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Nuclear coordinate dependence of electronic wave function studied by high-resolution electron momentum spectroscopy

Research Project

Project/Area Number 24750004
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Physical chemistry
Research InstitutionTohoku University

Principal Investigator

YAMAZAKI MASAKAZU  東北大学, 多元物質科学研究所, 助教 (00533465)

Project Period (FY) 2012-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2013: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2012: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Keywords電子状態 / 電子分光 / 電子衝突 / 分子軌道 / 波動関数 / 原子・分子物理 / 化学物理 / 電子線散乱
Research Abstract

In this study, in order to investigate correlation between nuclear and electron motions in a molecule, we have developed a high-resolution electron momentum spectroscopy that would be capable of measuring nuclear coordinate dependent electronic wave functions. As a result, the resolution of electron binding energy has been improved from 2.7 eV to 1.1 eV by improving energy resolution of an electron analyzer incorporated with a monochromatized incident electron beam. To achieve higher resolution, it is found to be fundamental to develop a new electron analyzer with reduced aberrations and advanced electron optics as well as to introduce highly stable voltage supplies.

Report

(3 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • Research Products

    (57 results)

All 2014 2013 2012 Other

All Journal Article (9 results) (of which Peer Reviewed: 7 results) Presentation (43 results) (of which Invited: 5 results) Book (2 results) Remarks (3 results)

  • [Journal Article] 電子のオービタルパターンを見る2014

    • Author(s)
      山﨑優一
    • Journal Title

      パリティ

      Volume: 29巻 Pages: 13-15

    • URL

      http://pub.maruzen.co.jp/book_magazine/magazine/parity-back/parity2014/2014_01/1401_cont.html

    • Related Report
      2013 Final Research Report
  • [Journal Article] Development of an (e,2e) electron momentum spectroscopy apparatus using an ultrashort pulsed electron gun2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Journal Title

      Rev. Sci. Instrum.

      Volume: Vol.84, 063105 Issue: 6 Pages: 1-10

    • DOI

      10.1063/1.4809792

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Interatomic resonant Auger effects in core-level photoemission from NO and CS2 molecules2013

    • Author(s)
      M. Yamazaki, J. Adachi, T. Teramoto, A. Yagishita
    • Journal Title

      Journal of Physics B: Atomic, Molecular and Optical Physics

      Volume: VOL. 46 Issue: 11 Pages: 1-10

    • DOI

      10.1088/0953-4075/46/11/115101

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Molecular-frame (e,2e) experiment for N2 at large momentum transfer2013

    • Author(s)
      D. B. Jones, M. Yamazaki, N. Watanabe, M. Takahashi
    • Journal Title

      Physical Review A

      Volume: 87 Issue: 2 Pages: 1-5

    • DOI

      10.1103/physreva.87.022714

    • Related Report
      2013 Final Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] 電子のオービタルパターンを見る2013

    • Author(s)
      山崎優一
    • Journal Title

      パリティ

      Volume: 29巻 Pages: 13-15

    • Related Report
      2013 Annual Research Report
  • [Journal Article] Electron-impact ionization of N2 at large momentum transfer above the double-ionization threshold2012

    • Author(s)
      D. B. Jones, M. Yamazaki, N. Watanabe, M. Takahashi
    • Journal Title

      Physical Review A

      Volume: 86巻 Issue: 6 Pages: 1-7

    • DOI

      10.1103/physreva.86.062707

    • Related Report
      2013 Final Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Vibrational effects on valence electron momentum distributions of ethylene2012

    • Author(s)
      N. Watanabe, M. Yamazaki, M. Takahashi
    • Journal Title

      Journal of Chemical Physics

      Volume: 137 Issue: 11 Pages: 1-8

    • DOI

      10.1063/1.4752653

    • Related Report
      2013 Final Research Report 2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Recoil frame photoelectron angular distributions in core O 1s ionozation of H2CO2012

    • Author(s)
      M. Stener
    • Journal Title

      J. Phys. B: At. Mol. Opt. Phys.

      Volume: 45 Issue: 19 Pages: 194004-194004

    • DOI

      10.1088/0953-4075/45/19/194004

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] C Is photoelectron angular distributions from fixed-in-space CO molecules in the high-energy continuum >50 eV2012

    • Author(s)
      J. Adachi, M. Kazama. T. Teramoto, N. Miyauchi, T. Mizuno, M. Yamazaki, T. Fujikawa, A. Yagishita
    • Journal Title

      Journal of Physics B

      Volume: 45 Issue: 19 Pages: 194007-194007

    • DOI

      10.1088/0953-4075/45/19/194007

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] アセトンの光解離反応の時間分解電子運動量分光:反応ダイナミクスを取り入れた散乱理論解析2014

    • Author(s)
      中澤博之、大石慶也、山崎優一、朱超原、高橋正彦
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学(平塚)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解(e,2e)電子運動量分光の開発による化学反応におけるフロンティア電子運動の可視化2013

    • Author(s)
      山﨑優一, 髙橋正彦
    • Organizer
      原子衝突学会第38回年会
    • Place of Presentation
      埼玉
    • Year and Date
      2013-11-16
    • Related Report
      2013 Final Research Report
  • [Presentation] 時間分解電子運動量分光によるアセトンの光解離ダイナミクス2013

    • Author(s)
      山﨑優一, 大石慶也, 中澤博之, 葛西裕治, 髙橋正彦
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都
    • Year and Date
      2013-09-26
    • Related Report
      2013 Final Research Report
  • [Presentation] Development of time-resolved electron momentum spectroscopy : Preliminary results for the photodissociation dynamics of several molecules2013

    • Author(s)
      M. Yamazaki, M. Takahashi
    • Organizer
      International Symposium on (e,2e), Double Photo-ionization and Related Topics & 17th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions
    • Place of Presentation
      中国・合肥市
    • Year and Date
      2013-08-01
    • Related Report
      2013 Final Research Report
  • [Presentation] Development of time-resolved electron momentum spectroscopy : a tool for visualizing the motion of electrons during a chemical reaction2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Organizer
      XXVIII International Conference on Photonic, Electronic and Atomic Collisions
    • Place of Presentation
      中国・蘭州市
    • Year and Date
      2013-07-25
    • Related Report
      2013 Final Research Report
  • [Presentation] Development of time-resolved (e,2e) electron momentum spectroscopy : Preliminary results for the photodissociation dynamics of several molecules2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Organizer
      29th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      仙台
    • Year and Date
      2013-06-06
    • Related Report
      2013 Final Research Report
  • [Presentation] 多次元電子分光による電子波動関数の立体特性に関する研究2013

    • Author(s)
      山﨑優一
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      東広島
    • Year and Date
      2013-03-27
    • Related Report
      2013 Final Research Report 2012 Research-status Report
  • [Presentation] 時間分解電子運動量分光法の開発による化学反応の電子レベルでの可視化:アセトンの光解離反応2013

    • Author(s)
      山崎優一、高橋正彦
    • Organizer
      附置研究所間アライアンス 平成24年度成果報告会
    • Place of Presentation
      北海道大学(札幌)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Vibronic effects on electron momentum distributions of ethylene2013

    • Author(s)
      N. Watanabe, M. Yamazaki, M. Takahashi
    • Organizer
      29th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of laser-assisted electron momentum spectroscopy: the present status of experimental and theoretical progress2013

    • Author(s)
      M. Yamazaki, K. Kouzakov, Yu. Popov, H. Ohmura, M. Takahashi
    • Organizer
      29th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of a high-intensity target beam source for time-resolved (e,2e) electron momentum spectroscopy2013

    • Author(s)
      H. Nakazawa, M. Yamazaki, M. Takahashi
    • Organizer
      29th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of time-resolved (e,2e) electron momentum spectroscopy: Preliminary results for the photodissociation dynamics of several molecules2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Organizer
      29th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of time-resolved electron momentum spectroscopy: a tool for visualizing the motion of electrons during a chemical reaction2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Organizer
      XXVIII International Conference on Photonic, Electronic and Atomic Collisions
    • Place of Presentation
      中国、蘭州
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Development of time-resolved electron momentum spectroscopy: Preliminary results for the photodissociation dynamics of several molecules2013

    • Author(s)
      M. Yamazaki, M. Takahashi
    • Organizer
      International Symposium on (e,2e), Double Photo-ionization and Related Topics & 17th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions
    • Place of Presentation
      中国、合肥
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Development of time-resolved (e,2e) electron momentum spectroscopy: a tool for visualizing the motion of electrons during a chemical reaction2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Organizer
      International Symposium on (e,2e), Double Photo-ionization and Related Topics & 17th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions
    • Place of Presentation
      中国、合肥
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of time-resolved electron momentum spectroscopy: the present status of experimental and theoretical progress2013

    • Author(s)
      M. Yamazaki, K. A. Kouzakov, Yu. V. Popov, H. Ohmura, M. Takahashi
    • Organizer
      International Symposium on (e,2e), Double Photo-ionization and Related Topics & 17th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions
    • Place of Presentation
      中国、合肥
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解電子運動量分光の開発:化学反応途中の分子軌道の観測を目指して2013

    • Author(s)
      山崎優一
    • Organizer
      分子科学最前線2013
    • Place of Presentation
      コープ.イン.京都(京都)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 時間分解電子運動量分光によるアセトンの光解離ダイナミクス:データ解析と理論計算2013

    • Author(s)
      大石慶也、山崎優一、中澤博之、葛西裕治、高橋正彦
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解電子運動量分光によるアセトンの光解離ダイナミクス2013

    • Author(s)
      山崎優一、大石慶也、中澤博之、葛西裕治、高橋正彦
    • Organizer
      第7回分子科学討論会
    • Place of Presentation
      京都テルサ(京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of a high-intensity molecular beam source for time-resolved (e,2e) electron momentum spectroscopy2013

    • Author(s)
      H. Nakazawa, M. Yamazaki, M. Takahashi
    • Organizer
      International Symposium for the 70th Anniversary of the Tohoku Branch of the Chemical Society of Japan
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Development of time-resolved (e,2e) electron momentum spectroscopy: a tool for visualizing the electron motion during a chemical reaction2013

    • Author(s)
      M. Yamazaki, Y. Kasai, K. Oishi, H. Nakazawa, M. Takahashi
    • Organizer
      International Symposium for the 70th Anniversary of the Tohoku Branch of the Chemical Society of Japan
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解(e,2e)電子運動量分光の開発による化学反応におけるフロンティア電子運動の可視化2013

    • Author(s)
      山崎優一、高橋正彦
    • Organizer
      原子衝突学会第38回年会
    • Place of Presentation
      理化学研究所(和光)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Development of laser-assisted electron momentum spectroscopy: the present status of experimental and theoretical progress (II)2013

    • Author(s)
      M. Yamazaki, K. Oishi, H. Nakazawa, Y. Kasai, K. A. Kouzakov, Yu. V. Popov, H. Ohmura, C. Zhu, M. Takahashi
    • Organizer
      原子衝突学会第38回年会
    • Place of Presentation
      理化学研究所(和光)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解電子運動量分光によるアセトンの光解離過程:反応ダイナミクスを取り入れた理論解析2013

    • Author(s)
      中澤博之、大石慶也、山崎優一、高橋正彦
    • Organizer
      原子衝突学会第38回年会
    • Place of Presentation
      理化学研究所(和光)
    • Related Report
      2013 Annual Research Report
  • [Presentation] CO+-O+解離座標系で測定されたC 1s光電子角度分布の鏡映対称性の破れ2013

    • Author(s)
      水流翔太、風間美里、足立純一、宮内直弥、山崎優一、柳下明、藤川高志
    • Organizer
      原子衝突学会第38回年会
    • Place of Presentation
      理化学研究所(和光)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解電子運動量分光法の開発による物質内電子移動の可視化2013

    • Author(s)
      山崎優一、高橋正彦
    • Organizer
      附置研究所間アライアンス 平成25年度新エネルギー材料・デバイスプロジェクトグループ研究会
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解電子運動量分光と解離ダイナミクスを考慮した理論解析によるアセトンの光解離ダイナミクスの研究2013

    • Author(s)
      大石慶也、中澤博之、山崎優一、大村英樹、Chaoyuan Zhu、高橋正彦
    • Organizer
      第13回東北大学多元物質科学研究所研究発表会
    • Place of Presentation
      東北大学(仙台)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解電子運動量分光の開発 : 過渡状態電子運動の可視化へ向けて2012

    • Author(s)
      山﨑優一, 大石慶也, 葛西裕治, 川瀬裕也, 髙橋正彦
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京
    • Year and Date
      2012-09-18
    • Related Report
      2013 Final Research Report
  • [Presentation] Progress towards development of time-resolved (e,2e) electron momentum spectroscopy2012

    • Author(s)
      M. Yamazaki, M. Takahashi
    • Organizer
      International Conference on Many Particle Spectroscopy of Atoms, Molecules, Clusters and Surfaces
    • Place of Presentation
      ドイツ・ベルリン
    • Year and Date
      2012-08-29
    • Related Report
      2013 Final Research Report
  • [Presentation] Progress towards development of time-resolved electron momentum spectroscopy2012

    • Author(s)
      M. Yamazaki, K. Oishi, Y. Kasai, Y. Kawase, M. Takahashi
    • Organizer
      2nd International Symposium on Electron Momentum Spectroscopy
    • Place of Presentation
      ベルギー・ブリュッセル
    • Year and Date
      2012-08-23
    • Related Report
      2013 Final Research Report
  • [Presentation] 時間分解(e,2e)電子運動量分光の開発2012

    • Author(s)
      山﨑優一, 大石慶也, 葛西裕治, 川瀬裕也, 髙橋正彦
    • Organizer
      原子衝突学会第37回年会
    • Place of Presentation
      東京
    • Year and Date
      2012-07-29
    • Related Report
      2013 Final Research Report 2012 Research-status Report
  • [Presentation] Progress towards development of a time-resolved chemical reaction microscope using electron Compton scattering2012

    • Author(s)
      M. Yamazaki, Y. Kasai, Y. Kawase, M. Takahashi
    • Organizer
      28th Symposium on Chemical Kinetics and Dynamics
    • Place of Presentation
      福岡
    • Related Report
      2012 Research-status Report
  • [Presentation] 電子コンプトン散乱を用いた時間分解反応顕微鏡の開発2012

    • Author(s)
      山崎優一、大石慶也、葛西裕治、川瀬裕也、高橋正彦
    • Organizer
      第9回原子・分子・光化学(AMO)討論会
    • Place of Presentation
      埼玉
    • Related Report
      2012 Research-status Report
  • [Presentation] 超高感度電子運動量分光を用いたHeの励起イオン化過程の研究2012

    • Author(s)
      川瀬裕也、山崎優一、渡邉昇、高橋正彦
    • Organizer
      原子衝突学会第37回年会
    • Place of Presentation
      東京
    • Related Report
      2012 Research-status Report
  • [Presentation] Progress towards development of time-resolved electron momentum spectroscopy2012

    • Author(s)
      M. Yamazaki, K. Oishi, Y. Kasai, Y. Kawase, M. Takahashi
    • Organizer
      2nd International Symposium on Electron Momentum Spectroscopy
    • Place of Presentation
      ブリュッセル、ベルギー
    • Related Report
      2012 Research-status Report
  • [Presentation] Progress towards development of time-resolved (e,2e) electron momentum spectroscopy2012

    • Author(s)
      M. Yamazaki, M. Takahashi
    • Organizer
      International Conference on Many Particle Spectroscopy of Atoms, Molecules, Clusters and Surfaces
    • Place of Presentation
      ベルリン、ドイツ
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] Progress towards development of an apparatus for time-resolved (e,2e) electron momentum spectroscopy2012

    • Author(s)
      M. Yamazaki, K. Oishi, Y. Kasai, Y. Kawase, M. Takahashi
    • Organizer
      International Conference on Many Particle Spectroscopy of Atoms, Molecules, Clusters and Surfaces
    • Place of Presentation
      ベルリン、ドイツ
    • Related Report
      2012 Research-status Report
  • [Presentation] エチレンの電子運動量分布に対する分子振動の影響2012

    • Author(s)
      渡邉昇、山崎優一、高橋正彦
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京
    • Related Report
      2012 Research-status Report
  • [Presentation] 時間分解(e,2e)電子運動量分光装置と散乱理論の開発2012

    • Author(s)
      山崎優一、K. A. Kouzakov、Yu. V. Popov、高橋正彦
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京
    • Related Report
      2012 Research-status Report
  • [Presentation] 時間分解電子運動量分光の開発:過渡状態電子運動の可視化へ向けて2012

    • Author(s)
      山崎優一、大石慶也、葛西裕治、川瀬裕也、高橋正彦
    • Organizer
      第6回分子科学討論会
    • Place of Presentation
      東京
    • Related Report
      2012 Research-status Report
  • [Presentation] Development of time-resolved (e,2e) electron momentum spectroscopy: the present status of experimental and theoretical progress2012

    • Author(s)
      M. Yamazaki, K. A. Kouzakov, Yu. V. Popov, M. Takahashi
    • Organizer
      10th Asian International Seminar on Atomic and Molecular Physics
    • Place of Presentation
      台北、台湾
    • Related Report
      2012 Research-status Report
  • [Presentation] 時間分解電子運動量分光法の開発による化学反応の電子レベルでの可視化2012

    • Author(s)
      山崎優一、高橋正彦
    • Organizer
      新エネルギー材料・デバイスプロジェクトグループ分科会
    • Place of Presentation
      福岡
    • Related Report
      2012 Research-status Report
  • [Presentation] 時間分解電子運動量分光と散乱理論の開発2012

    • Author(s)
      山崎優一、大石慶也、中澤博之、大村英樹、K. A. Kouzakov、Yu. V. Popov、高橋正彦
    • Organizer
      第12回東北大学多元物質科学研究所研究発表会
    • Place of Presentation
      仙台
    • Related Report
      2012 Research-status Report
  • [Book] (e,2e) spectroscopy using fragmentation processes in"Fragmentation Processes (Topics in Atomic and Molecular Physics)"2013

    • Author(s)
      J. Lower, M. Yamazaki, M. Takahashi
    • Publisher
      Cambridge University Press
    • Related Report
      2013 Final Research Report
  • [Book] Fragmentation Processes (Topics in Atomic and Molecular Physics)2013

    • Author(s)
      J. Lower, M. Yamazaki, M. Takahashi
    • Publisher
      Cambridge University Press
    • Related Report
      2012 Research-status Report
  • [Remarks]

    • URL

      http://www.tagen.tohoku.ac.jp/modules/laboratory/index.php?laboid=42

    • Related Report
      2013 Final Research Report
  • [Remarks] 東北大学多元物質科学研究所業績データベース

    • URL

      http://db.tagen.tohoku.ac.jp/php/db/view-personal.php?pserial=2961

    • Related Report
      2013 Annual Research Report
  • [Remarks] 東北大学多元物質科学研究所業績データベース

    • URL

      http://db.tagen.tohoku.ac.jp/php/db/view-personal.php?pserial=2961

    • Related Report
      2012 Research-status Report

URL: 

Published: 2013-05-31   Modified: 2019-07-29  

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