organizer
      Workshop on Frustration and Topology in Condensed Matter
    • Place of Presentation
      National Cheng Kung University, Tainan (Taiwan)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] 量子スピンアイス系Yb2Ti2O7の新奇な強磁性転移と磁気相図2014

    • Author(s)
      濱地紀彰、安井幸夫、橘髙俊一郎、榊原俊郎、小野田繁樹
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学(神奈川県)
    • Related Report
      2013 Research-status Report
  • [Presentation] Hydrodynamic theory for Coulomb and Higgs-confining phases in quantum spin ice2013

    • Author(s)
      Shigeki Onoda
    • Organizer
      7th ISSP International Workshop and Symposium "Emergent Phases in Condensed Matter -- from topological to first principles approaches"
    • Place of Presentation
      東京大学物性研究所(千葉県)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Hydrodynamic theory for Coulomb and Higgs-confining phases in quantum spin ice2013

    • Author(s)
      Shigeki Onoda
    • Organizer
      NCTS Workshop on Quantum Condensation (QC13)
    • Place of Presentation
      National Center for Theoretical Sciences, National Cheng-Kung University, Tainan (Taiwan)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] 量子スピンアイスにおける磁気単極子と量子電磁気学・ヒッグス機構2013

    • Author(s)
      小野田繁樹
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学(徳島県)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] スピン軌道相互作用する電子系における電荷スピン熱輸送係数の理論2013

    • Author(s)
      小野田繁樹
    • Organizer
      日本磁気学会第193回研究会/第47回スピンエレクトロニクス専門研究会「スピンカロリトロニクス --磁気と熱の織り成す協調現象--」
    • Place of Presentation
      中央大学(東京都)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Topological magnetic insulators on the pyrochlore lattice: towards a first-principles design2013

    • Author(s)
      Shigeki Onoda
    • Organizer
      International Symposium on Computational Science 2013
    • Place of Presentation
      Kanazawa University, Kanazawa, Japan
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] 磁性体からカイラルスピン液体にわたる常ホール果の研究磁性体からカイラルスピン液体にわたる常ホール果の研究2013

    • Author(s)
      小野田繁樹
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学、広島、日本
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Topological phases with broken time-reversal symmetry in pyrochlore iridates2012

    • Author(s)
      Shigeki Onoda
    • Organizer
      International Workshop "Itinerant Spin-Orbital Systems: From Magnetic Frustration to Novel Superconductivity
    • Place of Presentation
      Max Planck Institute, Dresden, Germany
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Higgs transition from magnetic Coulomb liquid to ferromagnet in Yb2Ti2O72012

    • Author(s)
      Shigeki Onoda
    • Organizer
      9th International workshop on Polarised Neutrons in Condensed Matter Investigations
    • Place of Presentation
      Jean Monnet center, Paris, France
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Quantum spin ice2012

    • Author(s)
      Shigeki Onoda
    • Organizer
      KITP Program: "Frustrated Magnetism and Quantum Spin Liquids: From Theory and Models to Experiments
    • Place of Presentation
      Kavli Institute of Theoretical Physics, Santa Barbara, USA
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Topological phases with broken time-reversal symmetry in pyrochlore iridates2012

    • Author(s)
      Shigeki Onoda
    • Organizer
      Aspen Center for Physics, Summer Workshop "Spin-Orbit Physics in Correlated Electron Systems"
    • Place of Presentation
      Aspen Center for Physics, Aspen, USA
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Spontaneous and quantized anomalous Hall effects in magnetic pyrochlore iridates2012

    • Author(s)
      Shigeki Onoda
    • Organizer
      520. Wilhelm und Else Heraeus Seminar "Spin-orbit-driven transverse transport phenomena"
    • Place of Presentation
      Wilhelm und Else Heraeus-Stiftung, Bad Honnef, Germany
    • Related Report
      2012 Research-status Report
    • Invited
  • [Remarks] Melting of frozen frustration

    • URL

      http://www.riken.jp/en/research/rikenresearch/highlights/8138/

    • Related Report
      2015 Annual Research Report
  • [Remarks] プレスリリース「凍ったスピンをさらに冷やして量子効果で液体に融かす」

    • URL

      http://www.riken.jp/pr/press/2015/20150821_2/

    • Related Report
      2015 Annual Research Report
  • [Remarks] 量子スピンアイスの解説(理化学研究所・研究代表者ホームページ内)

    • URL

      http://www.riken.jp/lab-www/cond-mat-theory/onoda/Pr2TM2O7_2.htm

    • Related Report
      2013 Research-status Report
  • [Remarks] Higgs transition of north and south poles

    • URL

      http://www.riken.go.jp/engn/r-world/info/release/press/2012/120808/index.html

    • Related Report
      2012 Research-status Report
  • [Remarks] There's more to Higgs than bosons

    • URL

      http://www.rikenresearch.riken.jp/eng/research/7122.html

    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2022-01-27  

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