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Development of ultrafast photoelectrron diffraction

Research Project

Project/Area Number 25246041
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Quantum beam science
Research InstitutionHigh Energy Accelerator Research Organization

Principal Investigator

YAGISHITA AKIRA  大学共同利用機関法人高エネルギー加速器研究機構, その他部局等, 名誉教授 (80157966)

Co-Investigator(Kenkyū-buntansha) FUJIKAWA TAKASHI  千葉大学, 融合科学研究科, 名誉教授 (30114987)
TERAMOTO TAKAHIRO  立命館大学, 理工学部, 助教 (40467056)
KISHIMOTO NAOKI  東北大学, 理学系研究科, 准教授 (60302080)
Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥46,410,000 (Direct Cost: ¥35,700,000、Indirect Cost: ¥10,710,000)
Fiscal Year 2015: ¥8,320,000 (Direct Cost: ¥6,400,000、Indirect Cost: ¥1,920,000)
Fiscal Year 2014: ¥17,160,000 (Direct Cost: ¥13,200,000、Indirect Cost: ¥3,960,000)
Fiscal Year 2013: ¥20,930,000 (Direct Cost: ¥16,100,000、Indirect Cost: ¥4,830,000)
Keywords光電子回折法 / 配列分子 / X線自由電子レーザー / 分子構造 / 超高速光電子回折法 / 分子構造変化 / 光化学反応 / 単一配向分子
Outline of Final Research Achievements

We have measured deep inner-shell 2p X-ray photoelectron diffraction (XPD) profiles from laser-aligned I2 molecules using X-ray free-electron laser (XFEL) pulses. By applying our molecular structure determination methodology to the XPD profiles, which were measured for I2 molecular ensembles with high degree of alignment, we have succeeded in determining the inter-nuclear distance of the I2 molecules in the electric field of Nd:YAG laser for the alignment.
Thus, it was revealed that the inter-nuclear distance in the laser field is elongated by ca. 0.3Å, compared to that of the equilibrium geometry of the ground state.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • Research Products

    (30 results)

All 2016 2015 2014 2013 Other

All Journal Article (9 results) (of which Peer Reviewed: 9 results,  Acknowledgement Compliant: 4 results,  Open Access: 1 results) Presentation (19 results) (of which Int'l Joint Research: 3 results,  Invited: 6 results) Remarks (2 results)

  • [Journal Article] 分子座標系で観測する光電子放出の物理:基礎と応用2015

    • Author(s)
      柳下 明
    • Journal Title

      分光研究

      Volume: 64 Pages: 331-345

    • NAID

      40020484290

    • Related Report
      2015 Annual Research Report 2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoelectron angular distributions from single oriented molecules: Past, Present and future2015

    • Author(s)
      Akira Yagishita
    • Journal Title

      J. Electron Spectroscopy and Related Phenomena

      Volume: 200 Pages: 247-256

    • DOI

      10.1016/j.elspec.2015.04.016

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Photoelectron diffraction from laser-aligned molecules with X-ray free-electron laser pulses2015

    • Author(s)
      Kyo Nakajima
    • Journal Title

      Scientific Reports

      Volume: 5 Issue: 1 Pages: 140651-1406511

    • DOI

      10.1038/srep14065

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Photoelectron angular distributions from single oriented molecules: Past, present and future2015

    • Author(s)
      A. Yagishita
    • Journal Title

      J. Electron Spectroscopy & Related Phenomena

      Volume: 200

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Site-specific fragmentation probabilities deduced from O+ - CO+ molecular frame photoelectron angular distributions from CO22014

    • Author(s)
      S.Tsuru
    • Journal Title

      Chem. Phys. Lett.

      Volume: 608 Pages: 152-156

    • DOI

      10.1016/j.cplett.2014.05.086

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Off-resonance photoemission dynamics studied by recoil frame F1s and C1s photoelectron angular distributions of CH3F2014

    • Author(s)
      M. Stener
    • Journal Title

      J. Chem. Phys.

      Volume: 140 Issue: 4

    • DOI

      10.1063/1.4862267

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Geometrical effect on the issue of asymmetric C1s photoelectron angular distributions detected in coincidenvce wtih the fragment ion pairs of CO+- O+ for CO2 molecules2014

    • Author(s)
      S. Tsuru
    • Journal Title

      J. Phys. B: At. Mol. Opt. Phys.

      Volume: 47 Issue: 7 Pages: 071002-071002

    • DOI

      10.1088/0953-4075/47/7/071002

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoelectron diffraction from single oriented molecules: Towards ultrafast structure determination of molecules using x-ray free-electron lasers2013

    • Author(s)
      M. Kazama
    • Journal Title

      Physical Review A

      Volume: 87 Issue: 6

    • DOI

      10.1103/physreva.87.063417

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Interatomic resonant Auger effects in core-level photoemission from NO and CS2 molecules2013

    • Author(s)
      M. Yamazaki, J. Adachi, T. Teramoto, A. Yagishita
    • Journal Title

      Journal of Physics B: Atomic, Molecular and Optical Physics

      Volume: VOL. 46 Issue: 11 Pages: 1-10

    • DOI

      10.1088/0953-4075/46/11/115101

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] XFEL を用いた光電子回折法による高強度レーザー中の分子構造2016

    • Author(s)
      柳下 明
    • Organizer
      日本物理学会第 71 回年次 大会
    • Place of Presentation
      東北学院大学泉キャンパス、宮城県仙台市
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] 気相実験における XFEL とフェムト秒レーザー光との同期法の開発2016

    • Author(s)
      峰本紳一郎
    • Organizer
      日本物理学会第 71 回年次 大会
    • Place of Presentation
      東北学院大学泉キャンパス、宮城県仙台市
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Ultrafast structure determination of a molecule in an intense laser field by photoelectron diffraction imaging using XFEL2015

    • Author(s)
      S. Minemoto
    • Organizer
      International Conference on Electron Spectroscopy and Structure: ICESS2015
    • Place of Presentation
      Stony Brook University, New York, USA
    • Year and Date
      2015-09-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 超高速X線光電子回折の理論2015

    • Author(s)
      水流翔太
    • Organizer
      原子衝突学会第40回年会
    • Place of Presentation
      首都大学東京、東京都南大沢
    • Year and Date
      2015-09-28
    • Related Report
      2015 Annual Research Report
  • [Presentation] Photoelectron difraction from laser-aligned molecules using an x-ray free-electron laser2015

    • Author(s)
      K. Nakajima
    • Organizer
      ICPEAC satellites "International Symposium on (e,2e), Double Photo-ionization and Related Topics" and "18th International Symposium on Polarization and Corelation in Electronic and Atomic Collisions
    • Place of Presentation
      San Sebastian, Spain
    • Year and Date
      2015-07-30 – 2015-08-01
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Photoelectron diffraction from laser-aligned molecules using an x-ray free-electron laser2015

    • Author(s)
      K. Nakajima
    • Organizer
      ICPEAC satellites, International Symposium on (e,2e), Double Photo-ionization and Related Topics
    • Place of Presentation
      San Sebastian, Spain
    • Year and Date
      2015-07-30
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Theory of ultrafast x-ray photoelectron diffraction2015

    • Author(s)
      S. Tsuru
    • Organizer
      ICPEAC satellites, International Symposium on (e,2e), Double Photo-ionization and Related Topics
    • Place of Presentation
      San Sebastian, Spain
    • Year and Date
      2015-07-30
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 超高速光電子回折法の開発II2015

    • Author(s)
      中嶋 享
    • Organizer
      日本物理学会第70回年次大会
    • Place of Presentation
      東京(早稲田大学)
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] X線自由電子レーザーによる配列分子の光電子回折2015

    • Author(s)
      中嶋 享
    • Organizer
      第28回日本放射光学会年会放射光科学合同シンポジウム
    • Place of Presentation
      草津(立命館大学)
    • Year and Date
      2015-01-10 – 2015-01-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Photoelectron diffraction from laser-aligned molecules with an x-ray free-electron laser2014

    • Author(s)
      K. Nakajima
    • Organizer
      11th Asian International Seminar on Atomic and Molecular Physics (AISAMP 11)
    • Place of Presentation
      Sendai(Tohoku Univ.)
    • Year and Date
      2014-10-06 – 2014-10-10
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] A velocity map imaging apparatus for photoelectron difraction studies using x-ray free-electron laser2014

    • Author(s)
      K. Nakajima
    • Organizer
      原子衝突学会第39回年会/AISAMP 11
    • Place of Presentation
      仙台(東北大学)
    • Year and Date
      2014-10-04 – 2014-10-06
    • Related Report
      2014 Annual Research Report
  • [Presentation] F1s photoelectron angular distributions detected in coincidence with the BF2+-F+ ions of BF3 molecules: fragmentation-site dependence of them2014

    • Author(s)
      S. Tsuru
    • Organizer
      原子衝突学会第39回年会/AISAMP 11
    • Place of Presentation
      仙台(東北大学)
    • Year and Date
      2014-10-04 – 2014-10-06
    • Related Report
      2014 Annual Research Report
  • [Presentation] 超高速光電子回折法の開発2014

    • Author(s)
      中嶋 享
    • Organizer
      第8回分子科学討論会2014
    • Place of Presentation
      東広島(広島大学)
    • Year and Date
      2014-09-21 – 2014-09-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] O+-CO+解離座標系で測定されたO1s光電子角度分布におけるCO2のサイト選択的解離の研究2014

    • Author(s)
      水流翔太
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] Physics on photoemission from oriented molecules: past, present, and future2013

    • Author(s)
      A. Yagishita
    • Organizer
      第29回化学反応討論会
    • Place of Presentation
      東北大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Photoelectron Diffraction from Single Oriented Molecules2013

    • Author(s)
      A. Yagishita
    • Organizer
      CC3DMR 2013
    • Place of Presentation
      Jeju Island, South Korea
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] CO+-O+解離座標系で測定されたC1s光電子角度分布の鏡映対称性の破れ2013

    • Author(s)
      水流翔太
    • Organizer
      原子衝突学会第38回年会
    • Place of Presentation
      理化学研究所、和光
    • Related Report
      2013 Annual Research Report
  • [Presentation] Interatomic resonance Auger in core-level photoemission from small molecules

    • Author(s)
      A. Yagishita
    • Organizer
      50 Years of Atomic Physics with Synchrotron Radiation
    • Place of Presentation
      NIST, Gaithersburg, MD, USA
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 超高速光電子回折法の開発 I

    • Author(s)
      中嶋享
    • Organizer
      日本物理学会第69回年次大会
    • Place of Presentation
      東海大学湘南キャンパス
    • Related Report
      2013 Annual Research Report
  • [Remarks] 柳下・基礎光化学物理研究室

    • URL

      http://molecule.kek.jp

    • Related Report
      2015 Annual Research Report
  • [Remarks] 柳下・基礎光化学物理研究室

    • URL

      http://molecule.kek.jp

    • Related Report
      2013 Annual Research Report

URL: 

Published: 2013-05-15   Modified: 2019-07-29  

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