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Study on the attosecond multi-level tunnel ionization processes that form an electron wavepacket.

Research Project

Project/Area Number 25247069
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Atomic/Molecular/Quantum electronics
Research InstitutionWaseda University

Principal Investigator

Hiromichi Niikura  早稲田大学, 理工学術院, 教授 (10500598)

Co-Investigator(Kenkyū-buntansha) Morishita Toru  電気通信大学, 情報理工学(系)研究科, 准教授 (20313405)
IWAKURA Izumi  神奈川大学, 工学部, 准教授 (40517083)
Co-Investigator(Renkei-kenkyūsha) Madesen L. B.  Aarhus University
Tolstikhin O. I.  Moscow institute of physics and technology
Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥45,890,000 (Direct Cost: ¥35,300,000、Indirect Cost: ¥10,590,000)
Fiscal Year 2015: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2014: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2013: ¥36,660,000 (Direct Cost: ¥28,200,000、Indirect Cost: ¥8,460,000)
Keywordsトンネルイオン化 / アト秒科学 / 高次高調波 / 再衝突電子 / アト秒イオン化 / アト秒高次高調波 / トンネルイオン化過程 / 数サイクルパルス / 極端紫外光 / 分子軌道イメージング / 分子動力学 / 分子軌道
Outline of Final Research Achievements

We have developed the experimental and theoretical approaches to study the multi-level tunnel ionization process induced by intense, laser pulses. First, we have measured the two-dimensional high-harmonic spectra emitted from aligned molecules using two-color intense laser pulses. By controlling the alignment angle, we control the contribution of the levels that are related to the tunnel ionization and high-harmonic generation. Next, using the attosecond high-harmonics combined with the intense laser pulse, we have explored that a particular ionization channel is predominantly selected, that allows us to observe an phase-resolved electron wavefunction image with attosecond time-resolution. We have also developed the theoretical treatments regarding to the multi-level tunnel ionization process that includes the multi-electron effect.

Report

(5 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • Products Report
  • Research Products

    (37 results)

All 2018 2017 2016 2015 2014 2013 Other

All Journal Article (21 results) (of which Int'l Joint Research: 6 results,  Peer Reviewed: 21 results,  Acknowledgement Compliant: 10 results) Presentation (14 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results) Remarks (2 results)

  • [Journal Article] Coherent imaging of an attosecond electron wave packet2017

    • Author(s)
      D. M. Villeneuve, Paul. Hockett, M. J. J. Vrakking, Hiromichi Niikura
    • Journal Title

      Science

      Volume: 356 Issue: 6343 Pages: 1150-1153

    • DOI

      10.1126/science.aam8393

    • Related Report
      Products Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Pulsed Nd : YAG laser-induced photoreaction of cis, cis-1, 3-cyclooctadiene at 266 nm : selective cyclization to cis-bicyclo [4.2.0] oct-7-ene2017

    • Author(s)
      Keiko Komor-Orisaku, Yui Hirose, Izumi Iwakura
    • Journal Title

      Photochemical & Photobiological Sciences

      Volume: 16 Issue: 2 Pages: 146-150

    • DOI

      10.1039/c6pp00323k

    • Related Report
      Products Report
    • Peer Reviewed
  • [Journal Article] Contribution of multiple electron trajectories to high-harmonic generation in the few-cycle regime2015

    • Author(s)
      A. Naumov, D. Villeneuve, H. Niikura
    • Journal Title

      Physical Review A

      Volume: 91 Issue: 6

    • DOI

      10.1103/physreva.91.063421

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Numerical simulation of the double-to-single ionization ratio for the helium atom in strong laser fields2015

    • Author(s)
      Z. Chen, Y. Zheng, W. Yang, X. Song, J. Xu, L. F. DiMauro, O. Zatsarinny, K. Bartschat, T. Morishita, S.-F. Zhao, and C. D. Lin
    • Journal Title

      Phys. Rev. A

      Volume: 92 Issue: 6

    • DOI

      10.1103/physreva.92.063427

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Analysis of a shift of the maximum of photoelectron momentum distributions generated by intense circularly polarized pulses2015

    • Author(s)
      M. Ohmi, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev. A 92

      Volume: 92 Issue: 4

    • DOI

      10.1103/physreva.92.043402

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Weak-field asymptotic theory of tunneling ionization including the first-order correction terms: Application to molecules2015

    • Author(s)
      V. H. Trinh, V. N. T. Pham, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 91 Issue: 6

    • DOI

      10.1103/physreva.91.063410

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Hyperspherical calculations of ultralow-energy collisions in Coulomb three-body systems2015

    • Author(s)
      Y. Zhou, S. Watanabe, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 92 Issue: 3

    • DOI

      10.1103/physreva.92.032713

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Structure factors for tunneling ionization rates of diatomic molecules2015

    • Author(s)
      R. Saito, O. I. Tolstikhin, L. B. Madsen, and ,T. Morishita
    • Journal Title

      Atomic Data and Nuclear Data Tables

      Volume: 103-104 Pages: 4-49

    • DOI

      10.1016/j.adt.2015.02.001

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Weak-field asymptotic theory of tunneling ionization: benchmark analytical results for two-electron atoms2015

    • Author(s)
      V. H. Trinh, O. I. Tolstikhin, and T. Morishit
    • Journal Title

      J. Phys. B: At. Mol. Opt. Phys

      Volume: 48 Pages: 061003-061003

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Application of the many-electron weak-field asymptotic theory of tunneling ionization to atoms2014

    • Author(s)
      I. Y. Tolstikhina,T. Morishita, and O. I. Tolstikhin
    • Journal Title

      Physical Review A

      Volume: 90 Issue: 5 Pages: 053413-053413

    • DOI

      10.1103/physreva.90.053413

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Rydberg states in the strong field ionization of hydrogen by 800, 1200 and 1600 nm lasers2014

    • Author(s)
      Q. Li, X.-M. Tong, T. Morishita, C. Jin, H. Wei and C. D. Lin
    • Journal Title

      J. Phys. B: At. Mol. Opt. Phys

      Volume: 47 Pages: 204019-204019

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Universality of Returning Electron Wave Packet in High-Order Harmonic2014

    • Author(s)
      A.-T. Le, H. Wei, C. Jin, V. N. Tuoc, T. Morishita, and C. D. Lin
    • Journal Title

      Physical Review Letters

      Volume: 113 Issue: 3 Pages: 033001-033001

    • DOI

      10.1103/physrevlett.113.033001

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Probing dipole-forbidden autoionizing states by isolated attosecond pulses2014

    • Author(s)
      W.-C. Chu, T. Morishita, and C. D. Lin
    • Journal Title

      Phys. Rev. A

      Volume: 89 Issue: 3

    • DOI

      10.1103/physreva.89.033427

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular Siegert states in an electric field. II. Transverse momentum distribution of the ionized electrons2014

    • Author(s)
      V. N. T. Pham, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev

      Volume: A89 Issue: 3 Pages: 33426-33426

    • DOI

      10.1103/physreva.89.033426

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Application of the weak-field asymptotic theory to tunneling ionization of H2O2014

    • Author(s)
      L. B. Madsen, Frank Jensen, O. I. Tolstikhin, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 89 Issue: 3 Pages: 33412-33412

    • DOI

      10.1103/physreva.89.033412

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fine structures in the intensity dependence of excitation and ionization probabilities of hydrogen atoms in intense 800-nm laser pulses2014

    • Author(s)
      Q. Li, X.-M. Tong, T. Morishita, H. Wei, and C. D. Lin
    • Journal Title

      Phys. Rev. A

      Volume: 89 Issue: 2

    • DOI

      10.1103/physreva.89.023421

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Weak-field asymptotic theory of tunneling ionization in many-electron atomic and molecular systems2014

    • Author(s)
      O. I. Tolstikhin, L. B. Madsen, and T. Morishita
    • Journal Title

      Phys. Rev

      Volume: A89 Issue: 1 Pages: 13421-13421

    • DOI

      10.1103/physreva.89.013421

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular tunneling ionization of the carbonyl sulfide molecule by double-frequency phase-controlled laser fields2014

    • Author(s)
      H. Ohmura, N. Sato, and T. Morishita
    • Journal Title

      Phy. Rev. A

      Volume: 89 Issue: 1

    • DOI

      10.1103/physreva.89.013405

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photoelectron spectra and high Rydberg states of lithium generated by intense lasers in the over-the-barrier ionization regime2013

    • Author(s)
      T. Morishita and C. D. Lin
    • Journal Title

      Phy. Rev. A

      Volume: 87 Issue: 6

    • DOI

      10.1103/physreva.87.063405

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] First-order correction terms in the weak-field asymptotic theory of tunneling ionization2013

    • Author(s)
      V. H. Trinh, O. I. Tolstikhin, L. B. Madsen, and T. Morishita
    • Journal Title

      Phys. Rev

      Volume: A87 Issue: 4 Pages: 43426-43426

    • DOI

      10.1103/physreva.87.043426

    • NAID

      110009754754

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] "Effect of nuclear motion on tunneling ionization rates of molecules"2013

    • Author(s)
      O. I. Tolstikhin, H. J. Worner, and T. Morishita
    • Journal Title

      Phys. Rev. A

      Volume: 87, 041401(R) Issue: 4

    • DOI

      10.1103/physreva.87.041401

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] Phase-resolved imaging of an attosecond electron wavepacket2018

    • Author(s)
      H. Niikura, P. Hockett, S. Patchkovskii, M.J.J. Vrakking and D. Villeneuve
    • Organizer
      Symposium on Recollision Physics 2018
    • Related Report
      Products Report
  • [Presentation] アト秒位相分解波動関数イメージング2018

    • Author(s)
      新倉弘倫
    • Organizer
      レーザー学会学術講演会第39次年会
    • Related Report
      Products Report
  • [Presentation] Phase-resolved electron wavepacket imaging using attosecond pulse2016

    • Author(s)
      P. Hockett, D. Villeneuve and H. Niikura
    • Organizer
      Gordon Research Conference (Multiphoton Processes)
    • Place of Presentation
      Proctor Academy,NH, USA
    • Year and Date
      2016-06-19
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Transition state spectroscopy of the reactions induced by coherent molecular vibration in the electronic ground state2015

    • Author(s)
      Izumi Iwakura
    • Organizer
      EMN Ultrafast Meeting
    • Place of Presentation
      Las Vegas, USA
    • Year and Date
      2015-11-16
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Time-dependent photoelectron momentum structures with attosecond time-resolution2015

    • Author(s)
      H. Niikura and T. Morishita
    • Organizer
      5th International conference on. Attosecond Physics
    • Place of Presentation
      St-Sauveur, Canada
    • Year and Date
      2015-07-06
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] A simple approach to time-dependent photoelectron momentum spectroscopy combined with attosecond laser pulses2015

    • Author(s)
      H. Niikura
    • Organizer
      Ultrafast Dynamic Imaging of Matter
    • Place of Presentation
      Grindelwald, Swiss
    • Year and Date
      2015-03-07 – 2015-03-14
    • Related Report
      2014 Annual Research Report
  • [Presentation] Atomic and molecular tunneling ionization in a static electric field: From tunneling to over-the-barrier regimes2014

    • Author(s)
      T. Morishita
    • Organizer
      International Workshop on Strong Field Physics and Ultrafast Phenomena
    • Place of Presentation
      Zhangjiajie, China
    • Year and Date
      2014-10-31 – 2014-11-04
    • Related Report
      2014 Annual Research Report
  • [Presentation] Laser induced rescattering electron spectroscopy for ultrafast atomic and molecular imaging2014

    • Author(s)
      T. Morishita
    • Organizer
      Atomic and molecular physics: a joint Japanese and French view over 120 years
    • Place of Presentation
      Cernay la Ville - France
    • Year and Date
      2014-07-21 – 2014-07-23
    • Related Report
      2014 Annual Research Report
  • [Presentation] Atomic and molecular tunneling ionization in a static electric field:2014

    • Author(s)
      T. Morishita
    • Organizer
      LPHYS 14, 23 th International Laser Physics Workshop
    • Place of Presentation
      Sofia, Burgaria
    • Year and Date
      2014-07-14 – 2014-07-18
    • Related Report
      2014 Annual Research Report
  • [Presentation] Controlling attosecond electron wave packet in a molecule2014

    • Author(s)
      H. Niikura
    • Organizer
      Ultra-fast phenomena
    • Place of Presentation
      Okinawa, Japan
    • Year and Date
      2014-07-07 – 2014-07-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] Atomic and Molecular Ionization by Intense Laser Fields: From Tunneling to Over-the-Barrier Regimes2014

    • Author(s)
      T. Morishita
    • Organizer
      Gordon Research Conference, Photoionization & Photodetachment, Probing Electronic and Nuclear Dynamics
    • Place of Presentation
      Hotel Galvez, Galveston, TX
    • Related Report
      2013 Annual Research Report
  • [Presentation] Control of attosecond electron wave packet in polyatomic molecules2013

    • Author(s)
      H. Niikura
    • Organizer
      4th International Conference on Attosecond Physics
    • Place of Presentation
      pasteur, pari, France
    • Related Report
      2013 Annual Research Report
  • [Presentation] Two-electron dynamics in nonlinear double excitation of helium by intense ultrashort extreme-ultraviolet pulses2013

    • Author(s)
      T. Morishita
    • Organizer
      International Symposium on (e,2e), Double Photoionization and Related Topics & 17th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions
    • Place of Presentation
      He Fei, China
    • Related Report
      2013 Annual Research Report
  • [Presentation] Atomic and molecular ionization in a static electric field: From tunneling to over-the-barrier regimes

    • Author(s)
      T. Morishita
    • Organizer
      The workshop on Strong Laser Physics, Shang-tou university
    • Place of Presentation
      Shang-tou, China
    • Related Report
      2013 Annual Research Report
  • [Remarks] サイエンス誌との契約により

    • URL

      http://www.f.waseda.jp/niikura/en/pubaE.htm

    • Related Report
      Products Report
  • [Remarks] [1]の論文(Coherent imaging of an attosecond electron wave packet)は、からダウンロード可能になっている。

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      Products Report

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Published: 2013-05-15   Modified: 2019-07-29  

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