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Studying and controlling photoluminescence blinking of quantum dots by using intense THz pulses

Research Project

Project/Area Number 24760042
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Applied optics/Quantum optical engineering
Research InstitutionKyoto University

Principal Investigator

HIRORI Hideki  京都大学, 物質-細胞統合システム拠点, 准教授 (00512469)

Project Period (FY) 2012-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2013: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2012: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
KeywordsTHz分光 / 非線形分光 / 高強度THz発生 / 半導体光物性 / 量子井戸 / 量子ドット / 光物性 / 半導体 / 超高速分光 / テラヘルツ非線形光学 / 半導体量子ドット
Research Abstract

The purpose of this study is studying and controlling the photoluminescence phenomena of quantum dots or wells, which has expected for the applications of electro-optic devices. The excitation density dependence of photoluminescence (PL) blinking of single CdSe/ZnS quantum dots indicates that the biexciton generation is a precursor of the trion state and not of the OFF state. Also, the THz electric field dependence and the relaxation dynamics of the PL flash intensity of GaAs quantum wells suggest that the strong electric field of the THz pulse ionizes impurity states during the one-picosecond period of the THz pulse and release carriers from a giant reservoir containing impurity states in the AlGaAs layers.

Report

(3 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • Research Products

    (27 results)

All 2014 2013 2012

All Journal Article (12 results) (of which Peer Reviewed: 10 results) Presentation (15 results) (of which Invited: 3 results)

  • [Journal Article] Terahertz-induced optical emission of photoexcited undoped GaAs quantum wells2013

    • Author(s)
      K. Shinokita, H. Hirori, K. Tanaka, T. Mochizuki, C. Kim, H. Akiyama, L. N. Pfeiffer, and K. W. West
    • Journal Title

      Physical Review Letters誌

      Volume: 111巻

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Electric field ionization of gallium acceptors in germanium induced by single-cycle terahertz pulses2013

    • Author(s)
      Y. Mukai, H. Hirori, K. Tanaka
    • Journal Title

      Physical Review B Rapid Communications誌

      Volume: 87巻

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Biexciton state causes photoluminescence fluctuations in CdSe/ZnS core/shell quantum dots at high photoexcitation densities2013

    • Author(s)
      N. Yoshikawa, H. Hirori, H. Watanabe, T. Aoki, T. Ihara, R. Kusuda, C. Wolpert, T. K. Fujiwara, A. Kusumi, Y. Kanemitsu, and K. Tanaka
    • Journal Title

      Physical Review B

      Volume: 88巻

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] High-power THz pulse generation and nonlinear THz spectroscopy2013

    • Author(s)
      K. Shinokita, H. Hirori, K. Tanaka, T. Mochizuki, C. Kim, H. Akiyama, L. N. Pfeiffer, K. W. West.
    • Journal Title

      Proceedings of the International Society for Optics and Photonics (SPIE)

      Volume: 8604巻

    • Related Report
      2013 Final Research Report
  • [Journal Article] Terahertz-Induced Optical Emission of Photoexcited Undoped GaAs Quantum Wells2013

    • Author(s)
      K. Shinokita, H. Hirori, K. Tanaka, T. Mochizuki, C. Kim, H. Akiyama, L. N. Pfeiffer and K. W. West
    • Journal Title

      Phys. Rev. Lett.

      Volume: 111 Issue: 6 Pages: 67401-67401

    • DOI

      10.1103/physrevlett.111.067401

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electric field ionization of gallium acceptors in germanium induced by single-cycle terahertz pulses2013

    • Author(s)
      Y. Mukai, H. Hirori, K. Tanaka
    • Journal Title

      Physical Review B Rapid Communications

      Volume: 87 Issue: 20

    • DOI

      10.1103/physrevb.87.201202

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Biexciton state causes photoluminescence fluctuations in CdSe/ZnS core/shell quantum dots at high photoexcitation densities2013

    • Author(s)
      N. Yoshikawa, H. Hirori, H. Watanabe, T. Aoki, T. Ihara, R. Kusuda, C. Wolpert, T. K. Fujiwara, A. Kusumi, Y. Kanemitsu, and K. Tanaka
    • Journal Title

      Physical Review B

      Volume: Vol.88 Issue: 15

    • DOI

      10.1103/physrevb.88.155440

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nonlinear Optical Phenomena Induced by Intense Single-Cycle Terahertz Pulses2013

    • Author(s)
      H. Hirori and K. Tanaka
    • Journal Title

      IEEE Journal of Selected Topics in Quantum Electronics

      Volume: 19 Issue: 1 Pages: 8401110-8401110

    • DOI

      10.1109/jstqe.2012.2221685

    • NAID

      120005241438

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-power THz pulse generation and nonlinear THz spectroscopy2013

    • Author(s)
      K. Shinokita, H. Hirori, K. Tanaka, T. Mochizuki, C. Kim, H. Akiyama, L. N. Pfeiffer, K. W. West
    • Journal Title

      Proceedings of the International Society for Optics and Photonics (SPIE)

      Volume: 8604 Pages: 86040B-86040B

    • DOI

      10.1117/12.2008309

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nonlinear optical phenomena induced by intense single-cycle terahertz pulses2012

    • Author(s)
      H. Hirori, K. Tanaka.
    • Journal Title

      IEEE Journal of Selected Topics in Quantum Electronics誌

      Volume: 19巻

    • NAID

      120005241438

    • Related Report
      2013 Final Research Report
  • [Journal Article] Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3 and applications to nonlinear optics2012

    • Author(s)
      H. Hirori, K. Tanaka
    • Journal Title

      Proc. SPIE誌

      Volume: 8240巻

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] 高強度THzパルスで誘起する非線形光学現象2012

    • Author(s)
      廣理英基,田中耕一郎
    • Journal Title

      応用物理学会誌(解説)

      Volume: 81巻第4号 Pages: 291-297

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Presentation] 超高強度THz光源の開発とTHz非線形分光、応用物理学会2014

    • Author(s)
      廣理英基、田中耕一郎
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学相模原キャンパス
    • Related Report
      2013 Final Research Report
  • [Presentation] 超高強度THz光源の開発とTHz非線形分光2014

    • Author(s)
      廣理英基、田中耕一郎
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] High-power Terahertz Pulse Generation and Application to Nonlinear THz Spectroscopy2013

    • Author(s)
      H. Hirori, K. Tanaka
    • Organizer
      Nonlinear Optics
    • Place of Presentation
      The Fairmont Orchid, Kohala Coast, Hawaii (アメリカ)
    • Related Report
      2013 Final Research Report
  • [Presentation] High-power Terahertz Pulse Generation and Application to Nonlinear THz Spectroscopy2013

    • Author(s)
      H. Hirori, K. Tanaka
    • Organizer
      The 18th International Conference on Electron Dynamics in Semiconductors, Optoelectronics and Nanostructures (EDISON18)
    • Place of Presentation
      くにびきメッセ,松江市,島根県(日本)
    • Related Report
      2013 Final Research Report
  • [Presentation] High-power THz pulse generation and nonlinear THz spectroscopy2013

    • Author(s)
      H. Hirori, K. Tanaka
    • Organizer
      2013 Photonics West
    • Place of Presentation
      The Moscone Center, San Francisco (アメリカ)(8604-10)
    • Related Report
      2013 Final Research Report
  • [Presentation] 超高強度THz光源の開発と非線形光学現象への応用に関する研究(第7回日本物理学会若手奨励賞受賞記念講演)2013

    • Author(s)
      廣理英基
    • Organizer
      第68回日本物理学会
    • Place of Presentation
      広島大学、東広島市
    • Related Report
      2013 Final Research Report
  • [Presentation] CdSe/ZnS単一量子ドットにおける高強度励起下でのトリオン生成2013

    • Author(s)
      吉川尚孝,廣理英基,渡邊浩,青木隆朗,Christian Wolpert,田中耕一郎
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Final Research Report
  • [Presentation] 希土類オルソフェライトHoFeO3における高強度テラヘルツ磁場誘起マグノン生成2013

    • Author(s)
      向井佑,廣理英基,山本隆文,陰山洋,田中耕一郎
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Final Research Report
  • [Presentation] Dynamics of Optically Excited Carriers under Intense Terahertz Pulse in GaAs Quantum Wells2013

    • Author(s)
      K. Shinokita, H. Hirori, T. Mochizuki, H. Akiyama, L. N. Pfeiffer, K. W. West, and K. Tanaka
    • Organizer
      International Workshop on Optical Terahertz Science and Technology 2013(OTST2013)
    • Place of Presentation
      Kyoto Terssa, Japan
    • Related Report
      2013 Final Research Report
  • [Presentation] Photoluminescence Flash Induced by Intense Single-Cycle Terahertz Pulses in Undoped GaAs Quantum Wells2013

    • Author(s)
      K. Shinokita, H. Hirori, K. Tanaka,T. Mochizuki, H. Akiyama, K. W. West, L. N. Pfeiffer
    • Organizer
      CLEO-PR & OECC/PS 2013
    • Place of Presentation
      Kyoto International Conference Center, Kyoto
    • Related Report
      2013 Annual Research Report 2013 Final Research Report
  • [Presentation] GaAs量子井戸の励起子内部準位における過渡的ACシュタルク効果の観測2013

    • Author(s)
      内田健人,廣理英基,篠北啓介,望月敏光,金昌秀,吉田正裕,秋山英文,L.N.Pfeiffer,K.W.WestE,田中耕一郎
    • Organizer
      日本物理学会2013年秋季大会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Final Research Report
  • [Presentation] High-power Terahertz Pulse Generation and Application to Nonlinear THz Spectroscopy2013

    • Author(s)
      H. Hirori, K. Tanaka
    • Organizer
      Nonlinear Optics (NLO2013)
    • Place of Presentation
      The Fairmont Orchid, Kohala Coast, Hawaii (アメリカ)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] High-power Terahertz Pulse Generation and Application to Nonlinear THz Spectroscopy2013

    • Author(s)
      H. Hirori, K. Tanaka
    • Organizer
      The 18th International Conference on Electron Dynamics in Semiconductors (EDISON18)
    • Place of Presentation
      くにびきメッセ, 松江市, 島根県 (日本)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Dynamics of Optically Excited Carriers under Intense Terahertz Pulse in GaAs Quantum Wells2013

    • Author(s)
      K. Shinokita, H. Hirori, T. Mochizuki, H. Akiyama, L. N. Pfeiffer, K. W. West, K. Tanaka
    • Organizer
      International Workshop on Optical Terahertz Science and Technology 2013(OTST2013)
    • Place of Presentation
      Kyoto Terssa, Kyoto
    • Related Report
      2013 Annual Research Report
  • [Presentation] CdSe/ZnS単一量子ドットにおける明滅現象の励起光強度依存性2013

    • Author(s)
      吉川尚孝
    • Organizer
      日本物理学会 2013年 春季大会
    • Place of Presentation
      広島大学(東広島市)
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2019-07-29  

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