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Plasmon hybridization near-field Raman microscopy

Research Project

Project/Area Number 25286008
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Nanostructural physics
Research InstitutionOsaka University

Principal Investigator

Verma Prabhat  大阪大学, 工学(系)研究科(研究院), 教授 (60362662)

Co-Investigator(Kenkyū-buntansha) 齊藤 結花  大阪大学, 工学(系)研究科(研究院), 准教授 (90373307)
Project Period (FY) 2013-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥19,370,000 (Direct Cost: ¥14,900,000、Indirect Cost: ¥4,470,000)
Fiscal Year 2015: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2014: ¥9,490,000 (Direct Cost: ¥7,300,000、Indirect Cost: ¥2,190,000)
Fiscal Year 2013: ¥5,200,000 (Direct Cost: ¥4,000,000、Indirect Cost: ¥1,200,000)
Keywordsナノプローブ / 近接場光学顕微鏡 / Plasmon resonance / plasmon resonance tuning / enhanced spectroscopy / TERS / ナノマイクロ科学 / ナノ構造物理 / 近接場顕微鏡
Outline of Final Research Achievements

Tuning of plasmon resonant wavelength of a metallic tip in near-field scanning optical microscopy is highly important to make it more practical and reliable. In this research, we applied plasmon hybridization in near-field scanning optical microscopy for wide-range tuning of plasmon resonance. Plasmon hybridization between a metallic tip and a thin metallic substrate allows to tune plasmon resonant wavelength over wide frequency range, just by changing metal thickness. We have performed FDTD simulation to optimize controllability of plasmon resonance, where kind of material, apex size, and metal thickness were investigated. Also, we have found out an optical conditions to fabricate extremely smooth metal film on a glass substrate, by adjusting evaporation conditions such as evaporation angle and rate. We have controlled plasmon resonant wavelength from 450 nm to 650 nm through the plasmon hybridization technique.

Report

(5 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Annual Research Report
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • Research Products

    (49 results)

All 2017 2016 2015 2014 2013

All Journal Article (16 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 12 results,  Acknowledgement Compliant: 5 results) Presentation (33 results) (of which Int'l Joint Research: 15 results,  Invited: 28 results)

  • [Journal Article] A Review on Tip-Enhanced Raman Spectroscopy2017

    • Author(s)
      P. Verma
    • Journal Title

      Chem. Rev.

      Volume: 1 Pages: 1-1

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Near-field absorption imaging by a Raman nano-light source2016

    • Author(s)
      R. Kato, Y. Saito, and P. Verma
    • Journal Title

      RSC Adv.

      Volume: 6 Pages: 113139-113139

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Control of near-field polarizations for nanoscale molecular orientational imaging2016

    • Author(s)
      T. Mino, Y. Saito, and P. Verma
    • Journal Title

      Appl. Phys. Lett.

      Volume: 109 Pages: 041105-041105

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Highly efficient plasmonic tip design for plasmon nanofocusing in near-field optical microscopy2016

    • Author(s)
      T. Umakoshi, Y. Saito, and P. Verma
    • Journal Title

      Nanoscale

      Volume: 8 Pages: 5634-5634

    • Related Report
      2016 Annual Research Report 2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] High-sensitivity pesticide detection using particle-enhanced resonant Raman scattering2016

    • Author(s)
      B. Ranjan, Y. Saito, and P. Verma
    • Journal Title

      Appl. Phys. Exp.

      Volume: 9 Pages: 032401-032401

    • NAID

      210000137818

    • Related Report
      2016 Annual Research Report 2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Superhydrophobic SERS Substrates Based on Silver-Coated Reduced Graphene Oxide Gratings Prepared by Two-Beam Laser Interference2015

    • Author(s)
      Z. Yan, Y. Zhang, W. Wang, X. Fu, H. Jiang, Y. Liu, P. Verma, S. Kawata, and H. B. Sun
    • Journal Title

      ACS Appl. Mater. Interfaces

      Volume: 7 Pages: 27059-27059

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Optical Antennas with Multiple Plasmonic Nanoparticles for Tip-Enhanced Raman Microscopy2015

    • Author(s)
      A. Taguchi, Y. Jun, P. Verma and S. Kawata
    • Journal Title

      Nanoscale

      Volume: 7 Pages: 17424-17424

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Silver Hierarchical Structures Grown on Microstructured Silicon in Chip for Microfluidic Integrated Catalyst and SERS Detector2015

    • Author(s)
      Z. Yan, C. Li, Y. Luo, J. Zhao, H. Yang, P. Verma, and S. Kawata
    • Journal Title

      Chinese Optics Letters

      Volume: 13 Pages: 102401-102401

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Temperature-dependent Photodegradation in UV-resonance Raman Spectroscopy2015

    • Author(s)
      H. Yoshino, Y. Saito, Y. Kumamoto, A. Taguchi, P. Verma, and S. Kawata
    • Journal Title

      Analytical Sciences

      Volume: 31 Pages: 451-451

    • NAID

      130005067341

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Optical antennas for tunable enhancement in tip-enhanced Raman spectroscopy imaging2015

    • Author(s)
      I. Maouli, A. Taguchi, Y. Saito, S. Kawata and P. Verma
    • Journal Title

      Appl. Phys. Express

      Volume: 8 Pages: 032401-032401

    • NAID

      210000137427

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temperature dependent photodegradation in UV resonant Raman spectroscopy2015

    • Author(s)
      H. Yoshino, Y. Saito, Y. Kumamoto, A. Taguchi, P. Verma and S. Kawata
    • Journal Title

      Analytical Science

      Volume: 印刷中

    • NAID

      130005067341

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantitative Analysis of Polarization-Controlled Tip-Enhanced Raman Imaging Through the Evaluation of Tip Dipole2014

    • Author(s)
      T. Mino, Y. Saito, and P. Verma
    • Journal Title

      ACS Nano

      Volume: 8 Pages: 10187-10187

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tip-enhanced Raman investigation of extremely localized semiconductor-to-metal transition of carbon nanotube2013

    • Author(s)
      Y. Okuno, Y. Saito, S. Kawata, and P. Verma
    • Journal Title

      Phys. Rev. Lett.

      Volume: 111 Pages: 216101-216101

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tip-enhanced nano-Raman analytical imaging of locally-induced strain distribution in carbon nanotubes2013

    • Author(s)
      T. Yano, T. Ichimura, S. Kuwahara, F. H'Dhili, K. Uetsuki, Y. Okuno, P. Verma, and S. Kawata
    • Journal Title

      Nature Commun

      Volume: 4 Pages: 2592-2592

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Far-field free tapping-mode tip-enhanced Raman microscopy2013

    • Author(s)
      J. Yu, Y. Saito, T. Ichimura, S. Kawata and P. Verma
    • Journal Title

      Appl. Phys. Lett.

      Volume: 102 Pages: 123110-123110

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Evaluation of the interlayer interactions of few layers of graphene2013

    • Author(s)
      J. Tsurumi, Y. Saito and P. Verma
    • Journal Title

      Chem. Phys. Lett.

      Volume: 557 Pages: 114-114

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] Nano-optical imaging with Tip-Enhanced Raman Spectroscopy2017

    • Author(s)
      Prabhat Verma
    • Organizer
      The 6th Conference on Nanomaterials
    • Place of Presentation
      Bangkok, Thailand
    • Year and Date
      2017-01-03
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Optical Imaging at Nanoscale Using Tip-Enhanced Raman Spectroscopy2016

    • Author(s)
      Prabhat Verma
    • Organizer
      Photonics 2016
    • Place of Presentation
      Kanpur, India
    • Year and Date
      2016-12-04
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Nanoimaging with tip-enhanced Raman spectroscopy: Seeing what others don’t2016

    • Author(s)
      Prabhat Verma
    • Organizer
      International Conference on Perspectives in Vibrational Spectroscopy
    • Place of Presentation
      Lucknow, India
    • Year and Date
      2016-11-05
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] White Nano-light-source for Optical Nanoimaging with TERS2016

    • Author(s)
      Prabhat Verma
    • Organizer
      34th Annual Meeting of SPP4th Annual Meeting of SPP
    • Place of Presentation
      Iloilo, Philippines
    • Year and Date
      2016-08-18
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] White Nano-light-source for TERS Nanoimaging2016

    • Author(s)
      Prabhat Verma
    • Organizer
      The 13th Progress in Electromagnetics Research Symposium
    • Place of Presentation
      Shanghai, China
    • Year and Date
      2016-08-08
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Broadband Nano-Light-Source through Plasmon Nanofocusing for Background-Free NSOM and TERS Imaging2016

    • Author(s)
      Prabhat Verma
    • Organizer
      The 6th International Multidisciplinary Conference on Optofluidics
    • Place of Presentation
      Beijing, China
    • Year and Date
      2016-07-24
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] White Nano-light-source through Plasmon Nano-focusing for TERS2016

    • Author(s)
      Prabhat Verma
    • Organizer
      International Conference on Electronic Materials
    • Place of Presentation
      Singapore
    • Year and Date
      2016-07-04
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] High-Resolution Nanoimaging with Tip-Enhanced Raman Spectroscopy2016

    • Author(s)
      Prabhat Verma
    • Organizer
      The 9th International Conference on Nanophotonics
    • Place of Presentation
      Taipei, Taiwan
    • Year and Date
      2016-03-21
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] High-Resolution Optical Nanoimaging with Tip-Enhanced Raman Spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      The International Conference on Small Science
    • Place of Presentation
      Phuket, Thailand
    • Year and Date
      2015-11-04
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] “Optical Imaging at the Nanometer Scale: Seeing What Light Cannot SeeOptical Imaging at the Nanometer Scale: Seeing What Light Cannot See2015

    • Author(s)
      Prabhat Verma
    • Organizer
      3M Nano 2016
    • Place of Presentation
      Changchun, China
    • Year and Date
      2015-10-05
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Nanophotonics with Tip-enhanced Raman Spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      International Conference on Optical MEMS and Nanophotonics
    • Place of Presentation
      Jerusalem, Israel,
    • Year and Date
      2015-08-02
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Manipulating light at optical antenna in tip-enhances Raman spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      The 7th International Conference on Information Optics and Photonics
    • Place of Presentation
      Nanjing, China
    • Year and Date
      2015-07-12
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Nano-scale optical imaging with tip-enhanced Raman spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      Nano Korea 2015 Symposium
    • Place of Presentation
      Seoul, Korea
    • Year and Date
      2015-07-01
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Controlling Nano-antennas In Tip-enhanced Raman Spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      International Conference on Materials for Advanced Technologies
    • Place of Presentation
      Singapore
    • Year and Date
      2015-06-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Optical Imaging at the Nanometer Scale through Tip-Enhanced Raman Spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      33rd Physics Congress of the Physics Society of the Philippines
    • Place of Presentation
      Vigan, Philippines
    • Year and Date
      2015-06-03
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Optical antennas for tip-enhanced Raman spectroscopy2015

    • Author(s)
      Prabhat Verma
    • Organizer
      Workshop on Functional Nanophotonics
    • Place of Presentation
      Rabat, Morocco
    • Year and Date
      2015-02-25 – 2015-02-26
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Seeing what light cannot see2015

    • Author(s)
      Prabhat Verma
    • Organizer
      OPTO Osaka 2015
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2015-01-14
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Polarization in Tip-enhanced Raman spectroscopy2014

    • Author(s)
      Prabhat Verma
    • Organizer
      Singapore-Japan International Workshop on Nanohotonics, Plasmonics and Metamaterials
    • Place of Presentation
      Singapore
    • Year and Date
      2014-12-11 – 2014-12-12
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Plasmon focusing for background-free near-field microscopy2014

    • Author(s)
      Takayuki Umakoshi, Yuika Saito, Prabhat Verma
    • Organizer
      Japan-Singapore International Workshop on Nanophotonics, Plasmonics and Metamaterials
    • Place of Presentation
      Nanyang Technological Univ. Singapore
    • Year and Date
      2014-12-10 – 2014-12-13
    • Related Report
      2014 Annual Research Report
  • [Presentation] Techniques in tip-enhanced Raman spectroscopy2014

    • Author(s)
      Prabhat Verma
    • Organizer
      KAST Frontier Scientists Symposium on Photonic Nanostructures
    • Place of Presentation
      Seoul, South Korea
    • Year and Date
      2014-12-04 – 2014-12-05
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Tip-enhanced Raman spectroscopy at extremely high spatial resolution2014

    • Author(s)
      Prabhat Verma
    • Organizer
      OSJ Optics&Photonics Japan 2014
    • Place of Presentation
      Tokyo, Japan
    • Year and Date
      2014-11-05 – 2014-11-07
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Optimization of plasmonic tip structure for background-free nano imaging2014

    • Author(s)
      Takayuki Umakoshi, Yuika Saito, Prabhat Verma
    • Organizer
      The 13th International Conference on Near-field Optics, Nanophotonics and Related techniques
    • Place of Presentation
      Salt Lake City, USA
    • Year and Date
      2014-10-18 – 2014-10-25
    • Related Report
      2014 Annual Research Report
  • [Presentation] Nanoscale optical investigation of electronic properties of carbon nanotubes2014

    • Author(s)
      Prabhat Verma
    • Organizer
      SPIE Photonics Asia 2014
    • Place of Presentation
      Beijing, China
    • Year and Date
      2014-10-09 – 2014-10-11
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] プラズモンフォーカシングによる光学ナノイメージング2014

    • Author(s)
      馬越貴之、齊藤結花、プラブハット バルマ
    • Organizer
      2014年秋季第75回応用物理学会学術講演会
    • Place of Presentation
      北海道大学
    • Year and Date
      2014-09-16 – 2014-09-21
    • Related Report
      2014 Annual Research Report
  • [Presentation] Optical nano-imaging via plasmon forcusing on metallic tip2014

    • Author(s)
      Takayuki Umakoshi, Yuika Saito and Prabhat Verma
    • Organizer
      International OSA Network of Students Asia 5 Hokkaido
    • Place of Presentation
      Clark Memorial Student center, Hokkaido, Japan
    • Year and Date
      2014-09-14 – 2014-09-21
    • Related Report
      2014 Annual Research Report
  • [Presentation] Tip-Enhanced Raman Spectroscopy at Extremely High Spatial Resolution2014

    • Author(s)
      Prabhat Verma
    • Organizer
      5th International Conference on Prospectives in Vibrational Spectroscopy
    • Place of Presentation
      Trivandrum, India
    • Year and Date
      2014-07-08 – 2014-07-12
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Tip-Enhanced Raman Investigation of the Localization of Electronic Properties in Carbon Nanotubes2014

    • Author(s)
      Prabhat Verma
    • Organizer
      META 20 14, The 5th International Conference on Metamaterials, Photonic Crystals and Plasmonics
    • Place of Presentation
      Singapore
    • Year and Date
      2014-05-20 – 2014-05-23
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Tip-enhanced Raman investigation of localized electronic properties in ‘X’-shaped carbon nanotubes2014

    • Author(s)
      Verma Prabhat
    • Organizer
      International Symposium on Nanophotonics and Nanomaterials
    • Place of Presentation
      Beijing
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Tip-enhanced Raman investigation of localized electronic properties in carbon nanotubes2014

    • Author(s)
      Verma Prabhat
    • Organizer
      Japan-Taiwan Bilateral Conference: Biomedical and Plasmonic Imaging
    • Place of Presentation
      Taipei
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Tip-enhanced Raman investigation of localized semiconductor-to-metal transition in carbon nanotubes2014

    • Author(s)
      Verma Prabhat
    • Organizer
      The Third International Conference on Frontiers of Plasmonics
    • Place of Presentation
      Xiamen
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Tip-enhanced Fluorescence imaging with nanometric control on tip-sample separation2013

    • Author(s)
      Verma Prabhat
    • Organizer
      The 9th Asia-Pacific Conference on Near-field Optics
    • Place of Presentation
      Singapore
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Nanometric control on tip-sample separation for TERS and tip-enhanced fluorescence imaging2013

    • Author(s)
      Verma Prabhat
    • Organizer
      TERS III - 3rd Meeting on Tip Enhanced Raman Spectroscopy
    • Place of Presentation
      Zurich
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Some improved techniques for better nanoimaging through tip-enhanced Raman scattering2013

    • Author(s)
      Verma Prabhat
    • Organizer
      Nanoimaging and Nanospectroscopy, SPIE Optics + Photonics
    • Place of Presentation
      San Diego
    • Related Report
      2013 Annual Research Report
    • Invited

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Published: 2013-05-21   Modified: 2019-07-29  

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