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Electron spectroscopic studies of magnetic electrode interfaces in graphene spintronics for enhanced spin injection.

Research Project

Project/Area Number 24760033
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionJapan Atomic Energy Agency

Principal Investigator

OHTOMO MANABU  独立行政法人日本原子力研究開発機構, 原子力科学研究部門 先端基礎研究センター, 博士研究員 (20610299)

Project Period (FY) 2012-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2013: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2012: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Keywordsスピン偏極ヘリウム脱励起分光法 / 六方晶窒化ホウ素 / グラフェン / スピントロニクス / 磁性 / 準安定原子線 / 準安定原子 / スピン偏極準安定ヘリウム脱励起分光 / 表面科学
Research Abstract

The hexagonal boron nitride (h-BN) is a promising spin-injection barrier material for graphene spintronics. In this study, the spin-polarized metastable de-excitation spectroscopy (SPMDS) was employed to elucidate the spin-dependent electronic states induced at the h-BN/magnetic metal interfaces which have considerable effects on the spin injection efficiency.
The extreme surface sensitivity of the method enabled us to prove the orbital mixing and in-gap states formation on h-BN monolayer independently from strong signals from magnetic metals (Ni and Co). It was revealed that the in-gap states are spin-polarized parallel to the majority spins of Ni and Co. This result is essential for understanding the sign and magnitude of magnetoresistance of spintronics devices with h-BN tunnel barriers.

Report

(3 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • Research Products

    (25 results)

All 2014 2013 2012 Other

All Journal Article (7 results) (of which Peer Reviewed: 7 results) Presentation (16 results) Remarks (2 results)

  • [Journal Article] Contact-induced spin polarization of monolayer hexagonal boron nitride on ni(111)2014

    • Author(s)
      M. Ohtomo, Y. Yamauchi, A. A. Kuzubov, N. S. Eliseeva, P. V. Avramov, S. Entani, Y. Matsumoto, H. Naramoto and S. Sakai
    • Journal Title

      Appl. Phys. Lett.

      Volume: 104 (5) Issue: 5 Pages: 51604-51604

    • DOI

      10.1063/1.4863324

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] The adsorption of h-bn monolayer on the ni(111) surface studied by density functional theory2014

    • Author(s)
      X. Sun, A. Pratt, Z. Y. Li, M. Ohtomo, S. Sakai and Y. Yamauchi
    • Journal Title

      J. Appl. Phys.

      Volume: 115 Issue: 17

    • DOI

      10.1063/1.4866237

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] High spin polarization at the Fe/C60 interface in the Fe-doped C60 film.2013

    • Author(s)
      S. Sakai, Y. Matsumoto, M. Ohtomo, S. Entani, P. V. Avramov, P. B. Sorokin, H. Naramoto
    • Journal Title

      Synthetic Metals

      Volume: in press

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Contact-induced spin polarization in graphene/h-BN/Ni Nanocomposites2012

    • Author(s)
      P.V. Avramov, A.A. Kuzubov, S. Sakai, H. Naramoto, M. Ohtomo, S. Entani, Y. Matsumoto, P.B. Sorokin
    • Journal Title

      J. Appl. Phys.

      Volume: 112 Issue: 11 Pages: 114303-114303

    • DOI

      10.1063/1.4767134

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Intrinsic edge asymmetry in narrow zigzag hexagonal heteroatomic nanoribbons causes their subtle uniform curvature2012

    • Author(s)
      P.V. Avramov, D.G. Fedorov, P.B. Sorokin, S. Sakai, H. Naramoto, M. Ohtomo, S. Entani, Y. Matsumoto, H. Naramoto
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 3 Issue: 15 Pages: 2003-2003

    • DOI

      10.1021/jz300625t

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] High hydrogen-adsorption-rate material based on graphene decorated with alkali metals2012

    • Author(s)
      L.Y. Antipina, P.V. Avramov, S. Sakai, H. Naramoto, M. Ohtomo, S. Entani, Y. Matsumoto, P.B. Sorokin
    • Journal Title

      Phys. Rev. B

      Volume: 86 Issue: 8 Pages: 85435-85435

    • DOI

      10.1103/physrevb.86.085435

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Bias voltage dependence of tunneling magnetoresistance in granular C_<60>-Co films with current-perpendicular-to-plane geometry2012

    • Author(s)
      S. Sakai, S. Mitani, Y. Matsumoto, S. Entani, P.V. Avramov, M. Ohtomo, H. Naramoto, K. Takanashi
    • Journal Title

      J. Magn. Magn. Mater

      Volume: 324 Issue: 12 Pages: 1970-1970

    • DOI

      10.1016/j.jmmm.2012.01.033

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] Spin Polarization of Monolayer Hexagonal Boron Nitride on Ni(111) Studied by Spin-polarized Metastable De-excitation Spectroscopy2014

    • Author(s)
      M. Ohtomo, P.V. Avramov, S. Entani, Y. Matsumoto, H. Naramoto, Y. Yamauchi, and S. Sakai
    • Organizer
      Physics and Chemistry of Surface and Interfaces (PCSI-41)
    • Place of Presentation
      Santa Fe, New Mexico (USA)(口頭発表)
    • Related Report
      2013 Final Research Report
  • [Presentation] 六方晶窒化ホウ素単層膜の水素化と電子・スピン状態評価2014

    • Author(s)
      大伴真名歩,山内泰,圓谷志郎,松本吉弘,楢本洋,境誠司
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学相模原キャンパス(口頭発表)
    • Related Report
      2013 Final Research Report
  • [Presentation] Spin Polarization of Monolayer Hexagonal Boron Nitride on Ni(111) Studied by Spin-polarized Metastable De-excitation Spectroscopy2014

    • Author(s)
      M. Ohtomo, P.V. Avramov, S. Entani, Y. Matsumoto, H. Naramoto, Y. Yamauchi, and S. Sakai
    • Organizer
      Physics and Chemistry of Surface and Interfaces
    • Place of Presentation
      Santa Fe, New Mexico (USA)
    • Related Report
      2013 Annual Research Report
  • [Presentation] 六方晶窒化ホウ素単層膜の水素化と電子・スピン状態評価2014

    • Author(s)
      大伴真名歩,山内泰,圓谷志郎,松本吉弘,楢本洋,境誠司
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学相模原キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] Spin polarization of monolayer hexagonal boron nitride on Ni(111) studied by spin-polarized metastable de-excitation spectroscopy2013

    • Author(s)
      Manabu Ohtomo, Pavel V. Avramov, Shiro Entani, Yoshihiro Matsumoto, Hiroshi Naramoto, Yasushi Yamauchi, Seiji Sakai
    • Organizer
      5th international conference on recent progress in graphene research (RPGR2013)
    • Place of Presentation
      Tokyo (Japan)(ポスター)
    • Related Report
      2013 Final Research Report
  • [Presentation] 最表面敏感なスピン偏極準安定ヘリウム脱励起分光による単層六方晶窒化ホウ素/ニッケル接合のスピン偏極測定2013

    • Author(s)
      大伴真名歩,パヴェルアブラモフ,圓谷志郎,松本吉弘,楢本洋,山内泰,境誠司
    • Organizer
      第74回応用物理学会学術講演会
    • Place of Presentation
      同志社大学(口頭発表)
    • Related Report
      2013 Final Research Report
  • [Presentation] 六方晶窒化ホウ素‐磁性金属界面のスピン偏極状態2013

    • Author(s)
      大伴真名歩、山内泰、山村野百合、Pavel V. Avramov、松本吉弘、圓谷志郎、小出明広、楢本洋、雨宮健太、藤川高志、境誠司
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(口頭発表)
    • Related Report
      2013 Final Research Report
  • [Presentation] Spin polarization of hexagonal boron nitride/Ni(111) interface studied by spin-polarized meta -stable de-excitation spectroscopy2013

    • Author(s)
      大伴真名歩,山内泰,,圓谷志郎,松本吉弘,楢本洋,境誠司
    • Organizer
      第44回フラーレン・ナノチューブ・グラフェン総合シンポジウム
    • Place of Presentation
      東京大学(ポスター)
    • Related Report
      2013 Final Research Report
  • [Presentation] Spin polarization of monolayer hexagonal boron nitride on Ni(111) studied by spin-polarized metastable de-excitation spectroscopy.2013

    • Author(s)
      Manabu Ohtomo, Pavel V. Avramov, Shiro Entani, Yoshihiro Matsumoto, Hiroshi Naramoto, Yasushi Yamauchi, Seiji Sakai
    • Organizer
      5th international conference on recent progress in graphene research
    • Place of Presentation
      東京大学本郷キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] 最表面敏感なスピン偏極準安定ヘリウム脱励起分光による単層六方晶窒化ホウ素/ニッケル接合のスピン偏極測定2013

    • Author(s)
      大伴真名歩,パヴェル アブラモフ,圓谷志郎,松本吉弘,楢本洋,山内泰,境誠司
    • Organizer
      第74回応用物理学会学術講演会
    • Place of Presentation
      同志社大学京田辺キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] 六方晶窒化ホウ素‐磁性金属界面のスピン偏極状態2013

    • Author(s)
      大伴真名歩、山内泰、山村野百合、Pavel V. Avramov、松本吉弘、圓谷志郎、小出明広、楢本洋、雨宮健太、藤川高志、境誠司
    • Organizer
      日本物理学会第68 回年次大会
    • Place of Presentation
      広島大学
    • Related Report
      2012 Research-status Report
  • [Presentation] Spin polarization of hexagonal boron nitride/Ni(111) interface studied by spin-polarized metastable de-excitation spectroscopy.2013

    • Author(s)
      大伴 真名歩, 山内 泰,, 圓谷 志郎, 松本 吉弘, 楢本 洋, 境 誠司
    • Organizer
      第44回 フラーレン・ナノチューブ・グラフェン総合シンポジウム
    • Place of Presentation
      東京大学
    • Related Report
      2012 Research-status Report
  • [Presentation] X-ray magnetic circular dichroism studies of monolayer hexagonal boron nitride / magnetic metal interface2012

    • Author(s)
      Manabu Ohtomo, Yoshihiro Matsumoto, Shiro Entani, Pavel V. Avramov, Hiroshi Naramoto, Kenta Amemiya and Seiji Sakai
    • Organizer
      4th International Meeting on Spins in Organic Semiconductor (SpinOS 2012)
    • Place of Presentation
      London (United Kingdom)(ポスター)
    • Related Report
      2013 Final Research Report
  • [Presentation] X-ray Magnetic Circular Dichroism Studies of Hexagonal Boron Nitride / Ni(111) Hetero Interfaces2012

    • Author(s)
      Manabu Ohtomo, Yoshihiro Matsumoto, Noyuri Yamamura, Shiro Entani, Pavel V. Avramov, Hiroshi Naramoto, Kenta Amemiya, Takashi Fujikawa, and Seiji Sakai
    • Organizer
      XAFS theory workshop : XAFS theory and nanoparticles
    • Place of Presentation
      Chiba (Japan)(ポスター)
    • Related Report
      2013 Final Research Report
  • [Presentation] X-ray Magnetic Circular Dichroism Studies of Hexagonal Boron Nitride / Ni(111) Hetero Interfaces2012

    • Author(s)
      Manabu Ohtomo, Yoshihiro Matsumoto, Noyuri Yamamura, Shiro Entani, Pavel V. Avramov, Hiroshi Naramoto, Kenta Amemiya, Takashi Fujikawa, and Seiji Sakai
    • Organizer
      XAFS theory workshop: XAFS theory and nanoparticles
    • Place of Presentation
      千葉大学
    • Related Report
      2012 Research-status Report
  • [Presentation] X-ray magnetic circular dichroism studies of monolayer hexagonal boron nitride / magnetic metal interfaces.2012

    • Author(s)
      Manabu Ohtomo, Yoshihiro Matsumoto, Shiro Entani, Pavel V. Avramov, Hiroshi Naramoto, Kenta Amemiya and Seiji Sakai
    • Organizer
      4th International Meeting on Spins in Organic Semiconductor
    • Place of Presentation
      University of London
    • Related Report
      2012 Research-status Report
  • [Remarks] 分子スピントロニクス研究Grウェブサイト

    • URL

      http://asrc.jaea.go.jp/soshiki/gr/sakai-gr/index.html

    • Related Report
      2013 Annual Research Report
  • [Remarks] 分子スピントロニクス研究Grウェブサイト

    • URL

      http://asrc.jaea.go.jp/soshiki/gr/sakai-gr/index.html

    • Related Report
      2012 Research-status Report

URL: 

Published: 2013-05-31   Modified: 2019-07-29  

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