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Development on low dimensional thermoelectric thin films

Research Project

Project/Area Number 25289043
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Thermal engineering
Research InstitutionKyushu Institute of Technology

Principal Investigator

Miyazaki Koji  九州工業大学, 工学(系)研究科(研究院), 教授 (70315159)

Co-Investigator(Kenkyū-buntansha) TAKASHIRI Masayuki  東海大学, 工学部, 准教授 (50631818)
YABUKI Tomohide  九州工業大学, 大学院工学研究院, 助教 (70734143)
TANAKA Saburo  日本大学, 工学部, 助教 (30713127)
Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥16,250,000 (Direct Cost: ¥12,500,000、Indirect Cost: ¥3,750,000)
Fiscal Year 2015: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2014: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2013: ¥8,450,000 (Direct Cost: ¥6,500,000、Indirect Cost: ¥1,950,000)
Keywordsナノマイクロ熱工学 / 低次元半導体 / 熱電変換 / 薄膜生成 / ナノインプリント
Outline of Final Research Achievements

Bismuth telluride thin films were made by using vacuum arc plasma deposition method. Bismuth telluride film with 10nm thickness was deposited on glass substrate heated at 200℃ during the deposition process. The thermoelectric properties of the films were measured, and the maximum Seebeck coefficient was 167 microW/K. The Seebeck coefficient was increased when the film thickness was decreased. However, the increase of the Seebeck coefficient can be explained well by classical carrier transport model. The measured ZT was only 0.5 at 300K. It was lower than the expected value of a low dimensional Bismuth telluride film. We demonstrated fabrication of nano-wire of Bismuth telluride by depositing the film on a nano-structured substrate. The Bismuth telluride nano-wire with 50nm diameter was fabricated successfully.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • Research Products

    (28 results)

All 2016 2015 2014 2013 Other

All Journal Article (8 results) (of which Peer Reviewed: 8 results,  Acknowledgement Compliant: 1 results) Presentation (18 results) (of which Int'l Joint Research: 4 results,  Invited: 6 results) Book (1 results) Remarks (1 results)

  • [Journal Article] Enhanced thermoelectric properties of phase-separating bismuth selenium telluride thin films via a two-step method2015

    • Author(s)
      Masayuki Takashiri,Kensuke Kurita,Harutoshi Hagino,Saburo Tanaka,Koji Miyazaki
    • Journal Title

      Journal of Applied Physics

      Volume: 118 Issue: 6 Pages: 065301-065301

    • DOI

      10.1063/1.4928311

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Thermal design of a thermoelectric micro-generator2015

    • Author(s)
      Shota Hama, Tomohide Yabuki, Laurent Tranchant, Koji Miyazaki
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 660 Pages: 012088-012088

    • DOI

      10.1088/1742-6596/660/1/012088

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Comparison of crystal growth and thermoelectric properties of n-type Bi-Se-Te and p-type Bi-Sb-Te nanocrystalline thin films: Effects of homogeneous irradiation with an electron beam2014

    • Author(s)
      Masayuki Takashiri, Kazuo Imai, Masato Uyama, Harutoshi Hagino, Saburo Tanaka, Koji Miyazaki, Yoshitake Nishi
    • Journal Title

      Journal of Applied Physics

      Volume: 115 Issue: 21 Pages: 214311-214311

    • DOI

      10.1063/1.4881676

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Effects of homogeneous irradiation of electron beam on crystal growth and thermoelectric properties of nanocrystalline bismuth selenium telluride thin films2014

    • Author(s)
      Masayuki Takashiri, Kazuo Imai, Masato Uyama, Harutoshi Hagino, Saburo Tanaka, Koji Miyazaki, Yoshitake Nishi
    • Journal Title

      Journal of Alloys and Compounds

      Volume: 612 Pages: 98-102

    • DOI

      10.1016/j.jallcom.2014.05.146

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Strain and grain size effects on thermal transport in highly-oriented nanocrysatalline bisumuth antimony telluride thin films2014

    • Author(s)
      Masayuki Takashiri, Saburo Tanaka, Harutoshi Hagino, Koji Miyazaki
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 76 Pages: 376-384

    • DOI

      10.1016/j.ijheatmasstransfer.2014.04.048

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication by Coaxial-Type Vacuum Arc Evaporation Method and Characterization of Bismuth Telluride Thin Films2013

    • Author(s)
      Michitaka Uchino, Kunihisa Kato, Harutoshi Hagino, and Koji Miyazaki
    • Journal Title

      Journal of Electronic Materials

      Volume: 42 Issue: 7 Pages: 1814-1819

    • DOI

      10.1007/s11664-012-2438-2

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Determination of the origin of crystal orientation for nanocrystalline bismuth telluride-based thin films prepared by use of the flash evaporation method2013

    • Author(s)
      Masayuki Takashiri, Saburo Tanaka, Koji Miyazaki
    • Journal Title

      Journal of Electronic Materials

      Volume: 未定 Issue: 6 Pages: 1881-1889

    • DOI

      10.1007/s11664-013-2896-1

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Growth of single-crystalline bismuth antimony telluride nanoplates on the surface of nanoparticle thin films2013

    • Author(s)
      Masayuki Takashiri, Saburo Tanaka, Koji Miyazaki
    • Journal Title

      Journal of Crystal Growth

      Volume: 372 Pages: 199-204

    • DOI

      10.1016/j.jcrysgro.2013.03.028

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Presentation] Enhanced Figure of Merit of a Self-assembled Micro-porous Bismuth Telluride Thin Film2016

    • Author(s)
      Koji Miyazaki
    • Organizer
      The 1st Pacific Rim Thermal Engineering Conference
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2016-03-13
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] めっき法を用いたビスマステルライド系薄膜及び熱電モジュールに及ぼす熱処理の影響2015

    • Author(s)
      初田 直樹, 和地 誠, 竹森 大地, 高尻 雅之
    • Organizer
      第7回マイクロ・ナノ工学シンポジウム
    • Place of Presentation
      新潟
    • Year and Date
      2015-10-28
    • Related Report
      2015 Annual Research Report
  • [Presentation] Bismuth Telluride thin films and their applications2015

    • Author(s)
      Koji Miyazaki, Kunihiro Yamada, Shota Hama, Tomohide Yabuki
    • Organizer
      14th International Union of Materials Research Societies-International Conference on Advanced Materials
    • Place of Presentation
      Jeju, Korea
    • Year and Date
      2015-10-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 基板加熱アークプラズマ蒸着によるBi2Te3薄膜の生成2015

    • Author(s)
      山田晋弘,濱翔太,矢吹智英,Laurent Tranchant,宮崎康次
    • Organizer
      第12回日本熱電学会学術講演会
    • Place of Presentation
      福岡
    • Year and Date
      2015-09-07
    • Related Report
      2015 Annual Research Report
  • [Presentation] Heat conduction in a micro-porous Si thin film2015

    • Author(s)
      Koji Miyazaki
    • Organizer
      International symposium on micro and nano technology
    • Place of Presentation
      Calgary, Canda
    • Year and Date
      2015-06-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] The influence of substrate temperature on thermoelectric properties of bismuth telluride thin films2015

    • Author(s)
      K. Yamada, S. Hama, T. Yabuki, L. Tranchant, K. Miyazaki
    • Organizer
      34th International Conference on Thermoelectrics
    • Place of Presentation
      Dresden, Germany
    • Year and Date
      2015-06-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 真空アーク蒸着法による低次元熱電薄膜の生成と評価2014

    • Author(s)
      山田晋弘,濱翔太,矢吹智英,宮崎康次
    • Organizer
      日本機械学会第6回マイクロ・ナノ工学シンポジウム
    • Place of Presentation
      松江
    • Year and Date
      2014-10-20
    • Related Report
      2014 Annual Research Report
  • [Presentation] Inorganic-organic Composite for a Flexible Thermoelectric Device2014

    • Author(s)
      Koji Miyazaki
    • Organizer
      7th Taiwan-Japan Workshop on Mechanical and Aerospace Engineering
    • Place of Presentation
      Taipei, Taiwan
    • Year and Date
      2014-09-13
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] 熱電変換素子の基礎と応用2014

    • Author(s)
      宮崎 康次
    • Organizer
      IEEE 2014 International Meeting for Future of Electron Devices, Kansai
    • Place of Presentation
      京都
    • Year and Date
      2014-06-19
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Organic-Inorganic Nano-structured Composite for Thermoelectrics2014

    • Author(s)
      Koji Miyazaki
    • Organizer
      2014 Energy Materials Nanotechnology East Meeting
    • Place of Presentation
      Beijing, China
    • Year and Date
      2014-05-12
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] ビスマス・テルライド系薄膜の構造・熱電特性における電子線照射の効果2014

    • Author(s)
      今井和朗,宇山将人,萩野春俊,田中三郎,宮崎康次,西義武,高尻雅之
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      相模原
    • Related Report
      2013 Annual Research Report
  • [Presentation] 電子線照射したビスマス・テルライド系薄膜熱電素子の構造・熱電特性の評価2014

    • Author(s)
      今井和朗,宇山将人,西義武,高尻雅之
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      相模原
    • Related Report
      2013 Annual Research Report
  • [Presentation] アークプラズマガンによる熱電薄膜の生成と評価2013

    • Author(s)
      内野道隆,山田晋弘,山本明宏,加藤邦久,宮崎康次
    • Organizer
      第34回日本熱物性シンポジウム
    • Place of Presentation
      富山
    • Related Report
      2013 Annual Research Report
  • [Presentation] ナノ構造ビスマステルライドの格子熱伝導率2013

    • Author(s)
      田中三郎,高尻雅之,宮崎康次,佐々木直栄
    • Organizer
      第5回マイクロ・ナノ工学シンポジウム
    • Place of Presentation
      仙台
    • Related Report
      2013 Annual Research Report
  • [Presentation] ビスマステルライド系薄膜の格子熱伝導率における応力とナノサイズ効果2013

    • Author(s)
      鄭東,田中三郎,宮崎康次,高尻雅之
    • Organizer
      第5回マイクロ・ナノ工学シンポジウム
    • Place of Presentation
      仙台
    • Related Report
      2013 Annual Research Report
  • [Presentation] ビスマステルライド薄膜の面方向熱伝導率測定2013

    • Author(s)
      萩野春俊,内野道隆,高尻雅之,田中三郎,宮崎康次
    • Organizer
      第10回日本熱電学会
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
  • [Presentation] めっき法によるビスマス・テルライド系薄膜熱電素子の作製と物性評価2013

    • Author(s)
      初田直樹,松岡健,高尻雅之
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      相模原
    • Related Report
      2013 Annual Research Report
  • [Presentation] ナノ結晶ビスマステルライド系薄膜の熱輸送における残留応力の効果2013

    • Author(s)
      高尻雅之,田中三郎,宮崎康次
    • Organizer
      第10回日本熱電学会
    • Place of Presentation
      名古屋
    • Related Report
      2013 Annual Research Report
  • [Book] 熱電変換材料 実用・活用を目指した設計と開発2014

    • Author(s)
      黒崎健ら 他28名
    • Total Pages
      249
    • Publisher
      情報機構
    • Related Report
      2014 Annual Research Report
  • [Remarks] 九州工業大学 熱デバイス研究室

    • URL

      http://www.mech.kyutech.ac.jp/tdl/study/index.html

    • Related Report
      2015 Annual Research Report

URL: 

Published: 2013-05-21   Modified: 2019-07-29  

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